摘要
铁基超导体呈现丰富的电子相图,各种有序态相互交叠.本文主要介绍利用核磁共振手段在空穴型和电子型掺杂的BaFe2As2以及LaFeAsO1-xFx这三种具有代表性的铁基超导体中探测到的反铁磁序与超导序的微观共存、量子临界点和量子临界行为.实验发现,无论在空穴型还是电子型掺杂的铁基超导体中,反铁磁相变温度都随着掺杂被抑制,并最终在某个掺杂量降到零温而形成量子临界点.在反铁磁转变温度之上存在结构相变,其转变温度也随着掺杂而降低.核磁共振谱证实结构相变也形成一个量子临界点.本文介绍核磁共振及输运测量揭示的这两种量子临界点附近存在的量子临界行为,共存态下奇异的超导性质等.
In the past several decades, quantum phase transition and the associated fluctuations have emerged as a major challenge to our understanding of condensed matter. Such transition is tuned by an external parameter such as pressure,chemical doping or magnetic field. The transition point, called quantum critical point（QCP）, is only present at absolute zero temperature（T）, but its influence（quantum criticality） is spread to nonzero temperature region. Quite often,new stable orders of matter, such as superconductivity, emerge around the QCP, whose relationship to the quantum fluctuations is one of the most important issues.Iron-pnictide superconductors are the second class of high-temperature-superconductor family whose phase diagram is very similar to the first class, the copper-oxides. Superconductivity emerges in the vicinity of exotic orders, such as antiferromagnetic, structural or nematic order. Therefore, iron-pnictides provide us a very good opportunity to study quantum criticality. Here we review nuclear magnetic resonance（NMR） study on the coexistence of states and quantum critical phenomena in both hole-doped system Ba1-xKxFe2As2 as well as electron-doped systems BaFe2-xNixAs2 and La Fe As O1-xFx. Firstly, we found that the 75 As NMR spectra split or are broadened for H//c-axis, and shift to a higher frequency for H//ab-plane below a certain temperature in the underdoped region of both hole-doped Ba1-xKxFe2As2 and electron-doped BaFe2-xNixAs2, which indicate that an internal magnetic field develops along the c-axis due to an antiferromagnetic order. Upon further cooling, the spin-lattice relaxation rate 1/T1 measured at the shifted peak shows a distinct decrease below the superconducting critical temperature Tc. These results show unambiguously that the antiferromagnetic order and superconductivity coexist microscopically, which is the essential condition for a magnetic QCP. Moreover, the much weaker T-dependence of 1/T1 in the superconducting state compared with the optimal doping sample sug
出处
《物理学报》
SCIE
EI
CAS
CSCD
北大核心
2015年第21期82-95,共14页
Acta Physica Sinica
基金
中科院先导B项目(批准号:XDB07020200)
国家重点基础研究发展计划(批准号:2012CB821402
2015CB921304)
国家自然科学基金(批准号:11104336)资助的课题~~
关键词
核磁共振
铁基超导体
自旋涨落
量子临界性
nuclear magnetic resonance
iron-based superconductor
spin fluctuations
quantum critical phenomena
