摘要
利用从紫细菌Rb.sphaeroides601所提取出的外周捕光天线LH2以及其不同pH值酸化样品(部分和全部去除B800分子LH2)并采用不同波长下的飞秒单色抽运探测技术详细研究了LH2中B800吸收带内的激发态动力学过程。通过对野生型与部分/完全去B800分子LH2的比较研究,分析了B800吸收带激发后所表现出的丰富变化的动力学过程,研究结果表明激发B800带的动力学过程中包含着B850上激子带的直接激发而产生的对激发态动力学的贡献。
Photodynamics of two kinds of peripheral antenna complexes light harvesting 2 （LH2） of Rb. Sphaeroides 601, namely the native LH2 and B800-released LH2, where B800-BChls were partially or completely removed with different pH treatments, were studied using femtosecond pump-probe technique at different laser wavelengths. The obtained results for these samples demonstrate that under the excitation around B800 absorption band, the photoabsorption and photobleaching dynamics are caused by the direct excitation of upper excitonic levels of B850 and excited state of B800 pigments, respectively.
出处
《物理学报》
SCIE
EI
CAS
CSCD
北大核心
2006年第9期4472-4477,共6页
Acta Physica Sinica
基金
国家自然科学基金(批准号:10274013)资助的课题.~~
关键词
紫细菌外周捕光天线LH2
部分和全部去除B800分子LH2
激发态动力学的演变
飞秒抽运探测
peripheral light harvesting complexes （LH2） from Rb. Sphaeroides 601, BS00 partially or completely released LH2, excited-state dynamical evolution, femtosecond pump-probe
