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Helicity dependent directional surface plasmon polariton excitation using a metasurface with interfacial phase discontinuity 被引量:35
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作者 Lingling Huang Xianzhong Chen +4 位作者 Benfeng Bai Qiaofeng Tan Guofan Jin Thomas Zentgraf Shuang Zhang 《Light(Science & Applications)》 SCIE EI CAS 2013年第1期197-203,共7页
Surface plasmon polaritons(SPPs)have been widely exploited in various scientific communities,ranging from physics,chemistry to biology,due to the strong confinement of light to the metal surface.For many applications,... Surface plasmon polaritons(SPPs)have been widely exploited in various scientific communities,ranging from physics,chemistry to biology,due to the strong confinement of light to the metal surface.For many applications,it is important that the free space photon can be coupled to SPPs in a controllable manner.In this Letter,we apply the concept of interfacial phase discontinuity for circularly polarizations on a metasurface to the design of a novel type of polarization-dependent SPP unidirectional excitation at normal incidence.Selective unidirectional excitation of SPPs along opposite directions is experimentally demonstrated at optical frequencies by simply switching the helicity of the incident light.This approach,in conjunction with dynamic polarization modulation techniques,opens gateway towards integrated plasmonic circuits with electrically reconfigurable functionalities. 展开更多
关键词 METAMATERIALS metasurface surface plasmon
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科学家合作网络的聚类分析 被引量:14
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作者 张鹏 李梦辉 +2 位作者 吴金闪 狄增如 樊瑛 《复杂系统与复杂性科学》 EI CSCD 2005年第2期30-34,共5页
在自建的经济物理学科学家合作网络的基础上,实现了层次聚类法和介数聚类法,并将他们应用到对经济物理学科学家合作网络结构的聚类分析中,在理论层次对两种方法进行了比较,同时将两种算法的计算结果与现实进行对照,发现介数聚类的结果... 在自建的经济物理学科学家合作网络的基础上,实现了层次聚类法和介数聚类法,并将他们应用到对经济物理学科学家合作网络结构的聚类分析中,在理论层次对两种方法进行了比较,同时将两种算法的计算结果与现实进行对照,发现介数聚类的结果与现实吻合得较好。在充分理解Newm an提出的Q函数的基础上,讨论了聚类过程中的最佳集团数。 展开更多
关键词 复杂网络 集团结构 聚类 经济物理
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Malus-metasurface-assisted polarization multiplexing 被引量:12
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作者 Liangui Deng Juan Deng +12 位作者 Zhiqiang Guan Jin Tao Yang Chen Yan Yang Daxiao Zhang Jibo Tang Zhongyang Li Zile Li Shaohua Yu Guoxing Zheng Hongxing Xu Cheng-Wei Qiu Shuang Zhang 《Light(Science & Applications)》 SCIE EI CAS CSCD 2020年第1期1038-1046,共9页
Polarization optics plays a pivotal role in diffractive,refractive,and emerging flat optics,and has been widely employed in contemporary optical industries and daily life.Advanced polarization manipulation leads to ro... Polarization optics plays a pivotal role in diffractive,refractive,and emerging flat optics,and has been widely employed in contemporary optical industries and daily life.Advanced polarization manipulation leads to robust control of the polarization direction of light.Nevertheless,polarization control has been studied largely independent of the phase or intensity of light.Here,we propose and experimentally validate a Malus-metasurface-assisted paradigm to enable simultaneous and independent control of the intensity and phase properties of light simply by polarization modulation.The orientation degeneracy of the classical Malus’s law implies a new degree of freedom and enables us to establish a one-to-many mapping strategy for designing anisotropic plasmonic nanostructures to engineer the Pancharatnam–Berry phase profile,while keeping the continuous intensity modulation unchanged.The proposed Malus metadevice can thus generate a near-field greyscale pattern,and project an independent far-field holographic image using an ultrathin and single-sized metasurface.This concept opens up distinct dimensions for conventional polarization optics,which allows one to merge the functionality of phase manipulation into an amplitudemanipulation-assisted optical component to form a multifunctional nano-optical device without increasing the complexity of the nanostructures.It can empower advanced applications in information multiplexing and encryption,anti-counterfeiting,dual-channel display for virtual/augmented reality,and many other related fields. 展开更多
关键词 OPTICS enable unchanged
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Optical observations of LIGO source GW 170817 by the Antarctic Survey Telescopes at Dome A,Antarctica 被引量:8
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作者 lei hu xuefeng wu +30 位作者 igor andreoni michael c.b.ashley jeff cooke xiangqun cui fujia du zigao dai bozhong gu yi hu haiping lu xiaoyan li zhengyang li ensi liang liangduan liu bin ma zhaohui shang tianrui sun n.b.suntzeff charling tao syed a.uddin lifan wang xiaofeng wang haikun wen di xiao jin xu ji yang shihai yang xiangyan yuan hongyan zhou hui zhang jilin zhou zonghong zhu 《Science Bulletin》 SCIE EI CAS CSCD 2017年第21期1433-1438,共6页
The LIGO detection of gravitational waves(GW) from merging black holes in 2015 marked the beginning of a new era in observational astronomy. The detection of an electromagnetic signal from a GW source is the critical ... The LIGO detection of gravitational waves(GW) from merging black holes in 2015 marked the beginning of a new era in observational astronomy. The detection of an electromagnetic signal from a GW source is the critical next step to explore in detail the physics involved. The Antarctic Survey Telescopes(AST3),located at Dome A, Antarctica, is uniquely situated for rapid response time-domain astronomy with its continuous night-time coverage during the austral winter. We report optical observations of the GW source(GW 170817) in the nearby galaxy NGC 4993 using AST3. The data show a rapidly fading transient at around 1 day after the GW trigger, with the i-band magnitude declining from 17:23 ± 0:13 magnitude to 17:72 ± 0:09 magnitude in ~1:8 h. The brightness and time evolution of the optical transient associated with GW 170817 are broadly consistent with the predictions of models involving merging binary neutron stars. We infer from our data that the merging process ejected about ~10^(-2) solar mass of radioactive material at a speed of up to 30% the speed of light. 展开更多
关键词 Gravitational waves Binary neutron stars Gamma-ray bursts
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The ALMaQUEST Survey ⅩⅤ:The dependence of the molecular-to-atomic gas ratios on resolved optical diagnostics
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作者 Niankun Yu Zheng Zheng +14 位作者 Chao-Wei Tsai Pei Zuo Sara L.Ellison David V.Stark Di Li Jingwen Wu Karen L.Masters Ting Xiao Yinghui Zheng Zongnan Li Kai Zhang Hongying Chen Shu Liu Sihan Jiao Fanyi Meng 《Science China(Physics,Mechanics & Astronomy)》 SCIE EI CAS CSCD 2024年第9期174-196,共23页
The atomic-to-molecular gas conversion is a critical step in the baryon cycle of galaxies,which sets the initial conditions for subsequent star formation and influences the multi-phase interstellar medium.We compiled ... The atomic-to-molecular gas conversion is a critical step in the baryon cycle of galaxies,which sets the initial conditions for subsequent star formation and influences the multi-phase interstellar medium.We compiled a sample of 94 nearby galaxies with observations of multi-phase gas contents by utilizing public H_(Ⅰ),CO,and optical IFU data from the Ma NGA survey together with new FAST H_(Ⅰ)observations.In agreement with previous results,our sample shows that the global molecular-to-atomic gas ratio(R_(mol)≡log M_(H2)/M_(H_(Ⅰ)))is correlated with the global stellar mass surface densityμ_*with a Kendall'sτcoefficient of 0.25 and p<10^(-3),less tightly but still correlated with stellar mass and NUV-r color,and not related to the specific star formation rate(sSFR).The cold gas distribution and kinematics inferred from the H_(Ⅰ)and CO global profile asymmetry and shape do not significantly rely on R_(mol).Thanks to the availability of kpc-scale observations of MaNGA,we decompose galaxies into H_(Ⅱ),composite,and AGN-dominated regions by using the BPT diagrams.With increasing R_(mol),the fraction of H_(Ⅱ)regions within 1.5 effective radius decreases slightly;the density distribution in the spatially resolved BPT diagram also changes significantly,suggesting changes in metallicity and ionization states.Galaxies with high R_(mol)tend to have high oxygen abundance,both at one effective radius with a Kendall'sτcoefficient of 0.37(p<10^(-3))and their central regions.Among all parameters investigated here,the oxygen abundance at one effective radius has the strongest relation with global R_(mol).The dependence of gas conversion on gas distribution and galaxy ionization states is weak.In contrast,the observed positive relation between oxygen abundance(μ_(*))and R_(mol)indicates that the gas conversion is efficient in regions of high metallicity(density). 展开更多
关键词 GALAXIES baryon cycle radio lines H_(Ⅰ)21 cm atomic-to-molecular gas conversion
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The CCD instrument background of the SMILE SXI 被引量:2
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作者 M.W.J.Hubbard O.Hetherington +6 位作者 D.J.Hall T.W.Buggey S.Parsons T.Arnold A.Holland C.Pagani S.Sembay 《Earth and Planetary Physics》 EI CSCD 2024年第1期15-24,共10页
The ESA and CAS SMILE mission orbit is highly elliptical and will pass through multiple radiation environments.The Soft X-ray Imager(SXI)instrument aboard has a radiation shutter door designed to close when the surrou... The ESA and CAS SMILE mission orbit is highly elliptical and will pass through multiple radiation environments.The Soft X-ray Imager(SXI)instrument aboard has a radiation shutter door designed to close when the surrounding radiation flux is high.The shutter door will close when passing below an altitude threshold to protect against trapped particles in the Earth’s Van Allen Belts.Therefore,two radiation environments can be approximated based on the shutter door position:open and closed.The instrument background for the CCDs(Charge-Coupled Devices)that form the focal plane array of the SXI were evaluated for the two environments.Due to the correlation of the space environment with the solar cycle,the solar minima and maxima,the background was also evaluated at these two extremes.The results demonstrated that the highest instrument background will occur during solar minima due to the main contributing source being Galactic Cosmic Rays(GCRs).It was also found that the open background was highest for solar minima and that the closed background was highest during solar maxima.This is due to the radiation shutter door acting as a scattering centre and the changes in the energy flux distribution of the GCRs between the two solar extremes. 展开更多
关键词 instrument background X-ray astronomy space radiation
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Atlas of dynamic spectra of fast radio burst FRB 20201124A
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作者 王铂钧 胥恒 +64 位作者 姜金辰 徐江伟 牛佳瑞 陈平 李柯伽 张冰 朱炜玮 东苏勃 张春风 傅海 周德江 张永坤 王培 冯毅 李晔 李冬子 鲁文宾 杨元培 RNCaballero 蔡策 陈卯蒸 戴子高 艾力·伊沙木丁 甘恒谦 韩金林 郝龙飞 黄玉祥 姜鹏 李承奎 李菂 李辉 李新乔 李志玄 刘志勇 罗睿 门云鹏 牛晨辉 彭文溪 钱磊 宋黎明 孙京海 王发印 汪敏 王娜 王维扬 吴雪峰 肖硕 熊少林 徐永华 徐仁新 杨俊 杨轩 姚蕊 易祁彬 岳友岭 于东俊 余文飞 袁建平 张彬彬 张松波 张双南 赵一 郑伟康 朱岩 邹金航 《Chinese Physics B》 SCIE EI CAS CSCD 2023年第2期1-4,共4页
Fast radio bursts(FRBs) are highly dispersed millisecond-duration radio bursts,[1,2]of which the physical origin is still not fully understood. FRB 20201124A is one of the most actively repeating FRBs. In this paper, ... Fast radio bursts(FRBs) are highly dispersed millisecond-duration radio bursts,[1,2]of which the physical origin is still not fully understood. FRB 20201124A is one of the most actively repeating FRBs. In this paper, we present the collection of 1863 burst dynamic spectra of FRB 20201124A measured with the Five-hundred-meter Aperture Spherical radio Telescope(FAST). The current collection, taken from the observation during the FRB active phase from April to June 2021, is the largest burst sample detected for any FRB so far. The standard PSRFITs format is adopted, including dynamic spectra of the burst, and the time information of the dynamic spectra, in addition, mask files help readers to identify the pulse positions are also provided. The dataset is available in Science Data Bank, with the link https://www.doi.org/10.57760/sciencedb.j00113.00076. 展开更多
关键词 fast radio burst FAST
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On the apparent line-of-sight alignment of the peak X-ray intensity of the magnetosheath and the tangent to the magnetopause,as viewed by SMILE-SXI 被引量:2
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作者 Andrew Read 《Earth and Planetary Physics》 EI CSCD 2024年第1期155-172,共18页
The Soft X-ray Imager(SXI)on board the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE)spacecraft will be able to view the Earth’s magnetosheath in soft X-rays.Simulated images of the X-ray emission visible f... The Soft X-ray Imager(SXI)on board the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE)spacecraft will be able to view the Earth’s magnetosheath in soft X-rays.Simulated images of the X-ray emission visible from the position of SMILE are created for a range of solar wind densities by using 3 years of the SMILE mission orbit,together with models of the expected X-ray emissivity from the Earth’s magnetosheath.Results from global magnetohydrodynamic simulations and a simple model for exospheric neutral densities are used to compare the locations of the lines of sight along which integrated soft X-ray intensities peak with the lines of sight lying tangent to surfaces(defined here to be the magnetopause)along which local soft X-ray intensities peak or exhibit their strongest gradients,or both,for strongly southward interplanetary magnetic field conditions when no depletion or low-latitude boundary layers are expected.Where,in the parameter space of the various times and seasons,orbital phases,solar wind conditions,and magnetopause models,the alignment of the X-ray emission peak with the magnetopause tangent is good,or is not,is presented.The main results are as follows.The spacecraft needs to be positioned well outside the magnetopause;low-altitude times near perigee are not good.In addition,there are seasonal aspects:dayside-apogee orbits are generally very good because the spacecraft travels out sunward at high altitude,but nightside-apogee orbits,behind the Earth,are bad because the spacecraft only rarely leaves the magnetopause.Dusk-apogee and dawnapogee orbits are intermediate.Dayside-apogee orbits worsen slightly over the first three mission years,whereas nightside-apogee orbits improve slightly.Additionally,many more times of good agreement with the peak-to-tangent hypothesis occur when the solar wind is in a high-density state,as opposed to a low-density state.In a high-density state,the magnetopause is compressed,and the spacecraft is more often a good distance outside the magnetopause. 展开更多
关键词 X-rays MAGNETOSPHERE MAGNETOSHEATH MAGNETOPAUSE Solar wind Magnetosphere Ionosphere Link Explorer(SMILE) Earth solar wind charge exchange
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Planar matrices and arrays of Feynman diagrams:poles for higher k
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作者 Alfredo Guevara Yong Zhang 《Communications in Theoretical Physics》 SCIE CAS CSCD 2024年第4期1-13,共13页
Planar arrays of tree diagrams were introduced as a generalization of Feynman diagrams that enable the computation of biadjoint amplitudes m_(n)(^(k))for k>2.In this follow-up work,we investigate the poles of m_(n)... Planar arrays of tree diagrams were introduced as a generalization of Feynman diagrams that enable the computation of biadjoint amplitudes m_(n)(^(k))for k>2.In this follow-up work,we investigate the poles of m_(n)(^(k))from the perspective of such arrays.For general k,we characterize the underlying polytope as a Flag Complex and propose a computation of the amplitude-based solely on the knowledge of the poles,whose number is drastically less than the number of the full arrays.As an example,we first provide all the poles for the cases(k,n)=(3,7),(3,8),(3,9),(3,10),(4,8)and(4,9)in terms of their planar arrays of degenerate Feynman diagrams.We then implement simple compatibility criteria together with an addition operation between arrays and recover the full collections/arrays for such cases.Along the way,we implement hard and soft kinematical limits,which provide a map between the poles in kinematic space and their combinatoric arrays.We use the operation to give a proof of a previously conjectured combinatorial duality for arrays in(k,n)and(n-k,n).We also outline the relation to boundary maps of the hypersimplex Δ_(k,n) and rays in the tropical Grassmannian Tr(k,n). 展开更多
关键词 Feynman diagrams biadjoint amplitudes POLES
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Surface-modified Ag@Ru-P25 for photocatalytic CO_(2) conversion with high selectivity over CH_(4) formation at the solid–gas interface 被引量:1
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作者 Chaitanya B.Hiragond Sohag Biswas +8 位作者 Niket SPowar Junho Lee Eunhee Gong Hwapyong Kim Hong Soo Kim Jin-Woo Jung Chang-Hee Cho Bryan M.Wong Su-Il In 《Carbon Energy》 SCIE EI CAS CSCD 2024年第1期182-196,共15页
Systematic optimization of the photocatalyst and investigation of the role of each component is important to maximizing catalytic activity and comprehending the photocatalytic conversion of CO_(2) reduction to solar f... Systematic optimization of the photocatalyst and investigation of the role of each component is important to maximizing catalytic activity and comprehending the photocatalytic conversion of CO_(2) reduction to solar fuels.A surface-modified Ag@Ru-P25 photocatalyst with H_(2)O_(2) treatment was designed in this study to convert CO_(2) and H_(2)O vapor into highly selective CH4.Ru doping followed by Ag nanoparticles(NPs)cocatalyst deposition on P25(TiO_(2))enhances visible light absorption and charge separation,whereas H_(2)O_(2) treatment modifies the surface of the photocatalyst with hydroxyl(–OH)groups and promotes CO_(2) adsorption.High-resonance transmission electron microscopy,X-ray photoelectron spectroscopy,X-ray absorption near-edge structure,and extended X-ray absorption fine structure techniques were used to analyze the surface and chemical composition of the photocatalyst,while thermogravimetric analysis,CO_(2) adsorption isotherm,and temperature programmed desorption study were performed to examine the significance of H_(2)O_(2) treatment in increasing CO_(2) reduction activity.The optimized Ag1.0@Ru1.0-P25 photocatalyst performed excellent CO_(2) reduction activity into CO,CH4,and C2H6 with a~95%selectivity of CH4,where the activity was~135 times higher than that of pristine TiO_(2)(P25).For the first time,this work explored the effect of H_(2)O_(2) treatment on the photocatalyst that dramatically increases CO_(2) reduction activity. 展开更多
关键词 gas-phase CO_(2) reduction H_(2)O_(2) treatment plasmonic nanoparticles solar fuel photocatalyst surface modification
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Tuning structural,electrical,dielectric and magnetic properties of Mg-Cu-Co ferrites via dysprosium(Dy^(3+))doping
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作者 Maria Akhtar M.S.Hasan +2 位作者 Nasir Amin N.A.Morley Muhammad Imran Arshad 《Journal of Rare Earths》 SCIE EI CAS CSCD 2024年第1期137-146,I0005,共11页
In current research work,Dy3+substituted Mg0.5Cu0.25Co0.25Fe2-xDyxO4(0.0≤x≤0.04 with the step interval of 0.01)soft ferrites were synthesized by the sol-gel auto combustion method.The prepared samples were character... In current research work,Dy3+substituted Mg0.5Cu0.25Co0.25Fe2-xDyxO4(0.0≤x≤0.04 with the step interval of 0.01)soft ferrites were synthesized by the sol-gel auto combustion method.The prepared samples were characterized by the techniques using X-ray diffraction(XRD),scanning electron microscopy(SEM),energy dispersive X-ray spectroscopy(EDS),Fourier transform infrared(FTIR)spectroscopy,curre nt-voltage(Ⅰ-Ⅴ)measurement,LCR meter,vibrating sample magnetometer(VSM)and Raman.XRD data reveal that the average crystallite size is 49.71 nm and the lattice constant is 0.83703 nm for sample x=0.03.The non-uniform grain growth was demonstrated by micrographs and impurity-free elemental composition was observed from EDX analysis.The DC resistivity has an increasing and decreasing trend in ferromagnetic and paramagnetic regions with an increase in temperature.Moreover,the high resistivity is observed with the order of 1010Ω·cm,and the activation energy is 0.944 eV for samples x=0.03.The dielectric parameters including dielectric constant,dielectric losses,and impedance gradually decrease with the increase in frequency from 8 Hz to 8 MHz.The minimum dielectric loss at high frequency is found for sample x=0.03.The coercivity(Hc)and saturation magnetization(Ms)are found in the ranges of 520.82-544.02 Oe and 20.5841-21.1473 emu/g,respectively.These observations confirm that dysprosium(x=0.03)doped MCC-soft ferrites may be applicable in transformer cores,microwave absorbance,and telecommunication devices. 展开更多
关键词 Soft ferrites DC resistivity Dielectric loss IMPEDANCE COERCIVITY Rare earths
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Sodium metals for single emitter strong coupling:Alternative plasmonic candidates beyond noble metals
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作者 Yi Zhang Shuying Chen +2 位作者 Yuning Han Xiulai Xu Lin Zhou 《Science China(Physics,Mechanics & Astronomy)》 SCIE EI CAS CSCD 2024年第8期106-117,共12页
This work provides a theoretical investigation into the strong coupling between a single quantum emitter(QE)and the surface plasmons of sodium metals in two representative plasmonic systems,i.e.,the semi-infinite meta... This work provides a theoretical investigation into the strong coupling between a single quantum emitter(QE)and the surface plasmons of sodium metals in two representative plasmonic systems,i.e.,the semi-infinite metal-dielectric interface and the metal nanoparticles(NPs)of monomer/dimer configuration.In both configurations,sodium metals exhibit distinctly stronger coupling strength and lower optical loss in the optical region than their noble metal counterparts,demonstrating the ideal candidate characteristics for single-molecule-level strong couplings with distinctly facile operation conditions.Our results provide new insights into extreme light-matter interactions with potential applications in quantum information,optical sensors,quantum chemistry,etc. 展开更多
关键词 sodium metals PLASMONICS single quantum emitter strong coupling pseudomode
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Properties of Flare Events on M Stars from LAMOST Spectral Survey Based on Kepler and TESS Light Curves
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作者 Gang Meng Li-Yun Zhang +7 位作者 Tianhao Su Zilu Yang Xianming LHan Prabhakar Misra Liu Long Qingfeng Pi Zhongzhong Zhu Linyan Jiang 《Research in Astronomy and Astrophysics》 SCIE CAS CSCD 2023年第5期1-18,共18页
A catalog of M stars has been published from the Large Sky Area Multi-Object Fiber Spectroscopic Telescope data release 7(LAMOST DR7).We cross-matched the LAMOST M catalog with Kepler,Kepler 2(K2)and Transiting Exopla... A catalog of M stars has been published from the Large Sky Area Multi-Object Fiber Spectroscopic Telescope data release 7(LAMOST DR7).We cross-matched the LAMOST M catalog with Kepler,Kepler 2(K2)and Transiting Exoplanet Survey Satellite(TESS)surveys.We obtained the light curves from the Kepler and TESS surveys.We detected 20,047 flare events from 4053 M stars and calculated their durations,amplitudes,and energies.We analyzed the distribution of the flare durations and energies.The distributions of flare duration for Kepler,K2 and TESS peak are at 3–3.5 hr,4–6 hr and 1–1.5 hr,respectively.This may be the result of the different cadences for the three data sets.The highest regions of the flare energies of Kepler,K2 and TESS are 32–32.5,32–32.5 and31–31.5 erg in Log format,respectively.A linear relationship between flare duration and energy emerges from our analysis.The ratio of flare duration to total observational time is approximately 0.2%–0.3%for the Kepler,K2 and TESS surveys.The occurrence rate of a star with a flare event increases from the M0 to M4 subtypes.We also determined the spatial distribution of the flare rate of M stars in the Milky Way.It seems that the flare rate decreases as the vertical height increases.The power index of the flare energies is in the region of 1.53–2.32,which is similar to previous result for solar type star(2.0).Further,we examined the relationship between the flare amplitude and chromospheric intensity.The flare activity increases rapidly with the increase in the HαEW at the lower values(less approximately 2?)and it increases slowly at the higher values. 展开更多
关键词 STARS activity-stars flare-stars LOW-MASS
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Direct observation of interlayer coherent acoustic phonon dynamics in bilayer and few-layer PtSe2 被引量:5
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作者 XIN CHEN SAIFENG ZHANG +9 位作者 LEI WANG YI-FAN HUANG HUIYAN LIU JIAWEI HUANG NINGNING DONG WEIMIN LIU IVAN MKISLYAKOV JEAN MICHEL NUNZI LONG ZHANG JUN WANG 《Photonics Research》 SCIE EI CSCD 2019年第12期1416-1424,共9页
This work reports the real-time observation of the interlayer lattice vibrations in bilayer and few-layer PtSe_2 by means of the coherent phonon method. The layer-breathing mode and standing wave mode of the interlaye... This work reports the real-time observation of the interlayer lattice vibrations in bilayer and few-layer PtSe_2 by means of the coherent phonon method. The layer-breathing mode and standing wave mode of the interlayer vibrations are found to coexist in such a kind of group-10 transition metal dichalcogenides(TMDCs). The interlayer breathing force constant standing for perpendicular coupling(per effective atom) is derived as 7.5 N/m,2.5 times larger than that of graphene. The interlayer shearing force constant is comparable to the interlayer breathing force constant, which indicates that PtSe2 has nearly isotropic interlayer coupling. The low-frequency Raman spectroscopy elucidates the polarization behavior of the layer-breathing mode that is assigned to have A1 g symmetry. The standing wave mode shows redshift with the increasing number of layers, which successfully determines the out-of-plane sound velocity of PtSe2 experimentally. Our results manifest that the coherent phonon method is a good tool to uncover the interlayer lattice vibrations, beyond the conventional Raman spectroscopy limit. The strong interlayer interaction in group-10 TMDCs reveals their promising potential in high-frequency(~terahertz) micro-mechanical resonators. 展开更多
关键词 POLARIZATION INTERLAYER COHERENT
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Metal to insulator transition for conducting polymers in plasmonic nanogaps
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作者 Yuling Xiong Rohit Chikkaraddy +5 位作者 Charlie Readman Shu Hu Kunli Xiong Jialong Peng Qianqi Lin Jeremy J.Baumberg 《Light(Science & Applications)》 SCIE EI CSCD 2024年第1期23-32,共10页
Conjugated polymers are promising material candidates for many future applications in flexible displays, organic circuits, and sensors. Their performance is strongly affected by their structural conformation including... Conjugated polymers are promising material candidates for many future applications in flexible displays, organic circuits, and sensors. Their performance is strongly affected by their structural conformation including both electrical and optical anisotropy. Particularly for thin layers or close to crucial interfaces, there are few methods to track their organization and functional behaviors. Here we present a platform based on plasmonic nanogaps that can assess the chemical structure and orientation of conjugated polymers down to sub-10 nm thickness using light. We focus on a representative conjugated polymer, poly(3,4-ethylenedioxythiophene) (PEDOT), of varying thickness (2-20 nm) while it undergoes redox in situ. This allows dynamic switching of the plasmonic gap spacer through a metal-insulator transition. Both dark-field (DF) and surface-enhanced Raman scattering (SERS) spectra track the optical anisotropy and orientation of polymer chains close to a metallic interface. Moreover, we demonstrate how this influences both optical and redox switching for nanothick PEDOT devices. 展开更多
关键词 TRANSITION INSULATOR CONJUGATED
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Recent advances in graphene and other 2D materials 被引量:5
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作者 Pablo Ares Kostya S.Novoselov 《Nano Materials Science》 EI CAS CSCD 2022年第1期3-9,共7页
The isolation of the first two-dimensional material, graphene-a monolayer of carbon atoms arranged in a hexagonal lattice-opened new exciting opportunities in the field of condensed matter physics and materials. Its i... The isolation of the first two-dimensional material, graphene-a monolayer of carbon atoms arranged in a hexagonal lattice-opened new exciting opportunities in the field of condensed matter physics and materials. Its isolation and subsequent studies demonstrated that it was possible to obtain sheets of atomically thin crystals and that these were stable, and they also began to show its outstanding properties, thus opening the door to a whole new family of materials, known as two-dimensional materials or 2D materials. The great interest in different 2D materials is motivated by the variety of properties they show, being candidates for numerous applications.Additionally, the combination of 2D crystals allows the assembly of composite, on-demand materials, known as van der Waals heterostructures, which take advantage of the properties of those materials to create functionalities that otherwise would not be accessible. For example, the combination of 2D materials, which can be done with high precision, is opening up opportunities for the study of new challenges in fundamental physics and novel applications. Here we review the latest fundamental discoveries in the area of 2D materials and offer a perspective on the future of the field. 展开更多
关键词 2D materials GRAPHENE Molybdenum disulphide Tarition mebl dichalogenides Hexagonal boron nitride van der waals heterostructus Ulrathin nanomaterials
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K_(3)La(PO_(4))_(2)基质中Tb^(3+)的发光和能量传递 被引量:5
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作者 欧奕意 王笑军 梁宏斌 《发光学报》 EI CAS CSCD 北大核心 2022年第9期1350-1360,I0001,共12页
采用高温固相方法合成了不同浓度Tb^(3+)掺杂的单斜结构K_(3)La(PO_(4))_(2)荧光粉,利用XRD表征了其相纯度,并对基质化合物进行了结构精修。研究了Tb^(3+)掺杂样品在不同温度下的发光性质及不同掺杂浓度样品在室温下的发光性质。发现在... 采用高温固相方法合成了不同浓度Tb^(3+)掺杂的单斜结构K_(3)La(PO_(4))_(2)荧光粉,利用XRD表征了其相纯度,并对基质化合物进行了结构精修。研究了Tb^(3+)掺杂样品在不同温度下的发光性质及不同掺杂浓度样品在室温下的发光性质。发现在室温、373 nm激发下,Tb^(3+)离子表现为^(5)D_(3)⁃7F_(J)(J=5,4,3,2)和^(5)D_(4)⁃^(7)F_(J)'(J'=6,5,4,3)等两组发射。不同温度下低掺样品的光谱测试表明,多声子弛豫对5D_(3)能级发射的猝灭贡献有限。随着掺杂浓度增加,Tb^(3+)离子5D_(3)发射减弱而5D_(4)发射增强,样品表现出从青光到绿光的光色调控性质,这主要是由Tb^(3+)能级间的交叉弛豫过程导致的;进一步通过Inokuti⁃Hirayama模型和扩展的Yokota⁃Tanimoto模型对5D_(3)发光衰减曲线进行拟合,结果表明能量传递的主要作用方式为电偶极⁃四极作用,临界传递距离约为1.03 nm。 展开更多
关键词 Tb^(3+) K_(3)La(PO_(4))_(2) 发光 能量传递 多声子弛豫 交叉弛豫
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Luminescence regulation of Sb^(3+)in 0D hybrid metal halides by hydrogen bond network for optical anti-counterfeiting
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作者 Dehai Liang Saif M.H.Qaid +5 位作者 Xin Yang Shuangyi Zhao Binbin Luo Wensi Cai Qingkai Qian Zhigang Zang 《Opto-Electronic Advances》 SCIE EI CAS CSCD 2024年第3期15-25,共11页
The Sb^(3+) doping strategy has been proven to be an effective way to regulate the band gap and improve the photophysical properties of organic-inorganic hybrid metal halides(OIHMHs).However,the emission of Sb^(3+) io... The Sb^(3+) doping strategy has been proven to be an effective way to regulate the band gap and improve the photophysical properties of organic-inorganic hybrid metal halides(OIHMHs).However,the emission of Sb^(3+) ions in OIHMHs is primarily confined to the low energy region,resulting in yellow or red emissions.To date,there are few reports about green emission of Sb^(3+)-doped OIHMHs.Here,we present a novel approach for regulating the luminescence of Sb^(3+) ions in 0D C_(10)H_(2)_(2)N_(6)InCl_(7)·H_(2)O via hydrogen bond network,in which water molecules act as agents for hydrogen bonding.Sb^(3+)-doped C_(10)H_(2)2N_(6)InCl_(7)·H_(2)O shows a broadband green emission peaking at 540 nm and a high photoluminescence quantum yield(PLQY)of 80%.It is found that the intense green emission stems from the radiative recombination of the self-trapped excitons(STEs).Upon removal of water molecules with heat,C_(10)H_(2)_(2)N_(6)In_(1-x)Sb_(x)Cl_(7) generates yellow emis-sion,attributed to the breaking of the hydrogen bond network and large structural distortions of excited state.Once water molecules are adsorbed by C_(10)H_(2)_(2)N_(6)In_(1-x)Sb_(x)Cl_(7),it can subsequently emit green light.This water-induced reversible emission switching is successfully used for optical security and information encryption.Our findings expand the under-standing of how the local coordination structure influences the photophysical mechanism in Sb^(3+)-doped metal halides and provide a novel method to control the STEs emission. 展开更多
关键词 indium-based halides Sb^(3+)doping hydrogen bonding network optical anti-counterfeiting
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Baseline design of the KunLun Turbulence Profiler instrument
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作者 Xiaohui Guo Yi Hu +2 位作者 Jing Li Xu Yang Zhengzhou Yan 《Astronomical Techniques and Instruments》 CSCD 2024年第4期218-226,共9页
Adaptive optics systems are the most powerful tools to counteract the image blurring caused by atmospheric turbulence,allowing ground-based telescopes to capture high-resolution images.A critical parameter influencing... Adaptive optics systems are the most powerful tools to counteract the image blurring caused by atmospheric turbulence,allowing ground-based telescopes to capture high-resolution images.A critical parameter influencing adaptive optics system performance is the atmospheric refractive index structure constant,C_(n)^(2),which characterizes the intensity of atmospheric optical turbulence as a function of altitude.Given its simplicity,the lunar scintillometer is the preferred method for detecting atmospheric turbulence in challenging environments like Dome A in Antarctica,where sites are still in the developmental stages and local environmental conditions are extremely harsh.However,optimizing the performance of such instruments requires carefully determining the baseline configuration of photon sensors according to each site's specific optical turbulence profile characteristics.This study uses a Monte Carlo method to identify the optimal configuration for the KunLun Turbulence Profiler(KLTP),an instrument comparable to the lunar scintillometer,developed for use at Dome A.Simulations conducted using the obtained optimal baseline configuration recovered three different model optical turbulence profiles,demonstrating the effectiveness of our method in obtaining an optimal baseline configuration.Our approach can be easily applied to baseline design for similar turbulence profilers at other sites. 展开更多
关键词 KunLun Turbulence Profiler Monte Carlo Simulation Turbulence profile
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Accretion in strong field gravity with eXTP 被引量:1
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作者 Alessandra De Rosa Phil Uttley +99 位作者 LiJun Gou Yuan Liu Cosimo Bambi Didier Barret Tomaso Belloni Emanuele Berti Stefano Bianchi Ilaria Caiazzo Piergiorgio Casella Marco Feroci Valeria Ferrari Leonardo Gualtieri Jeremy Heyl Adam Ingram Vladimir Karas FangJun Lu Bin Luo Giorgio Matt Sara Motta Joseph Neilsen Paolo Pani Andrea Santangelo XinWen Shu JunFeng Wang Jian-Min Wang YongQuan Xue YuPeng Xu WeiMin Yuan YeFei Yuan Shuang-Nan Zhang Shu Zhang Ivan Agudo Lorenzo Amati Nils Andersson Cristina Baglio Pavel Bakala Altan Baykal Sudip Bhattacharyya Ignazio Bombaci NiccolóBucciantini Fiamma Capitanio Riccardo Ciolfi Wei K.Cui Filippo D'Ammando Thomas Dauser Melania Del Santo Barbara De Marco Tiziana Di Salvo Chris Done Michal Dovciak Andrew C.Fabian Maurizio Falanga Angelo Francesco Gambino Bruce Gendre Victoria Grinberg Alexander Heger Jeroen Homan Rosario Iaria JiaChen Jiang ChiChuan Jin Elmar Koerding Manu Linares Zhu Liu Thomas J.Maccarone Julien Malzac Antonios Manousakis Frédéric Marin Andea Marinucci Missagh Mehdipour Mariano Méndez Simone Migliari Cole Miller Giovanni Miniutti Emanuele Nardini Paul T.O'Brien Julian P.Osborne Pierre Olivier Petrucci Andrea Possenti Alessandro Riggio Jerome Rodriguez Andrea Sanna LiJing Shao Malgosia Sobolewska Eva Sramkova Abigail L.Stevens Holger Stiele Giulia Stratta Zdenek Stuchlik Jiri Svoboda Fabrizio Tamburini Thomas M.Tauris Francesco Tombesi Gabriel Torok Martin Urbanec Frederic Vincent QingWen Wu Feng Yuan Jean J.M.in't Zand Andrzej A.Zdziarski XinLin Zhou 《Science China(Physics,Mechanics & Astronomy)》 SCIE EI CAS CSCD 2019年第2期45-73,共29页
In this paper we describe the potential of the enhanced X-ray Timing and Polarimetry(eXTP) mission for studies related to accretion flows in the strong field gravity regime around both stellar-mass and supermassive bl... In this paper we describe the potential of the enhanced X-ray Timing and Polarimetry(eXTP) mission for studies related to accretion flows in the strong field gravity regime around both stellar-mass and supermassive black-holes. eXTP has the unique capability of using advanced "spectral-timing-polarimetry" techniques to analyze the rapid variations with three orthogonal diagnostics of the flow and its geometry, yielding unprecedented insight into the inner accreting regions, the effects of strong field gravity on the material within them and the powerful outflows which are driven by the accretion process. 展开更多
关键词 X-ray black holes physics ACCRETION
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