The development of self-powered water purification technologies for decentralized applications is crucial for ensuring the provision of drinking water in resource-limited regions. The elimination of the dependence on ...The development of self-powered water purification technologies for decentralized applications is crucial for ensuring the provision of drinking water in resource-limited regions. The elimination of the dependence on external energy inputs and the attainment of self-powered status significantly expands the applicability of the treatment system in real-world scenarios. Hybrid energy harvesters, which convert multiple ambient energies simultaneously, show the potential to drive self-powered water purification facilities under fluctuating actual conditions. Here, we propose recent advancements in hybrid energy systems that simultaneously harvest various ambient energies (e.g., photo irradiation, flow kinetic, thermal, and vibration) to drive water purification processes. The mechanisms of various energy harvesters and point-of-use water purification treatments are first outlined. Then we summarize the hybrid energy harvesters that can drive water purification treatment. These hybrid energy harvesters are based on the mechanisms of mechanical and photovoltaic, mechanical and thermal, and thermal and photovoltaic effects. This review provides a comprehensive understanding of the potential for advancing beyond the current state-of-the-art of hybrid energy harvester-driven water treatment processes. Future endeavors should focus on improving catalyst efficiency and developing sustainable hybrid energy harvesters to drive self-powered treatments under unstable conditions (e.g., fluctuating temperatures and humidity).展开更多
Over the years,the Shaying River Basin has experienced frequent instances of river pollution.The presence of numerous critical pollutant discharge enterprises and sewage-treatment plants in the vicinity of the Shaying...Over the years,the Shaying River Basin has experienced frequent instances of river pollution.The presence of numerous critical pollutant discharge enterprises and sewage-treatment plants in the vicinity of the Shaying River has transformed it a major tributary with relatively serious pollution challenge within the upper reaches of Huaihe River Basin.To study the sources of manganese(Mn),chromium(Cr),nickel(Ni),arsenic(As),cadmium(Cd)and lead(Pb)in Shaying River water,123 sets of surface water samples were collected from 41 sampling points across the entire basin during three distinct phases from 2019 to 2020,encompassing normal water period,dry season and wet season.The primary origins of heavy metals in river water were determined by analyzing the heavy metal contents in urban sewage wastewater,industrial sewage wastewater,groundwater,mine water,and the heavy metal contributions from agricultural non-point source pollution.The analytical findings reveal that Mn primarily originates from shallow groundwater used for agricultural irrigation,While Cr mainly is primarily sourced from urban sewage treatment plant effluents,coal washing wastewater,tannery wastewater,and industrial discharge related to metal processing and manufacturing.Ni is mainly contributed by urban sewage treatment plant effluents and industrial wastewater streams associated with machinery manufacturing and metal processing.Cd primarily linked to industrial wastewater,particularly from machinery manufacturing and metal processing facilities,while Pb is predominantly associated with urban sewage treatment plant effluents and wastewater generated in Pb processing and recycling wastewater.These research provides a crucial foundation for addressing the prevention and control of dissolved heavy metals at their sources in the Shaying River.展开更多
基金supported by the National Key R&D Program of China(No.2022YFC3205400)the National Natural Science Foundation of China(Grant No.52200079).
文摘The development of self-powered water purification technologies for decentralized applications is crucial for ensuring the provision of drinking water in resource-limited regions. The elimination of the dependence on external energy inputs and the attainment of self-powered status significantly expands the applicability of the treatment system in real-world scenarios. Hybrid energy harvesters, which convert multiple ambient energies simultaneously, show the potential to drive self-powered water purification facilities under fluctuating actual conditions. Here, we propose recent advancements in hybrid energy systems that simultaneously harvest various ambient energies (e.g., photo irradiation, flow kinetic, thermal, and vibration) to drive water purification processes. The mechanisms of various energy harvesters and point-of-use water purification treatments are first outlined. Then we summarize the hybrid energy harvesters that can drive water purification treatment. These hybrid energy harvesters are based on the mechanisms of mechanical and photovoltaic, mechanical and thermal, and thermal and photovoltaic effects. This review provides a comprehensive understanding of the potential for advancing beyond the current state-of-the-art of hybrid energy harvester-driven water treatment processes. Future endeavors should focus on improving catalyst efficiency and developing sustainable hybrid energy harvesters to drive self-powered treatments under unstable conditions (e.g., fluctuating temperatures and humidity).
基金funded and supported by the Youth Science and Technology Project of Henan Provincial Bureau of Geology and Mineral Resources,YDKQKC[2008]No.8.
文摘Over the years,the Shaying River Basin has experienced frequent instances of river pollution.The presence of numerous critical pollutant discharge enterprises and sewage-treatment plants in the vicinity of the Shaying River has transformed it a major tributary with relatively serious pollution challenge within the upper reaches of Huaihe River Basin.To study the sources of manganese(Mn),chromium(Cr),nickel(Ni),arsenic(As),cadmium(Cd)and lead(Pb)in Shaying River water,123 sets of surface water samples were collected from 41 sampling points across the entire basin during three distinct phases from 2019 to 2020,encompassing normal water period,dry season and wet season.The primary origins of heavy metals in river water were determined by analyzing the heavy metal contents in urban sewage wastewater,industrial sewage wastewater,groundwater,mine water,and the heavy metal contributions from agricultural non-point source pollution.The analytical findings reveal that Mn primarily originates from shallow groundwater used for agricultural irrigation,While Cr mainly is primarily sourced from urban sewage treatment plant effluents,coal washing wastewater,tannery wastewater,and industrial discharge related to metal processing and manufacturing.Ni is mainly contributed by urban sewage treatment plant effluents and industrial wastewater streams associated with machinery manufacturing and metal processing.Cd primarily linked to industrial wastewater,particularly from machinery manufacturing and metal processing facilities,while Pb is predominantly associated with urban sewage treatment plant effluents and wastewater generated in Pb processing and recycling wastewater.These research provides a crucial foundation for addressing the prevention and control of dissolved heavy metals at their sources in the Shaying River.
