南海南部低海平面时期巽他陆架陆源碎屑的物源区变化,对于研究海陆变迁过程古环境演化具有重要意义.选择巽他陆架外缘对海平面变化影响非常敏感的氧同位素3期岩心记录(18282-2孔),开展高分辨率陆源碎屑粘土矿物分析,以期获得海平面变化...南海南部低海平面时期巽他陆架陆源碎屑的物源区变化,对于研究海陆变迁过程古环境演化具有重要意义.选择巽他陆架外缘对海平面变化影响非常敏感的氧同位素3期岩心记录(18282-2孔),开展高分辨率陆源碎屑粘土矿物分析,以期获得海平面变化影响下的物源区演化历史.研究结果显示,在氧同位素3期44.5~36.0 cal ka BP期间,巽他陆架外缘含有较高的蒙脱石(29%~44%)与中等含量的高岭石(21%~27%)、伊利石(19%~27%)和绿泥石(14%~20%).物源区分析表明,这个时期的蒙脱石主要由苏门答腊岛和泰国中部河流提供,高岭石主要由马来半岛、苏门答腊岛和婆罗洲西部河流提供,而伊利石和绿泥石主要由湄公河提供.在此期间,海平面长时间位于-80 m以下,巽他出露陆架上发育的大型古河流(北巽他河、古昭披耶河及古湄公河)可将来自周边物源区的陆源碎屑物质直接输送到陆架外缘.研究岩心的蒙脱石/(伊利石+绿泥石)比值与海平面变化具有良好的对应关系:当海平面下降时,蒙脱石/(伊利石+绿泥石)比值增大;反之亦然.这一现象表明海平面变化是影响巽他陆架外缘氧同位素3期沉积环境演化的最重要因素,即海平面升降引起的海陆格局变化,特别是古岸线的迁移可显著影响古河流与研究站位间的搬运距离,从而导致周边物源区对陆架外缘的陆源碎屑物质相对贡献量发生变化.展开更多
The compositions of grain size,clay minerals,and geochemical elements in core sediments(TS4)from the southwestern Taiwan Basin(South China Sea)were investigated to assess the response of terrigenous sediment input to ...The compositions of grain size,clay minerals,and geochemical elements in core sediments(TS4)from the southwestern Taiwan Basin(South China Sea)were investigated to assess the response of terrigenous sediment input to sea level change and the East Asian monsoon evolution since 30 kyr.The chronology was discussed based on foraminiferal AMS14C dates.Our results indi-cated that rivers in Taiwan have been the major sediment contributors since 30 kyr,followed by the Pearl River;and Luzon Island contribute little sediments to the southwestern Taiwan Basin.In this study,we reconstructed the variations in terrigenous sediment input by using the proxies such as Al2O_(3)(%),F1 score,and TiO_(2)/CaO.The F1 score can be used to indicate the flux of terrigenous sediments.The contribution of Taiwan Residents rivers and the Pearl River were evaluated by using the value of(illite+chlorite)/kaolinite.The variations of Al2O_(3)(%),F1 score,and TiO_(2)/CaO values along the core were clearly correlated to the evolution of the East Asian summer monsoon since 30 kyr.Based on these records,we recognized three evolutionary stages of terrigenous sediment input in the southwestern Taiwan Basin.During stage Ⅰ(29-24kyr),the input of terrigenous sediments continued to increase.During stage Ⅱ(24-11.5 kyr),the sediment input decreased at first and then increased,with the lowest value during the last glacial period(21-17kyr).Terrigenous sediment input during stage Ⅲ(11.5 kyr-)showed the decreasing first and then increasing trends,generally higher than those in the first and second stages.The variations of terrigenous sediment input in the study area corresponded well with the evolu-tion of the East Asian summer monsoon since 30 kyr.Increased terrigenous sediment input during 4-1.8 kyr was suggested to be caused by the enhanced ENSO activity.Sea level change does not alter the overall trend of terrigenous sediment input,but does change the relative contributions of rivers in Taiwan and the Pearl River.展开更多
The area of East China Sea(ECS)inner shelf is an important sink of suspended particulates from Yangtze River(YR)and materials originated from YR basin.In this study,the parameters of lignin and alkane biomarkers in su...The area of East China Sea(ECS)inner shelf is an important sink of suspended particulates from Yangtze River(YR)and materials originated from YR basin.In this study,the parameters of lignin and alkane biomarkers in surface sediment samples from ECS inner shelf were determined to distinguish the sources and to trace the transport of terrigenous organic matters in the region.Our dataset showed that total alkanes with carbon numbers from 10 to 38(T-alkanes)were significantly correlated to both TAR(terrigenous/aquatic ratio)and HMW/LMW(the ratio of high molecular weight to low molecular weight alkanes)(r=0.88,P<0.05 for both),indicating that the majority of T-alkanes was predominantly originated from terrestrial sources,and T-alkanes are important constituents of terrestrial organic matters in the study area.The area was probably affected by petroleum pollution to a certain degree,as indicated by the values of carbon preference index(CPI),odd-over-even carbon number predominance(OEP)and the ratio of pristane to phytane(Pr/Ph).The values of Pr/n-C_(17) and Ph/n-C_(18) suggested a strong reductive sedimentary condition in the region with no obvious biodegradation.The content of eight lignin phenols(Σ8)decreased from the coast to the open sea,indicative of riverine input and hydrodynamic transport of terrigenous organic matters.Lignin degradation parameters presented an increasing trend from the coastline toward the open sea.The lignin vegetation parameters and alkane index(AI)suggested the predominance of non-woody angiosperms in the YR basin.The obvious correlation betweenΛ8(Σ8 normalized to 100 mg organic carbon),TAR and HMW/LMW reveals the significantly concurrent input of lignin and alkanes from terrestrial sources.展开更多
文摘南海南部低海平面时期巽他陆架陆源碎屑的物源区变化,对于研究海陆变迁过程古环境演化具有重要意义.选择巽他陆架外缘对海平面变化影响非常敏感的氧同位素3期岩心记录(18282-2孔),开展高分辨率陆源碎屑粘土矿物分析,以期获得海平面变化影响下的物源区演化历史.研究结果显示,在氧同位素3期44.5~36.0 cal ka BP期间,巽他陆架外缘含有较高的蒙脱石(29%~44%)与中等含量的高岭石(21%~27%)、伊利石(19%~27%)和绿泥石(14%~20%).物源区分析表明,这个时期的蒙脱石主要由苏门答腊岛和泰国中部河流提供,高岭石主要由马来半岛、苏门答腊岛和婆罗洲西部河流提供,而伊利石和绿泥石主要由湄公河提供.在此期间,海平面长时间位于-80 m以下,巽他出露陆架上发育的大型古河流(北巽他河、古昭披耶河及古湄公河)可将来自周边物源区的陆源碎屑物质直接输送到陆架外缘.研究岩心的蒙脱石/(伊利石+绿泥石)比值与海平面变化具有良好的对应关系:当海平面下降时,蒙脱石/(伊利石+绿泥石)比值增大;反之亦然.这一现象表明海平面变化是影响巽他陆架外缘氧同位素3期沉积环境演化的最重要因素,即海平面升降引起的海陆格局变化,特别是古岸线的迁移可显著影响古河流与研究站位间的搬运距离,从而导致周边物源区对陆架外缘的陆源碎屑物质相对贡献量发生变化.
基金This study was financially supported by the National Key Research and Development Program(No.2017YFC 0306703)the National Natural Science Foundation of China(No.41706065).
文摘The compositions of grain size,clay minerals,and geochemical elements in core sediments(TS4)from the southwestern Taiwan Basin(South China Sea)were investigated to assess the response of terrigenous sediment input to sea level change and the East Asian monsoon evolution since 30 kyr.The chronology was discussed based on foraminiferal AMS14C dates.Our results indi-cated that rivers in Taiwan have been the major sediment contributors since 30 kyr,followed by the Pearl River;and Luzon Island contribute little sediments to the southwestern Taiwan Basin.In this study,we reconstructed the variations in terrigenous sediment input by using the proxies such as Al2O_(3)(%),F1 score,and TiO_(2)/CaO.The F1 score can be used to indicate the flux of terrigenous sediments.The contribution of Taiwan Residents rivers and the Pearl River were evaluated by using the value of(illite+chlorite)/kaolinite.The variations of Al2O_(3)(%),F1 score,and TiO_(2)/CaO values along the core were clearly correlated to the evolution of the East Asian summer monsoon since 30 kyr.Based on these records,we recognized three evolutionary stages of terrigenous sediment input in the southwestern Taiwan Basin.During stage Ⅰ(29-24kyr),the input of terrigenous sediments continued to increase.During stage Ⅱ(24-11.5 kyr),the sediment input decreased at first and then increased,with the lowest value during the last glacial period(21-17kyr).Terrigenous sediment input during stage Ⅲ(11.5 kyr-)showed the decreasing first and then increasing trends,generally higher than those in the first and second stages.The variations of terrigenous sediment input in the study area corresponded well with the evolu-tion of the East Asian summer monsoon since 30 kyr.Increased terrigenous sediment input during 4-1.8 kyr was suggested to be caused by the enhanced ENSO activity.Sea level change does not alter the overall trend of terrigenous sediment input,but does change the relative contributions of rivers in Taiwan and the Pearl River.
基金This study was financially supported by the National Natural Science Foundation of China(Nos.41276067,41020164005)the National Basic Research Program of China(973 Program,No.2010CB428901).
文摘The area of East China Sea(ECS)inner shelf is an important sink of suspended particulates from Yangtze River(YR)and materials originated from YR basin.In this study,the parameters of lignin and alkane biomarkers in surface sediment samples from ECS inner shelf were determined to distinguish the sources and to trace the transport of terrigenous organic matters in the region.Our dataset showed that total alkanes with carbon numbers from 10 to 38(T-alkanes)were significantly correlated to both TAR(terrigenous/aquatic ratio)and HMW/LMW(the ratio of high molecular weight to low molecular weight alkanes)(r=0.88,P<0.05 for both),indicating that the majority of T-alkanes was predominantly originated from terrestrial sources,and T-alkanes are important constituents of terrestrial organic matters in the study area.The area was probably affected by petroleum pollution to a certain degree,as indicated by the values of carbon preference index(CPI),odd-over-even carbon number predominance(OEP)and the ratio of pristane to phytane(Pr/Ph).The values of Pr/n-C_(17) and Ph/n-C_(18) suggested a strong reductive sedimentary condition in the region with no obvious biodegradation.The content of eight lignin phenols(Σ8)decreased from the coast to the open sea,indicative of riverine input and hydrodynamic transport of terrigenous organic matters.Lignin degradation parameters presented an increasing trend from the coastline toward the open sea.The lignin vegetation parameters and alkane index(AI)suggested the predominance of non-woody angiosperms in the YR basin.The obvious correlation betweenΛ8(Σ8 normalized to 100 mg organic carbon),TAR and HMW/LMW reveals the significantly concurrent input of lignin and alkanes from terrestrial sources.
