摘要
采集了太湖地区污染与非污染稻田表土,采用原状土低能量分离-分散技术提取土壤团聚体粒组,分析土壤中不同粒径团聚体颗粒组质量组成和Pb、Cd、Hg、As等重金属元素的含量,讨论重金属污染下土壤团聚体组成和重金属团聚体分配的变化.结果表明：在重金属污染下,供试水稻土砂粒级团聚体减少,而较细粒径团聚体相对增多;4种重金属元素在不同粒径团聚体颗粒组中的含量存在差异,但随粒径的变化趋势基本一致,即在＆lt;0.002 mm粒径的颗粒组中最高,其次是0.2~2 mm粒径的颗粒组,而在0.02~0.2 mm和0.002~0.02 mm粒径的团聚体中呈现亏缺现象（富集系数为0.56~0.96）.表明重金属污染可能减弱了较大土壤团聚体的形成,导致细粒径团聚体相对增多,从而明显提高了重金属元素在粉砂和粘粒组团聚体中的分配,这可能进一步提高了污染农田重金属的水迁移和大气颗粒物迁移的风险.对于重金属污染对稻田土壤生物物理和生物化学过程的影响及其机制还需要进一步研究.
Topsoil samples were collected from a polluted and an adjacent non-polluted paddy field in the Taihu Lake region of China. Different particle size fractions of soil aggregates were separated by low-energy dispersion procedure, and their mass composition and Pb, Cd, Hg, and As concentrations were determined. Under heavy metals pollution, the mass composition of sand-sized frac- tions reduced, while that of clay-sized fractions increased. The concentrations of test metals in different particle size fractions differed, with the highest in 〈 0. 002 mm fraction, followed by in 2-0. 2 mm fraction. In 0. 02-0. 002 mm and 0. 2-0. 02 mm fractions, all the test metals were relatively deficient, with an enrichment index of 0. 56-0. 96. The present study showed that the aggregation of fine particles could be depressed by heavy metals pollution, which in turn, led to a relative increase in the mass composition of fine particles and the associated allocation of heavy metals in weakly aggregated silt particles, and further, increased the risks of heavy metals translocation from polluted farmland into water and atmosphere. Further studies should be made on the impacts of heavy metals pollution on soil biophysical and biochemical processes and related mechanisms.
出处
《应用生态学报》
CAS
CSCD
北大核心
2009年第11期2806-2812,共7页
Chinese Journal of Applied Ecology
基金
国家自然科学基金项目(40671180)
科技部科技支撑计划项目(2006BAD17B06)资助.
关键词
土壤污染
水稻土
重金属
微团聚体
颗粒组
迁移风险
soil pollution
paddy soil
heavy metal
micro-aggregate
particle size fraction
translocation risk.
