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Reactions between graphene oxide sheets cause irreversible agglomeration 被引量:2

自反应决定石墨烯团聚的不可逆
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摘要 Graphene has received increased attention recently owing to its wide range of significant applications.Graphene is comprised of planar sheets of carbon atoms arranged in six-membered ring networks(Fig.1a).An atomically thin sheet of this substance can be regarded as molecular entity,in which nanometer-scale corrugations and defects create different physical and chemical environments.Knowledge about how these sheets interact with solvent molecules and how the defects govern these interactions is a critical component of understanding and predicting the liquid-phase chemistry of graphene.Contact angle measurements have been typically utilized to gain macroscopic information about interfacial interactions occurring between water and graphene.Owing to its one carbon atom thickness,the top single-layer of graphene is wetting transparent to the underlying substrates[1,2].The surface hydrophobicity of graphene can be induced by adsorption of airborne pollutants(e.g.,hydrocarbons)[3].In addition,graphenebased interfacial materials having either superhydrophobicity or superhydrophilicity have been developed.
作者 Ying Dong Jing Li Xiao-Yu Yang 董莹;李静;阳晓宇(Department of Forensic Medicine,Huazhong University of Science and Technology,Wuhan 430030,China;Hubei Province Key Laboratory of Coal Conversion and New Carbon Materials,School of Chemistry and Chemical Engineering,Wuhan University of Science and Technology,Wuhan 430081,China;State Key Laboratory of Advanced Technology for Materials Synthesis and Processing&Shenzhen Research Institute&Joint Laboratory for Marine Advanced Materials in National Laboratory for Marine Science and Technology(Qingdao),Wuhan University of Technology,Wuhan 430070,China;School of Engineering and Applied Sciences,Harvard University,Cambridge,MA 02138,USA)
出处 《Science Bulletin》 SCIE EI CAS CSCD 2022年第19期1943-1945,共3页 科学通报(英文版)
基金 supported by the National Natural Science Foundation of China(51861135313) the National 111 Project(B20002) the Program for Changjiang Scholars and Innovative Research Team in University(IRT_15R52) the Sino-German Centre’s COVID-19 Related Bilateral Collaborative Project(C-0046) the Guangdong Province International Scientific and Technological Cooperation Projects(2020A0505100036) the Guangdong Basic and Applied Basic Research Foundation(2022A1515010137) the Shenzhen Science and Technology Program(JCYJ20210324142010029 and GJHZ20210705143204014)。
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