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An in-situ analysis and measurement of thorium-234,uranium isotopes in seawater 被引量:5

An in-situ analysis and measurement of thorium-234,uranium isotopes in seawater
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摘要 A low-level β counting-or spectrum apparatus used for the detection of the β radiation of thorium-234 and α spectrum of thorium- 228 simultaneously and an easy operating procedure for the enrichment, radiochemical separating, sampling and measurement of thorium-234 and uranium-238 in the ocean are developed based on the requirements of analyzing export productivity in the eupho- ric zone via thorium-234 - uranium-238 radioactivity disequilibrium. The detecting efficiency both of 13 and α radiation is higher than 20%. The background of βradiation is less than 0. 5 min ^-1 , and the energy resolution of ct detector is better than 1%. Total recycle ratio of thorium-234 is about 75%. Using the above apparatus and procedure, the radioactivities of dissolved thorium-234 and uranium-238, particle thorium-234 and uranium-238 in seawater of the South China Sea, the Southern Ocean and the Arctic Ocean were analyzed. A low-level β counting-or spectrum apparatus used for the detection of the β radiation of thorium-234 and α spectrum of thorium- 228 simultaneously and an easy operating procedure for the enrichment, radiochemical separating, sampling and measurement of thorium-234 and uranium-238 in the ocean are developed based on the requirements of analyzing export productivity in the eupho- ric zone via thorium-234 - uranium-238 radioactivity disequilibrium. The detecting efficiency both of 13 and α radiation is higher than 20%. The background of βradiation is less than 0. 5 min ^-1 , and the energy resolution of ct detector is better than 1%. Total recycle ratio of thorium-234 is about 75%. Using the above apparatus and procedure, the radioactivities of dissolved thorium-234 and uranium-238, particle thorium-234 and uranium-238 in seawater of the South China Sea, the Southern Ocean and the Arctic Ocean were analyzed.
出处 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2007年第3期73-83,共11页 海洋学报(英文版)
基金 This project was supported by the State Social Commonweal Grant(project name:the comprehensive investigation of Nansha Islands waters) the Natural Science Foundation of Fujian Province of China under contract No.2006J0287 This study was also supported,in part,by the National Natural Science Foundation of China from key program under contract No.40531007 general program under contract Nos 40406014 and 40276001 State Social Commonweal Grant under contract No.2004DIB5178.
关键词 OCEAN β counting-or spectrum apparatus radiochemical separating thorium-234 uranium-238 ocean, β counting-or spectrum apparatus, radiochemical separating, thorium-234, uranium-238
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  • 1S. M. Pike,K. O. Buesseler,J. Andrews,N. Savoye.Quantification of 234Th recovery in small volume sea water samples by inductively coupled plasma-mass spectrometry[J].Journal of Radioanalytical and Nuclear Chemistry.2005(2) 被引量:1
  • 2C. R. Benitez-Nelson,K. O. Buesseler,M. Rutgers van der Loeff,J. Andrews,L. Ball,G. Crossin,M. A. Charette.Testing a new small-volume technique for determining 234Th in seawater[J].Journal of Radioanalytical and Nuclear Chemistry.2001(3) 被引量:1

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