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低光照强度下氧化石墨烯-g-C_3N_4/PVDF膜的光催化降解性能研究 被引量:5

Synthesis of Graphene Oxide Doped g-C_3N_4/ PVDF Membrane and Photodegradation in Low Light Intensity
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摘要 基于π-π非共价掺杂的原理,采用半封闭高温烧结法制备了GO/g-C3N4。结构分析表明,GO与g-C3N4发生了相互作用。考察了GO引入前后g-C3N4在低光照强度下紫外光降解甲基橙的光催化活性。结果表明,掺杂适量的GO能够提高g-C3N4的光催化活性,当烧结温度为500℃、GO掺杂量为0.5wt%,热解温度为500℃时光催化降解率最高,达到39.50%。 Graphite oxide (GO) doped C3N4 was composed by semi - closed method based on π-π stacking interaction between GO and g-C3N4. The structural analysis results proved the π-π stacking interaction. The photocatalytic activities of g-C3N4 before and after GO modification were compared after composed with PVDF membranein low light intensity. The results showed that photocatalytic activity of g-C3N4 can be improved by doping right amount of GO, the photodegradation rate of GO/g-C3N4 reached its maximum value 39.50% at 0.5wt% GO and 500 ℃, for the MO photodegradation.
出处 《科学技术与工程》 北大核心 2015年第16期1-6,共6页 Science Technology and Engineering
基金 江苏省自然科学基金(BK20130747) 江苏省科技支撑计划项目(BE2014039) 南京工程学院大学生科技创新基金(N20150231)资助
关键词 Fe掺杂g-C3N4 PVDF复合膜 低光照强度 光催化降解 GO doped g-C3N4 PVDF composite membrane low light intensity photocatalytic degradation
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参考文献18

  • 1Lim S H, Elim H I, Gao X Y, et al. Electronic and optical properties of nitrogen-doped multiwalled carbon nanotubes. Physical Review B, 2006; 73(4) : 45402(1-6). 被引量:1
  • 2Xiao K, Liu Y, Hu Pinghn, et al. n-type field-effect transistors made of an individual nitrogen-doped muhiwalled carbon nanotube. Journal of the American Chemical Society,2005 ; 127(24) : 8614-8617. 被引量:1
  • 3Deifallah M, Mcmillan P F, Cora F. Electronic and structural proper- ties of two-dimensional carbon nitride graphenes. Journal of Hysical Hemistry C ,2008 ; 112(14) : 5447-5453. 被引量:1
  • 4Enoki T, Kobayashi Y. Magnetic nanographite: an approach to molec- ular magnetism. Journal of Materials Chemistry, 2005 ; 15 ( 37 ) : 3999--4002. 被引量:1
  • 5Tomita S, Sakurai T, Ohta H, et al. Structure and electronic proper- ties of carbon onions. The Journal of Chemical Physics,2001; 114: 7477-7482. 被引量:1
  • 6Endo M, Hayashi T, Hong S H, et al. Scanning tunneling microscope study of boron-doped highly oriented pyrolytic graphite. Journal of Ap- olied Physics.2001 : 90 : 5670. 被引量:1
  • 7田蒙奎,上官文峰,欧阳自远,王世杰.光解水制氢半导体光催化材料的研究进展[J].功能材料,2005,36(10):1489-1492. 被引量:19
  • 8Liao G, Chen S, Quan X, et al. Graphene oxide modified g-C3 N4 hy- brid with enhanced photocatalytic capability under visible light irradi- ation. Journal of Materials Chemistry, 2012 ; 22 ( 6 ) : 2721 -2726. 被引量:1
  • 9Du A, Sanvito S, Li Z, et al. Hybrid graphene and graphitic carbon nitride nanocomposite : gap opening, electron-hole puddle, interracial charge transfer, and enhanced visible light response. Journal of the AmericanChemical Society,2012 ; 134 (9) : 4393--4397. 被引量:1
  • 10Liu Q, Zhang J. Graphene supported Co-g-C3 N4 as a novel metal- macrocyclic electrocatalyst for the oxygen reduction reaction in fuel cells. Langmuir,2013 ; 29( 11 ) : 3821-3828. 被引量:1

二级参考文献54

  • 1李杰,曹传宝,朱鹤荪.三维大孔氮化碳材料的制备及其血液相容性[J].北京科技大学学报,2007,29(2):142-145. 被引量:8
  • 2沈伟韧 赵文宽 贺飞 方佑龄.化学进展(Shen W R.Zhao W K,He F,Fang Y L.Progr Chem),1998,10(4):349-349. 被引量:1
  • 3符小荣 宋世庚 王学燕 谭辉 武光明 陶明德.感光科学与光化学(Fu X R,Song Sh G,Wang X Y,Tan H,Wu G M,Tao M D.Photogr Sci Photochem),1997,15(3):234-234. 被引量:1
  • 4张新荣 赵梦月 陈士夫.感光科学与光化学(Zhang X R,Zhao M Y,Chen Sh F.Photogr Sci Photochem),2000,18(4):297-297. 被引量:1
  • 5赵文宽 覃榆森 方佑龄 董庆华.催化学报(Zhao W K,Tan Y S,Fang Y L,Dong Q H.Chin J Cata1),1999,20(3):368-368. 被引量:1
  • 6戴清 路春娥 翁葵平 袁春伟.催化学报(Dai Q,Lu Ch E,Weng K P,Yuan Ch W.Chin J Cata1),1999,20(3):313-313. 被引量:1
  • 7Liu A Y,Cohen M L. Prediction of new low compressibility solids [ J ]. Science, 1989,245:841-842. 被引量:1
  • 8Teter D M, Hemley R J. Low-compressibility carbon nitrides [ J ]. Science, 1996,271 : 53-55. 被引量:1
  • 9Vinu A,Ariga K,Mori T,et al. Preparation and characterization of well-ordered hexagonal mesopomus carbon nitride[ J]. Advanced Materials,2005 ,17 :1648-1652. 被引量:1
  • 10Zimerman J L, Williams R, Khabashesku V N, et al. Synthesis of spherical carbon nitride nanostructures [J]. Nano Letters,2001,1(12) :731-734. 被引量:1

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