The two-dimensional steady-state discrete phase mathematical model is developed to analyze gas-particle flow and combustion characteristics of coal particles, as well as components concentration and temperature distri...The two-dimensional steady-state discrete phase mathematical model is developed to analyze gas-particle flow and combustion characteristics of coal particles, as well as components concentration and temperature distribu- tion of coal gas in the process of pulverized coal injection of blast furnace raceway. The results show that a great deal of coal gas discharges on the top of raceway away from the tuyere, and the residence time of coal particles in the re- gion of blowpipe and tuyere is 20 ms or so and 50 ms when it reaches raceway boundary. The pressure is the highest at the bottom of raceway and the maximal temperature is about 2 423 K. The char combustion is mainly carried out in the raceway and the maximum of char burn-out rate attains 3× 10-4 kg/s.展开更多
To better understand the characteristics and transformation mechanisms of secondary inorganic aerosols,hourly mass concentrations of water-soluble inorganic ions(WSIIs)in PM_(2.5)and their gaseous precursors were meas...To better understand the characteristics and transformation mechanisms of secondary inorganic aerosols,hourly mass concentrations of water-soluble inorganic ions(WSIIs)in PM_(2.5)and their gaseous precursors were measured online from 2016 to 2018 at an urban site in Beijing.Seasonal and diurnal variations in water-soluble ions and gaseous precursors were discussed and their gas-particle conversion and partitioning were also examined,some related parameters were characterized.The(TNH_(3))Rich was also defined to describe the variations of the excess NH_(3)in different seasons.In addition,a sensitivity test was carried out by using ISORROPIA II to outline the driving factors of gas-particle partitioning.In Beijing,the relative contribution of nitrate to PM_(2.5)has increased markedly in recent years,especially under polluted conditions.In the four seasons,only a small portion of NO_(2)in the atmosphere was converted into total nitrate(TNO_(3)),and more than 80%of TNO_(3)occurred in the form of nitrate due to the abundant ammonia.The concentration of total ammonia(TNH_(3))was much higher than that required to neutralize acid gases,and most of the TNH_(3)occurred as gaseous NH_(3).The nitrous acid(HONO)concentration was highly correlated with NH_(3)concentration and had increased significantly in Beijing compared with previous studies.The total chloride(TCl)was the highest in winter,andε(Cl^(-))was more sensitive to variations in the ambient temperature(T)and relative humidity(RH)thanε(NO_(3)^(-)).展开更多
Based on a kinetic energy equation of particle turbulence, a k-ε-kk model for turbulent gas-particle flows is proposed. The prediction of confined plane gas-particle jets shows a good agreement with experimental data...Based on a kinetic energy equation of particle turbulence, a k-ε-kk model for turbulent gas-particle flows is proposed. The prediction of confined plane gas-particle jets shows a good agreement with experimental data. This model is proved to be far superior to the presently used k-ε-A.P. model based on the algebraic model of particle turbulence.展开更多
Particle-laden gas flows past a circular cylinder at the Reynolds number of 2×10^(5) were numerically investigated. The Discrete Vortex Method (DVM) was employed to evaluate the unsteady gas flow fields and a Lag...Particle-laden gas flows past a circular cylinder at the Reynolds number of 2×10^(5) were numerically investigated. The Discrete Vortex Method (DVM) was employed to evaluate the unsteady gas flow fields and a Lagrangian approach was applied for tracking individual solid particles. The vortex patterns and the distributions of particles with different Stokes numbers were obtained. Numerical results show that: (1) at small Stokes number (St=0.01) the particles move with the fluid and could be found evenly throughout the flow, (2) the regions around the vortex cores, where few particles exist, become wider as the stokes number of particles increases from 0.01 to 1.0, (3) at middle Stokes number (St=1.0, 10) centrifugal forces throw the particles out of the wake vortices, (4) at high Stokes number (St=100, 1000) the particles are not affected by the vortices,and their motion is determined by their inertia effects.展开更多
A two-scale second-order moment two-phase turbulence model was developed and used to simulate gas-particle flow in a sudden-expansion chamber and a channel. The simulation results were in agreement with the experiment...A two-scale second-order moment two-phase turbulence model was developed and used to simulate gas-particle flow in a sudden-expansion chamber and a channel. The simulation results were in agreement with the experimental results, and the results were compared with those of the single-scale second-order moment two-phase turbulence model. Several improved features show that the two-scale model is to a certain extent better than the single-scale model, which may be attributed to the fact that particle turbulence is well characterized by the two-scale turbulence model.展开更多
Polychlorinated biphenyls （PCBs） were measured in atmospheric samples collected from the North Pacific to the Arctic Ocean between July and September 2012 to study the atmospheric concentration characteris-tics of P...Polychlorinated biphenyls （PCBs） were measured in atmospheric samples collected from the North Pacific to the Arctic Ocean between July and September 2012 to study the atmospheric concentration characteris-tics of PCBs and their gas/particle partitioning. The mean concentration of 26 PCBs （vapor plus particulate phase） （∑PCBs） was 19.116 pg/m^3with a standard deviation of 13.833 pg/m^3. Three most abundant conge-ners were CB-28, -52 and -77, accounting for 43.0% to∑PCBs. The predominance of vapor PCBs （79.0% to∑PCBs） in the atmosphere was observed.∑PCBs were negative correlated with the latitudes and inverse of the absolute temperature （1/T）. The significant correlation for most congeners was also observed between the logarithm of gas/particle partition coefficient （logKp） and 1/T. Shallower slopes （from ∑0.15 to ∑0.46, average ∑0.27） were measured from the regression of the logarithm of sub-cooled liquid vapor pressures （logpoL） and logKP for all samples. The difference of the slopes and intercepts among samples was insignifi-cant （p〉0.1）, implying adsorption and/or absorption processes and the aerosol composition did not differ significantly among different samples. By comparing three models, the J-P adsorption model, the octanol/air partition coefficient （KOA） based model and the soot-air model, the gas/particle partitioning of PCBs in the Arctic atmosphere was simulated more precisely by the soot-air model, and the adsorption onto el-emental carbon is more sensitive than the absorption into organic matters of aerosols, especially for low-chlorinated PCB congeners.展开更多
A two-fluid particle-wall collision model with consideration of wall roughness is pro- posed.It takes into account the effects of the friction,restitution and in particular the wall roughness, and hence the redistribu...A two-fluid particle-wall collision model with consideration of wall roughness is pro- posed.It takes into account the effects of the friction,restitution and in particular the wall roughness, and hence the redistribution of Reynolds stress in different directions,the absorption of turbulent en- ergy from the mean motion and the attenuation of particle motion by the wall.The proposed model is used to simulate sudden-expansion and swirling gas-particle flows and is validated by comparing with experimental results.The results show that the proposed model gives better results than those obtained by the presently used zero-gradient condition.Hence,it is suggested that the proposed model should be used as the wall boundary condition for the particle phase in place of the presently used boundary condition.展开更多
A two-scale second-order moment two-phase turbulence model accounting for inter-particle collision is developed, based on the concepts of particle large-scale fluctuation due to turbulence and particle small-scale flu...A two-scale second-order moment two-phase turbulence model accounting for inter-particle collision is developed, based on the concepts of particle large-scale fluctuation due to turbulence and particle small-scale fluctuation due to collision and through a unified treatment of these two kinds of fluctuations. The proposed model is used to simulate gas-particle flows in a channel and in a downer. Simulation results are in agreement with the experimental results reported in references and are near the results obtained using the sin- gle-scale second-order moment two-phase turbulence model superposed with a particle collision model （USM-θ model） in most regions.展开更多
A semi-empirical turbulence enhancement model accounting for the particle-wake effect was incorporated into the second-order moment two-phase turbulence model and employed to simulate gas-particle flows in a swirling ...A semi-empirical turbulence enhancement model accounting for the particle-wake effect was incorporated into the second-order moment two-phase turbulence model and employed to simulate gas-particle flows in a swirling sudden-expansion chamber. The simulated results for two-phases mean velocities and fluctuation velocities coincide well with the experiment ones, which demonstrates that this model, in comparison with the turbulence model not accounting for the wake effect, leads to higher calculating accuracy.展开更多
A particle nonlinear two-scale kp-εp turbulence model is proposed for simulating the anisotropic turbulent two-phase flow. The particle kinetic energy equation for two-scale fluctuation, particle energy transfer rate...A particle nonlinear two-scale kp-εp turbulence model is proposed for simulating the anisotropic turbulent two-phase flow. The particle kinetic energy equation for two-scale fluctuation, particle energy transfer rate equation for large-scale fluctuation, and particle turbulent kinetic energy dissipation rate equation for small-scale fluctuation are derived and closed. This model is used to simulate gas-particle flows in a sudden-expansion chamber. The simulation is com- pared with the experiment and with those obtained by using another two kinds of tow-phase turbulence model, such as the single-scale k-ε two-phase turbulence model and the particle two-scale second-order moment （USM） two-phase turbulence model. It is shown that the present model gives simulation in much better agreement with the experiment than the single-scale k-ε two-phase turbulence model does and is almost as good as the particle two-scale USM turbu-lence model.展开更多
A new second-order moment two- phase turbulence model accounting for particle wake effect was established and used to simulate gas-particle flow in a horizontal channel for different values of wall roughness. The resu...A new second-order moment two- phase turbulence model accounting for particle wake effect was established and used to simulate gas-particle flow in a horizontal channel for different values of wall roughness. The results show that compared with the model without considering the particle wake effect, the present model gives simulation results agreeing much better with the experimental results for the gas turbulence modulation, but the predicted results for particle motion with the two kinds of models are quite close.展开更多
The gas-particle flow in the primary air pipe （PAP） of a low NOx swirl burner was investigated using the computational fluid dynamics （CFD） coupled with the discrete element method （DEM）. The mathematical models...The gas-particle flow in the primary air pipe （PAP） of a low NOx swirl burner was investigated using the computational fluid dynamics （CFD） coupled with the discrete element method （DEM）. The mathematical models were validated using the measured values obtained at the outlet of the primary pipe through a phase Doppler anemometer （PDA） system. Particles of different Stokes numbers in the primary air pipe （PAP） were investigated, and the effects of the structure of the primary air pipe and the particle-particle interaction on particle dispersion were analyzed. The results indicate that particles under the combined effects of the Venturi pipe and the spindle body are concentrated into a narrow band area and that the PAP structure can more efficiently concentrate particles with large Stokes numbers. The formed fuel rich/lean jet persists for a long distance out of the burner, thereby favoring of air-staged combustion and NOx reduction. The particle collision frequency and its fluctuation range increase as the particle Stokes number increases. The collisions among particles result in an increase of the spanwise dispersion of particles. Experimental results indicate that the models that take particle-particle collision into consideration are more able to predict particle concentration.展开更多
In this paper the present authors measured the gas-particle two-phase velocity correlation in sudden expansion gas-particle flows with a phase Doppler particle anemometer （PDPA） and simulated the system behavior by ...In this paper the present authors measured the gas-particle two-phase velocity correlation in sudden expansion gas-particle flows with a phase Doppler particle anemometer （PDPA） and simulated the system behavior by using both a Reynolds-averaged Navier-Stokes （RANS） model and a large-eddy simulation （LES）. The results of the measurements yield the axial and radial time-averaged velocities as well as the fluctuation velocities of gas and three particle-size groups （30μm, 50μm, and 95μm） and the gasparticle velocity correlation for 30μm and 50μm particles. From the measurements, theoretical analysis, and simulation, it is found that the two-phase velocity correlation of sudden-expansion flows, like that of jet flows, is less than the gas and particle Reynolds stresses. What distinguishes the two-phase velocity correlations of sudden-expansion flow from those of jet and channel flows is the absence of a clear relationship between the two-phase velocity correlation and particle size in sudden-expansion flows. The measurements, theoretical analysis, and numerical simulation all lead to the above-stated conclusions. Quantitatively, the results of the LES are better than those of the RANS model.展开更多
The weighted-sum-of-gray-gas(WSGG)model and Mie theory are applied to study the influents of particle size on the radiative transfer in high temperature homogeneous gas-particle mixtures,such as the flame in aero-engi...The weighted-sum-of-gray-gas(WSGG)model and Mie theory are applied to study the influents of particle size on the radiative transfer in high temperature homogeneous gas-particle mixtures,such as the flame in aero-engine combustor.The radiative transfer equation is solved by the finite volume method.The particle size is assumed to obey uniform distribution and logarithmic normal(L-N)distribution,respectively.Results reveal that when particle size obeys uniform distribution,increasing particle size with total particle volume fraction fvunchanged will result in the decreasing of the absolute value of radiative heat transfer properties,and the effect of ignoring particle scattering will also be weakened.Opposite conclusions can be obtained when total particle number concentration N0 is unchanged.Moreover,if particle size obeys L-N distribution,increasing the narrowness indexσor decreasing the characteristic diameter Dˉwith the total particle volume fraction fvunchanged will increase the absolute value of radiative heat transfer properties.With total particle number concentration N0 unchanged,opposite conclusions for radiative heat source and incident radiation terms can be obtained except for radiative heat flux term.As a whole,the effects of particle size on the radiative heat transfer in the high-temperature homogeneous gas-particle mixtures are complicated,and the particle scattering cannot be ignoring just according to the particle size.展开更多
A k - ε-PDF model based on statistical theory for turbulent gas-particle flows is proposed,and a numerical procedure combining the finite difference and finite fluctuating-velocity -group methods is used.The obtained...A k - ε-PDF model based on statistical theory for turbulent gas-particle flows is proposed,and a numerical procedure combining the finite difference and finite fluctuating-velocity -group methods is used.The obtained statistically averaged equations have the same form as those obtained by using the Reynolds averaging.Using the k -ε-PDF model (PDF particle turbulence model combined with the k - ε gas turbulence model),many terms,such as the diffusion term in particle Reynolds Stress equations,can be accurately calculated for verifying the second-moment-closure model.The k - ε- PDF model is used to simulate sudden-expansion particle-laded flow.comparison of the predictions using both k -ε-PDF and the k - ε- kp models with experimental results shows that the k - ε-PDF model give more reasonable non-isotropic features of particle turbulence.展开更多
In the suburbs of Kitakyushu,Japan,the inorganic aerosol mass concentration(IAM)was about 32.7μg/m^(3),with the aerosol pH of 3.3.To study the thermodynamics of aerosol when its individual components'concentratio...In the suburbs of Kitakyushu,Japan,the inorganic aerosol mass concentration(IAM)was about 32.7μg/m^(3),with the aerosol pH of 3.3.To study the thermodynamics of aerosol when its individual components'concentration is reduced,sensitive tests were performed using the ISORROPIAⅡmodel,in which the seven control species—TNaCl,TNH_(4)^(+),TSO_(4)^(2-),TNO_(3)^(-),TMg^(2+),TK^(+),and TCa^(2+)—were taken into account.IAM and inorganic aerosol pH after reducing TNaCl,TNO_(3)^(-),TMg^(2+),TK^(+),and TCa^(2+)responded linearly(0%≤concentration reduction ratio(CRR)≤100%,with the exception of 100%in TNaCl);the nonlinear variations of these two parameters could be observed by controlling TNH_(4)^(+)and TSO_(4)^(2-).Unexpected aerosol behavior occurred at 100%reduction of TNaCl,which was caused by the sudden increase of NO_(3)^(-),NH_(4)^(+),and aerosol liquid water content(ALWC);the increase of IAM was also observed after controlling TSO_(4)^(2-)(60%≤CRR≤100%)and TCa^(2+)(0%≤CRR≤100%),which was mainly related to the variation of ALWC driven by the response of CaSO_(4).Multiple regression analysis showed that ALWC was statistically and strongly related to the variations of NO_(3)^(-),Cl-,SO_(4)^(2-),HSO_(4)^(-),HNO_(3),and NH_(3)(P<0.05),with regression coefficients of 1.68,5.23,1.83,2.81,0.34,and 0.57,respectively.The highest coefficient(5.23)was found for Cl^(-),revealing that sea salts significantly influenced particle responses.Overall,this study comprehensively investigated aerosol characteristics and inner responses for the reduction of components,which is of great significance for a better understanding of atmospheric chemistry in Kitakyushu,Japan.展开更多
Sub-grid effective drag,filtered and residual stresses in the meso-scale of gas-particle fluidized flows are intrinsically affected by underlying micro-scale conditions as well as non-local effects related to macro-sc...Sub-grid effective drag,filtered and residual stresses in the meso-scale of gas-particle fluidized flows are intrinsically affected by underlying micro-scale conditions as well as non-local effects related to macro-scale conditions.In this work we applied microscopic two-fluid modeling to experiment with particle Froude number in order to evaluate the impact of this micro-scale condition over the concerning meso-scale derived sub-grid parameters.We performed highly resolved simulations in periodic domains for particle Froude numbers from 12.21 to 799.22,for a wide range of macro-scale conditions.Results were filtered and classified by ranges of meso-scale markers for the various particle Froude numbers.The particle Froude number was found to considerably affect the structural refinement of the heterogeneous flow fields thereby directly impacting effective drag,filtered and residual stresses.All of those parameters showed systematic behaviors in relation to particle Froude number,thereby providing sound data for new sub-grid modeling propositions.展开更多
The interaction between nozzle design and fluidization gas composition significantly influences the dynamics within a powder fuel scramjet's combustion chamber.To investigate this relationship,an experimental stud...The interaction between nozzle design and fluidization gas composition significantly influences the dynamics within a powder fuel scramjet's combustion chamber.To investigate this relationship,an experimental study utilized high-speed shadow imaging technology to explore the macroscopic aspects of powder fuel injection.The investigation examined various convergence angles,nozzle throat lengths,and fluidized gas compositions.Key findings include:During jet development,powder fuel initially concentrates near the axis,with non-convergence angle nozzles exhibiting longer concentrated distribution periods than convergence angle conditions.Decreasing nozzle convergence angles lead to increased penetration distance,frontal velocity,and radial diffusion distance during the initial stages of jet development.Additionally,stable jet shapes show larger divergence angles as nozzle convergence angle decreases,with the largest divergence angle observed atα=60°.In the initial 0-7 ms of jet development,the powder fuel jet demonstrates greater penetration distance and frontal velocity under certain conditions.Moreover,penetration distance and frontal velocity increase with throat length from 7 to 20 ms,accompanied by changes in divergence angles.Specifically,at a throat length(l)of 2 mm,the near-field divergence angle measures 46.50°,and the far-field divergence angle is 22.25°.Conversely,at l=8mm,the near-field divergence angle is 33.49°,and the far-field divergence angle is 23.21°.The fluidization gas composition minimally affects jet penetration distance and frontal velocity during the initial 0-3 ms.However,due to hydrogen's low density,hydrogen/powder fuel jets exhibit shorter distances and velocities compared to nitrogen/powder fuel jets.Hydrogen fluidization also results in larger divergence angles,particularly in the near field.These findings underscore the importance of nozzle design and fluidization gas composition in optimizing scramjet performance and efficiency.展开更多
The turbulence enhancement by particle wake effect is studied by large eddy simulation （LES） of turbulent gas flows passing a single particle. The predicted time-averaged and root-mean-square fluctuation velocities ...The turbulence enhancement by particle wake effect is studied by large eddy simulation （LES） of turbulent gas flows passing a single particle. The predicted time-averaged and root-mean-square fluctuation velocities behind the particle are in agreement with the Reynolds-averaged Navier-Stokes modeling results and experimental results. A semi-empirical turbulence enhancement model is proposed by the present-authors based on the LES resuits. This model is incorporated into the second-order moment two-phase turbulence model for simulating vertical gas-particle pipe flows and horizontal gas-particle channel flows. The simulation results show that compared with the model not accounting for the particle wake effect, the present model gives simulation results for the gas turbulence modulation in much better agreement with the experimental results.展开更多
The basic equations of turbulent gas-solid flows are derived by using the pseudo-fluid model of particle phase with a refined two-phase turbulence model.These equations are then applied to swirling gas-particle flows ...The basic equations of turbulent gas-solid flows are derived by using the pseudo-fluid model of particle phase with a refined two-phase turbulence model.These equations are then applied to swirling gas-particle flows for analyzing the collection efficiency in cyclone separators.展开更多
基金Item Sponsored by National Natural Science Foundation of China and Shanghai Baosteel Group Co Ltd United Research Foundation(50374085)
文摘The two-dimensional steady-state discrete phase mathematical model is developed to analyze gas-particle flow and combustion characteristics of coal particles, as well as components concentration and temperature distribu- tion of coal gas in the process of pulverized coal injection of blast furnace raceway. The results show that a great deal of coal gas discharges on the top of raceway away from the tuyere, and the residence time of coal particles in the re- gion of blowpipe and tuyere is 20 ms or so and 50 ms when it reaches raceway boundary. The pressure is the highest at the bottom of raceway and the maximal temperature is about 2 423 K. The char combustion is mainly carried out in the raceway and the maximum of char burn-out rate attains 3× 10-4 kg/s.
基金supported by the National Natural Science Foundation of China(No.42005079,41675131)the Beijing Natural Science Foundation(No.8131003)the Beijing Talents Fund(No.2014000021223ZK49)。
文摘To better understand the characteristics and transformation mechanisms of secondary inorganic aerosols,hourly mass concentrations of water-soluble inorganic ions(WSIIs)in PM_(2.5)and their gaseous precursors were measured online from 2016 to 2018 at an urban site in Beijing.Seasonal and diurnal variations in water-soluble ions and gaseous precursors were discussed and their gas-particle conversion and partitioning were also examined,some related parameters were characterized.The(TNH_(3))Rich was also defined to describe the variations of the excess NH_(3)in different seasons.In addition,a sensitivity test was carried out by using ISORROPIA II to outline the driving factors of gas-particle partitioning.In Beijing,the relative contribution of nitrate to PM_(2.5)has increased markedly in recent years,especially under polluted conditions.In the four seasons,only a small portion of NO_(2)in the atmosphere was converted into total nitrate(TNO_(3)),and more than 80%of TNO_(3)occurred in the form of nitrate due to the abundant ammonia.The concentration of total ammonia(TNH_(3))was much higher than that required to neutralize acid gases,and most of the TNH_(3)occurred as gaseous NH_(3).The nitrous acid(HONO)concentration was highly correlated with NH_(3)concentration and had increased significantly in Beijing compared with previous studies.The total chloride(TCl)was the highest in winter,andε(Cl^(-))was more sensitive to variations in the ambient temperature(T)and relative humidity(RH)thanε(NO_(3)^(-)).
文摘Based on a kinetic energy equation of particle turbulence, a k-ε-kk model for turbulent gas-particle flows is proposed. The prediction of confined plane gas-particle jets shows a good agreement with experimental data. This model is proved to be far superior to the presently used k-ε-A.P. model based on the algebraic model of particle turbulence.
文摘Particle-laden gas flows past a circular cylinder at the Reynolds number of 2×10^(5) were numerically investigated. The Discrete Vortex Method (DVM) was employed to evaluate the unsteady gas flow fields and a Lagrangian approach was applied for tracking individual solid particles. The vortex patterns and the distributions of particles with different Stokes numbers were obtained. Numerical results show that: (1) at small Stokes number (St=0.01) the particles move with the fluid and could be found evenly throughout the flow, (2) the regions around the vortex cores, where few particles exist, become wider as the stokes number of particles increases from 0.01 to 1.0, (3) at middle Stokes number (St=1.0, 10) centrifugal forces throw the particles out of the wake vortices, (4) at high Stokes number (St=100, 1000) the particles are not affected by the vortices,and their motion is determined by their inertia effects.
基金Project supported by the Special Funds for Major State Basic Research (Grant No: G-1999-0222-08), China Postdoctoral Science Foundation (Grant No: 2004036239).
文摘A two-scale second-order moment two-phase turbulence model was developed and used to simulate gas-particle flow in a sudden-expansion chamber and a channel. The simulation results were in agreement with the experimental results, and the results were compared with those of the single-scale second-order moment two-phase turbulence model. Several improved features show that the two-scale model is to a certain extent better than the single-scale model, which may be attributed to the fact that particle turbulence is well characterized by the two-scale turbulence model.
基金The Chinese Polar Environment Comprehensive Investigation and Assessment Programs under contract Nos 02-01,03-04,04-01 and 04-03the National Natural Science Fundation of China under contract No.21377032
文摘Polychlorinated biphenyls （PCBs） were measured in atmospheric samples collected from the North Pacific to the Arctic Ocean between July and September 2012 to study the atmospheric concentration characteris-tics of PCBs and their gas/particle partitioning. The mean concentration of 26 PCBs （vapor plus particulate phase） （∑PCBs） was 19.116 pg/m^3with a standard deviation of 13.833 pg/m^3. Three most abundant conge-ners were CB-28, -52 and -77, accounting for 43.0% to∑PCBs. The predominance of vapor PCBs （79.0% to∑PCBs） in the atmosphere was observed.∑PCBs were negative correlated with the latitudes and inverse of the absolute temperature （1/T）. The significant correlation for most congeners was also observed between the logarithm of gas/particle partition coefficient （logKp） and 1/T. Shallower slopes （from ∑0.15 to ∑0.46, average ∑0.27） were measured from the regression of the logarithm of sub-cooled liquid vapor pressures （logpoL） and logKP for all samples. The difference of the slopes and intercepts among samples was insignifi-cant （p〉0.1）, implying adsorption and/or absorption processes and the aerosol composition did not differ significantly among different samples. By comparing three models, the J-P adsorption model, the octanol/air partition coefficient （KOA） based model and the soot-air model, the gas/particle partitioning of PCBs in the Arctic atmosphere was simulated more precisely by the soot-air model, and the adsorption onto el-emental carbon is more sensitive than the absorption into organic matters of aerosols, especially for low-chlorinated PCB congeners.
基金The project supported by the Special Funds for the Major State Basic Research,China (G-1999-0222-08)
文摘A two-fluid particle-wall collision model with consideration of wall roughness is pro- posed.It takes into account the effects of the friction,restitution and in particular the wall roughness, and hence the redistribution of Reynolds stress in different directions,the absorption of turbulent en- ergy from the mean motion and the attenuation of particle motion by the wall.The proposed model is used to simulate sudden-expansion and swirling gas-particle flows and is validated by comparing with experimental results.The results show that the proposed model gives better results than those obtained by the presently used zero-gradient condition.Hence,it is suggested that the proposed model should be used as the wall boundary condition for the particle phase in place of the presently used boundary condition.
基金The project supported by the Special Funds for Major State Basic Research,China(G-1999-0222-08)the Postdoctoral Science Foundation(2004036239)
文摘A two-scale second-order moment two-phase turbulence model accounting for inter-particle collision is developed, based on the concepts of particle large-scale fluctuation due to turbulence and particle small-scale fluctuation due to collision and through a unified treatment of these two kinds of fluctuations. The proposed model is used to simulate gas-particle flows in a channel and in a downer. Simulation results are in agreement with the experimental results reported in references and are near the results obtained using the sin- gle-scale second-order moment two-phase turbulence model superposed with a particle collision model （USM-θ model） in most regions.
基金the China Postdoctoral Science Foundation (Grant No.2004036239).
文摘A semi-empirical turbulence enhancement model accounting for the particle-wake effect was incorporated into the second-order moment two-phase turbulence model and employed to simulate gas-particle flows in a swirling sudden-expansion chamber. The simulated results for two-phases mean velocities and fluctuation velocities coincide well with the experiment ones, which demonstrates that this model, in comparison with the turbulence model not accounting for the wake effect, leads to higher calculating accuracy.
文摘A particle nonlinear two-scale kp-εp turbulence model is proposed for simulating the anisotropic turbulent two-phase flow. The particle kinetic energy equation for two-scale fluctuation, particle energy transfer rate equation for large-scale fluctuation, and particle turbulent kinetic energy dissipation rate equation for small-scale fluctuation are derived and closed. This model is used to simulate gas-particle flows in a sudden-expansion chamber. The simulation is com- pared with the experiment and with those obtained by using another two kinds of tow-phase turbulence model, such as the single-scale k-ε two-phase turbulence model and the particle two-scale second-order moment （USM） two-phase turbulence model. It is shown that the present model gives simulation in much better agreement with the experiment than the single-scale k-ε two-phase turbulence model does and is almost as good as the particle two-scale USM turbu-lence model.
基金the China Postdoctoral Science Foundation (Grant No.2004036239)the Foundation of Jiangxi Educational Committee (Grant No.GJJ08230)
文摘A new second-order moment two- phase turbulence model accounting for particle wake effect was established and used to simulate gas-particle flow in a horizontal channel for different values of wall roughness. The results show that compared with the model without considering the particle wake effect, the present model gives simulation results agreeing much better with the experimental results for the gas turbulence modulation, but the predicted results for particle motion with the two kinds of models are quite close.
基金supported by Key Technologies Research and Development Program of China(2011BAA04B01)Zhejiang Provincial Natural Science Foundation of China(LZ12E06002)
文摘The gas-particle flow in the primary air pipe （PAP） of a low NOx swirl burner was investigated using the computational fluid dynamics （CFD） coupled with the discrete element method （DEM）. The mathematical models were validated using the measured values obtained at the outlet of the primary pipe through a phase Doppler anemometer （PDA） system. Particles of different Stokes numbers in the primary air pipe （PAP） were investigated, and the effects of the structure of the primary air pipe and the particle-particle interaction on particle dispersion were analyzed. The results indicate that particles under the combined effects of the Venturi pipe and the spindle body are concentrated into a narrow band area and that the PAP structure can more efficiently concentrate particles with large Stokes numbers. The formed fuel rich/lean jet persists for a long distance out of the burner, thereby favoring of air-staged combustion and NOx reduction. The particle collision frequency and its fluctuation range increase as the particle Stokes number increases. The collisions among particles result in an increase of the spanwise dispersion of particles. Experimental results indicate that the models that take particle-particle collision into consideration are more able to predict particle concentration.
基金supported by the National Natural Science Foundation of China (50606026 and 50736006)
文摘In this paper the present authors measured the gas-particle two-phase velocity correlation in sudden expansion gas-particle flows with a phase Doppler particle anemometer （PDPA） and simulated the system behavior by using both a Reynolds-averaged Navier-Stokes （RANS） model and a large-eddy simulation （LES）. The results of the measurements yield the axial and radial time-averaged velocities as well as the fluctuation velocities of gas and three particle-size groups （30μm, 50μm, and 95μm） and the gasparticle velocity correlation for 30μm and 50μm particles. From the measurements, theoretical analysis, and simulation, it is found that the two-phase velocity correlation of sudden-expansion flows, like that of jet flows, is less than the gas and particle Reynolds stresses. What distinguishes the two-phase velocity correlations of sudden-expansion flow from those of jet and channel flows is the absence of a clear relationship between the two-phase velocity correlation and particle size in sudden-expansion flows. The measurements, theoretical analysis, and numerical simulation all lead to the above-stated conclusions. Quantitatively, the results of the LES are better than those of the RANS model.
基金supported by the National Natural Science Foundation of China (No: 51806103)Jiangsu Provincial Natural Science Foundation(No: BK20170800)Open Funds of Aero-engine Thermal Environment and Structure Key Laboratory of Ministry of Industry and Information Technology (No. CEPE2018005)
文摘The weighted-sum-of-gray-gas(WSGG)model and Mie theory are applied to study the influents of particle size on the radiative transfer in high temperature homogeneous gas-particle mixtures,such as the flame in aero-engine combustor.The radiative transfer equation is solved by the finite volume method.The particle size is assumed to obey uniform distribution and logarithmic normal(L-N)distribution,respectively.Results reveal that when particle size obeys uniform distribution,increasing particle size with total particle volume fraction fvunchanged will result in the decreasing of the absolute value of radiative heat transfer properties,and the effect of ignoring particle scattering will also be weakened.Opposite conclusions can be obtained when total particle number concentration N0 is unchanged.Moreover,if particle size obeys L-N distribution,increasing the narrowness indexσor decreasing the characteristic diameter Dˉwith the total particle volume fraction fvunchanged will increase the absolute value of radiative heat transfer properties.With total particle number concentration N0 unchanged,opposite conclusions for radiative heat source and incident radiation terms can be obtained except for radiative heat flux term.As a whole,the effects of particle size on the radiative heat transfer in the high-temperature homogeneous gas-particle mixtures are complicated,and the particle scattering cannot be ignoring just according to the particle size.
文摘A k - ε-PDF model based on statistical theory for turbulent gas-particle flows is proposed,and a numerical procedure combining the finite difference and finite fluctuating-velocity -group methods is used.The obtained statistically averaged equations have the same form as those obtained by using the Reynolds averaging.Using the k -ε-PDF model (PDF particle turbulence model combined with the k - ε gas turbulence model),many terms,such as the diffusion term in particle Reynolds Stress equations,can be accurately calculated for verifying the second-moment-closure model.The k - ε- PDF model is used to simulate sudden-expansion particle-laded flow.comparison of the predictions using both k -ε-PDF and the k - ε- kp models with experimental results shows that the k - ε-PDF model give more reasonable non-isotropic features of particle turbulence.
文摘In the suburbs of Kitakyushu,Japan,the inorganic aerosol mass concentration(IAM)was about 32.7μg/m^(3),with the aerosol pH of 3.3.To study the thermodynamics of aerosol when its individual components'concentration is reduced,sensitive tests were performed using the ISORROPIAⅡmodel,in which the seven control species—TNaCl,TNH_(4)^(+),TSO_(4)^(2-),TNO_(3)^(-),TMg^(2+),TK^(+),and TCa^(2+)—were taken into account.IAM and inorganic aerosol pH after reducing TNaCl,TNO_(3)^(-),TMg^(2+),TK^(+),and TCa^(2+)responded linearly(0%≤concentration reduction ratio(CRR)≤100%,with the exception of 100%in TNaCl);the nonlinear variations of these two parameters could be observed by controlling TNH_(4)^(+)and TSO_(4)^(2-).Unexpected aerosol behavior occurred at 100%reduction of TNaCl,which was caused by the sudden increase of NO_(3)^(-),NH_(4)^(+),and aerosol liquid water content(ALWC);the increase of IAM was also observed after controlling TSO_(4)^(2-)(60%≤CRR≤100%)and TCa^(2+)(0%≤CRR≤100%),which was mainly related to the variation of ALWC driven by the response of CaSO_(4).Multiple regression analysis showed that ALWC was statistically and strongly related to the variations of NO_(3)^(-),Cl-,SO_(4)^(2-),HSO_(4)^(-),HNO_(3),and NH_(3)(P<0.05),with regression coefficients of 1.68,5.23,1.83,2.81,0.34,and 0.57,respectively.The highest coefficient(5.23)was found for Cl^(-),revealing that sea salts significantly influenced particle responses.Overall,this study comprehensively investigated aerosol characteristics and inner responses for the reduction of components,which is of great significance for a better understanding of atmospheric chemistry in Kitakyushu,Japan.
基金supported by The State of Sao Paulo Research Foundation (FAPESP)The National Council for Scientific and Technological Development (CNPq),both from Brazil.
文摘Sub-grid effective drag,filtered and residual stresses in the meso-scale of gas-particle fluidized flows are intrinsically affected by underlying micro-scale conditions as well as non-local effects related to macro-scale conditions.In this work we applied microscopic two-fluid modeling to experiment with particle Froude number in order to evaluate the impact of this micro-scale condition over the concerning meso-scale derived sub-grid parameters.We performed highly resolved simulations in periodic domains for particle Froude numbers from 12.21 to 799.22,for a wide range of macro-scale conditions.Results were filtered and classified by ranges of meso-scale markers for the various particle Froude numbers.The particle Froude number was found to considerably affect the structural refinement of the heterogeneous flow fields thereby directly impacting effective drag,filtered and residual stresses.All of those parameters showed systematic behaviors in relation to particle Froude number,thereby providing sound data for new sub-grid modeling propositions.
基金the China Scholarship Council,the Fundamental Research Funds for the Central Universities(grant No.30920041102).
文摘The interaction between nozzle design and fluidization gas composition significantly influences the dynamics within a powder fuel scramjet's combustion chamber.To investigate this relationship,an experimental study utilized high-speed shadow imaging technology to explore the macroscopic aspects of powder fuel injection.The investigation examined various convergence angles,nozzle throat lengths,and fluidized gas compositions.Key findings include:During jet development,powder fuel initially concentrates near the axis,with non-convergence angle nozzles exhibiting longer concentrated distribution periods than convergence angle conditions.Decreasing nozzle convergence angles lead to increased penetration distance,frontal velocity,and radial diffusion distance during the initial stages of jet development.Additionally,stable jet shapes show larger divergence angles as nozzle convergence angle decreases,with the largest divergence angle observed atα=60°.In the initial 0-7 ms of jet development,the powder fuel jet demonstrates greater penetration distance and frontal velocity under certain conditions.Moreover,penetration distance and frontal velocity increase with throat length from 7 to 20 ms,accompanied by changes in divergence angles.Specifically,at a throat length(l)of 2 mm,the near-field divergence angle measures 46.50°,and the far-field divergence angle is 22.25°.Conversely,at l=8mm,the near-field divergence angle is 33.49°,and the far-field divergence angle is 23.21°.The fluidization gas composition minimally affects jet penetration distance and frontal velocity during the initial 0-3 ms.However,due to hydrogen's low density,hydrogen/powder fuel jets exhibit shorter distances and velocities compared to nitrogen/powder fuel jets.Hydrogen fluidization also results in larger divergence angles,particularly in the near field.These findings underscore the importance of nozzle design and fluidization gas composition in optimizing scramjet performance and efficiency.
基金Supported by the Major Project of National Natural Science Foundation of China (No.10632070) the Postdoctoral ScienceFoundation (No.2004036239).
文摘The turbulence enhancement by particle wake effect is studied by large eddy simulation （LES） of turbulent gas flows passing a single particle. The predicted time-averaged and root-mean-square fluctuation velocities behind the particle are in agreement with the Reynolds-averaged Navier-Stokes modeling results and experimental results. A semi-empirical turbulence enhancement model is proposed by the present-authors based on the LES resuits. This model is incorporated into the second-order moment two-phase turbulence model for simulating vertical gas-particle pipe flows and horizontal gas-particle channel flows. The simulation results show that compared with the model not accounting for the particle wake effect, the present model gives simulation results for the gas turbulence modulation in much better agreement with the experimental results.
文摘The basic equations of turbulent gas-solid flows are derived by using the pseudo-fluid model of particle phase with a refined two-phase turbulence model.These equations are then applied to swirling gas-particle flows for analyzing the collection efficiency in cyclone separators.
