CO_(2)捕集、利用与封存(CO_(2)Capture, Utilization and Storage, CCUS)技术是减少碳排放的有效手段之一,是实现中国“双碳”目标的重要技术保障,其中CO_(2)管道输送是最重要的一环。从CCUS技术和CO_(2)管道设计两个维度综述了国内外C...CO_(2)捕集、利用与封存(CO_(2)Capture, Utilization and Storage, CCUS)技术是减少碳排放的有效手段之一,是实现中国“双碳”目标的重要技术保障,其中CO_(2)管道输送是最重要的一环。从CCUS技术和CO_(2)管道设计两个维度综述了国内外CO_(2)捕集、CO_(2)运输、CO_(2)封存和CO_(2)利用的研究进展,针对运输过程,着重从工艺设计、杂质、含水量、止裂控制和风险评估等方面梳理了CO_(2)管道设计的研究成果。中国目前正在大力推进CCUS技术,中国石油、中国石化和中国海洋石油等机构分别成立了相关的研究机构,聚焦CCUS发展的各个环节。虽然中国尚处于技术发展的初级阶段,但相信随着科研人员的努力会很快赶超发达国家,跻身第一方阵。研究结果旨在为中国的CCUS技术发展提供参考,促进中国CCUS技术的推广实施和CO_(2)管道的合理设计。展开更多
The life-cycle assessment method,which originates from general products and services,has gradually come to be applied to investigations of the life-cycle carbon emissions(LCCE)of buildings.A literature review was cond...The life-cycle assessment method,which originates from general products and services,has gradually come to be applied to investigations of the life-cycle carbon emissions(LCCE)of buildings.A literature review was conducted to clarify LCCE implications,calculations,and reductions in the context of buildings.A total of 826 global building carbon emission calculation cases were obtained from 161 studies based on the framework of the building life-cycle stage division stipulated by ISO 21930 and the basic principles of the emission factor(EF)approach.The carbon emission calculation methods and results are discussed herein,based on the modules of production,construction,use,end-of-life,and supplementary benefits.According to the hotspot distribution of a building’s carbon emissions,carbon reduction strategies are classified into six groups for technical content and benefits analysis,including reducing the activity data pertaining to building materials and energy,reducing the carbon EFs of the building materials and energy,and exploiting the advantages of supplementary benefits.The research gaps and challenges in current building LCCE studies are summarized in terms of research goals and ideas,calculation methods,basic parameters,and carbon reduction strategies;development suggestions are also proposed.展开更多
The lifecycle greenhouse gas(GHG)emissions(Well-to-Wake)from maritime transport must be reduced by at least 50%in absolute values by 2050 to contribute to the ambitions of the Paris Agreement(2015).A transition from c...The lifecycle greenhouse gas(GHG)emissions(Well-to-Wake)from maritime transport must be reduced by at least 50%in absolute values by 2050 to contribute to the ambitions of the Paris Agreement(2015).A transition from conventional fuels to alternative fuels with zero or lower GHG emissions is viewed as the most promising avenue to reach the GHG reductions.Whereas GHG and toxic pollutants emitted from the use of fossil fuels(heavy fuel oil(HFO)and marine gas/diesel oil(MGO/MDO))are generally well understood,the emissions associated with the new fuel options are only now being measured and communicated.This review provides an outlook on fuels that could help shipping respond to the decarbonization effort including Liquefied Petroleum Gas(LPG),Liquefied Natural Gas(LNG),methanol,ammonia,and hydrogen.A quantification of the pollutants associated from the use of these fuels is provided and challenges and barriers to their uptake are discussed.展开更多
In China,there has been insufficient study of whole food system greenhouse gas(GHG)accounting,which limits the development of mitigation strategies and may preclude the achievement of carbon peak and carbon neutrality...In China,there has been insufficient study of whole food system greenhouse gas(GHG)accounting,which limits the development of mitigation strategies and may preclude the achievement of carbon peak and carbon neutrality goals.The paper presents the development of a carbon extension of NUFER(NUtrient flows in Food chain,Environment and Resources use model),a food system GHG emission accounting model that covers land use and land-use change,agricultural production,and post-production subsectors.The spatiotemporal characteristics of GHG emissions were investigated for the Chinese food system(CFS)from 1992 to 2017,with a focus on GHG emissions from the entire system.The potential to achieve a low-carbon food system in China was explored.The net GHG emissions from the CFS increased from 785Tg CO_(2)equivalent(CO_(2)-eq)in 1992 to 1080 Tg CO_(2)-eq in 2017.Agricultural activities accounted for more than half of the total emissions during the study period,while agricultural energy was the largest contributor to the GHG increase.In 2017,highest emitting regions were located in central and southern China(Guangdong and Hunan),the North China Plain(Shandong,Henan and Jiangsu)and Northeast China(Heilongjiang and Inner Mongolia)and contributed to over half of the total GHG emissions.Meanwhile,Xinjiang,Qinghai and Tibet are shown as carbon sink areas.It was found that foodsystem GHG emissions could be reduced to 355 Tg CO_(2)-eq,where enhancing endpoint mitigation technologies,transforming social-economic and diet conditions,and increasing agricultural productivities can contribute to 60%,25%and 15%,respectively.Synergistic mitigation effects were found to exist in agricultural activities.展开更多
Climate financing is a key issue in current negotiations on climate protection. This study establishes a climate financing model based on a mechanism in which donor countries set up funds for climate financing and rec...Climate financing is a key issue in current negotiations on climate protection. This study establishes a climate financing model based on a mechanism in which donor countries set up funds for climate financing and recipient countries use the funds exclusively for carbon emission reduction. The burden-sharing principles are based on GDP, historical emissions, and consumption- based emissions. Using this model, we develop and analyze a series of scenario simulations, including a financing program negotiated at the Cancun Climate Change Conference （2010） and several subsequent programs. Results show that sustained climate financing can help to combat global climate change. However, the Cancun Agreements are projected to result in a reduction of only 0.0I^C in global warming by 2100 compared to the scenario without climate financing. Longer-term climate financing programs should be established to achieve more significant benefits. Our model and simulations also show that climate financing has economic benefits for develop- ing countries. Developed countries will suffer a slight GDP loss in the early stages of climate financing, but the long- term economic growth and the eventual benefits of climate mitigation will compensate for this slight loss. Different burden-sharing principles have very similar effects on global temperature change and economic growth of recipient countries, but they do result in differences in GDP changes for Japan and the FSU. The GDP-based principle results in a larger share of financial burden for Japan, while the historical emissions-based principle results in a larger share of financial burden for the FSU. A larger burden share leads to a greater GDP loss.展开更多
Emission intensity and climate change control the transport flux and fate of persistent organic pollutants(POPs)inmultiple environmental compartments.This study applied amultimedia model(BETR model)to explore alternat...Emission intensity and climate change control the transport flux and fate of persistent organic pollutants(POPs)inmultiple environmental compartments.This study applied amultimedia model(BETR model)to explore alternations in the spatio-temporal trends of concentrations and transport flux of benzopyrene(BaP),phenanthrene(Phe),perfluorooctane sulfonates(PFOS)and polychlorinated biphenyls(PCBs)in the Chaohu watershed,located in the lower reaches of the Yangtze River,China in response to changes in source emissions and climate.The potential historic and future risks of these pollutants also were assessed.The results suggest that current trends in concentrations and transport were similar to that of their emissions between 2005 and 2018.During the next 100 years,temporal trends and spatial patterns were not predicted to change significantly,which is consistent with climate change.Based on sensitivity and correlation analyses,climate change had significant effects on multi-media concentrations and transport fluxes of BaP,Phe,PFOS and PCBs,and rainfall intensity was the predominant controlling factor.Risk quotients(RQs)of BaP and Phe-in soil increased from 0.42 to 0.95 and 0.06 to 0.35,respectively,from 2005 to 2090,indicating potential risks.The RQs of the other examined contaminants exhibited little potential risk in soil,water,or sediment.Based on spatial patterns,it was inferred that the ecosystem around Lake Chaohu is the most at risk.The study provides insights needed for local pollution control of POPs in the Chaohu watershed.In addition,the developed approach can be applied to other watersheds world-wide.展开更多
In this contribution, we use a coupled air quality modelling system (AQM) as a tool to design and develop an air quality plan in Madrid. AQM has allowed us to obtain a preliminary evaluation of the effect of mitigatio...In this contribution, we use a coupled air quality modelling system (AQM) as a tool to design and develop an air quality plan in Madrid. AQM has allowed us to obtain a preliminary evaluation of the effect of mitigation measures over regional and local air quality levels. To achieve these goals, we have prepared a sophisticated AQM, coupling the meteorological model WRF, the emission model AEMM, and the photochemical model CMAQ. AQM was evaluated using the whole modelling year 2010 working with high horizontal resolution, 3 km for the region of Madrid and 1km for urban metropolitan area of Madrid. Two different analyses have been realized: a source apportionment exercise following a zero-out methodology to obtain the contribution to the air quality levels of the different emission sector;and an evaluation of the main mitigation measures considered in the air quality plan using sensitivity analysis. The air quality plan was focused on the improvement of NO<sub>2</sub> levels and AQM analyzed the effect of the mitigation measures during ten episodes of 2011 where NO<sub>2</sub> or O<sub>3</sub> levels were the highest of the year;so we analyzed the effect of the mitigation plan in worst conditions. Results provided by the AQM system show that it accomplishes the European Directive modelling uncertainty requirements and the mean absolute gross error for 1-h maximum daily NO<sub>2</sub> is 31% over locations with higher levels of this atmospheric pollutant;the road traffic is the main contributor to the air quality levels providing a 81% for NO<sub>2</sub>, 67% for CO and 46% for PM<sub>10</sub>;measures defined in the plan achieve to reduce up to 11 μgm<sup>-3</sup> NO<sub>2</sub> levels offering highest reductions over urban areas with traffic influence.展开更多
The overall objective of this study was to establish the effects of steel industrial effluent on Nairobi metropolitan water system and its impact to the society. The study sought to identify various types of wastes pr...The overall objective of this study was to establish the effects of steel industrial effluent on Nairobi metropolitan water system and its impact to the society. The study sought to identify various types of wastes produced by factories, assess how the waste generated is managed and disposed</span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;">,</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;"> examine the effects of effluent discharge on Nairobi River and finally propose mitigation measures. The research adopted a qualitative design and employed a number of methods: direct observations, document reviews to content analysis of the past studies, which in the end generated invaluable data. The study revealed that there are four categories of waste generated</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;">:</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;"> solid waste, liquid waste, footbath chemicals as well as thermal wastes. It was also found that waste management in place w</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;">as</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;"> not effective enough leading to water and soil pollution. Other causes of pollution were found out to emanate from gasses contamination to the air and chemicals used during steel processing. The findings will inform the community of the harmful effects of untreated water and how it impacts on their health and productivity. It will also help the stakeholders in the environmental conservation to articulate issues of policy and influence agenda setting in the national and sub-national levels.展开更多
文摘CO_(2)捕集、利用与封存(CO_(2)Capture, Utilization and Storage, CCUS)技术是减少碳排放的有效手段之一,是实现中国“双碳”目标的重要技术保障,其中CO_(2)管道输送是最重要的一环。从CCUS技术和CO_(2)管道设计两个维度综述了国内外CO_(2)捕集、CO_(2)运输、CO_(2)封存和CO_(2)利用的研究进展,针对运输过程,着重从工艺设计、杂质、含水量、止裂控制和风险评估等方面梳理了CO_(2)管道设计的研究成果。中国目前正在大力推进CCUS技术,中国石油、中国石化和中国海洋石油等机构分别成立了相关的研究机构,聚焦CCUS发展的各个环节。虽然中国尚处于技术发展的初级阶段,但相信随着科研人员的努力会很快赶超发达国家,跻身第一方阵。研究结果旨在为中国的CCUS技术发展提供参考,促进中国CCUS技术的推广实施和CO_(2)管道的合理设计。
基金supported by the National Natural Science Foundation of China(51825802,52130803,52278020,and 72374121)the China National Key Research and Development Program(2018YFE0106100)+1 种基金the China Postdoctoral Science Foundation(2022M711815)the New Cornerstone Science Foundation through the XPLORER PRIZE.
文摘The life-cycle assessment method,which originates from general products and services,has gradually come to be applied to investigations of the life-cycle carbon emissions(LCCE)of buildings.A literature review was conducted to clarify LCCE implications,calculations,and reductions in the context of buildings.A total of 826 global building carbon emission calculation cases were obtained from 161 studies based on the framework of the building life-cycle stage division stipulated by ISO 21930 and the basic principles of the emission factor(EF)approach.The carbon emission calculation methods and results are discussed herein,based on the modules of production,construction,use,end-of-life,and supplementary benefits.According to the hotspot distribution of a building’s carbon emissions,carbon reduction strategies are classified into six groups for technical content and benefits analysis,including reducing the activity data pertaining to building materials and energy,reducing the carbon EFs of the building materials and energy,and exploiting the advantages of supplementary benefits.The research gaps and challenges in current building LCCE studies are summarized in terms of research goals and ideas,calculation methods,basic parameters,and carbon reduction strategies;development suggestions are also proposed.
文摘The lifecycle greenhouse gas(GHG)emissions(Well-to-Wake)from maritime transport must be reduced by at least 50%in absolute values by 2050 to contribute to the ambitions of the Paris Agreement(2015).A transition from conventional fuels to alternative fuels with zero or lower GHG emissions is viewed as the most promising avenue to reach the GHG reductions.Whereas GHG and toxic pollutants emitted from the use of fossil fuels(heavy fuel oil(HFO)and marine gas/diesel oil(MGO/MDO))are generally well understood,the emissions associated with the new fuel options are only now being measured and communicated.This review provides an outlook on fuels that could help shipping respond to the decarbonization effort including Liquefied Petroleum Gas(LPG),Liquefied Natural Gas(LNG),methanol,ammonia,and hydrogen.A quantification of the pollutants associated from the use of these fuels is provided and challenges and barriers to their uptake are discussed.
基金supported by the National Natural Science Foundation of China(NSFC)(31872403)the Foundation for Youth Innovation Promotion Association of the Chinese Academy of Sciences(2019101)+2 种基金the UNCNET—a project funded under the JPI Urban Europe/China collaboration,project numbers 71961137011(NSFC,China)and 870234(FFG,Austria)the FABLE Consortiumthe financial support of the Norwegian Ministry of Climate and Environment。
文摘In China,there has been insufficient study of whole food system greenhouse gas(GHG)accounting,which limits the development of mitigation strategies and may preclude the achievement of carbon peak and carbon neutrality goals.The paper presents the development of a carbon extension of NUFER(NUtrient flows in Food chain,Environment and Resources use model),a food system GHG emission accounting model that covers land use and land-use change,agricultural production,and post-production subsectors.The spatiotemporal characteristics of GHG emissions were investigated for the Chinese food system(CFS)from 1992 to 2017,with a focus on GHG emissions from the entire system.The potential to achieve a low-carbon food system in China was explored.The net GHG emissions from the CFS increased from 785Tg CO_(2)equivalent(CO_(2)-eq)in 1992 to 1080 Tg CO_(2)-eq in 2017.Agricultural activities accounted for more than half of the total emissions during the study period,while agricultural energy was the largest contributor to the GHG increase.In 2017,highest emitting regions were located in central and southern China(Guangdong and Hunan),the North China Plain(Shandong,Henan and Jiangsu)and Northeast China(Heilongjiang and Inner Mongolia)and contributed to over half of the total GHG emissions.Meanwhile,Xinjiang,Qinghai and Tibet are shown as carbon sink areas.It was found that foodsystem GHG emissions could be reduced to 355 Tg CO_(2)-eq,where enhancing endpoint mitigation technologies,transforming social-economic and diet conditions,and increasing agricultural productivities can contribute to 60%,25%and 15%,respectively.Synergistic mitigation effects were found to exist in agricultural activities.
基金This work was supported by the National Basic Research Program of China （No. 2012CB955800）, the National Social Science Foundation of China （Grant No. 14CGJ025） and the CAS Strategic Priority Research Program （Grant No. XDA05150900）.
文摘Climate financing is a key issue in current negotiations on climate protection. This study establishes a climate financing model based on a mechanism in which donor countries set up funds for climate financing and recipient countries use the funds exclusively for carbon emission reduction. The burden-sharing principles are based on GDP, historical emissions, and consumption- based emissions. Using this model, we develop and analyze a series of scenario simulations, including a financing program negotiated at the Cancun Climate Change Conference （2010） and several subsequent programs. Results show that sustained climate financing can help to combat global climate change. However, the Cancun Agreements are projected to result in a reduction of only 0.0I^C in global warming by 2100 compared to the scenario without climate financing. Longer-term climate financing programs should be established to achieve more significant benefits. Our model and simulations also show that climate financing has economic benefits for develop- ing countries. Developed countries will suffer a slight GDP loss in the early stages of climate financing, but the long- term economic growth and the eventual benefits of climate mitigation will compensate for this slight loss. Different burden-sharing principles have very similar effects on global temperature change and economic growth of recipient countries, but they do result in differences in GDP changes for Japan and the FSU. The GDP-based principle results in a larger share of financial burden for Japan, while the historical emissions-based principle results in a larger share of financial burden for the FSU. A larger burden share leads to a greater GDP loss.
基金supported by the National Key Research and Development Program of China(No.2017YFA0605003)the National Natural Science Foundation of China(Nos.51922010,41521003).
文摘Emission intensity and climate change control the transport flux and fate of persistent organic pollutants(POPs)inmultiple environmental compartments.This study applied amultimedia model(BETR model)to explore alternations in the spatio-temporal trends of concentrations and transport flux of benzopyrene(BaP),phenanthrene(Phe),perfluorooctane sulfonates(PFOS)and polychlorinated biphenyls(PCBs)in the Chaohu watershed,located in the lower reaches of the Yangtze River,China in response to changes in source emissions and climate.The potential historic and future risks of these pollutants also were assessed.The results suggest that current trends in concentrations and transport were similar to that of their emissions between 2005 and 2018.During the next 100 years,temporal trends and spatial patterns were not predicted to change significantly,which is consistent with climate change.Based on sensitivity and correlation analyses,climate change had significant effects on multi-media concentrations and transport fluxes of BaP,Phe,PFOS and PCBs,and rainfall intensity was the predominant controlling factor.Risk quotients(RQs)of BaP and Phe-in soil increased from 0.42 to 0.95 and 0.06 to 0.35,respectively,from 2005 to 2090,indicating potential risks.The RQs of the other examined contaminants exhibited little potential risk in soil,water,or sediment.Based on spatial patterns,it was inferred that the ecosystem around Lake Chaohu is the most at risk.The study provides insights needed for local pollution control of POPs in the Chaohu watershed.In addition,the developed approach can be applied to other watersheds world-wide.
文摘In this contribution, we use a coupled air quality modelling system (AQM) as a tool to design and develop an air quality plan in Madrid. AQM has allowed us to obtain a preliminary evaluation of the effect of mitigation measures over regional and local air quality levels. To achieve these goals, we have prepared a sophisticated AQM, coupling the meteorological model WRF, the emission model AEMM, and the photochemical model CMAQ. AQM was evaluated using the whole modelling year 2010 working with high horizontal resolution, 3 km for the region of Madrid and 1km for urban metropolitan area of Madrid. Two different analyses have been realized: a source apportionment exercise following a zero-out methodology to obtain the contribution to the air quality levels of the different emission sector;and an evaluation of the main mitigation measures considered in the air quality plan using sensitivity analysis. The air quality plan was focused on the improvement of NO<sub>2</sub> levels and AQM analyzed the effect of the mitigation measures during ten episodes of 2011 where NO<sub>2</sub> or O<sub>3</sub> levels were the highest of the year;so we analyzed the effect of the mitigation plan in worst conditions. Results provided by the AQM system show that it accomplishes the European Directive modelling uncertainty requirements and the mean absolute gross error for 1-h maximum daily NO<sub>2</sub> is 31% over locations with higher levels of this atmospheric pollutant;the road traffic is the main contributor to the air quality levels providing a 81% for NO<sub>2</sub>, 67% for CO and 46% for PM<sub>10</sub>;measures defined in the plan achieve to reduce up to 11 μgm<sup>-3</sup> NO<sub>2</sub> levels offering highest reductions over urban areas with traffic influence.
文摘The overall objective of this study was to establish the effects of steel industrial effluent on Nairobi metropolitan water system and its impact to the society. The study sought to identify various types of wastes produced by factories, assess how the waste generated is managed and disposed</span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;">,</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;"> examine the effects of effluent discharge on Nairobi River and finally propose mitigation measures. The research adopted a qualitative design and employed a number of methods: direct observations, document reviews to content analysis of the past studies, which in the end generated invaluable data. The study revealed that there are four categories of waste generated</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;">:</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;"> solid waste, liquid waste, footbath chemicals as well as thermal wastes. It was also found that waste management in place w</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;">as</span></span></span><span style="font-family:Verdana;"><span style="font-family:Verdana;"><span style="font-family:Verdana;"> not effective enough leading to water and soil pollution. Other causes of pollution were found out to emanate from gasses contamination to the air and chemicals used during steel processing. The findings will inform the community of the harmful effects of untreated water and how it impacts on their health and productivity. It will also help the stakeholders in the environmental conservation to articulate issues of policy and influence agenda setting in the national and sub-national levels.
