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Effect of Au film pre-deposited at different durations as inner electrode on the electrical properties and interface microstructures of Na_2O-PbO-Nb_2O_5-SiO_2 multi-layer glass-ceramic capacitors

Effect of Au film pre-deposited at different durations as inner electrode on the electrical properties and interface microstructures of Na_2O-PbO-Nb_2O_5-SiO_2 multi-layer glass-ceramic capacitors
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摘要 To further study the effect of sputtered Au film as transition electrode layer on the electrical properties and interface microstructures of Na20-PbO-Nb2O5-SiO2 multilayer glass-ceramic capacitors, Au films pre-deposited at different time were prepared by DC magnetron sputtering. Compared with the single paste electrode structure, samples with Au films pre-deposited from 6 to 18 min have the consistent perfor- mance to effectively improve the electrical properties of the capacitors, resulting in the doubled breakdown strength, an increase of equivalent capacitance by 22% and a decrease of leakage current by an order of magnitude. SEM observations indicate that the Au films with deposition time from 6 to 18 min would all help the formation of a dense electrode/dielectric interface and inhibit the diffusion of Ag. The results reveal that Au film pre-deposited for 6 min as inner electrode was sufficient to improve the interface microstructure and therefore to inhibit the Ag diffusion and enhance the overall performance of the multi-layer glass-ceramic capacitors. To further study the effect of sputtered Au film as transition electrode layer on the electrical properties and interface microstructures of Na20-PbO-Nb2O5-SiO2 multilayer glass-ceramic capacitors, Au films pre-deposited at different time were prepared by DC magnetron sputtering. Compared with the single paste electrode structure, samples with Au films pre-deposited from 6 to 18 min have the consistent perfor- mance to effectively improve the electrical properties of the capacitors, resulting in the doubled breakdown strength, an increase of equivalent capacitance by 22% and a decrease of leakage current by an order of magnitude. SEM observations indicate that the Au films with deposition time from 6 to 18 min would all help the formation of a dense electrode/dielectric interface and inhibit the diffusion of Ag. The results reveal that Au film pre-deposited for 6 min as inner electrode was sufficient to improve the interface microstructure and therefore to inhibit the Ag diffusion and enhance the overall performance of the multi-layer glass-ceramic capacitors.
出处 《Acta Metallurgica Sinica(English Letters)》 SCIE EI CAS CSCD 2011年第6期449-456,共8页 金属学报(英文版)
基金 financially supported by the National High Technical Research and Development Programme of China (No.2008AA03A236)
关键词 Inner electrode Deposition time GLASS-CERAMIC Multi-layer capacitor Inner electrode Deposition time Glass-ceramic Multi-layer capacitor
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  • 1A. C Caballero,E Nieto,P Duran,C Moure,M Kosec,Z Samardzija,G Drazic. Ceramic–electrode interaction in PZT and PNN–PZT multilayer piezoelectric ceramics with AG/PD 70/30 inner electrode[J] 1997,Journal of Materials Science(12):3257~3262 被引量:1

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