It is attractive and encouraging to develop new fluorescent carbon dots(CDs)with excellent optical properties and promising applications prospects.Herein,highly-efficient green emissive CDs(m-CDs)with a high quantum y...It is attractive and encouraging to develop new fluorescent carbon dots(CDs)with excellent optical properties and promising applications prospects.Herein,highly-efficient green emissive CDs(m-CDs)with a high quantum yield(QY)of 71.7%in water are prepared through a facile solvothermal method.Interestingly,the m-CDs exhibit excellent fluorescence stability in the pH range of 1–9.However,the fluorescence intensity of the m-CDs is almost completely quenched as the pH is increased from 9 to 10.The mechanism of the unique pH-responsive behavior is discussed in detail and a plausible mechanism is proposed.Owing to the unique pH-responsive behavior,the m-CDs are used as a on-off fluorescent probe for water quality identification.By combining the reversible pH-ultrasensitive optical properties of the m-CDs in the pH range of 9–10 with the glucose oxidase-mimicking(GOx-mimicking)ability of Au nanoparticles(AuNPs),glucose can be quantitatively detected.Finally,two environment-friendly starch-based solid-state fluorescence materials(powder and film)are developed through green preparation routes.展开更多
This paper proposes a scheme for entanglement concentration of unknown triparticle W class states with a certain probability. This protocol is mainly based on the coincidences of single-photon detectors and requires s...This paper proposes a scheme for entanglement concentration of unknown triparticle W class states with a certain probability. This protocol is mainly based on the coincidences of single-photon detectors and requires single-photon detectors and linear optical elements. The scheme is feasible within current technology.展开更多
We propose two schemes for the generation of the Wn state with three atoms separately trapped in two distant cavities coupled by an optical fibre. One is implemented by controlling the interaction time, the other is i...We propose two schemes for the generation of the Wn state with three atoms separately trapped in two distant cavities coupled by an optical fibre. One is implemented by controlling the interaction time, the other is implemented via the adiabatic passage. The influence of various decoherence processes, such as spontaneous emission of the utoma and photon leakages of the cavities and the optical fibre, on the fidelity is also investigated. It is found that the Wn state can be generated with high fidelity even when these decoherence processes are present.展开更多
基金supported by the National Natural Science Foundation of China(Nos.21375123,21675151,and 21721003)the Ministry of Science and Technology of China(No.2016YFA0203203).
文摘It is attractive and encouraging to develop new fluorescent carbon dots(CDs)with excellent optical properties and promising applications prospects.Herein,highly-efficient green emissive CDs(m-CDs)with a high quantum yield(QY)of 71.7%in water are prepared through a facile solvothermal method.Interestingly,the m-CDs exhibit excellent fluorescence stability in the pH range of 1–9.However,the fluorescence intensity of the m-CDs is almost completely quenched as the pH is increased from 9 to 10.The mechanism of the unique pH-responsive behavior is discussed in detail and a plausible mechanism is proposed.Owing to the unique pH-responsive behavior,the m-CDs are used as a on-off fluorescent probe for water quality identification.By combining the reversible pH-ultrasensitive optical properties of the m-CDs in the pH range of 9–10 with the glucose oxidase-mimicking(GOx-mimicking)ability of Au nanoparticles(AuNPs),glucose can be quantitatively detected.Finally,two environment-friendly starch-based solid-state fluorescence materials(powder and film)are developed through green preparation routes.
基金Project supported by the Natural Science Foundation of the Education Department of Anhui Province, China （Grant No 2006kj070A） and Anhui Provincial Natural Science Foundation, China （Grant No 03042401） and the Talent Foundation of Anhui University, China.
文摘This paper proposes a scheme for entanglement concentration of unknown triparticle W class states with a certain probability. This protocol is mainly based on the coincidences of single-photon detectors and requires single-photon detectors and linear optical elements. The scheme is feasible within current technology.
基金Project supported by the National Natural Science Foundation of China (Grant No. 11074072)
文摘We propose two schemes for the generation of the Wn state with three atoms separately trapped in two distant cavities coupled by an optical fibre. One is implemented by controlling the interaction time, the other is implemented via the adiabatic passage. The influence of various decoherence processes, such as spontaneous emission of the utoma and photon leakages of the cavities and the optical fibre, on the fidelity is also investigated. It is found that the Wn state can be generated with high fidelity even when these decoherence processes are present.
