期刊文献+

氮气气氛下旋转滑动弧重整甲烷制氢实验研究 被引量:7

Experimental Research of Hydrogen Production From Methane Reforming in Nitrogen Using a Rotating Gliding Arc Reactor
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摘要 本文采用切向气流和磁场协同驱动的旋转滑动弧低温等离子体,以氮气为载气,进行了甲烷重整制氢的研究。考察了进气流量,CH_4/N_2比和外加电阻对制氢效果的影响,结果表明,随着进气流量的增加,甲烷转化率逐渐降低;随着CH_4/N_2比的增大,外加电阻为40 kΩ时,甲烷转化率逐渐降低,最大可达87.49%,而外加电阻为70 kΩ时,甲烷转化率却先降低后增大;减小外加电阻有利于增加甲烷转化率和氢气选择性,但会造成能耗的增加。 A rotating gliding arc co-driven by tangential flow and magnetic field was used for hydrogen production from methane reforming in nitrogen. Effect of gas flow, CH4/N2 ratio and resistance on performance of methane reforming was investigated. The results show that, as gas flow rate grows, methane conversion decreases.For the 40 kΩ resistance, methane conversion decreases with rising CH4/N2 ratio. The maximum value is up to 87.48%. Whereas, for the 70 kΩ resistance, methane conversion first decreases and then increases for CH4/N2 increasing. A lower resistance is beneficial for methane conversion and hydrogen selectivity, but leads to higher energy consumption simultaneously.
出处 《工程热物理学报》 EI CAS CSCD 北大核心 2013年第4期787-790,共4页 Journal of Engineering Thermophysics
基金 国家自然科学基金资助项目(No.51076142)
关键词 旋转滑动弧 甲烷重整 制氢 rotating gliding arc methane reforming hydrogen production
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参考文献11

  • 1Gangoli S P, Gutsol A F, Fridman A A. A Non- Equilibrium Plasma Source: Magnetically Stabilized Glid- ing Arc Discharge: I . Design and Diagnostics [J]. Plasma Sources Sci Technol, 2010, 19(6): 1-7. 被引量:1
  • 2FridmanA, Nester S, Kennedy L A, et al. Gliding Arc Gas Discharge [J]. Progress in Energy Comb Sci, 1999, 25(2): 211-231. 被引量:1
  • 3Yan J H, Liu Y N, Bo Z, et al. Degradation of Gas-Liquid Gliding Arc Discharge on Acid Orange II [J]. Journal of Hazardous Materials, 2008, 157(2): 441-447. 被引量:1
  • 4XU G F, DING X W. Syngas Production from Methane Using AC Gliding Arc Reactor [C]// Power Energy Eng Conf. Wuhan: China, 2011:1-4. 被引量:1
  • 5KalraC S, GustolA F, PridmanAA. Gliding Arc Dis- charges as a Source of the Intermediate Plasma for Methane Partial Oxidation [J]. IEEE Trans Plasma Sci- ence, 2005, 33:32-41. 被引量:1
  • 6Rusu I, Cormier J M. On a Possible Mechanism of the Methane Steam Reforming in a Gliding Arc Reactor [J]. Chem En J, 2003, 91:23- 31. 被引量:1
  • 7颜士鑫,李晓东,钟犁,余量,严建华,岑可法.滑动弧等离子体协助甲烷蒸汽重整制氢[J].太阳能学报,2011,32(5):766-770. 被引量:5
  • 8Streethawong T, Thakonpatthanakun P, Chavadej S. Par- tial Oxidation of Methane with Air for Synthesis Gas Pro- duction in a Multistage Gliding Arc Discharge System [J]. Int J Hydrogen Energy, 2007, 32:1067-1079. 被引量:1
  • 9ZHANG J Q, YANG Y J, ZHANG J S, et al. Non- Oxidative Coupling of Methane to C2 Hydrocarbons Un- der Above-Atmospheric Pressure Using Pulsed Microwave Plasma [J]. Energy Fuels, 2002, 16:687-693. 被引量:1
  • 10Rueangjitt N, Streethawong T, Chavadej S, et al. Non- Oxidative Reforming of Methane in a Mini-Gliding Arc Discharge Reactor: Effects of Feed Methane Concentra- tion, Feed Flow Rate, Electrode Gap Distance, Residence Time, and Catalyst Distance [J]. Plasma Chem Plasma Process, 2011, 31:517-534. 被引量:1

二级参考文献10

  • 1毛宗强.氢能及其近期应用前景[J].科技导报,2005,23(2):34-38. 被引量:36
  • 2Yan J H,Liu Y N,Bo Z,et al.Degradation of gas-liquid gliding arc discharge on Acid Orange II[J].Journal of Hazardous Materials,2008,157(2):441-447. 被引量:1
  • 3Bo Zheng,Yan Jianhua,Li Xiaodong,et al.Plasma assisted dry methane reforming using gliding arc gas discharge:Effect of feed gases proportion[J].Internation Journal of Hydrogen Energy,2008,33(20):5545-5553. 被引量:1
  • 4SreethawongT,Thakonpatthanakun P,Chavadej S.Partial oxidation of methane with air for synthesis gas production in a multistage gliding arc discharge system[J].International Journal of Hydrogen Energy,2007,32:1067-1079. 被引量:1
  • 5Rusu I,Cormier J M.On a possible mechanism of the methane steam reforming in a gliding arc reactor[J].Chemical Engineering Journal,2003,91:23-31. 被引量:1
  • 6Gallagher M J,Geiger R,Polevich A,et al.On-board plasma-assisted conversion of heavy hydrocarbons into synthesis gas[J].Fuel,2009,89(6):1187-1192. 被引量:1
  • 7Fridman A,Nester S,Lawrence A,et al.Gliding arc gas discharge[J].Progress in Energy and Combustion,1999,25(2):211-231. 被引量:1
  • 8Bo Zheng,Yan Jianhua,Li Xiaodong,et al.Nitrogen dioxide formation in the gliding arc discharge-assisted decomposition of volatile organic compounds[J].Journal of Hazardous Materials,2009,166(2-3):1210-1216. 被引量:1
  • 9Kado S,Urasaki K,Sekine Y,et al.Reaction mechanism of methane activation using non-equilibrium pulsed discharge at room temperature[J].Fuel,2003,82(18):2291-297. 被引量:1
  • 10蔡炽柳.氢能及其应用前景分析[J].能源与环境,2008(5):39-41. 被引量:12

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