摘要
The authors investigated size-dependent amplified spontaneous emission（ASE） from organic crystals. Specifically, N-（4-{4-[4-（diphenylamino）styryl]styryl}phenyl）-N-phenylbenzene amine（Ph-TPA2） organic crystals were used in the experiment. The ASE threshold was decreased with the decrease of the width of the crystal at the same gain length, which reflects that total internal reflection plays an important role on the ASE properties in these slab organic crystals. The ASE properties pumped by one- and two-photon were also comparatively studied. We found that the thresholds of ASE in two-photon pumping condition are less size-dependent than those in singlephoton condition because of the nonlinear light generation processes in two-photon absorption processes.
The authors investigated size-dependent amplified spontaneous emission（ASE） from organic crystals. Specifically, N-（4-{4-[4-（diphenylamino）styryl]styryl}phenyl）-N-phenylbenzene amine（Ph-TPA2） organic crystals were used in the experiment. The ASE threshold was decreased with the decrease of the width of the crystal at the same gain length, which reflects that total internal reflection plays an important role on the ASE properties in these slab organic crystals. The ASE properties pumped by one- and two-photon were also comparatively studied. We found that the thresholds of ASE in two-photon pumping condition are less size-dependent than those in singlephoton condition because of the nonlinear light generation processes in two-photon absorption processes.
基金
Supported by the National High-Tech Research and Development Program of China(No.2009AA03Z401)
the National Natural Science Foundation of China(Nos.61077002, 60807030)
the Project of National Lab for Tsinghua Information Tech-nologies, China
