Partial pressure of CO2(pCO2) was investigated in the Changjiang(Yangtze River) Estuary,Hangzhou Bay and their adjacent areas during a cruise in August 2004,China.The data show that pCO2 in surface waters of the studi...Partial pressure of CO2(pCO2) was investigated in the Changjiang(Yangtze River) Estuary,Hangzhou Bay and their adjacent areas during a cruise in August 2004,China.The data show that pCO2 in surface waters of the studied area was higher than that in the atmosphere with only exception of a patch east of Zhoushan Archipelago.The pCO2 varied from 168 to 2 264 μatm,which fell in the low range compared with those of other estuaries in the world.The calculated sea-air CO2 fluxes decreased offshore and varied from -10.0 to 88.1 mmol m-2 d-1 in average of 24.4 ± 16.5 mmol m-2 d-1.Although the area studied was estimated only 2 × 104 km2,it emitted(5.9 ± 4.0) × 103 tons of carbon to the atmosphere every day.The estuaries and their plumes must be further studied for better understanding the role of coastal seas playing in the global oceanic carbon cycle.展开更多
In the northwestern North Pacific,annual net air-sea CO_(2) flux is greatest in the Kuroshio Extension(KE)zone,owing to its low annual mean partial pressure of CO_(2)(pCO_(2)),and it decreases southward across the bas...In the northwestern North Pacific,annual net air-sea CO_(2) flux is greatest in the Kuroshio Extension(KE)zone,owing to its low annual mean partial pressure of CO_(2)(pCO_(2)),and it decreases southward across the basin.To quantify the influences of factors controlling the latitudinal gradient in CO_(2) uptake,sea surface pCO_(2) and related parameters were investigated in late spring of 2018 in a study spanning the KE,Kuroshio Recirculation(KR),and subtropical zones.We found that the sea-to-air pCO_(2) difference(ΔpCO_(2))was negative and at its lowest in the KE zone.ΔpCO_(2) gradually increased southward across the KR zone,and the sea surface was nearly in air-equilibrium with atmospheric CO_(2) in the subtropical zone.We found that northward cooling and vertical mixing were the two major processes governing the latitudinal gradient in surface pCO_(2) and ΔpCO_(2),while biological influences were relatively minor.In the KE zone affected by upwelling,the vertical-mixing-induced increase in surface pCO_(2) likely canceled out approximately 61%of the decrease in surface pCO_(2) caused by cooling and biological activities.Moreover,the prolonged air-sea equilibration for CO_(2) and relatively short hydraulic retention time jointly led to the low surface pCO_(2) in the KE zone in spring.Ultimately,the cooling KE current flows out of the region before it can be re-equilibrated with atmospheric CO_(2).展开更多
A wave rotor is suitable for compact and efficient pressure-exchange between gas flows.This work measured the circumferential pressure distribution of the rotor/stator interfaces and utilized a CFD method to simulate ...A wave rotor is suitable for compact and efficient pressure-exchange between gas flows.This work measured the circumferential pressure distribution of the rotor/stator interfaces and utilized a CFD method to simulate the unsteady pressure waves.The experimental and CFD results showed some slopes in the circumferential pressure distributions,and the slopes indicated the traces of specific unsteady pressure waves.Such traces varied regularly if the rotational speed varied within a range from-11%to+11%off the baseline value,but they were seriously disturbed if the rotational speed varied by-45%from the baseline value.It verified that a pressure wave in a wave rotor tended to keep its pressure ratio and propagation velocity unchanged if the rotational speed varied by a small extent,and that the pressure wave could not keep its propagation patterns if the rotational speed varied by a large extent.Because of the pressure wave behaviors,the wave rotor demonstrated specific regulations of the rotational speed effects on its operational states.展开更多
With the rapid development of the nuclear industry,more-stringent requirements are proposed for highlevel radioactive waste liquid treatment and the enrichment of isotope products.High-pressure ion exchange chromatogr...With the rapid development of the nuclear industry,more-stringent requirements are proposed for highlevel radioactive waste liquid treatment and the enrichment of isotope products.High-pressure ion exchange chromatography has been widely accepted for the fine separation of elements and nuclides due to its advantages,such as high efficiency,environmental friendliness,ease of operation,and feasibility for large-scale industrial applications.Here,we summarized the evolution of high-pressure ion exchange chromatography and the relevant research progress in ion exchange equilibrium and related separation technology.The prospects for application of high-pressure ion exchange chromatography to rare earth elements,actinide elements and isotope separation were discussed.High-pressure ion exchange chromatography represents a promising strategy for the extraction of rare earth elements and actinide elements from high-level radioactive waste liquid,as well as being an effective method for the automated production of high purity isotope products with great environmental benefits.展开更多
基金Supported by the National Basic Research Program of China (973 Program, No. 2005CB407305)the open foundation of the Key Laboratory of Marine Sedimentology & Environmental Geology, SOA (No. MASEG200606)+1 种基金the Qingdao Special Program for Leading Scientists (No. 05-2-JC-90)the 100-Talent Project of the Chinese Academy of Sciences
文摘Partial pressure of CO2(pCO2) was investigated in the Changjiang(Yangtze River) Estuary,Hangzhou Bay and their adjacent areas during a cruise in August 2004,China.The data show that pCO2 in surface waters of the studied area was higher than that in the atmosphere with only exception of a patch east of Zhoushan Archipelago.The pCO2 varied from 168 to 2 264 μatm,which fell in the low range compared with those of other estuaries in the world.The calculated sea-air CO2 fluxes decreased offshore and varied from -10.0 to 88.1 mmol m-2 d-1 in average of 24.4 ± 16.5 mmol m-2 d-1.Although the area studied was estimated only 2 × 104 km2,it emitted(5.9 ± 4.0) × 103 tons of carbon to the atmosphere every day.The estuaries and their plumes must be further studied for better understanding the role of coastal seas playing in the global oceanic carbon cycle.
基金The Senior User Project of R/V Kexue of the Center for Ocean Mega-Science,Chinese Academy of Sciences under contract No.KEXUE2020G07the Open Fund Project of the State Key Laboratory of Tropical Oceanography,South China Sea Institute of Oceanology,Chinese Academy of Sciences under contract No.LTO1906the Survey Project of Environmental Radioactivity Detection in the Western Pacific(R/V Xiangyanghong 3)of the Laboratory of Marine Isotopic Technology and Environmental Risk Assessment,Third Institute of Oceanography,Ministry of Natural Resource.
文摘In the northwestern North Pacific,annual net air-sea CO_(2) flux is greatest in the Kuroshio Extension(KE)zone,owing to its low annual mean partial pressure of CO_(2)(pCO_(2)),and it decreases southward across the basin.To quantify the influences of factors controlling the latitudinal gradient in CO_(2) uptake,sea surface pCO_(2) and related parameters were investigated in late spring of 2018 in a study spanning the KE,Kuroshio Recirculation(KR),and subtropical zones.We found that the sea-to-air pCO_(2) difference(ΔpCO_(2))was negative and at its lowest in the KE zone.ΔpCO_(2) gradually increased southward across the KR zone,and the sea surface was nearly in air-equilibrium with atmospheric CO_(2) in the subtropical zone.We found that northward cooling and vertical mixing were the two major processes governing the latitudinal gradient in surface pCO_(2) and ΔpCO_(2),while biological influences were relatively minor.In the KE zone affected by upwelling,the vertical-mixing-induced increase in surface pCO_(2) likely canceled out approximately 61%of the decrease in surface pCO_(2) caused by cooling and biological activities.Moreover,the prolonged air-sea equilibration for CO_(2) and relatively short hydraulic retention time jointly led to the low surface pCO_(2) in the KE zone in spring.Ultimately,the cooling KE current flows out of the region before it can be re-equilibrated with atmospheric CO_(2).
基金co-supported by the National Natural Science Foundation of China(No.51906007)the National Key Laboratory Foundation of China(No.6142702190204)。
文摘A wave rotor is suitable for compact and efficient pressure-exchange between gas flows.This work measured the circumferential pressure distribution of the rotor/stator interfaces and utilized a CFD method to simulate the unsteady pressure waves.The experimental and CFD results showed some slopes in the circumferential pressure distributions,and the slopes indicated the traces of specific unsteady pressure waves.Such traces varied regularly if the rotational speed varied within a range from-11%to+11%off the baseline value,but they were seriously disturbed if the rotational speed varied by-45%from the baseline value.It verified that a pressure wave in a wave rotor tended to keep its pressure ratio and propagation velocity unchanged if the rotational speed varied by a small extent,and that the pressure wave could not keep its propagation patterns if the rotational speed varied by a large extent.Because of the pressure wave behaviors,the wave rotor demonstrated specific regulations of the rotational speed effects on its operational states.
基金The financial supports from National Natural Science Foundation of China(Nos.22176077,U1730245)Natural Science Foundation of Gansu Province,China(No.20JR10RA615)the fundamental research funds for the central universities(No.lzujbky-2021-sp29)are acknowledged。
文摘With the rapid development of the nuclear industry,more-stringent requirements are proposed for highlevel radioactive waste liquid treatment and the enrichment of isotope products.High-pressure ion exchange chromatography has been widely accepted for the fine separation of elements and nuclides due to its advantages,such as high efficiency,environmental friendliness,ease of operation,and feasibility for large-scale industrial applications.Here,we summarized the evolution of high-pressure ion exchange chromatography and the relevant research progress in ion exchange equilibrium and related separation technology.The prospects for application of high-pressure ion exchange chromatography to rare earth elements,actinide elements and isotope separation were discussed.High-pressure ion exchange chromatography represents a promising strategy for the extraction of rare earth elements and actinide elements from high-level radioactive waste liquid,as well as being an effective method for the automated production of high purity isotope products with great environmental benefits.
