The coupled-channels optical method for positron scattering has been applied to investigate resonance states with unnatural parities in a positron-excited hydrogen system. The positronium formation channels and contin...The coupled-channels optical method for positron scattering has been applied to investigate resonance states with unnatural parities in a positron-excited hydrogen system. The positronium formation channels and continuum channel are included via a complex equivalent local potential. Resonance states with angular momenta L =- 1 to L = 2 and parities (-1)L+1 are calculated. Resonance energies and widths are reported and compared with other theoretical calculations. We found that the opening positronium formation channels play an important role in forming nondipole Feshbach resonances.展开更多
The effect of carbon black (CB) and graphite (G) powders on the macroscopic and nano-scale free volume properties of silicone rubber based on poly(di-methylsiloxane) (PDMS) was studied through thermal and cycl...The effect of carbon black (CB) and graphite (G) powders on the macroscopic and nano-scale free volume properties of silicone rubber based on poly(di-methylsiloxane) (PDMS) was studied through thermal and cyclic mechanical measurements, as well as with positron annihilation lifetime spectroscopy (PALS). The melting temperature of the composites (Tm) and the endothermic enthalpy of melting (ΔHm) were estimated by differential scanning calorimetry (DSC). Tm and the degree of crystallinity (χc) of PDMS composites were found to decrease with increasing the CB content. This can be explained due to the increase in physical cross-linking which results in a decrease in the crystallite thickness. Besides, χc was found to be dependent on the filler type. Cyclic stress-strain behavior of PDMS loaded with different contents of filler has been studied. Mullins ratio (RM) was found to be dependent on the filler type and content. It was found that, RM increases with increasing the filler content due to the increase in physical cross-linking which results in a decrease in the size of free volume, as observed through a decrease of the o-Ps lifetime τ3 measured by PALS. Moreover, the hysteresis in PDMS-CB composites was more pronounced than in PDMS-G composites. Furthermore, a correlation was established between the free volume Vf and the mechanical properties of PDMS composites containing different fillers. A negative correlation was observed between Vf and RM.展开更多
Positron scattering with atomic lithium is investigated by using a coupled-channel optical method.The ionization continuum and positronium formation channels are taken into account via a complex equivalent-local optic...Positron scattering with atomic lithium is investigated by using a coupled-channel optical method.The ionization continuum and positronium formation channels are taken into account via a complex equivalent-local optical potential.The positronium formation cross sections and the ionization cross sections,as well as the total scattering cross sections,are reported at energies above 3 eV and compared with available experimental and theoretical data.展开更多
An attempt to predict the new atomic dark matter lines is done on the example of a dark lepton atom-positronium. Its Layman-alpha line with the energy near 3 GeV may be observable if the appropriate conditions are rea...An attempt to predict the new atomic dark matter lines is done on the example of a dark lepton atom-positronium. Its Layman-alpha line with the energy near 3 GeV may be observable if the appropriate conditions are realized. For this we have studied a γ-ray excess in the center of our galaxy. In principle, this excess may be produced by the Lα line of a dark positronium in the medium with Compton scattering. The possibility of observations of an annihilation line (E^300 TeV) of dark positronium is also predicted. Other proposals to observe the atomic dark matter are shortly described. Besides, Hα line (1.3μ) of usual positronum must be observable in the direction on the center of our galaxy.展开更多
Positron lifetime measurements have been made in natural polymer-Nistari silk fibers as a function of isochronalannealing temperature in the range of 27℃ to 280℃. The variations in the positron results indicate the ...Positron lifetime measurements have been made in natural polymer-Nistari silk fibers as a function of isochronalannealing temperature in the range of 27℃ to 280℃. The variations in the positron results indicate the structural changesoccurring in the Nistari silk fibers and determine the glass transition temperature as 170℃. Activation energies weremeasured separately for the crystalline and amorphous regions indicating the versatility of the technique. These values areclose to the N--H bond dissociation energy, suggesting N--H bond dissociation as the most probable process occurringduring thermal treatment As an extension of the positron results, the molecular weight of the Nistari silk fibers wasdetermined to be 10.7×10~5 based on free volume, which lies within the range suggested for the silk fibers. There seems to bean indication that cross-linking changes the spiral structure of cotton fibers to network type. However, this needs to be validated by other techniques.展开更多
Positronium time of flight spectroscopy(Ps-TOF)is an effective technique for porous material research.It has advantages over other techniques for analyzing the porosity and pore tortuosity of materials.This paper de...Positronium time of flight spectroscopy(Ps-TOF)is an effective technique for porous material research.It has advantages over other techniques for analyzing the porosity and pore tortuosity of materials.This paper describes a design for Ps-TOF apparatus based on the Beijing intense slow positron beam,supplying a new material characterization technique.In order to improve the time resolution and increase the count rate of the apparatus,the detector system is optimized.For 3 eV o-Ps,the time broadening is 7.66 ns and the count rate is 3 cps after correction.展开更多
The results of a series of experiments on 3-photon annihilation of positrons and electrons, including the energy-angular correlation, angular distribution, energy spectrum and linear polarization of the annihilation p...The results of a series of experiments on 3-photon annihilation of positrons and electrons, including the energy-angular correlation, angular distribution, energy spectrum and linear polarization of the annihilation photons, the method of measuring the intensities of 3-photon annihilation, and the upper limit of axion production in the triplet positronium decay, are reported.展开更多
The inelastic scattering of positrons by excited lithium alkali atoms Li*(2p) have been investigated within the frame work of the coupled-static and frozen-core approximations with the assumption that the elastic and ...The inelastic scattering of positrons by excited lithium alkali atoms Li*(2p) have been investigated within the frame work of the coupled-static and frozen-core approximations with the assumption that the elastic and rearrangement channels are open. In the present work, a rather complicated computer code is developed based on the coupled-static, frozen-core and Green’s function partial wave expansion technique. The partial and total elastic and positronium (Ps) formation cross sections of e+-Li*(2p) are calculated through a wide range of incident energy of positrons ranging from 0.3 eV to 1000 eV. Also, we have calculated the partial and total elastic and rearrangement (reversal of the Ps formation) cross sections of Ps-Li+ collisions through the low, intermediate and high energy regions. The effect of polarization potential of the Ps atom is taken into our consideration. The total cross sections which corresponding to twelve partial cross sections (calculated at twelve values of the total angular momentum l = 0 to l = 11) are calculated for each channel. Our calculated total positronium formation cross sections are compared with experimental results and those calculated by other authors. The present calculations encourage the experimental physicists to carry out positron-lithium experiments by taking the excited lithium target into accounts in order to obtain more positronium especially in the low and intermediate energy regions.展开更多
Formed in silica aerogels, positronium annihilation in oxygen and nitrogen mixture is studied by a simple and convenient method. The results show that ortho-positronium (o-Ps) lifetime is significantly shortened whe...Formed in silica aerogels, positronium annihilation in oxygen and nitrogen mixture is studied by a simple and convenient method. The results show that ortho-positronium (o-Ps) lifetime is significantly shortened when some oxygen is introduced into ni- trogen gas and that the o-Ps collisional quenching rate for an oxy- gen molecule is (28.0±0.4) ±ts%amagat(1 amagat 2.69± 1025 m-3). It is found that the o-Ps annihilation rate in oxygen of latin at room temperature is (25.5±0.5) us-1 and that the effective num- ber of electrons per oxygen molecule available for 27 annihilation of positron in the o-Ps is (34.6±0.4).展开更多
A high-performance positron age-momentum correlation (AMOC) spectrometer was newly developed. The counting rate is increased up to 200 cps much larger than the value 20 cps reported by other international groups. An...A high-performance positron age-momentum correlation (AMOC) spectrometer was newly developed. The counting rate is increased up to 200 cps much larger than the value 20 cps reported by other international groups. And at the same time, the time resolution still keeps at the international level of 220 ps. Furthermore, positronium (Ps) annihilation in silica aerogel was investigated by AMOC, which indicates: (1) Ps annihilation between the grains dominantly undergoes pick-off process and spin conversion from o-Ps to p-Ps; (2) Annealing below 400 ℃ changes the grain surface conditions, i. e. the desorption of hydrogen and the decrease of the defect centers concentration.展开更多
I describe a method for the observation of Positronium (Ps) involvement in the solar radiation spectrum. In this method, Rydberg-Ritz’s principle and Planck’s radiation formula are used to acquire information of the...I describe a method for the observation of Positronium (Ps) involvement in the solar radiation spectrum. In this method, Rydberg-Ritz’s principle and Planck’s radiation formula are used to acquire information of the atomic transitions of Ps alike Hydrogen and Helium. In order to perform this experiment, an advanced solar spectrum monitor is constructed by utilizing light emitting diodes (LED) of various colors. A detailed study on this method provides qualitative agreement with experimental data, giving insight to the physical process involved in the solar radiation spectrum and confirming the existence of solar Ps.展开更多
Void nucleation and positronium formation are studied by positron annihilationlifetime technique in α-Al<sub>2</sub>O<sub>3</sub> irradiated by E<sub>n</sub>≥1 MeV fast neutrons t...Void nucleation and positronium formation are studied by positron annihilationlifetime technique in α-Al<sub>2</sub>O<sub>3</sub> irradiated by E<sub>n</sub>≥1 MeV fast neutrons to a fluence of 3×10<sup>20</sup> n/cm<sup>2</sup>.The voids of 0.7 nm are observed in the irradiated α-Al<sub>2</sub>O<sub>3</sub> after the post-irradiationannealing at 850℃ and the positronium is formed in the voids.展开更多
The momentum space coupled channels optical(CCO) method for positron scattering has been extended to study the scattering of positrons by metastable helium for impact energies in the range from the positronium thres...The momentum space coupled channels optical(CCO) method for positron scattering has been extended to study the scattering of positrons by metastable helium for impact energies in the range from the positronium threshold up to high energies. Both the positronium formation and ionization continuum channels are included in the calculations via a complex equivalent local potential. The positronium formation, ionization, elastic and 2~3S–2~3P excitation, and total scattering cross sections are all presented and compared with the available information.展开更多
Depth profiled positronium (Ps) annihilation lifetime spectroscopy (PALS) is an extremely useful probe of the pore characteristics in nanoporous low-dielectric (low-k) constant thin films. PALS has also been con...Depth profiled positronium (Ps) annihilation lifetime spectroscopy (PALS) is an extremely useful probe of the pore characteristics in nanoporous low-dielectric (low-k) constant thin films. PALS has also been considered as a potential probe to investigate diffusion barrier integrity and the structural changes of porous low-k films during their integration with Cu. Hence, it is essential to understand the diffusion behaviour of positronium/Cu atoms in the films. In this work, based on the fact that porous materials possess characteristics of statistical self-similarity, a fractal model, the Menger sponge model, has been applied to simulate the structure of a promising dielectric, porous methylsilsesquioxane (MSQ) films. The diffusion behaviour of Ps out of the fractal model and into the surrounding vacuum is studied by means of the diffusion equation and traditional adveetive diffusive theory. Predictive results from our model show good agreement with measurement data.展开更多
A brief survey is made to highlight the recent interests in positron, positronium and antimatter physics. Positron is the first antiparticle observed which was predicted by Dirac. Positronium is itself its antiparticl...A brief survey is made to highlight the recent interests in positron, positronium and antimatter physics. Positron is the first antiparticle observed which was predicted by Dirac. Positronium is itself its antiparticle and bi-positronium molecule is recently observed in laboratory which was predicted by Wheeler in 1946. The simplest antiatom i.e. antihydrogen is observed in the laboratory and the process to achieve the stable confinement of antihydrogen within the trap are in progress to test the standard model.展开更多
Taking the accurate values of γ energies of ^(192)Ir as a comparison standard, the mean values of the radiation energies of positron annihilation in silica aerogel with and without oxygen filled have been measured wi...Taking the accurate values of γ energies of ^(192)Ir as a comparison standard, the mean values of the radiation energies of positron annihilation in silica aerogel with and without oxygen filled have been measured witha high purity Ge γ spectrometer. The γ energy in parapositronium 2γ decay has been determined and the value of electron rest mass obtained, m_0c^2=510998.80±0.74 eV, which is in good agreement with the value recently adjusted within errors.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.10674055)
文摘The coupled-channels optical method for positron scattering has been applied to investigate resonance states with unnatural parities in a positron-excited hydrogen system. The positronium formation channels and continuum channel are included via a complex equivalent local potential. Resonance states with angular momenta L =- 1 to L = 2 and parities (-1)L+1 are calculated. Resonance energies and widths are reported and compared with other theoretical calculations. We found that the opening positronium formation channels play an important role in forming nondipole Feshbach resonances.
文摘The effect of carbon black (CB) and graphite (G) powders on the macroscopic and nano-scale free volume properties of silicone rubber based on poly(di-methylsiloxane) (PDMS) was studied through thermal and cyclic mechanical measurements, as well as with positron annihilation lifetime spectroscopy (PALS). The melting temperature of the composites (Tm) and the endothermic enthalpy of melting (ΔHm) were estimated by differential scanning calorimetry (DSC). Tm and the degree of crystallinity (χc) of PDMS composites were found to decrease with increasing the CB content. This can be explained due to the increase in physical cross-linking which results in a decrease in the crystallite thickness. Besides, χc was found to be dependent on the filler type. Cyclic stress-strain behavior of PDMS loaded with different contents of filler has been studied. Mullins ratio (RM) was found to be dependent on the filler type and content. It was found that, RM increases with increasing the filler content due to the increase in physical cross-linking which results in a decrease in the size of free volume, as observed through a decrease of the o-Ps lifetime τ3 measured by PALS. Moreover, the hysteresis in PDMS-CB composites was more pronounced than in PDMS-G composites. Furthermore, a correlation was established between the free volume Vf and the mechanical properties of PDMS composites containing different fillers. A negative correlation was observed between Vf and RM.
基金Project supported by National Natural Science Foundation of China (Grant No. 10674055)
文摘Positron scattering with atomic lithium is investigated by using a coupled-channel optical method.The ionization continuum and positronium formation channels are taken into account via a complex equivalent-local optical potential.The positronium formation cross sections and the ionization cross sections,as well as the total scattering cross sections,are reported at energies above 3 eV and compared with available experimental and theoretical data.
文摘An attempt to predict the new atomic dark matter lines is done on the example of a dark lepton atom-positronium. Its Layman-alpha line with the energy near 3 GeV may be observable if the appropriate conditions are realized. For this we have studied a γ-ray excess in the center of our galaxy. In principle, this excess may be produced by the Lα line of a dark positronium in the medium with Compton scattering. The possibility of observations of an annihilation line (E^300 TeV) of dark positronium is also predicted. Other proposals to observe the atomic dark matter are shortly described. Besides, Hα line (1.3μ) of usual positronum must be observable in the direction on the center of our galaxy.
文摘Positron lifetime measurements have been made in natural polymer-Nistari silk fibers as a function of isochronalannealing temperature in the range of 27℃ to 280℃. The variations in the positron results indicate the structural changesoccurring in the Nistari silk fibers and determine the glass transition temperature as 170℃. Activation energies weremeasured separately for the crystalline and amorphous regions indicating the versatility of the technique. These values areclose to the N--H bond dissociation energy, suggesting N--H bond dissociation as the most probable process occurringduring thermal treatment As an extension of the positron results, the molecular weight of the Nistari silk fibers wasdetermined to be 10.7×10~5 based on free volume, which lies within the range suggested for the silk fibers. There seems to bean indication that cross-linking changes the spiral structure of cotton fibers to network type. However, this needs to be validated by other techniques.
基金Supported by NSFC (10835006, 60606011, 10705031)
文摘Positronium time of flight spectroscopy(Ps-TOF)is an effective technique for porous material research.It has advantages over other techniques for analyzing the porosity and pore tortuosity of materials.This paper describes a design for Ps-TOF apparatus based on the Beijing intense slow positron beam,supplying a new material characterization technique.In order to improve the time resolution and increase the count rate of the apparatus,the detector system is optimized.For 3 eV o-Ps,the time broadening is 7.66 ns and the count rate is 3 cps after correction.
文摘The results of a series of experiments on 3-photon annihilation of positrons and electrons, including the energy-angular correlation, angular distribution, energy spectrum and linear polarization of the annihilation photons, the method of measuring the intensities of 3-photon annihilation, and the upper limit of axion production in the triplet positronium decay, are reported.
文摘The inelastic scattering of positrons by excited lithium alkali atoms Li*(2p) have been investigated within the frame work of the coupled-static and frozen-core approximations with the assumption that the elastic and rearrangement channels are open. In the present work, a rather complicated computer code is developed based on the coupled-static, frozen-core and Green’s function partial wave expansion technique. The partial and total elastic and positronium (Ps) formation cross sections of e+-Li*(2p) are calculated through a wide range of incident energy of positrons ranging from 0.3 eV to 1000 eV. Also, we have calculated the partial and total elastic and rearrangement (reversal of the Ps formation) cross sections of Ps-Li+ collisions through the low, intermediate and high energy regions. The effect of polarization potential of the Ps atom is taken into our consideration. The total cross sections which corresponding to twelve partial cross sections (calculated at twelve values of the total angular momentum l = 0 to l = 11) are calculated for each channel. Our calculated total positronium formation cross sections are compared with experimental results and those calculated by other authors. The present calculations encourage the experimental physicists to carry out positron-lithium experiments by taking the excited lithium target into accounts in order to obtain more positronium especially in the low and intermediate energy regions.
基金Supported by the National Natural Science Foundation of China(10975108and10974149)the Research Fund for the Doctoral Program of Higher Education of China(20090141120069)
文摘Formed in silica aerogels, positronium annihilation in oxygen and nitrogen mixture is studied by a simple and convenient method. The results show that ortho-positronium (o-Ps) lifetime is significantly shortened when some oxygen is introduced into ni- trogen gas and that the o-Ps collisional quenching rate for an oxy- gen molecule is (28.0±0.4) ±ts%amagat(1 amagat 2.69± 1025 m-3). It is found that the o-Ps annihilation rate in oxygen of latin at room temperature is (25.5±0.5) us-1 and that the effective num- ber of electrons per oxygen molecule available for 27 annihilation of positron in the o-Ps is (34.6±0.4).
基金Supported by NSFC (10575112, 10705031, 60606011)
文摘A high-performance positron age-momentum correlation (AMOC) spectrometer was newly developed. The counting rate is increased up to 200 cps much larger than the value 20 cps reported by other international groups. And at the same time, the time resolution still keeps at the international level of 220 ps. Furthermore, positronium (Ps) annihilation in silica aerogel was investigated by AMOC, which indicates: (1) Ps annihilation between the grains dominantly undergoes pick-off process and spin conversion from o-Ps to p-Ps; (2) Annealing below 400 ℃ changes the grain surface conditions, i. e. the desorption of hydrogen and the decrease of the defect centers concentration.
文摘I describe a method for the observation of Positronium (Ps) involvement in the solar radiation spectrum. In this method, Rydberg-Ritz’s principle and Planck’s radiation formula are used to acquire information of the atomic transitions of Ps alike Hydrogen and Helium. In order to perform this experiment, an advanced solar spectrum monitor is constructed by utilizing light emitting diodes (LED) of various colors. A detailed study on this method provides qualitative agreement with experimental data, giving insight to the physical process involved in the solar radiation spectrum and confirming the existence of solar Ps.
文摘Void nucleation and positronium formation are studied by positron annihilationlifetime technique in α-Al<sub>2</sub>O<sub>3</sub> irradiated by E<sub>n</sub>≥1 MeV fast neutrons to a fluence of 3×10<sup>20</sup> n/cm<sup>2</sup>.The voids of 0.7 nm are observed in the irradiated α-Al<sub>2</sub>O<sub>3</sub> after the post-irradiationannealing at 850℃ and the positronium is formed in the voids.
基金Project supported by the Natural Science Foundation of Heilongjiang Province of China(Grant No.12541160)
文摘The momentum space coupled channels optical(CCO) method for positron scattering has been extended to study the scattering of positrons by metastable helium for impact energies in the range from the positronium threshold up to high energies. Both the positronium formation and ionization continuum channels are included in the calculations via a complex equivalent local potential. The positronium formation, ionization, elastic and 2~3S–2~3P excitation, and total scattering cross sections are all presented and compared with the available information.
基金Project supported by the National Natural Science Foundation of China (Grant No. 60476011)
文摘Depth profiled positronium (Ps) annihilation lifetime spectroscopy (PALS) is an extremely useful probe of the pore characteristics in nanoporous low-dielectric (low-k) constant thin films. PALS has also been considered as a potential probe to investigate diffusion barrier integrity and the structural changes of porous low-k films during their integration with Cu. Hence, it is essential to understand the diffusion behaviour of positronium/Cu atoms in the films. In this work, based on the fact that porous materials possess characteristics of statistical self-similarity, a fractal model, the Menger sponge model, has been applied to simulate the structure of a promising dielectric, porous methylsilsesquioxane (MSQ) films. The diffusion behaviour of Ps out of the fractal model and into the surrounding vacuum is studied by means of the diffusion equation and traditional adveetive diffusive theory. Predictive results from our model show good agreement with measurement data.
文摘A brief survey is made to highlight the recent interests in positron, positronium and antimatter physics. Positron is the first antiparticle observed which was predicted by Dirac. Positronium is itself its antiparticle and bi-positronium molecule is recently observed in laboratory which was predicted by Wheeler in 1946. The simplest antiatom i.e. antihydrogen is observed in the laboratory and the process to achieve the stable confinement of antihydrogen within the trap are in progress to test the standard model.
基金Project supported by the National Natural Science Foundation of China.
文摘Taking the accurate values of γ energies of ^(192)Ir as a comparison standard, the mean values of the radiation energies of positron annihilation in silica aerogel with and without oxygen filled have been measured witha high purity Ge γ spectrometer. The γ energy in parapositronium 2γ decay has been determined and the value of electron rest mass obtained, m_0c^2=510998.80±0.74 eV, which is in good agreement with the value recently adjusted within errors.