Night-time OH levels have been determined for UK urban surface environments using two methods, the decay and steady state approximation methods. Measurement data from the UK National Environmental Technology Centre ar...Night-time OH levels have been determined for UK urban surface environments using two methods, the decay and steady state approximation methods. Measurement data from the UK National Environmental Technology Centre archive for four urban sites （Bristol, Harwell, London Eltham and Edinburgh） over the time period of 1996 to 2000 have been used in this study. Three reactive alkenes, namely isoprene, 1,3-butadiene and trans-2-pentene were chosen for the calculation of OH levels by the decay method. Hourly measurements of NO, NO〉 03, CO and 20 VOCs were used to determine night-time OH level using the steady state approximation method. Our results showed that the night-time OH levels were in the range of 1 × 10^3-1× 10^6 molecules/cm3 at these four urbap sites in the UK. The application of a t-test of these analyses indicated that except Bristol, there was no significant difference between the OH levels found from the decay and steady state approximation methods. Night-time levels of the OH radical appeared to peak in summer and spring time tracking the night-time 03 levels which also passed through a maximum at this time.展开更多
In this paper, we study a space-fractional anomalous diffusion in a variable area. The moving boundary is assumed moving with constant speed. The numerical scheme was present by changing the moving boundary to a fixed...In this paper, we study a space-fractional anomalous diffusion in a variable area. The moving boundary is assumed moving with constant speed. The numerical scheme was present by changing the moving boundary to a fixed one. The steady-state approximation was also given to show the properties of the diffusion process.展开更多
基金supported by the National Key R&D Program of China (2022YFE0102000)the National Natural Science Foundation of China (22121004 and U22A20409)+1 种基金Haihe Laboratory of Sustainable Chemical Transformations, the Program of Introducing Talents of Discipline to Universities (BP0618007)the XPLORER PRIZE for financial support。
文摘Night-time OH levels have been determined for UK urban surface environments using two methods, the decay and steady state approximation methods. Measurement data from the UK National Environmental Technology Centre archive for four urban sites （Bristol, Harwell, London Eltham and Edinburgh） over the time period of 1996 to 2000 have been used in this study. Three reactive alkenes, namely isoprene, 1,3-butadiene and trans-2-pentene were chosen for the calculation of OH levels by the decay method. Hourly measurements of NO, NO〉 03, CO and 20 VOCs were used to determine night-time OH level using the steady state approximation method. Our results showed that the night-time OH levels were in the range of 1 × 10^3-1× 10^6 molecules/cm3 at these four urbap sites in the UK. The application of a t-test of these analyses indicated that except Bristol, there was no significant difference between the OH levels found from the decay and steady state approximation methods. Night-time levels of the OH radical appeared to peak in summer and spring time tracking the night-time 03 levels which also passed through a maximum at this time.
文摘In this paper, we study a space-fractional anomalous diffusion in a variable area. The moving boundary is assumed moving with constant speed. The numerical scheme was present by changing the moving boundary to a fixed one. The steady-state approximation was also given to show the properties of the diffusion process.
