Atmospheric aerosols （acting as cloud condensation nuclei） can enhance the cloud droplet number concentration and reduce the cloud droplet size, and in turn affect the cloud optical depth, as well as the cloud albed...Atmospheric aerosols （acting as cloud condensation nuclei） can enhance the cloud droplet number concentration and reduce the cloud droplet size, and in turn affect the cloud optical depth, as well as the cloud albedo, and thereby exert a radiative influence on climate （the first indirect aerosol effect）. In this paper, based on various relationships between cloud droplet spectral dispersion （c） and cloud droplet number concentration （Nc）, we analytically derive the corresponding expressions of the cloud radiative forcing induced by changes in the cloud droplet number concentration. Further quantitative evaluation indicates that the cloud radiative forcing induced by aerosols for the different ^-Nc relationships varies from -29.1% to 25.2%, compared to the case without considering spectral dispersion （e = 0）. Our results suggest that an accurate description of e - Nc relationships helps to reduce the uncertainty of the first indirect aerosol effect and advances our scientific understanding of aerosol-cloud-radiation interactions.展开更多
The knowledge of two-phase cloud dispersion mechanism from HLG(hazardous liquefied gas) release is the prerequisite for accurate assessment and precise rescue of such accidents. In this paper, an experiment of two-pha...The knowledge of two-phase cloud dispersion mechanism from HLG(hazardous liquefied gas) release is the prerequisite for accurate assessment and precise rescue of such accidents. In this paper, an experiment of two-phase cloud dispersion from liquefied CO_(2) hole release is performed. The source terms, such as vapour mass fraction, release velocity and mean droplet diameter, are calculated based on thermodynamic theory. Taking phase transition of CO_(2) droplets to gas into account, CFD(computational fluid dynamics) model for two-phase cloud dispersion is established. The predicted cloud temperatures at the downstream agree well with the experimental data, with the maximum relative error of 5.8% and average relative error of 2.3%. The consequence distances in the downstream direction and in the crosswise direction calculated through two-phase model are larger than those through single-phase model,with the relative differences of 57.8% and 53.6% respectively. CO_(2) concentration calculated by twophase model is smaller in the vicinity of release hole, and larger beyond 0.135 m downstream. A smaller leakage rate results in a lower CO_(2) concentration and a higher cloud temperature.展开更多
The dispersion of the fuel due to the center high explosive, including several different physical stages, is analyzed by means of experimental results observed with a high speed motion analysis system, and the effect ...The dispersion of the fuel due to the center high explosive, including several different physical stages, is analyzed by means of experimental results observed with a high speed motion analysis system, and the effect of center high explosive charge is suggested. The process of the fuel dispersion process can be divided into three main stages, acceleration, deceleration and turbulence. Within a certain scope, the radius of the final fuel cloud dispersed is independent of the center explosive charge mass in an FAE (fuel air explosive) device, while only dependent both on the duration of acceleration stage and on that of the deceleration. In these two stages, the dispersion of the fuel dust mainly occurs along the radial direction. There is a close relation between the fuel dispersion process and the center explosive charge mass. To describe the motion of fuel for different stages of dispersion, different mechanical models should be applied.展开更多
From first principles, we find that the radar threshold reflectivity between nonprecipitating clouds and precipitating clouds is strongly related to not only the cloud droplet number concentration but also the spectra...From first principles, we find that the radar threshold reflectivity between nonprecipitating clouds and precipitating clouds is strongly related to not only the cloud droplet number concentration but also the spectral dispersion of cloud droplet size distributions. The further investigation indicates that the threshold value is an increasing function of spectral dispersion and cloud droplet number concentration. These results may improve our understanding of the cloud-precipitation interaction and the aerosol indirect effect.展开更多
The relative dispersion of the cloud droplet spectra or the shape parameter is usually assumed to be a constant in the two-parameter cloud microphysical scheme, or is derived through statistical analysis. However, obs...The relative dispersion of the cloud droplet spectra or the shape parameter is usually assumed to be a constant in the two-parameter cloud microphysical scheme, or is derived through statistical analysis. However, observations have revealed that the use of such methods is not applicable for all actual cases. In this study, formulas were derived based on cloud microphysics and the properties of gamma function to solve the average cloud droplet radius and the cloud droplet spectral shape parameter. The gamma distribution shape parameter, relative dispersion, and cloud droplet spectral distribution can be derived through solving the droplet spectral shape parameter equation using the average droplet radius, volume radius, and their ratio, thereby deriving an analytic solution. We further examined the equation for the droplet spectral shape parameter using the observational droplet spectral data, and results revealed the feasibility of the method. In addition, when the method was applied to the two-parameter cloud microphysical scheme of the Weather Research and Forecast(WRF) model to further examine its feasibility, the modeling results showed that it improved precipitation simulation performance, thereby indicating that it can be utilized in two-parameter cloud microphysical schemes.展开更多
Cloud droplet dispersion is an important parameter in estimating aerosol indirect effect on climate in general circulation models（GCMs）.This study investigates droplet dispersion in shallow cumulus clouds under diff...Cloud droplet dispersion is an important parameter in estimating aerosol indirect effect on climate in general circulation models（GCMs）.This study investigates droplet dispersion in shallow cumulus clouds under different aerosol conditions using three-dimensional large eddy simulations（LES）.It is found that cloud droplet mean radius,standard deviation,and relative dispersion generally decrease as aerosol mixing ratio increases from 25 mg-1（clean case） to 100 mg-1（moderate case）,and to 2000 mg-1（polluted case）.Under all the three simulated aerosol conditions,cloud droplet mean radius and standard deviation increase with height.However,droplet relative dispersion increases with height only in the polluted case,and does not vary with height in the clean and moderate cases.The mechanisms for cloud droplet dispersion are also investigated.An additional simulation without considering droplet collision-coalescence and sedimentation under the aerosol mixing ratio of 25 mg-1 shows smaller values of droplet mean radius,standard deviation,and relative dispersion as compared to the base clean case.This indicates that droplet collision-coalescence plays an important role in broadening droplet spectra.Results also suggest that the impact of homogeneous mixing on cumulus cloud droplet spectra is significant under all the three simulated aerosol conditions.In weak mixing（strong updraft） regions where clouds are closer to be adiabatic,cloud droplets tend to have larger mean radius,smaller standard deviation,and hence smaller relative dispersion than those in stronger mixing（downdraft or weak updraft） regions.The parameterized cloud optical depth in terms of cloud liquid water content,droplet number concentration,and relative dispersion is only slightly smaller than the result calculated from detailed droplet spectra,indicating that current parameterization of cloud optical depth as used in many GCMs is plausible for low clouds.展开更多
基金jointly supported by the National Natural Science Foundation of China (Grant No. 41105071)the CAS Strategic Priority Research Program (Grant No. XDA05110101)the National Basic Research Program of China (Grant No. 2011CB403406)
文摘Atmospheric aerosols （acting as cloud condensation nuclei） can enhance the cloud droplet number concentration and reduce the cloud droplet size, and in turn affect the cloud optical depth, as well as the cloud albedo, and thereby exert a radiative influence on climate （the first indirect aerosol effect）. In this paper, based on various relationships between cloud droplet spectral dispersion （c） and cloud droplet number concentration （Nc）, we analytically derive the corresponding expressions of the cloud radiative forcing induced by changes in the cloud droplet number concentration. Further quantitative evaluation indicates that the cloud radiative forcing induced by aerosols for the different ^-Nc relationships varies from -29.1% to 25.2%, compared to the case without considering spectral dispersion （e = 0）. Our results suggest that an accurate description of e - Nc relationships helps to reduce the uncertainty of the first indirect aerosol effect and advances our scientific understanding of aerosol-cloud-radiation interactions.
基金supported by the Natural Science Foundation of Shandong Province (ZR2021QB144)。
文摘The knowledge of two-phase cloud dispersion mechanism from HLG(hazardous liquefied gas) release is the prerequisite for accurate assessment and precise rescue of such accidents. In this paper, an experiment of two-phase cloud dispersion from liquefied CO_(2) hole release is performed. The source terms, such as vapour mass fraction, release velocity and mean droplet diameter, are calculated based on thermodynamic theory. Taking phase transition of CO_(2) droplets to gas into account, CFD(computational fluid dynamics) model for two-phase cloud dispersion is established. The predicted cloud temperatures at the downstream agree well with the experimental data, with the maximum relative error of 5.8% and average relative error of 2.3%. The consequence distances in the downstream direction and in the crosswise direction calculated through two-phase model are larger than those through single-phase model,with the relative differences of 57.8% and 53.6% respectively. CO_(2) concentration calculated by twophase model is smaller in the vicinity of release hole, and larger beyond 0.135 m downstream. A smaller leakage rate results in a lower CO_(2) concentration and a higher cloud temperature.
文摘The dispersion of the fuel due to the center high explosive, including several different physical stages, is analyzed by means of experimental results observed with a high speed motion analysis system, and the effect of center high explosive charge is suggested. The process of the fuel dispersion process can be divided into three main stages, acceleration, deceleration and turbulence. Within a certain scope, the radius of the final fuel cloud dispersed is independent of the center explosive charge mass in an FAE (fuel air explosive) device, while only dependent both on the duration of acceleration stage and on that of the deceleration. In these two stages, the dispersion of the fuel dust mainly occurs along the radial direction. There is a close relation between the fuel dispersion process and the center explosive charge mass. To describe the motion of fuel for different stages of dispersion, different mechanical models should be applied.
基金Project supported by the Special Foundation for China Nonprofit Industry (Grant No. GYHY200706036)the National Excellent Young Scientists Fund of the National Natural Science Foundation of China (Grant No. 40825008)the National Basic Research Program of China (Grant No. 2010CB833406)
文摘From first principles, we find that the radar threshold reflectivity between nonprecipitating clouds and precipitating clouds is strongly related to not only the cloud droplet number concentration but also the spectral dispersion of cloud droplet size distributions. The further investigation indicates that the threshold value is an increasing function of spectral dispersion and cloud droplet number concentration. These results may improve our understanding of the cloud-precipitation interaction and the aerosol indirect effect.
基金supported by National Basic Research Program of China(Grant No.2011CB403406)
文摘The relative dispersion of the cloud droplet spectra or the shape parameter is usually assumed to be a constant in the two-parameter cloud microphysical scheme, or is derived through statistical analysis. However, observations have revealed that the use of such methods is not applicable for all actual cases. In this study, formulas were derived based on cloud microphysics and the properties of gamma function to solve the average cloud droplet radius and the cloud droplet spectral shape parameter. The gamma distribution shape parameter, relative dispersion, and cloud droplet spectral distribution can be derived through solving the droplet spectral shape parameter equation using the average droplet radius, volume radius, and their ratio, thereby deriving an analytic solution. We further examined the equation for the droplet spectral shape parameter using the observational droplet spectral data, and results revealed the feasibility of the method. In addition, when the method was applied to the two-parameter cloud microphysical scheme of the Weather Research and Forecast(WRF) model to further examine its feasibility, the modeling results showed that it improved precipitation simulation performance, thereby indicating that it can be utilized in two-parameter cloud microphysical schemes.
基金Supported by the 11th Five-Year National Key Technology R&D Program of China under Grant No. 2006BAC12B003National Natural Science Foundation of China under Grant No. 40675004
文摘Cloud droplet dispersion is an important parameter in estimating aerosol indirect effect on climate in general circulation models（GCMs）.This study investigates droplet dispersion in shallow cumulus clouds under different aerosol conditions using three-dimensional large eddy simulations（LES）.It is found that cloud droplet mean radius,standard deviation,and relative dispersion generally decrease as aerosol mixing ratio increases from 25 mg-1（clean case） to 100 mg-1（moderate case）,and to 2000 mg-1（polluted case）.Under all the three simulated aerosol conditions,cloud droplet mean radius and standard deviation increase with height.However,droplet relative dispersion increases with height only in the polluted case,and does not vary with height in the clean and moderate cases.The mechanisms for cloud droplet dispersion are also investigated.An additional simulation without considering droplet collision-coalescence and sedimentation under the aerosol mixing ratio of 25 mg-1 shows smaller values of droplet mean radius,standard deviation,and relative dispersion as compared to the base clean case.This indicates that droplet collision-coalescence plays an important role in broadening droplet spectra.Results also suggest that the impact of homogeneous mixing on cumulus cloud droplet spectra is significant under all the three simulated aerosol conditions.In weak mixing（strong updraft） regions where clouds are closer to be adiabatic,cloud droplets tend to have larger mean radius,smaller standard deviation,and hence smaller relative dispersion than those in stronger mixing（downdraft or weak updraft） regions.The parameterized cloud optical depth in terms of cloud liquid water content,droplet number concentration,and relative dispersion is only slightly smaller than the result calculated from detailed droplet spectra,indicating that current parameterization of cloud optical depth as used in many GCMs is plausible for low clouds.
