The absorption spectrum of carbon dioxide at 2.004 μm has been recorded at sample temperatures between 218.0 K and room temperature, by using a high-resolution tunable diode laser absorption spectrometer（TDLAS） com...The absorption spectrum of carbon dioxide at 2.004 μm has been recorded at sample temperatures between 218.0 K and room temperature, by using a high-resolution tunable diode laser absorption spectrometer（TDLAS） combined with a temperature controlled cryogenically cooled absorption cell. The self-, N^（2-）, and air-broadening coefficients for nine transitions of ^（12）C^（16）O_2 belonging to the 20012←00001 band in the 4987 cm^（-1）–4998 cm^（-1） region have been measured at different temperatures. From these measurements, we have further determined the temperature dependence exponents of the pressure-broadening coefficients. To the best of our knowledge, the temperature dependence parameters of the collisional broadening coefficients are reported experimentally for the first time for these nine transitions. The measured halfwidth coefficients and the air temperature dependence exponents of these transitions are compared with the available values reported in the literature and HITRAN 2012 database. Agreements and discrepancies are also discussed.展开更多
In this work, a new full quantum method is proposed to calculate the broadening and shift coefficients of the D1 line in neutral collision. Based on the variable phase approach and Baranger theory, this method calcula...In this work, a new full quantum method is proposed to calculate the broadening and shift coefficients of the D1 line in neutral collision. Based on the variable phase approach and Baranger theory, this method calculates the scattering phase shift instead of scattering matrix elements in order to simplify the calculation. As an illustration, this method is used to calculate the broadening and shift coefficients of the absorption lines of alkali metal atom Rb, as it collides with buffer gas He and Ar, in a temperature range from 150 K to 800 K. With a comparison with other calculations and experiment measurements, the reasonable agreements in all cases demonstrate the validity and simplicity of this method.展开更多
The Monte Carlo simulation is performed to investigate the quantum mechanical （QM） effects on heat generation in nano-scale metal oxide semiconductor field effect transistors （MOSFETs） by solving the quantum Boltz...The Monte Carlo simulation is performed to investigate the quantum mechanical （QM） effects on heat generation in nano-scale metal oxide semiconductor field effect transistors （MOSFETs） by solving the quantum Boltzmann equation. The influence of QM effects both in real space and K space on the heat generation is investigated.展开更多
We modify a uniform model of single bubble sonoluminescence,in which heat diffusion,water vapor diffusion and chemical reactions are included to describe the bubble dynamics,and the processes of electron-atom bremsstr...We modify a uniform model of single bubble sonoluminescence,in which heat diffusion,water vapor diffusion and chemical reactions are included to describe the bubble dynamics,and the processes of electron-atom bremsstrahlung,electron-ion bremsstrahlung and recombination radiation,radiative attachment of electrons to atoms and molecules,line emissions of OH radicals and Na atoms are taken into account to calculate the light emission. With this model,we compute the light pulse width,the photon number per flash,the continuum and line spectra and the gas species as the products of chemical reactions,and try to compare with all the experimental data available. We obtain good agreement with the observations of Ar and Xe bubbles in many cases,but fail to match the experimental data of the photon number per flash. We also find that for He bubble the computed photon number is always too small to interpret the observations.展开更多
We apply two-photon resonant nondegenerate four-wave mixing with a resonant intermediate state to the obser-vation of the broadening and shifting of the barium Rydberg level 6s24d 1^D2 by collision with argon. The col...We apply two-photon resonant nondegenerate four-wave mixing with a resonant intermediate state to the obser-vation of the broadening and shifting of the barium Rydberg level 6s24d 1^D2 by collision with argon. The collision broadening and shifting cross sections are measured. This technique is purely optical, and can investigate the pressure dependence of the transverse relaxation rate-P21 between the Rydberg state and an intermediate state, as well as the transverse relaxation rate F20 between the Rydberg state and the ground state.展开更多
基金Project supported by the Young Scientists Fund of the National Natural Science Foundation of China(Grant Nos.41205021 and 61701006)the Youth Innovation Promotion Association of the Chinese Academy of Sciences(Grant No.2015264)the Scientific Research Foundation of the Higher Education Institutions of Anhui Province,China(Grant No.KJ2015A234)
文摘The absorption spectrum of carbon dioxide at 2.004 μm has been recorded at sample temperatures between 218.0 K and room temperature, by using a high-resolution tunable diode laser absorption spectrometer（TDLAS） combined with a temperature controlled cryogenically cooled absorption cell. The self-, N^（2-）, and air-broadening coefficients for nine transitions of ^（12）C^（16）O_2 belonging to the 20012←00001 band in the 4987 cm^（-1）–4998 cm^（-1） region have been measured at different temperatures. From these measurements, we have further determined the temperature dependence exponents of the pressure-broadening coefficients. To the best of our knowledge, the temperature dependence parameters of the collisional broadening coefficients are reported experimentally for the first time for these nine transitions. The measured halfwidth coefficients and the air temperature dependence exponents of these transitions are compared with the available values reported in the literature and HITRAN 2012 database. Agreements and discrepancies are also discussed.
基金Project supported by the National Natural Science Foundation of China(Grants Nos.11405077 and 11575073)
文摘In this work, a new full quantum method is proposed to calculate the broadening and shift coefficients of the D1 line in neutral collision. Based on the variable phase approach and Baranger theory, this method calculates the scattering phase shift instead of scattering matrix elements in order to simplify the calculation. As an illustration, this method is used to calculate the broadening and shift coefficients of the absorption lines of alkali metal atom Rb, as it collides with buffer gas He and Ar, in a temperature range from 150 K to 800 K. With a comparison with other calculations and experiment measurements, the reasonable agreements in all cases demonstrate the validity and simplicity of this method.
基金supported by the National Key Basic Research Program of China (Grant No 2006CB302705)the National Natural Science Foundation of China (Grant No 60776068)
文摘The Monte Carlo simulation is performed to investigate the quantum mechanical （QM） effects on heat generation in nano-scale metal oxide semiconductor field effect transistors （MOSFETs） by solving the quantum Boltzmann equation. The influence of QM effects both in real space and K space on the heat generation is investigated.
基金Supported by the National Natural Science Foundation of China (Grant Nos. 10674081 and 10434070)
文摘We modify a uniform model of single bubble sonoluminescence,in which heat diffusion,water vapor diffusion and chemical reactions are included to describe the bubble dynamics,and the processes of electron-atom bremsstrahlung,electron-ion bremsstrahlung and recombination radiation,radiative attachment of electrons to atoms and molecules,line emissions of OH radicals and Na atoms are taken into account to calculate the light emission. With this model,we compute the light pulse width,the photon number per flash,the continuum and line spectra and the gas species as the products of chemical reactions,and try to compare with all the experimental data available. We obtain good agreement with the observations of Ar and Xe bubbles in many cases,but fail to match the experimental data of the photon number per flash. We also find that for He bubble the computed photon number is always too small to interpret the observations.
基金Project supported by the Young Scientists Fund of the National Natural Science Foundation of China (Grant No. 10804025)the Natural Science Foundation of Hebei Province,China (Grant No. A2009000147)the Fundation for Photoelectronic Materia Research Base of Natural Science Foundation of Hebei Province,China (Grant Nos. 08B006 and 08B008)
文摘We apply two-photon resonant nondegenerate four-wave mixing with a resonant intermediate state to the obser-vation of the broadening and shifting of the barium Rydberg level 6s24d 1^D2 by collision with argon. The collision broadening and shifting cross sections are measured. This technique is purely optical, and can investigate the pressure dependence of the transverse relaxation rate-P21 between the Rydberg state and an intermediate state, as well as the transverse relaxation rate F20 between the Rydberg state and the ground state.
