摘要
Graphene has received increased attention recently owing to its wide range of significant applications.Graphene is comprised of planar sheets of carbon atoms arranged in six-membered ring networks(Fig.1a).An atomically thin sheet of this substance can be regarded as molecular entity,in which nanometer-scale corrugations and defects create different physical and chemical environments.Knowledge about how these sheets interact with solvent molecules and how the defects govern these interactions is a critical component of understanding and predicting the liquid-phase chemistry of graphene.Contact angle measurements have been typically utilized to gain macroscopic information about interfacial interactions occurring between water and graphene.Owing to its one carbon atom thickness,the top single-layer of graphene is wetting transparent to the underlying substrates[1,2].The surface hydrophobicity of graphene can be induced by adsorption of airborne pollutants(e.g.,hydrocarbons)[3].In addition,graphenebased interfacial materials having either superhydrophobicity or superhydrophilicity have been developed.
作者
Ying Dong
Jing Li
Xiao-Yu Yang
董莹;李静;阳晓宇(Department of Forensic Medicine,Huazhong University of Science and Technology,Wuhan 430030,China;Hubei Province Key Laboratory of Coal Conversion and New Carbon Materials,School of Chemistry and Chemical Engineering,Wuhan University of Science and Technology,Wuhan 430081,China;State Key Laboratory of Advanced Technology for Materials Synthesis and Processing&Shenzhen Research Institute&Joint Laboratory for Marine Advanced Materials in National Laboratory for Marine Science and Technology(Qingdao),Wuhan University of Technology,Wuhan 430070,China;School of Engineering and Applied Sciences,Harvard University,Cambridge,MA 02138,USA)
基金
supported by the National Natural Science Foundation of China(51861135313)
the National 111 Project(B20002)
the Program for Changjiang Scholars and Innovative Research Team in University(IRT_15R52)
the Sino-German Centre’s COVID-19 Related Bilateral Collaborative Project(C-0046)
the Guangdong Province International Scientific and Technological Cooperation Projects(2020A0505100036)
the Guangdong Basic and Applied Basic Research Foundation(2022A1515010137)
the Shenzhen Science and Technology Program(JCYJ20210324142010029 and GJHZ20210705143204014)。