Semiconductor perovskite films are now being widely investigated as light harvesters in solar cells with ever-increasing power conversion efficiencies,which have motivated the fabrication of other optoelectronic devic...Semiconductor perovskite films are now being widely investigated as light harvesters in solar cells with ever-increasing power conversion efficiencies,which have motivated the fabrication of other optoelectronic devices,such as light-emitting diodes,lasers,and photodetectors.Their superior material and optical properties are shared by the counterpart colloidal nanocrystals(NCs),with the additional advantage of quantum confinement that can yield size-dependent optical emission ranging from the near-UV to near-infrared wavelengths.So far,intensive research efforts have been devoted to the optical characterization of perovskite NC ensembles,revealing not only fundamental exciton relaxation and recombination dynamics but also lowthreshold amplified spontaneous emission and novel superfluorescence effects.Meanwhile,the application of single-particle spectroscopy techniques to perovskite NCs has helped to resolve a variety of optical properties for which there are few equivalents in traditional colloidal NCs,mainly including nonblinking photoluminescence,suppressed spectral diffusion,stable exciton fine structures,and coherent singlephoton emission.While the main purpose of ensemble optical studies is to guide the smooth development of perovskite NCs in classical optoelectronic applications,the rich observations from single-particle optical studies mark the emergence of a potential platform that can be exploited for quantum information technologies.展开更多
A significant step toward constructing high‐efficiency neuromorphic systems is the electronic emulation of advanced synaptic functions of the human brain.While previous studies have focused on mimicking the basic fun...A significant step toward constructing high‐efficiency neuromorphic systems is the electronic emulation of advanced synaptic functions of the human brain.While previous studies have focused on mimicking the basic functions of synapses using single‐gate transistors,multigate transistors offer an opportunity to simulate more complex and advanced memory‐forming behaviors in biological synapses.In this study,a simple and general method is used to assemble rubber semiconductors into suspended two‐phase composite films that are transferred to the surface of the ion‐conducting membrane to fabricate flexible multiterminal photoelectronic neurotransistors.The suspended ion conductive film is used as the gate dielectrics and supporting substrate.The prepared devices exhibit excellent electrical stability and mechanical flexibility after being bent.Basic photoelectronic synaptic behavior and pulse‐dependent plasticity are emulated.Furthermore,the device realizes the spatiotemporally integrated electrical and optical stimuli to mimic spatiotemporal information processing.This study provides a promising direction for constructing more complex spiking neural networks and more powerful neuromorphic systems with brain‐like dynamic spatiotemporal processing functions.展开更多
基金supported by the National Key R&D Program of China(Grant Nos.2019YFA0308700 and 2017YFA0303700)the National Natural Science Foundation of China(Grant Nos.61974058,11574147,and 11974164)the PAPD of Jiangsu Higher Education Institutions
文摘Semiconductor perovskite films are now being widely investigated as light harvesters in solar cells with ever-increasing power conversion efficiencies,which have motivated the fabrication of other optoelectronic devices,such as light-emitting diodes,lasers,and photodetectors.Their superior material and optical properties are shared by the counterpart colloidal nanocrystals(NCs),with the additional advantage of quantum confinement that can yield size-dependent optical emission ranging from the near-UV to near-infrared wavelengths.So far,intensive research efforts have been devoted to the optical characterization of perovskite NC ensembles,revealing not only fundamental exciton relaxation and recombination dynamics but also lowthreshold amplified spontaneous emission and novel superfluorescence effects.Meanwhile,the application of single-particle spectroscopy techniques to perovskite NCs has helped to resolve a variety of optical properties for which there are few equivalents in traditional colloidal NCs,mainly including nonblinking photoluminescence,suppressed spectral diffusion,stable exciton fine structures,and coherent singlephoton emission.While the main purpose of ensemble optical studies is to guide the smooth development of perovskite NCs in classical optoelectronic applications,the rich observations from single-particle optical studies mark the emergence of a potential platform that can be exploited for quantum information technologies.
基金supported by the National Natural Science Foundation of China(Nos.61975241 and 52173192)the Huxiang Youth Talent Program of Hunan Province(No.2020RC3010)+3 种基金the Science and Technology Innovation Program of Hunan Province(No.2020RC4004)the Special Funding for the Construction of Innovative Provinces in Hunan Province(No.2020GK2024)the National Key Research and Development Program of China(No.2017YFA0206600)Fundamental Research Funds for the Central Universities of Central South University(No.1053320213517).
文摘A significant step toward constructing high‐efficiency neuromorphic systems is the electronic emulation of advanced synaptic functions of the human brain.While previous studies have focused on mimicking the basic functions of synapses using single‐gate transistors,multigate transistors offer an opportunity to simulate more complex and advanced memory‐forming behaviors in biological synapses.In this study,a simple and general method is used to assemble rubber semiconductors into suspended two‐phase composite films that are transferred to the surface of the ion‐conducting membrane to fabricate flexible multiterminal photoelectronic neurotransistors.The suspended ion conductive film is used as the gate dielectrics and supporting substrate.The prepared devices exhibit excellent electrical stability and mechanical flexibility after being bent.Basic photoelectronic synaptic behavior and pulse‐dependent plasticity are emulated.Furthermore,the device realizes the spatiotemporally integrated electrical and optical stimuli to mimic spatiotemporal information processing.This study provides a promising direction for constructing more complex spiking neural networks and more powerful neuromorphic systems with brain‐like dynamic spatiotemporal processing functions.
