钍基熔盐堆(TMSR)核能系统项目是中科院未来10年先导研究专项之一,其研究目标是研发第四代裂变反应堆核能系统,计划至2020年之前建成2MW钍基熔盐实验堆,形成支撑未来TMSR核能系统发展的若干技术研发能力,并解决钍铀燃料循环和钍基熔盐...钍基熔盐堆(TMSR)核能系统项目是中科院未来10年先导研究专项之一,其研究目标是研发第四代裂变反应堆核能系统,计划至2020年之前建成2MW钍基熔盐实验堆,形成支撑未来TMSR核能系统发展的若干技术研发能力,并解决钍铀燃料循环和钍基熔盐堆相关重大技术挑战,研制出工业示范级钍基熔盐堆,实现钍资源的有效使用和核能的综合利用。钍基核燃料具有232Th/233U转换效率高、在热中子堆中也能增殖、产生较少的高毒性放射性核素、有利于防核扩散等优点,但也面临燃料制备困难、232U衰变子核的强γ辐射给乏燃料处理和燃料再加工带来的困难、钍铀转换反应链中间核233Pa会吸收堆内中子从而影响233U产量。核燃料利用的工作模式有开环模式、改进的开环模式和闭环模式。熔盐堆是第四代反应堆的6个候选堆型之一,非常适合用作钍铀燃料循环,熔盐堆加上干法在线分离技术有可能实现完全的钍铀燃料闭式循环。本世纪初提出的氟盐冷却高温堆(Fluoride salt-cooled High temperature Reactors,FHRs),用氟化熔盐作为冷却剂,采用TRISO燃料颗粒作为核燃料,其中球床型氟盐冷却高温堆可以在改进的开环模式实现钍铀燃料循环。熔盐堆良好的高温特性使其成为核能非电应用主要候选者之一,反应堆产生的高温热可直接用于页岩油开采和高温制氢等工业领域。展开更多
Heavy water-moderated molten salt reactors(HWMSRs)are novel molten salt reactors that adopt heavy water rather than graphite as the moderator while employing liquid fuel.Owing to the high moderating ratio of the heavy...Heavy water-moderated molten salt reactors(HWMSRs)are novel molten salt reactors that adopt heavy water rather than graphite as the moderator while employing liquid fuel.Owing to the high moderating ratio of the heavy water moderator and the utilization of liquid fuel,HWMSRs can achieve a high neutron economy.In this study,a large-scale small modular HWMSR with a thermal power of 500 MWth was proposed and studied.The criticality of the core was evaluated using an in-house critical search calculation code(CSCC),which was developed based on Standardized Computer Analyses for Licensing Evaluation,version 6.1.The preliminary fuel cycle performances(initial conversion ratio(CR),initialfissile fuel loading mass,and temperature coefficient)were investigated by varying the lattice pitch(P)and the molten salt volume fraction(VF).The results demonstrate that the temperature coefficient can be negative over the range of investigated Ps and VFs for both 233U-Th and LEU-Th fuels.A core with a P of 20 cm and a VF of 20%is recommended for 233U-Th and LEU-Th fuels to achieve a high performance of initial CR and fuel loading.Regarding TRU-Th fuel,a core with a smaller P(~5 cm)and larger VF(~24%)is recommended to obtain a negative temperature coefficient.展开更多
反应堆物理设计不确定度是第4代核能系统的QMU(quantification of margins and uncertainties)有效性认证所必须的参数之一,核数据不确定度是其重要来源。基于自主开发的耦合程序BUND(burnup uncertainty of nuclear data),将SCALE程序T...反应堆物理设计不确定度是第4代核能系统的QMU(quantification of margins and uncertainties)有效性认证所必须的参数之一,核数据不确定度是其重要来源。基于自主开发的耦合程序BUND(burnup uncertainty of nuclear data),将SCALE程序TRITON和TSUNAMI-3D模块耦合,完成了熔盐堆钍铀燃料循环、铀钚燃料循环核数据引起的有效增殖因数keff不确定度分析,并与ENDF/B-Ⅶ.1协方差数据库计算结果进行了对比。结果显示:初始时刻,两种燃料循环模式下,核数据导致的keff不确定度分别为0.490%和0.582%。随燃耗的增加,核数据引起的keff不确定度增加。寿期末,两种燃料循环模式下,对keff不确定度影响显著增加的反应道分别为239Pu(nubar)、(n,f)、(n,γ)、105 Rh(n,γ)、135 Xe(n,γ)和234 U(n,γ)、143 Nd(n,γ)、131,135 Xe(n,γ)等。展开更多
By using computer code WIMS/CENDL, the effects of some parameters, core configuration such as fuel element structure, neutron flux and burn-up, are discussed in this paper. It is shown that high neutron flux, small fu...By using computer code WIMS/CENDL, the effects of some parameters, core configuration such as fuel element structure, neutron flux and burn-up, are discussed in this paper. It is shown that high neutron flux, small fuel rod diameter, large volume ratio of coolant to fuel, seed-blank heterogeneous core arrangement and 231 Pa chemical separation are necessary for reducing 228Th production in reactor.展开更多
文摘钍基熔盐堆(TMSR)核能系统项目是中科院未来10年先导研究专项之一,其研究目标是研发第四代裂变反应堆核能系统,计划至2020年之前建成2MW钍基熔盐实验堆,形成支撑未来TMSR核能系统发展的若干技术研发能力,并解决钍铀燃料循环和钍基熔盐堆相关重大技术挑战,研制出工业示范级钍基熔盐堆,实现钍资源的有效使用和核能的综合利用。钍基核燃料具有232Th/233U转换效率高、在热中子堆中也能增殖、产生较少的高毒性放射性核素、有利于防核扩散等优点,但也面临燃料制备困难、232U衰变子核的强γ辐射给乏燃料处理和燃料再加工带来的困难、钍铀转换反应链中间核233Pa会吸收堆内中子从而影响233U产量。核燃料利用的工作模式有开环模式、改进的开环模式和闭环模式。熔盐堆是第四代反应堆的6个候选堆型之一,非常适合用作钍铀燃料循环,熔盐堆加上干法在线分离技术有可能实现完全的钍铀燃料闭式循环。本世纪初提出的氟盐冷却高温堆(Fluoride salt-cooled High temperature Reactors,FHRs),用氟化熔盐作为冷却剂,采用TRISO燃料颗粒作为核燃料,其中球床型氟盐冷却高温堆可以在改进的开环模式实现钍铀燃料循环。熔盐堆良好的高温特性使其成为核能非电应用主要候选者之一,反应堆产生的高温热可直接用于页岩油开采和高温制氢等工业领域。
基金supported by the Chinese TMSR Strategic Pioneer Science and Technology Project(No.XDA02010000)the National Natural Science Foundation of China(No.11905285)+1 种基金the National Natural Science Foundation of China(No.11790321)the Frontier Science Key Program of the Chinese Academy of Sciences(No.QYZDY-SSW-JSC016)。
文摘Heavy water-moderated molten salt reactors(HWMSRs)are novel molten salt reactors that adopt heavy water rather than graphite as the moderator while employing liquid fuel.Owing to the high moderating ratio of the heavy water moderator and the utilization of liquid fuel,HWMSRs can achieve a high neutron economy.In this study,a large-scale small modular HWMSR with a thermal power of 500 MWth was proposed and studied.The criticality of the core was evaluated using an in-house critical search calculation code(CSCC),which was developed based on Standardized Computer Analyses for Licensing Evaluation,version 6.1.The preliminary fuel cycle performances(initial conversion ratio(CR),initialfissile fuel loading mass,and temperature coefficient)were investigated by varying the lattice pitch(P)and the molten salt volume fraction(VF).The results demonstrate that the temperature coefficient can be negative over the range of investigated Ps and VFs for both 233U-Th and LEU-Th fuels.A core with a P of 20 cm and a VF of 20%is recommended for 233U-Th and LEU-Th fuels to achieve a high performance of initial CR and fuel loading.Regarding TRU-Th fuel,a core with a smaller P(~5 cm)and larger VF(~24%)is recommended to obtain a negative temperature coefficient.
文摘反应堆物理设计不确定度是第4代核能系统的QMU(quantification of margins and uncertainties)有效性认证所必须的参数之一,核数据不确定度是其重要来源。基于自主开发的耦合程序BUND(burnup uncertainty of nuclear data),将SCALE程序TRITON和TSUNAMI-3D模块耦合,完成了熔盐堆钍铀燃料循环、铀钚燃料循环核数据引起的有效增殖因数keff不确定度分析,并与ENDF/B-Ⅶ.1协方差数据库计算结果进行了对比。结果显示:初始时刻,两种燃料循环模式下,核数据导致的keff不确定度分别为0.490%和0.582%。随燃耗的增加,核数据引起的keff不确定度增加。寿期末,两种燃料循环模式下,对keff不确定度影响显著增加的反应道分别为239Pu(nubar)、(n,f)、(n,γ)、105 Rh(n,γ)、135 Xe(n,γ)和234 U(n,γ)、143 Nd(n,γ)、131,135 Xe(n,γ)等。
文摘By using computer code WIMS/CENDL, the effects of some parameters, core configuration such as fuel element structure, neutron flux and burn-up, are discussed in this paper. It is shown that high neutron flux, small fuel rod diameter, large volume ratio of coolant to fuel, seed-blank heterogeneous core arrangement and 231 Pa chemical separation are necessary for reducing 228Th production in reactor.
