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Broadband diffusion of terahertz waves by multi-bit coding metasurfaces 被引量:38
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作者 Li-Hua Gao Qiang Cheng +15 位作者 Jing Yang Shao-Jie Ma Jie Zhao Shuo Liu Hai-Bing Chen Qiong He Wei-Xiang Jiang Hui-Feng Ma Qi-Ye Wen Lan-Ju Liang Biao-Bing Jin Wei-Wei Liu Lei Zhou Jian-Quan Yao Pei-Heng Wu Tie-Jun Cui 《Light(Science & Applications)》 SCIE EI CAS CSCD 2015年第1期207-215,共9页
The terahertz region is a special region of the electromagnetic spectrum that incorporates the advantages of both microwaves and infrared light waves.In the past decade,metamaterials with effective medium parameters o... The terahertz region is a special region of the electromagnetic spectrum that incorporates the advantages of both microwaves and infrared light waves.In the past decade,metamaterials with effective medium parameters or gradient phases have been studied to control terahertz waves and realize functional devices.Here,we present a new approach to manipulate terahertz waves by using coding metasurfaces that are composed of digital coding elements.We propose a general coding unit based on a Minkowski closed-loop particle that is capable of generating 1-bit coding(with two phase states of 0 and 180°),2-bit coding(with four phase states of 0,90°,180°,and 270°),and multi-bit coding elements in the terahertz frequencies by using different geometric scales.We show that multi-bit coding metasurfaces have strong abilities to control terahertz waves by designing-specific coding sequences.As an application,we demonstrate a new scattering strategy of terahertz waves—broadband and wide-angle diffusion—using a 2-bit coding metasurface with a special coding design and verify it by both numerical simulations and experiments.The presented method opens a new route to reducing the scattering of terahertz waves. 展开更多
关键词 CODING DIFFUSION metasurface terahertz waves
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The role and significance of Magnesium in modern day research-A review 被引量:23
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作者 S V Satya Prasad S B Prasad +3 位作者 Kartikey Verma Raghvendra Kumar Mishra Vikas Kumar Subhash Singh 《Journal of Magnesium and Alloys》 SCIE EI CAS CSCD 2022年第1期1-65,共65页
Magnesium is one of the largely available elements in the earth’s crust. It has a low structural density with high specific strength. This unique material property has forced an increase in the use of magnesium and i... Magnesium is one of the largely available elements in the earth’s crust. It has a low structural density with high specific strength. This unique material property has forced an increase in the use of magnesium and its alloys in various applications pertaining to industrial sector,automobiles, aerospace and biomedical. Since magnesium is a highly reactive metal, it is prone to higher rate of corrosion as compared to its counterparts. Thus, it is essential to analyze the corrosion behavior of magnesium and its alloys in its applications. An appropriate process is to be followed in the design and development of magnesium alloys which overcome the limitations of magnesium and enhance the desired material properties in accordance to their applications. This review paper summarizes the importance of magnesium and its material properties. The influence of various alloying elements on the mechanical properties of magnesium is reviewed. The broad classification of Mg alloys and their behavioral trends are detailed. The corrosion behavior of magnesium and the influence of corrosion products on the material characteristics of magnesium, in aqueous medium, are discussed. The manufacturing techniques of magnesium alloys along with the secondary techniques are also covered. The various applications and the limitations of magnesium in these applications are covered. A complete section is dedicated towards detailing the recent trends of magnesium(Mg) alloys, i.e., the biodegradable nature and applications of Mg alloys. The influence of biocorrosion on Mg alloys and techniques to overcome it have been deliberated. This paper provides a thorough review on recent developments of magnesium with respect to engineering applications. 展开更多
关键词 Magnesium alloys Biodegradable alloys Magnesium corrosion BIOCORROSION
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EW-trending uplifts along the southern side of the central segment of the Altyn Tagh Fault, NW China: Insight into the rising mechanism of the Altyn Mountain during the Cenozoic 被引量:24
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作者 WU Lei XIAO AnCheng +4 位作者 WANG LiQun MAO LiGuang WANG Liang DONG YouPu XU Bo 《Science China Earth Sciences》 SCIE EI CAS 2012年第6期926-939,共14页
The Altyn Tagh Fault and the Altyn Mountain define respectively the tectonic and geographical northern edges of the Tibetan Plateau, and figure prominently in the growth and rising mechanism of the plateau. The rhombu... The Altyn Tagh Fault and the Altyn Mountain define respectively the tectonic and geographical northern edges of the Tibetan Plateau, and figure prominently in the growth and rising mechanism of the plateau. The rhombus-shaped Altyn Mountain has long been thought to have an intimate relation with the Altyn Tagh Fault; however, its formation mechanism remains unclear and debatable. In this paper, we focus on the EW-trending uplifts in the Altyn Mountain, and investigated three Cenozoic sedimentary sections in the vicinity of the EW-trending uplifts located along the southern side of the central segment of the Altyn Tagh Fault. Magnetostratigraphy and pollen analysis were used to constrain ages of the sediments. Clast composition of conglomerate and paleocurrents obtained from clast imbrications were applied to determine the provenance. We also established a geological section parallel to the Altyn Tagh Fault on sedimentary facies across the northwestern Qaidam Basin. The results indicate that these en-echelon EW-trending uplifts formed as early as ca. 36 Ma and were preferred to be under the control of basal shear of the Altyn Tagh Fault in the middle-lower crust, symbolizing the early uplift of the Altyn Mountain during the Cenozoic. Left-slip along the Altyn Tagh Fault occurring during the Miocene and afterwards displaced and altered these uplifts, shaping the Altyn Mountain to its present fabric. 展开更多
关键词 Northern Tibetan Plateau Altyn Tagh Fault Aityn Mountain EW-trending uplift Qaidam Basin
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3D non-isothermal phase-field simulation of microstructure evolution during selective laser sintering 被引量:12
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作者 Yangyiwei Yang Olav Ragnvaldsen +2 位作者 Yang Bai Min Yi Bai-Xiang Xu 《npj Computational Materials》 SCIE EI CSCD 2019年第1期442-453,共12页
During selective laser sintering(SLS),the microstructure evolution and local temperature variation interact mutually.Application of conventional isothermal sintering model is thereby insufficient to describe SLS.In th... During selective laser sintering(SLS),the microstructure evolution and local temperature variation interact mutually.Application of conventional isothermal sintering model is thereby insufficient to describe SLS.In this work,we construct our model from entropy level,and derive the non-isothermal kinetics for order parameters along with the heat transfer equation coupled with microstructure evolution.Influences from partial melting and laser-powder interaction are also addressed.We then perform 3D finite element non-isothermal phase-field simulations of the SLS single scan.To confront the high computation cost,we propose a novel algorithm analogy to minimum coloring problem and manage to simulate a system of 200 grains with grain tracking algorithm using as low as 8 non-conserved order parameters.Specifically,applying the model to SLS of the stainless steel 316L powder,we identify the influences of laser power and scan speed on microstructural features,including the porosity,surface morphology,temperature profile,grain geometry,and densification.We further validate the first-order kinetics of the transient porosity during densification,and demonstrate the applicability of the developed model in predicting the linkage of densification factor to the specific energy input during SLS. 展开更多
关键词 MICROSTRUCTURE ISOTHERMAL KINETICS
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Recent progress of energy transfer and luminescence intensity boosting mechanism in Nd3+-sensitized upconversion nanoparticles 被引量:11
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作者 Solomon Tiruneh Dibaba Xiaoqian Ge +1 位作者 Wei Ren Lining Sun 《Journal of Rare Earths》 SCIE EI CAS CSCD 2019年第8期791-805,I0001,共16页
Rare earth doped upconversion nanoparticles can be considered as the spice of research in the field of luminescence nanomaterials due to their unique optical properties such as near-infrared excitation.Enormous works ... Rare earth doped upconversion nanoparticles can be considered as the spice of research in the field of luminescence nanomaterials due to their unique optical properties such as near-infrared excitation.Enormous works have been reported about biomedical applications of 980 nm excited and Yb^3+-sensitized upconversion nanoparticles.However,980 nm excitation wavelength overlaps with the absorption band of water molecules in the biological environment,leading to overheating effect that can induce thermal damages of normal cells and tissues.Recently,Nd^3+-sensitized upconversion nanoparticles which can be excited with 808 nm has been widely investigated as alternative nanoparticles that can surmount this issue of overheating effect.Even though Nd^3+-sensitized upconversion nanoparticles can reduce the overheating effect by 20 fold as compared to Yb^3+-sensitized counterpart,there are several factors that reduce the upconversion luminescence intensity.In this review article,photon energy harvesting and transferring mechanisms in Nd^3+,Yb^3+and emitter ions co-doped upconversion nanoparticles under 808 nm excitation are briefly discussed.Factors that affect upconversion luminescence intensity and quantum yield of Nd^3+-sensitized upconversion nanoparticles are also addressed.Besides,some of the important strategies that have been recently utilized to boost upconversion luminescence intensity of Nd^3+sensitized upco nversion nanoparticles are tho roughly summarized.Lastly,the future challenges in the area and our perspectives are in sight. 展开更多
关键词 Rare earth UPCONVERSION NANOPARTICLES Nd^3+-sensitized Energy transfer
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An automatic grid generation approach over free-form surface for architectural design 被引量:11
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作者 苏亮 祝顺来 +1 位作者 肖南 高博青 《Journal of Central South University》 SCIE EI CAS 2014年第6期2444-2453,共10页
An essential step for the realization of free-form surface structures is to create an efficient structural gird that satisfies not only the architectural aesthetics,but also the structural performance.Employing the ma... An essential step for the realization of free-form surface structures is to create an efficient structural gird that satisfies not only the architectural aesthetics,but also the structural performance.Employing the main stress trajectories as the representation of force flows on a free-form surface,an automatic grid generation approach is proposed for the architectural design.The algorithm automatically plots the main stress trajectories on a 3D free-form surface,and adopts a modified advancing front meshing technique to generate the structural grid.Based on the proposed algorithm,an automatic grid generator named "St-Surmesh" is developed for the practical architectural design of free-form surface structure.The surface geometry of one of the Sun Valleys in Expo Axis for the Expo Shanghai 2010 is selected as a numerical example for validating the proposed approach.Comparative studies are performed to demonstrate how different structural grids affect the design of a free-form surface structure. 展开更多
关键词 grid generation free-form surface structure architectural geometry stress trajectory advancing front meshing technique
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SARISTU:Adaptive Trailing Edge Device(ATED)design process review 被引量:10
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作者 A.CONCILIO I.DIMINO R.PECORA 《Chinese Journal of Aeronautics》 SCIE EI CAS CSCD 2021年第7期187-210,共24页
SARISTU was a big cooperation project granted by the European Commission,7th Framework Programme,carried out between 2011 and 2015.It dealt with smart aeronautic structures,both morphing and sensored;its main target w... SARISTU was a big cooperation project granted by the European Commission,7th Framework Programme,carried out between 2011 and 2015.It dealt with smart aeronautic structures,both morphing and sensored;its main target was to demonstrate the feasibility of designing,manufacturing and operating in representative environment,instrumented structures.Till now,it represents the major effort carried out within the European Union on the development of adaptive architectures for air systems.Inside that big activity,the realization of an Adaptive Trailing Edge Device(ATED)for wing camber adaptations aimed at compensating the weight reduction following the fuel consumption during cruise was addressed.It made the core of investigations target variable geometry aircraft components together with two other analyses concerning the development of shape-changing winglet and droop nose.ATED activities were conducted by the Italian Aerospace Research Centre(CIRA)in tight cooperation with the University of Napoli,"Federico II",who coordinated a group of 12 different partners from 8 different nations(France,Germany,Greece,the Netherlands,Israel,Spain,Turkey,and Italy).In this paper,an integral synthesis of that work is reported,with a focus on the definition and realization of the components of the presented device.The publication is in fact meant as the first part of a series that is aimed at overviewing the whole adaptive trailing edge development,till wind tunnel tests execution.Such a concise report is a critical and harmonized review of what have been performed by many colleagues spread all over Europe,all of which are duly recalled in the reported bibliography where the reader may access more detailed information and descriptions.In detail,the paper starts with a general introduction of the concept and its aims,to move to the specs definition immediately after.Then,it deals with a short but comprehensive description of the main ATED components:structural skeleton,skin,actuation and sensing systems.It is worth remarking that the pa 展开更多
关键词 Actuator network Aeroelasticity Adaptive structures Adaptive systems design Adaptive trailing edge Kinematic systems MORPHING SARISTU Sensor network Skins
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Chiral metal nanostructures:synthesis,properties and applications 被引量:6
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作者 Sulaiman Umar Abbas Jun-Jun Li +8 位作者 Xing Liu Ayesha Siddique Yong-Xia Shi Man Hou Kai Yang Farhat Nosheen Xiao-Ya Cui Guang-Chao Zheng Zhi-Cheng Zhang 《Rare Metals》 SCIE EI CAS CSCD 2023年第8期2489-2515,共27页
Chirality,the property that an object cannot coincide with its mirror image arising from lack of mirror symmetry,is ubiquitous in nature at various length scales.The physical and chemical properties are strongly relat... Chirality,the property that an object cannot coincide with its mirror image arising from lack of mirror symmetry,is ubiquitous in nature at various length scales.The physical and chemical properties are strongly related to the nature of chiral complexes,playing a significant role in various fields such as photonics,biochemistry,medicine and catalysis.In particular,the recent flexible design of chiral metal nanostructures offers one platform for deeply understanding the origin of chirality and one roadmap for the precise construction of chiral nanomaterials directed by the applications.Herein,we summarize the different geometries and classical synthetic approaches to chiral noble metal nanomaterials.Moreover,chiroptical properties and potential applications of chiral metal nanostructures are discussed as well.Finally,the opportunities and challenges toward the synthesis and application of chiral metal nanostructures are proposed. 展开更多
关键词 Chiral metal nanostructures Circular dichroism(CD) ENANTIOMERS Chiroptical activity
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Numerical Study of a Novel Procedure for Installing the Tower and Rotor Nacelle Assembly of Offshore Wind Turbines Based on the Inverted Pendulum Principle 被引量:10
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作者 Wilson Guachamin Acero Zhen Gao Torgeir Moan 《Journal of Marine Science and Application》 CSCD 2017年第3期243-260,共18页
Current installation costs of offshore wind turbines(OWTs) are high and profit margins in the offshore wind energy sector are low, it is thus necessary to develop installation methods that are more efficient and pract... Current installation costs of offshore wind turbines(OWTs) are high and profit margins in the offshore wind energy sector are low, it is thus necessary to develop installation methods that are more efficient and practical. This paper presents a numerical study(based on a global response analysis of marine operations) of a novel procedure for installing the tower and Rotor Nacelle Assemblies(RNAs) on bottom-fixed foundations of OWTs. The installation procedure is based on the inverted pendulum principle. A cargo barge is used to transport the OWT assembly in a horizontal position to the site, and a medium-size Heavy Lift Vessel(HLV) is then employed to lift and up-end the OWT assembly using a special upending frame. The main advantage of this novel procedure is that the need for a huge HLV(in terms of lifting height and capacity) is eliminated. This novel method requires that the cargo barge is in the leeward side of the HLV(which can be positioned with the best heading) during the entire installation. This is to benefit from shielding effects of the HLV on the motions of the cargo barge, so the foundations need to be installed with a specific heading based on wave direction statistics of the site and a typical installation season. Following a systematic approach based on numerical simulations of actual operations, potential critical installation activities, corresponding critical events, and limiting(response) parameters are identified. In addition, operational limits for some of the limiting parameters are established in terms of allowable limits of sea states. Following a preliminary assessment of these operational limits, the duration of the entire operation, the equipment used, and weather-and water depth-sensitivity, this novel procedure is demonstrated to be viable. 展开更多
关键词 offshore wind turbine installation crane vessel shielding effects critical events limiting parameters inverted pendulum allowable sea states
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Ground motion spatial variability effects on seismic response control of cable-stayed bridges 被引量:10
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作者 Shehata E. Abdel Raheem Toshiro Hayashikawa Uwe Dorka 《Earthquake Engineering and Engineering Vibration》 SCIE EI CSCD 2011年第1期37-49,共13页
The spatial variability of input ground motion at supporting foundations plays a key role in the structural response of cable-stayed bridges (CSBs); therefore, spatial variation effects should be included in the ana... The spatial variability of input ground motion at supporting foundations plays a key role in the structural response of cable-stayed bridges (CSBs); therefore, spatial variation effects should be included in the analysis and design of effective vibration control systems. The control of CSBs represents a challenging and unique problem, with many complexities in modeling, control design and implementation, since the control system should be designed not only to mitigate the dynamic component of the structural response but also to counteract the effects of the pseudo-static component of the response. The spatial variability effects on the feasibility and efficiency of seismic control systems for the vibration control of CSBs are investigated in this paper. The assumption of uniform earthquake motion along the entire bridge may result in quantitative and qualitative differences in seismic response as compared with those produced by uniform motion at all supports. A systematic comparison of passive and active system performance in reducing the structural responses is performed, focusing on the effect of the spatially varying earthquake ground motion on the seismic response of a benchmark CSB model with different control strategies, and demonstrates the importance of accounting for the spatial variability of excitations. 展开更多
关键词 cable-stayed bridge vibration control earthquake spatial variation seismic design semi-active control
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Enhanced photoelectrochemical and photocatalytic activities of CdS nanowires by surface modification with MoS_2 nanosheets 被引量:9
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作者 Hongmei Wang1 2 +4 位作者 Sara Bonabi Naghadeh2 Chunhe Li3 Lu Ying1 A'Lester Allen2 Jin Zhong Zhang2 《Science China Materials》 SCIE EI CSCD 2018年第6期839-850,共12页
Nanocomposites composed of one-dimensional(1D) CdS nanowires(NWs) and 1 T-MoS2 nanosheets have been fabricated through a two-step solvothermal process. 5 mol% of MoS2 loading results in the best optical properties... Nanocomposites composed of one-dimensional(1D) CdS nanowires(NWs) and 1 T-MoS2 nanosheets have been fabricated through a two-step solvothermal process. 5 mol% of MoS2 loading results in the best optical properties,photoelectrochemical(PEC) as well as photocatalytic activities for hydrogen evolution reaction(HER). Compared with pure CdS NWs, the optimized nanocomposite shows 5.5 times enhancement in photocurrent and 86.3 times increase for HER in the presence of glucose and lactic acid as hole scavengers.The enhanced PEC and HER activities are attributed to the intimate contact between MoS2 and CdS that efficiently enhances charge carrier separation. In addition, ultrafast transient absorption(TA) measurements have been used to probe the charge carrier dynamics and gain deeper insight into the mechanism behind the enhanced PEC and photocatalytic performance. 展开更多
关键词 MoS2/CdS nanostructures surface modification photoelectrochemical activity photocatalytic hydrogen evolution glucose and lactic acid
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The quality traceability system for prefabricated buildings using blockchain:An integrated framework 被引量:9
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作者 Ziyao ZHANG Zhenmin YUAN +2 位作者 Guodong NI Han LIN Yujie LU 《Frontiers of Engineering Management》 2020年第4期528-546,共19页
The quality traceability of precast components has largely affected the widespread adoption of prefabricated buildings.Blockchain technology provides an effective solution to change the centralized storage mode of tra... The quality traceability of precast components has largely affected the widespread adoption of prefabricated buildings.Blockchain technology provides an effective solution to change the centralized storage mode of traditional traceability system and its related disadvantages.In this paper,we propose a framework of quality traceability system for precast components based on blockchain technology.The system framework adopts a hybrid blockchain architecture and dual storage mode,defines three types of smart contracts,and creates an interactive and efficient source tracing query method,which could effectively achieve the goals of decentralization,openness,and non-tamperability,as well as efficient traceability. 展开更多
关键词 quality traceability precast components blockchain FRAMEWORK
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Optomechanically induced transparency in a spinning resonator 被引量:8
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作者 HAO Lü YAJING JIANG +1 位作者 YU-ZHU WANG HUI JING 《Photonics Research》 SCIE EI 2017年第4期367-371,共5页
We study optomechanically induced transparency in a spinning microresonator. We find that in the presence of rotation-induced Sagnac frequency shift, both the transmission rate and the group delay of the signal are st... We study optomechanically induced transparency in a spinning microresonator. We find that in the presence of rotation-induced Sagnac frequency shift, both the transmission rate and the group delay of the signal are strongly affected, leading to a Fano-like spectrum of transparency. In particular, tuning the rotary speed leads to the emergence of nonreciprocal optical sidebands. This indicates a promising new way to control hybrid light–sound devices with spinning resonators. 展开更多
关键词 RATE
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Natural and Eco-Friendly Materials for Triboelectric Energy Harvesting 被引量:8
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作者 Vladislav Slabov Svitlana Kopyl +1 位作者 Marco PSoares dos Santos Andrei L.Kholkin 《Nano-Micro Letters》 SCIE EI CAS CSCD 2020年第3期179-196,共18页
Triboelectric nanogenerators(TENGs)are promising electric energy harvesting devices as they can produce renewable clean energy using mechanical excitations from the environment.Several designs of triboelectric energy ... Triboelectric nanogenerators(TENGs)are promising electric energy harvesting devices as they can produce renewable clean energy using mechanical excitations from the environment.Several designs of triboelectric energy harvesters relying on biocompatible and eco-friendly natural materials have been introduced in recent years.Their ability to provide customizable self-powering for a wide range of applications,including biomedical devices,pressure and chemical sensors,and battery charging appliances,has been demonstrated.This review summarizes major advances already achieved in the field of triboelectric energy harvesting using biocompatible and eco-friendly natural materials.A rigorous,comparative,and critical analysis of preparation and testing methods is also presented.Electric power up to 14 mW was already achieved for the dry leaf/polyvinylidene fluoride-based TENG devices.These findings highlight the potential of eco-friendly self-powering systems and demonstrate the unique properties of the plants to generate electric energy for multiple applications. 展开更多
关键词 Natural and eco-friendly materials Energy harvesting Triboelectric nanogenerators BIOCOMPATIBILITY
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Analytical Solutions of Cracks Emanating from an Elliptic Hole in an Infinite Plate under Tension 被引量:8
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作者 LIU Shuhong DUAN Shijie 《Chinese Journal of Mechanical Engineering》 SCIE EI CAS CSCD 2014年第5期1057-1063,共7页
It is a common phenomenon that the cracks originating from a hole can cause structural damage in engineering.However,the fracture mechanics studies of hole edge crack problems are not sufficient.The problem of an elli... It is a common phenomenon that the cracks originating from a hole can cause structural damage in engineering.However,the fracture mechanics studies of hole edge crack problems are not sufficient.The problem of an elliptical hole with two collinear edge cracks of unequal length in an infinite plate under uniform tension at infinity is investigated.Based on the complex variable method,the analytical solutions of stress functions and stress intensity factors are provided.The stress distribution along the axes and the edge of the elliptical hole is given graphically.The numerical results show that there is obvious stress concentration near the hole and cracks,and the stresses tend to applied loads at distances far from the defect,which conform to Saint-Venant’s principle.Hence,the stress functions are proved to be right.Under special conditions,the present configuration becomes the Griffith crack,two symmetrical cracks emanating from an elliptical hole,two cracks of unequal length emanating from a circular hole,a crack at the edge of a circular hole,or a crack emanating from an elliptical hole.Compared with available results,stress intensity factors for these special shapes of ellipses and cracks show good coincidence.The stress intensity factor for two cracks of unequal length at the edge of an elliptical hole increases with the crack length and the major-to-minor axis ratio of the elliptical hole.The stress distribution in an infinite plate containing an elliptic hole with unsymmetrical cracks is given for the first time. 展开更多
关键词 HOLE CRACK stress distribution stress intensity factor
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Ameliorating the re/dehydrogenation behaviour of MgH2 by zinc titanate addition 被引量:3
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作者 N.A.Ali N.A.Sazelee +4 位作者 M.F.Md Din M.M.Nasef A.A.Jalil Haizen Liu M.Ismail 《Journal of Magnesium and Alloys》 SCIE EI CAS CSCD 2023年第6期2205-2215,共11页
Magnesium hydride(MgH_(2))is the most feasible and effective solid-state hydrogen storage material,which has excellent reversibility but initiates decomposing at high temperatures and has slow kinetics performance.Her... Magnesium hydride(MgH_(2))is the most feasible and effective solid-state hydrogen storage material,which has excellent reversibility but initiates decomposing at high temperatures and has slow kinetics performance.Here,zinc titanate(Zn_(2)TiO_(4))synthesised by the solid-state method was used as an additive to lower the initial temperature for dehydrogenation and enhance the re/dehydrogenation behaviour of MgH_(2).With the presence of Zn_(2)TiO_(4),the starting temperature for the dehydrogenation of MgH_(2)was remarkably lowered to around 290℃–305℃.In addition,within 300 s,the MgH_(2)–Zn_(2)TiO_(4)sample absorbed 5.0 wt.%of H_(2)and 2.2–3.6 wt.%H_(2)was liberated from the composite sample in 30 min,which is faster by 22–36 times than as-milled MgH_(2).The activation energy of the MgH_(2)for the dehydrogenation process was also downshifted to 105.5 k J/mol with the addition of Zn_(2)TiO_(4)indicating a decrease of 22%than as-milled MgH_(2).The superior behaviour of MgH_(2)was due to the formation of Mg Zn_(2),MgO and MgTiO_(3),which are responsible for ameliorating the re/dehydrogenation behaviour of MgH_(2).These findings provide a new understanding of the hydrogen storage behaviour of the catalysed-MgH_(2)system. 展开更多
关键词 Hydrogen storage Solid-state storage MgH_(2) ADDITIVE Zn_(2)TiO_(4)
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Photoinduced large polaron transport and dynamics in organic-inorganic hybrid lead halide perovskite with terahertz probes 被引量:6
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作者 Zuanming Jin Yan Peng +14 位作者 Yuqing Fang Zhijiang Ye Zhiyuan Fan Zhilin Liu Xichang Bao Heng Gao Wei Ren Jing Wu Guohong Ma Qianli Chen Chao Zhang Alexey VBalakin Alexander PShkurinov Yiming Zhu Songlin Zhuang 《Light(Science & Applications)》 SCIE EI CAS CSCD 2022年第8期1853-1864,共12页
Organic-inorganic hybrid metal halide perovskites(MHPs)have attracted tremendous attention for optoelectronic applications.The long photocarrier lifetime and moderate carrier mobility have been proposed as results of ... Organic-inorganic hybrid metal halide perovskites(MHPs)have attracted tremendous attention for optoelectronic applications.The long photocarrier lifetime and moderate carrier mobility have been proposed as results of the large polaron formation in MHPs.However,it is challenging to measure the effective mass and carrier scattering parameters of the photogenerated large polarons in the ultrafast carrier recombination dynamics.Here,we show,in a one-step spectroscopic method,that the optical-pump and terahertz-electromagnetic probe(OPTP)technique allows us to access the nature of interplay of photoexcited unbound charge carriers and optical phonons in polycrystalline CH_(3)NH_(3)PbI_(3)(MAPbI_(3))of about 10μm grain size.Firstly,we demonstrate a direct spectral evidence of the large polarons in polycrystalline MAPbI_(3).Using the Drude-Smith-Lorentz model along with the Frӧhlich-type electron-phonon(e-ph)coupling,we determine the effective mass and scattering parameters of photogenerated polaronic carriers.We discover that the resulting moderate polaronic carrier mobility is mainly influenced by the enhanced carrier scattering,rather than the polaron mass enhancement.While,the formation of large polarons in MAPbI_(3)polycrystalline grains results in a long charge carrier lifetime at room temperature.Our results provide crucial information about the photo-physics of MAPbI3 and are indispensable for optoelectronic device development with better performance. 展开更多
关键词 POLARON PEROVSKITE INORGANIC
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Cenozoic tectonic and sedimentary evolution of southern Qaidam Basin, NE Tibetan Plateau and its implication for the rejuvenation of Eastern Kunlun Mountains 被引量:8
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作者 MAO LiGuang XIAO AnCheng +5 位作者 WU Lei LI BenLiang WANG LiQun LOU QianQian DONG YouPu QIN SuHua 《Science China Earth Sciences》 SCIE EI CAS 2014年第11期2726-2739,共14页
The Eastern Kunlun Mountains play an important role in the growth and eastward extrusion of the Tibetan Plateau. Tectonic and sedimentary study of the Cenozoic Qaidam Basin, especially the southern part, provides key ... The Eastern Kunlun Mountains play an important role in the growth and eastward extrusion of the Tibetan Plateau. Tectonic and sedimentary study of the Cenozoic Qaidam Basin, especially the southern part, provides key evidence for understanding their evolution. Here we present evidence including isopach maps, seismic sections and sedimentary analysis of single well to illustrate the sedimentary development of the basin and the structural features of its southern margin. The Qaidam Basin extended across Qiman Tagh-Eastern Kunlun Mountains in the early Cenozoic and withdrew northward at ca. 35.5 Ma, and then buckled as an EW striking elliptical depression since ca. 14.9 Ma, with the main depocenter migrating eastward. Our results support the view that the Kumukol and Hoh Xil basins joined the Qaidam Basin in the early Cenozoic time and we propose the Eastern Kunlun Mountains uplifted in the mid-Miocene. 展开更多
关键词 NE Tibetan Plateau Qaidam Basin Eastern Kunlun CENOZOIC mid-Miocene
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基于机器学习的氮掺杂石墨炔力学性能预测 被引量:1
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作者 张存 杨博林 +1 位作者 彭志龙 陈少华 《Science China Materials》 SCIE EI CAS CSCD 2024年第4期1129-1139,共11页
氮掺杂γ-石墨二炔(N-GDY)因其在能源、电子元器件和催化领域具有重要应用前景而备受关注.研究表明,N-GDY在不同的氮掺杂情况下会表现出迥异的物理化学性质.由于氮掺杂的多样性,N-GDY的理论及应用研究受到了极大的限制.鉴于此,本文采用... 氮掺杂γ-石墨二炔(N-GDY)因其在能源、电子元器件和催化领域具有重要应用前景而备受关注.研究表明,N-GDY在不同的氮掺杂情况下会表现出迥异的物理化学性质.由于氮掺杂的多样性,N-GDY的理论及应用研究受到了极大的限制.鉴于此,本文采用鄂维南等人提出的DeepMD方法训练得到了具有第一性原理精度、适用于N-GDY的机器学习势.利用该机器学习势,系统研究了氮掺杂模式对N-GDY力学性能的影响.研究发现,氮原子掺杂会导致N-GDY的抗拉强度降低.在单个碳链上掺杂氮原子时,N-GDY的抗拉强度随着氮原子掺杂位点到苯环的距离变小而减弱.相邻碳链氮原子共掺杂能够使N-GDY表现出更强的各向异性力学特征.本文研究结果对N-GDY在能源存储和柔性设备等领域的潜在应用提供了理论支持,同时也表明了机器学习势在从大规模数据集中学习并预测碳纳米材料复杂力学性质方面的潜力,为纳米材料设计及工程应用具有重要指导作用. 展开更多
关键词 机器学习 力学性能预测 氮掺杂 碳纳米材料 能源存储 力学特征 第一性原理 电子元器件
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Quantitatively mapping local quality of super-resolution microscopy by rolling Fourier ring correlation 被引量:3
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作者 Weisong Zhao Xiaoshuai Huang +14 位作者 Jianyu Yang Liying Qu Guohua Qiu Yue Zhao Xinwei Wang Deer Su Xumin Ding Heng Mao Yaming Jiu Ying Hu Jiubin Tan Shiqun Zhao Leiting Pan Liangyi Chen Haoyu Li 《Light(Science & Applications)》 SCIE EI CSCD 2023年第12期2826-2844,共19页
In fluorescence microscopy,computational algorithms have been developed to suppress noise,enhance contrast,and even enable super-resolution(SR).However,the local quality of the images may vary on multiple scales,and t... In fluorescence microscopy,computational algorithms have been developed to suppress noise,enhance contrast,and even enable super-resolution(SR).However,the local quality of the images may vary on multiple scales,and these differences can lead to misconceptions.Current mapping methods fail to finely estimate the local quality,challenging to associate the SR scale content.Here,we develop a rolling Fourier ring correlation(rFRC)method to evaluate the reconstruction uncertainties down to SR scale.To visually pinpoint regions with low reliability,a filtered rFRC is combined with a modified resolution-scaled error map(RSM),offering a comprehensive and concise map for further examination.We demonstrate their performances on various SR imaging modalities,and the resulting quantitative maps enable better SR images integrated from different reconstructions.Overall,we expect that our framework can become a routinely used tool for biologists in assessing their image datasets in general and inspire further advances in the rapidly developing field of computational imaging. 展开更多
关键词 RESOLUTION LOCAL enable
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