Volatile organic compounds(VOCs)released from the waste treatment facilities have become a significant issue because they are not only causing odor nuisance but may also hazard to human health.Non-thermal plasma(NTP)t...Volatile organic compounds(VOCs)released from the waste treatment facilities have become a significant issue because they are not only causing odor nuisance but may also hazard to human health.Non-thermal plasma(NTP)technologies are newly developed methods and became a research trend in recent years regarding the removal of VOCs from the air stream.Due to its unique characteristics,such as rapid response at room temperature,bulk homogenized volume,high reaction efficiency,dielectric barrier discharge(DBD)plasma technology is considered one of the most promising techniques of NTP.This paper reviews recent progress of DBD plasma technology for abatement of VOCs.The principle of plasma generation in DBD and its configurations(electrode,discharge gap,dielectric barrier material,etc.)are discussed in details.Based on previously published literature,attention has been paid on the effect of DBD configuration on the removal of VOCs.Effect of various process parameters such as initial concentration,gas feeding rate,oxygen content and input power on VOCs removal are also considered.Moreover,the role of catalysis and inhibitors in VOCs removal by DBD system are presented.Finally,a modified configuration of the DBD reactor,i.e.double dielectric barrier discharge(DDBD)for the abatement of VOCs is discussed.It was suggested that the DDBD plasma reactor could be used for higher conversion efficiency as well as for avoiding solid residue deposition on the electrode.These depositions can interfere with the performance of the reactor.展开更多
Dielectric barrier discharge（DBD） plasma is considered to be a promising method to synthesize solid catalysts. In this work, DBD plasma was used to synthesize a nitrogen‐vacancy‐doped g‐C3N4 catalyst in situ for ...Dielectric barrier discharge（DBD） plasma is considered to be a promising method to synthesize solid catalysts. In this work, DBD plasma was used to synthesize a nitrogen‐vacancy‐doped g‐C3N4 catalyst in situ for the first time. X‐ray diffraction, N2 adsorption, ultraviolet–visible spectroscopy, scanning electron microscopy, transmission electron microscopy, X‐ray photoelectron spectrosco‐py, electrochemical impedance spectroscopy, electron paramagnetic resonance, O2 tempera‐ture‐programmed desorption, and photoluminescence were used to characterize the obtained cat‐alysts. The photocatalytic H2O2 production ability of the as‐prepared catalyst was investigated. The results show that plasma treatment influences the morphology, structure, and optical properties of the as‐prepared catalyst. Nitrogen vacancies are active centers, which can adsorb reactant oxygen molecules, trap photoelectrons, and promote the transfer of photoelectrons from the catalyst to the adsorbed oxygen molecules for the subsequent reduction reaction. This work provides a new strat‐egy for synthesizing g‐C3N4‐based catalysts.展开更多
In order to simulate the flow control problem by using Nanosecond Pulsed Dielectric Barrier Discharge(NSDBD),a one-zone inhomogeneous phenomenological model is constructed based on the experimental and theoretical res...In order to simulate the flow control problem by using Nanosecond Pulsed Dielectric Barrier Discharge(NSDBD),a one-zone inhomogeneous phenomenological model is constructed based on the experimental and theoretical results.The model is coupled with the unsteady Navier-Stokes equations,which can well predict the compression-expansion wave structures and wave speed compared with experimental results and can be applied to the simulation of the flow control by using NSDBD.The model is adopted to investigate the separation control over NACA0015 airfoil using the NSDBD plasma actuator.The separation-control mechanisms are revealed that the spanwise vortices produced by the plasma actuation play the key role.Each plasma actuation can produce a spanwise vortex around the separation point near the leading edge.The spanwise vortices make the separated free-shear layer unstable and shed away,move downstream along the upper wall,control the flow near the wall,and bring outer flow with high kinetic energy into the near wall region to realize the effective separation control over the upper surface of the airfoil.展开更多
Conversion of methane by steam reforming was carried out by means of dielectric-barrier discharge.A systemic procedure was employed to determine the suitable experimental conditions.It was found that one of the plasma...Conversion of methane by steam reforming was carried out by means of dielectric-barrier discharge.A systemic procedure was employed to determine the suitable experimental conditions.It was found that one of the plasma generators can match the system best.A higher power input can always bring a higher conversion,but the selectivity to C2H6 decreased from 52.48% to 39.43% as the power increased from 20W to 49W.When discharge distance was 4mm,selectivities to almost all main products reached the max.The inner electrode made of stainless steel and the outer electrode with aluminum foil were one of the best options which can obviously enhance the conversion of methane.A larger flow rate always resulted in a lower conversion of methane.In the most time,19.93% steam promoted conversion of methane.展开更多
The present paper described an experimental investigation of separation control of an Unmanned Aerial Vehicle(UAV)at high wind speeds.The plasma actuator was based on Dielectric Barrier Discharge(DBD)and operated in a...The present paper described an experimental investigation of separation control of an Unmanned Aerial Vehicle(UAV)at high wind speeds.The plasma actuator was based on Dielectric Barrier Discharge(DBD)and operated in a steady manner.The flow over a wing of UAV was performed with smoke flow visualization in theΦ0.75 m low speed wind tunnel to reveal the flow structure over the wing so that the locations of plasma actuators could be optimized.A full model of the UAV was experimentally investigated in theΦ3.2 m low speed wind tunnel using a six-component internal strain gauge balance.The effects of the key parameters,including the locations of the plasma actuators,the applied voltage amplitude and the operating frequency,were obtained.The whole test model was made of aluminium and acted as a cathode of the actuator.The results showed that the plasma acting on the surface of UAV could obviously suppress the boundary layer separation and reduce the model vibration at the high wind speeds.It was found that the maximum lift coefficient of the UAV was increased by 2.5%and the lift/drag ratio was increased by about 80%at the wind speed of 100 m/s.The control mechanism of the plasma actuator at the test configuration was also analyzed.展开更多
Flow control using surface Dielectric Barrier Discharge(DBD)plasma actuators driven by a sinusoidal alternating-current power supply has gained significant attention from the aeronautic industry.The induced flow field...Flow control using surface Dielectric Barrier Discharge(DBD)plasma actuators driven by a sinusoidal alternating-current power supply has gained significant attention from the aeronautic industry.The induced flow field of the plasma actuator,with the starting vortex in the wall jet,plays an important role in flow control.However,the energy consumed for producing the induced flow field is only a small fraction of the total energy utilized by the plasma actuator,and most of the total energy is used in gas heating and dielectric heating.Therefore,an in-depth analysis of the thermal characteristics of the plasma actuator is the key to develop its potential capability further.In addition,compared with the investigation on the aerodynamic characteristics of the plasma actuator,there is a relative lack of detail in the study of its thermal characteristics.Understanding the thermal characteristics of the plasma actuator is of great interest for providing a deeper insight into the underlying working principles,advancing its numerical simulation model,prolonging its life,and achieving several potential engineering applications,such as antiicing and deicing.The present paper reviews the thermal characteristics of the plasma actuator,summarizes the influence of the dielectric film and actuation parameters on heating,and discusses the formation and transfer mechanism of the induced heating based on the discharge regimes of the plasma actuator in one cycle.展开更多
A plasma-assisted catalytic reactor was used to remove nitrogen oxides (NOx)from diesel engine exhaust operated under different load conditions. Initial studies were focused onplasma reactor (a dielectric barrier disc...A plasma-assisted catalytic reactor was used to remove nitrogen oxides (NOx)from diesel engine exhaust operated under different load conditions. Initial studies were focused onplasma reactor (a dielectric barrier discharge reactor) treatment of diesel exhaust at varioustemperatures. The nitric oxide (NO) removal efficiency was lowered when high temperature exhaust wastreated using plasma reactor. Also, NO removal efficiency decreased when 45% load exhaust wastreated. Studies were then made with plasma reactor combined with a catalytic reactor consisting ofa selective catalytic reduction (SCR) catalyst, V_2O_5/TiO_2. Ammonia was used as a reducing agentfor SCR process in a ratio of 1:1 to NOx. The studies were focused on temperatures of the SCRcatalytic reactor below 200℃. The plasma-assisted catalytic reactor was operated well to remove NOxunder no-load and load conditions. For an energy input of 96 J/l, the NOx removal efficienciesobtained under no-load and load conditions were 90% and 72% respectively at an exhaust temperatureof 100 ℃.展开更多
In this work,based on the role of pre-ionization of the non-uniform electric field and its effect of reducing the collisional ionization coefficient,a diffuse dielectric barrier discharge plasma is formed in the open ...In this work,based on the role of pre-ionization of the non-uniform electric field and its effect of reducing the collisional ionization coefficient,a diffuse dielectric barrier discharge plasma is formed in the open space outside the electrode structure at a lower voltage by constructing a three-dimensional non-uniform spatial electric field using a contact electrode structure.The air purification study is also carried out.Firstly,a contact electrode structure is constructed using a three-dimensional wire electrode.The distribution characteristics of the spatial electric field formed by this electrode structure are analyzed,and the effects of the non-uniform electric field and the different angles of the vertical wire on the generation of three-dimensional spatial diffuse discharge are investigated.Secondly,the copper foam contact electrode structure is constructed using copper foam material,and the effects of different mesh sizes on the electric field distribution are analyzed.The results show that as the mesh size of the copper foam becomes larger,a strong electric field region exists not only on the surface of the insulating layer,but also on the surface of the vertical wires inside the copper foam,i.e.,the strong electric field region shows a three-dimensional distribution.Besides,as the mesh size increases,the area of the vertical strong electric field also increases.However,the electric field strength on the surface of the insulating layer gradually decreases.Therefore,the appropriate mesh size can effectively increase the discharge area,which is conducive to improving the air purification efficiency.Finally,a highly permeable stacked electrode structure of multilayer wire-copper foam is designed.In combination with an ozone treatment catalyst,an air purification device is fabricated,and the air purification experiment is carried out.展开更多
The three-electrode sliding dielectric barrier discharge(TES-DBD) plasma actuator significantly enhances the ionization rate and momentum exchange between charged particles and neutral particles by incorporating a par...The three-electrode sliding dielectric barrier discharge(TES-DBD) plasma actuator significantly enhances the ionization rate and momentum exchange between charged particles and neutral particles by incorporating a parallel DC electrode into the standard DBD design. This design improves the body force and induced jet velocity while allowing flexible control of the induced jet angle, overcoming the limitations of discharge extension and uncontrollable direction in traditional DBD plasma actuators. An integrated plasma power supply has been designed specifically for TES-DBD plasma actuators, streamlining the power supply management. The methodology involves designing the circuit topology for the TES-DBD power supply, followed by simulating and validating its operating principles using Multisim software. The operational performance of the power supply is evaluated through a comprehensive analysis of its electrical,thermal, and aerodynamic properties specific to TES-DBD plasma actuation.展开更多
SF_(6) has excellent insulation performance and arc extinguishing ability,and is widely used in the power industry.However,its global warming potential is about 23,500 times that of C0_(2),it can exist stably in the a...SF_(6) has excellent insulation performance and arc extinguishing ability,and is widely used in the power industry.However,its global warming potential is about 23,500 times that of C0_(2),it can exist stably in the atmosphere,it is not easily degradable and is of great potential harm to the environment.Based on pulsed dielectric barrier discharge plasma technology,the effects of H_(2)O and 0_(2) on the degradation of SF_(6) were studied.Studies have shown that H_(2)O can effectively promote the decomposition of SF_(6) and improve its degradation rate and energy efficiency of degradation.Under the action of a pulse input voltage and input frequency of 15 kV and 15 kHz,respectively,when H_(2)O is added alone the effect of 1% H_(2)O is the best,and the rate and energy efficiency of degradation of SF_(6) reach their maximum values,which are 91.9% and 8.25 g kWh^(-1),respectively.The synergistic effect of H_(2)O and O_(2) on the degradation of SF_(6) was similar to that of H_(2)O.When the concentration of H_(2)O and O_(2) was 1%,the system obtained the best rate and energy efficiency of degradation,namely 89.7% and 8.05 g kWh~(-1),respectively.At the same time,different external gases exhibit different capabilities to regulate decomposition products.The addition of H_(2)O can effectively improve the selectivity of S0_(2).Under the synergistic effect of H_(2)O and O_(2),with increase in O_(2) concentration the degradation products gradually transformed into SO_(2)F_(2).From the perspective of harmless treatment of the degradation products of SF_(6),the addition of O_(2) during the SF_(6) degradation process should be avoided.展开更多
Dielectric barrier discharge(DBD)is considered as a promising technique to produce large volume uniform plasma at atmospheric pressure,and the dielectric barrier layer between the electrodes plays a key role in the DB...Dielectric barrier discharge(DBD)is considered as a promising technique to produce large volume uniform plasma at atmospheric pressure,and the dielectric barrier layer between the electrodes plays a key role in the DBD processes and enhancing discharge uniformity.In this work,the uniformity and discharge characteristics of the nanosecond(ns)pulsed DBD with dielectric barrier layers made of alumina,quartz glass,polycarbonate(PC),and polypropylene(PP)are investigated via discharge image observation,voltage-current waveform measurement and optical emission spectral diagnosis.Through analyzing discharge image by gray value standard deviation method,the discharge uniformity is quantitatively calculated.The effects of the space electric field intensity,the electron density(Ne),and the space reactive species on the uniformity are studied with quantifying the gap voltage Ug and the discharge current Ig,analyzing the recorded optical emission spectra,and simulating the temporal distribution of Ne with a one-dimensional fluid model.It is found that as the relative permittivity of the dielectric materials increases,the space electric field intensity is enhanced,which results in a higher Ne and electron temperature(Te).Therefore,an appropriate value of space electric field intensity can promote electron avalanches,resulting in uniform and stable plasma by the merging of electron avalanches.However,an excessive value of space electric field intensity leads to the aggregation of space charges and the distortion of the space electric field,which reduce the discharge uniformity.The surface roughness and the surface charge decay are measured to explain the influences of the surface properties and the second electron emission on the discharge uniformity.The results in this work give a comprehensive understanding of the effect of the dielectric materials on the DBD uniformity,and contribute to the selection of dielectric materials for DBD reactor and the realization of atmospheric pressure uniform,stable,and reactive plasma sources展开更多
The discharge morphology of pulsed dielectric barrier discharge(PDBD) plays important roles in its applications. Here, we systematically investigated the effects of the voltage amplitude,discharge gap, and O_(2)conten...The discharge morphology of pulsed dielectric barrier discharge(PDBD) plays important roles in its applications. Here, we systematically investigated the effects of the voltage amplitude,discharge gap, and O_(2)content on the PDBD morphology, and revealed the possible underlying mechanism of the U-shaped formation. First, the morphological evolution under different conditions was recorded. A unique U-shaped region appears in the middle edge region when the gap is larger than 2 mm, while the entire discharge region remains columnar under a 2 mm gap in He PDBD. The width of the discharge and the U-shaped region increase with the increase in voltage, and decrease with the increase of the gap and O_(2)content. To explain this phenomenon,a two-dimensional symmetric model was developed to simulate the spatiotemporal evolution of different species and calculate the electric thrust. The discharge morphology evolution directly corresponds to the excited-state atomic reduction process. The electric thrust on the charged particles mainly determines the reaction region and strongly influences the U-shaped formation.When the gap is less than 2 mm, the electric thrust is homogeneous throughout the entire region,resulting in a columnar shape. However, when the gap is larger than 2 mm or O_(2)is added, the electric thrust in the edge region becomes greater than that in the middle, leading to the U-shaped formation. Furthermore, in He PDBD, the charged particles generating electric thrust are mainly electrons and helium ions, while in He/O_(2)PDBD those that generate electric thrust at the outer edge of the electrode surface are mainly various oxygen-containing ions.展开更多
Ice accretion on aircraft encountering supercooled water droplets in clouds poses great risks to flight performance and safety.With the aim of optimizing the newly developed streamwise plasma heat knife method for ant...Ice accretion on aircraft encountering supercooled water droplets in clouds poses great risks to flight performance and safety.With the aim of optimizing the newly developed streamwise plasma heat knife method for anti-icing,a parametric investigation is carried out in this work.The influence of the detailed voltage profile on the heating effects of a Surface Dielectric Barrier Discharge driven by Nanosecond Pulses(NS-SDBD)is investigated,and a comparison of the antiicing performance among different configurations of streamwise plasma heat knife is made.The results show that columnar high-temperature regions produced by a multi-streamer discharge appear at small pulse rise time,but become diffuse as the pulse rise time increases.An optimal pulse rise time exists to provide a wide range and high value of temperature,which is found to be 150 ns for the setup in the present study.The influence of the pulse fall time is much weaker than that of the rise time.The range and value of the temperature decrease with increasing pulse fall time.A greater pulse width is found to improve the heating effect by increasing the discharge power.When a spanwise electrode is placed connecting the streamwise electrodes of the streamwise plasma heat knife at the airfoil leading edge,the anti-icing performance becomes poorer,whereas good performance is achieved when the spanwise electrode is at the edge of the streamwise electrodes.Based on this,a three-level configuration of the plasma heat knife is proposed,and its anti-icing performance is found to be much better than that of the original configuration.展开更多
Continuous processes which allow for large amount of wastewater to be treated to meet drainage standards while reducing treatment time and energy consumption are urgently needed. In this study, a dielectric barrier di...Continuous processes which allow for large amount of wastewater to be treated to meet drainage standards while reducing treatment time and energy consumption are urgently needed. In this study, a dielectric barrier discharge plasma water bed system was designed and then coupled with granular activated carbon (GAC) adsorption to rapidly remove acid fuchsine (AF) with high efficiency. Effects of feeding gases, treatment time and initial concentration of AF on removal efficiency were investigated. Results showed that compared to the N2 and air plasmas treatments, O2 plasma processing was most effective for AF degradation due to the strong oxidation ability of generated activated species, especially the OH radicals. The addition of GAC significantly enhanced the removal efficiency of AF in aqueous solution and shorten the required time by 50%. The effect was attributed to the ability of porous carbon to trap and concentrate the dye, increasing the time dye molecules were exposed to the plasma discharge zone, and to enhance the production of OH radicals on/in GAC to boost the degradation of dyes by plasma as well as in situ regenerate the exhausted GAC. The study offers a new opportunity for continuous effective remediation of wastewater contaminated with organic dyes using plasma technologies.展开更多
文摘Volatile organic compounds(VOCs)released from the waste treatment facilities have become a significant issue because they are not only causing odor nuisance but may also hazard to human health.Non-thermal plasma(NTP)technologies are newly developed methods and became a research trend in recent years regarding the removal of VOCs from the air stream.Due to its unique characteristics,such as rapid response at room temperature,bulk homogenized volume,high reaction efficiency,dielectric barrier discharge(DBD)plasma technology is considered one of the most promising techniques of NTP.This paper reviews recent progress of DBD plasma technology for abatement of VOCs.The principle of plasma generation in DBD and its configurations(electrode,discharge gap,dielectric barrier material,etc.)are discussed in details.Based on previously published literature,attention has been paid on the effect of DBD configuration on the removal of VOCs.Effect of various process parameters such as initial concentration,gas feeding rate,oxygen content and input power on VOCs removal are also considered.Moreover,the role of catalysis and inhibitors in VOCs removal by DBD system are presented.Finally,a modified configuration of the DBD reactor,i.e.double dielectric barrier discharge(DDBD)for the abatement of VOCs is discussed.It was suggested that the DDBD plasma reactor could be used for higher conversion efficiency as well as for avoiding solid residue deposition on the electrode.These depositions can interfere with the performance of the reactor.
基金supported by the Pilot Program of University of Liaoning Innovation and Education Reform~~
文摘Dielectric barrier discharge（DBD） plasma is considered to be a promising method to synthesize solid catalysts. In this work, DBD plasma was used to synthesize a nitrogen‐vacancy‐doped g‐C3N4 catalyst in situ for the first time. X‐ray diffraction, N2 adsorption, ultraviolet–visible spectroscopy, scanning electron microscopy, transmission electron microscopy, X‐ray photoelectron spectrosco‐py, electrochemical impedance spectroscopy, electron paramagnetic resonance, O2 tempera‐ture‐programmed desorption, and photoluminescence were used to characterize the obtained cat‐alysts. The photocatalytic H2O2 production ability of the as‐prepared catalyst was investigated. The results show that plasma treatment influences the morphology, structure, and optical properties of the as‐prepared catalyst. Nitrogen vacancies are active centers, which can adsorb reactant oxygen molecules, trap photoelectrons, and promote the transfer of photoelectrons from the catalyst to the adsorbed oxygen molecules for the subsequent reduction reaction. This work provides a new strat‐egy for synthesizing g‐C3N4‐based catalysts.
基金supported by the National Natural Science Foundation of China(Grant Nos.10972236,50906100)
文摘In order to simulate the flow control problem by using Nanosecond Pulsed Dielectric Barrier Discharge(NSDBD),a one-zone inhomogeneous phenomenological model is constructed based on the experimental and theoretical results.The model is coupled with the unsteady Navier-Stokes equations,which can well predict the compression-expansion wave structures and wave speed compared with experimental results and can be applied to the simulation of the flow control by using NSDBD.The model is adopted to investigate the separation control over NACA0015 airfoil using the NSDBD plasma actuator.The separation-control mechanisms are revealed that the spanwise vortices produced by the plasma actuation play the key role.Each plasma actuation can produce a spanwise vortex around the separation point near the leading edge.The spanwise vortices make the separated free-shear layer unstable and shed away,move downstream along the upper wall,control the flow near the wall,and bring outer flow with high kinetic energy into the near wall region to realize the effective separation control over the upper surface of the airfoil.
基金Supported by the National iqatural Science Foundation of China （20606023, 20490203）.
文摘Conversion of methane by steam reforming was carried out by means of dielectric-barrier discharge.A systemic procedure was employed to determine the suitable experimental conditions.It was found that one of the plasma generators can match the system best.A higher power input can always bring a higher conversion,but the selectivity to C2H6 decreased from 52.48% to 39.43% as the power increased from 20W to 49W.When discharge distance was 4mm,selectivities to almost all main products reached the max.The inner electrode made of stainless steel and the outer electrode with aluminum foil were one of the best options which can obviously enhance the conversion of methane.A larger flow rate always resulted in a lower conversion of methane.In the most time,19.93% steam promoted conversion of methane.
基金supported by the Exploration Foundation of Weapon Systems(Grant No.7130711)
文摘The present paper described an experimental investigation of separation control of an Unmanned Aerial Vehicle(UAV)at high wind speeds.The plasma actuator was based on Dielectric Barrier Discharge(DBD)and operated in a steady manner.The flow over a wing of UAV was performed with smoke flow visualization in theΦ0.75 m low speed wind tunnel to reveal the flow structure over the wing so that the locations of plasma actuators could be optimized.A full model of the UAV was experimentally investigated in theΦ3.2 m low speed wind tunnel using a six-component internal strain gauge balance.The effects of the key parameters,including the locations of the plasma actuators,the applied voltage amplitude and the operating frequency,were obtained.The whole test model was made of aluminium and acted as a cathode of the actuator.The results showed that the plasma acting on the surface of UAV could obviously suppress the boundary layer separation and reduce the model vibration at the high wind speeds.It was found that the maximum lift coefficient of the UAV was increased by 2.5%and the lift/drag ratio was increased by about 80%at the wind speed of 100 m/s.The control mechanism of the plasma actuator at the test configuration was also analyzed.
基金support by the National Natural Science Foundation of China(No.11902336)State Key Laboratory of Aerodynamics Foundation of China(Nos.SKLA2019020201,JBKYC190103)+1 种基金CARDC Fundamental and Frontier Technology Research Fund,China(No.PJD20180144)China Scholarship Council.
文摘Flow control using surface Dielectric Barrier Discharge(DBD)plasma actuators driven by a sinusoidal alternating-current power supply has gained significant attention from the aeronautic industry.The induced flow field of the plasma actuator,with the starting vortex in the wall jet,plays an important role in flow control.However,the energy consumed for producing the induced flow field is only a small fraction of the total energy utilized by the plasma actuator,and most of the total energy is used in gas heating and dielectric heating.Therefore,an in-depth analysis of the thermal characteristics of the plasma actuator is the key to develop its potential capability further.In addition,compared with the investigation on the aerodynamic characteristics of the plasma actuator,there is a relative lack of detail in the study of its thermal characteristics.Understanding the thermal characteristics of the plasma actuator is of great interest for providing a deeper insight into the underlying working principles,advancing its numerical simulation model,prolonging its life,and achieving several potential engineering applications,such as antiicing and deicing.The present paper reviews the thermal characteristics of the plasma actuator,summarizes the influence of the dielectric film and actuation parameters on heating,and discusses the formation and transfer mechanism of the induced heating based on the discharge regimes of the plasma actuator in one cycle.
文摘A plasma-assisted catalytic reactor was used to remove nitrogen oxides (NOx)from diesel engine exhaust operated under different load conditions. Initial studies were focused onplasma reactor (a dielectric barrier discharge reactor) treatment of diesel exhaust at varioustemperatures. The nitric oxide (NO) removal efficiency was lowered when high temperature exhaust wastreated using plasma reactor. Also, NO removal efficiency decreased when 45% load exhaust wastreated. Studies were then made with plasma reactor combined with a catalytic reactor consisting ofa selective catalytic reduction (SCR) catalyst, V_2O_5/TiO_2. Ammonia was used as a reducing agentfor SCR process in a ratio of 1:1 to NOx. The studies were focused on temperatures of the SCRcatalytic reactor below 200℃. The plasma-assisted catalytic reactor was operated well to remove NOxunder no-load and load conditions. For an energy input of 96 J/l, the NOx removal efficienciesobtained under no-load and load conditions were 90% and 72% respectively at an exhaust temperatureof 100 ℃.
基金supported by the Fundamental Research Funds for the Central Universities(No.2022YJS094)。
文摘In this work,based on the role of pre-ionization of the non-uniform electric field and its effect of reducing the collisional ionization coefficient,a diffuse dielectric barrier discharge plasma is formed in the open space outside the electrode structure at a lower voltage by constructing a three-dimensional non-uniform spatial electric field using a contact electrode structure.The air purification study is also carried out.Firstly,a contact electrode structure is constructed using a three-dimensional wire electrode.The distribution characteristics of the spatial electric field formed by this electrode structure are analyzed,and the effects of the non-uniform electric field and the different angles of the vertical wire on the generation of three-dimensional spatial diffuse discharge are investigated.Secondly,the copper foam contact electrode structure is constructed using copper foam material,and the effects of different mesh sizes on the electric field distribution are analyzed.The results show that as the mesh size of the copper foam becomes larger,a strong electric field region exists not only on the surface of the insulating layer,but also on the surface of the vertical wires inside the copper foam,i.e.,the strong electric field region shows a three-dimensional distribution.Besides,as the mesh size increases,the area of the vertical strong electric field also increases.However,the electric field strength on the surface of the insulating layer gradually decreases.Therefore,the appropriate mesh size can effectively increase the discharge area,which is conducive to improving the air purification efficiency.Finally,a highly permeable stacked electrode structure of multilayer wire-copper foam is designed.In combination with an ozone treatment catalyst,an air purification device is fabricated,and the air purification experiment is carried out.
基金supported by National Natural Science Foundation of China (Nos. 61971345 and 52107174)。
文摘The three-electrode sliding dielectric barrier discharge(TES-DBD) plasma actuator significantly enhances the ionization rate and momentum exchange between charged particles and neutral particles by incorporating a parallel DC electrode into the standard DBD design. This design improves the body force and induced jet velocity while allowing flexible control of the induced jet angle, overcoming the limitations of discharge extension and uncontrollable direction in traditional DBD plasma actuators. An integrated plasma power supply has been designed specifically for TES-DBD plasma actuators, streamlining the power supply management. The methodology involves designing the circuit topology for the TES-DBD power supply, followed by simulating and validating its operating principles using Multisim software. The operational performance of the power supply is evaluated through a comprehensive analysis of its electrical,thermal, and aerodynamic properties specific to TES-DBD plasma actuation.
基金supported by Guizhou Province (Ceneral), grant/award number Qian Ke He Zhi Cheng [2022] General 207, National Natural Science Foundation of China (No. 52307170)Natural Science Foundation of Hubei Province, China (No. 2023AFB382)。
文摘SF_(6) has excellent insulation performance and arc extinguishing ability,and is widely used in the power industry.However,its global warming potential is about 23,500 times that of C0_(2),it can exist stably in the atmosphere,it is not easily degradable and is of great potential harm to the environment.Based on pulsed dielectric barrier discharge plasma technology,the effects of H_(2)O and 0_(2) on the degradation of SF_(6) were studied.Studies have shown that H_(2)O can effectively promote the decomposition of SF_(6) and improve its degradation rate and energy efficiency of degradation.Under the action of a pulse input voltage and input frequency of 15 kV and 15 kHz,respectively,when H_(2)O is added alone the effect of 1% H_(2)O is the best,and the rate and energy efficiency of degradation of SF_(6) reach their maximum values,which are 91.9% and 8.25 g kWh^(-1),respectively.The synergistic effect of H_(2)O and O_(2) on the degradation of SF_(6) was similar to that of H_(2)O.When the concentration of H_(2)O and O_(2) was 1%,the system obtained the best rate and energy efficiency of degradation,namely 89.7% and 8.05 g kWh~(-1),respectively.At the same time,different external gases exhibit different capabilities to regulate decomposition products.The addition of H_(2)O can effectively improve the selectivity of S0_(2).Under the synergistic effect of H_(2)O and O_(2),with increase in O_(2) concentration the degradation products gradually transformed into SO_(2)F_(2).From the perspective of harmless treatment of the degradation products of SF_(6),the addition of O_(2) during the SF_(6) degradation process should be avoided.
基金supported by National Natural Science Foundation of China(Nos.52037004 and 52177148)Postgraduate Research&Practice Innovation Program of Jiangsu Province(No.KYCX23_1449).
文摘Dielectric barrier discharge(DBD)is considered as a promising technique to produce large volume uniform plasma at atmospheric pressure,and the dielectric barrier layer between the electrodes plays a key role in the DBD processes and enhancing discharge uniformity.In this work,the uniformity and discharge characteristics of the nanosecond(ns)pulsed DBD with dielectric barrier layers made of alumina,quartz glass,polycarbonate(PC),and polypropylene(PP)are investigated via discharge image observation,voltage-current waveform measurement and optical emission spectral diagnosis.Through analyzing discharge image by gray value standard deviation method,the discharge uniformity is quantitatively calculated.The effects of the space electric field intensity,the electron density(Ne),and the space reactive species on the uniformity are studied with quantifying the gap voltage Ug and the discharge current Ig,analyzing the recorded optical emission spectra,and simulating the temporal distribution of Ne with a one-dimensional fluid model.It is found that as the relative permittivity of the dielectric materials increases,the space electric field intensity is enhanced,which results in a higher Ne and electron temperature(Te).Therefore,an appropriate value of space electric field intensity can promote electron avalanches,resulting in uniform and stable plasma by the merging of electron avalanches.However,an excessive value of space electric field intensity leads to the aggregation of space charges and the distortion of the space electric field,which reduce the discharge uniformity.The surface roughness and the surface charge decay are measured to explain the influences of the surface properties and the second electron emission on the discharge uniformity.The results in this work give a comprehensive understanding of the effect of the dielectric materials on the DBD uniformity,and contribute to the selection of dielectric materials for DBD reactor and the realization of atmospheric pressure uniform,stable,and reactive plasma sources
基金financial support from the Interdisciplinary Fund of the Wuhan National High Magnetic Field Center (No. WHMFC202101)。
文摘The discharge morphology of pulsed dielectric barrier discharge(PDBD) plays important roles in its applications. Here, we systematically investigated the effects of the voltage amplitude,discharge gap, and O_(2)content on the PDBD morphology, and revealed the possible underlying mechanism of the U-shaped formation. First, the morphological evolution under different conditions was recorded. A unique U-shaped region appears in the middle edge region when the gap is larger than 2 mm, while the entire discharge region remains columnar under a 2 mm gap in He PDBD. The width of the discharge and the U-shaped region increase with the increase in voltage, and decrease with the increase of the gap and O_(2)content. To explain this phenomenon,a two-dimensional symmetric model was developed to simulate the spatiotemporal evolution of different species and calculate the electric thrust. The discharge morphology evolution directly corresponds to the excited-state atomic reduction process. The electric thrust on the charged particles mainly determines the reaction region and strongly influences the U-shaped formation.When the gap is less than 2 mm, the electric thrust is homogeneous throughout the entire region,resulting in a columnar shape. However, when the gap is larger than 2 mm or O_(2)is added, the electric thrust in the edge region becomes greater than that in the middle, leading to the U-shaped formation. Furthermore, in He PDBD, the charged particles generating electric thrust are mainly electrons and helium ions, while in He/O_(2)PDBD those that generate electric thrust at the outer edge of the electrode surface are mainly various oxygen-containing ions.
基金co-supported by the National Natural Science Foundation of China(Nos.12002384 and 11802341)National Science and Technology Major Project of China(No.J2019-Ⅱ-0014-0035)+1 种基金National Key Laboratory Fund of China(No.614220220200109)the Academician Workstation Foundation of the Green Aerotechnics Research Institute of Chongqing Jiaotong University,China(No.GATRI2020C06003)。
文摘Ice accretion on aircraft encountering supercooled water droplets in clouds poses great risks to flight performance and safety.With the aim of optimizing the newly developed streamwise plasma heat knife method for anti-icing,a parametric investigation is carried out in this work.The influence of the detailed voltage profile on the heating effects of a Surface Dielectric Barrier Discharge driven by Nanosecond Pulses(NS-SDBD)is investigated,and a comparison of the antiicing performance among different configurations of streamwise plasma heat knife is made.The results show that columnar high-temperature regions produced by a multi-streamer discharge appear at small pulse rise time,but become diffuse as the pulse rise time increases.An optimal pulse rise time exists to provide a wide range and high value of temperature,which is found to be 150 ns for the setup in the present study.The influence of the pulse fall time is much weaker than that of the rise time.The range and value of the temperature decrease with increasing pulse fall time.A greater pulse width is found to improve the heating effect by increasing the discharge power.When a spanwise electrode is placed connecting the streamwise electrodes of the streamwise plasma heat knife at the airfoil leading edge,the anti-icing performance becomes poorer,whereas good performance is achieved when the spanwise electrode is at the edge of the streamwise electrodes.Based on this,a three-level configuration of the plasma heat knife is proposed,and its anti-icing performance is found to be much better than that of the original configuration.
基金the National Natural Science Foundation of China (Grant No.51877184)the Central Analytical Research Facility operated by the Institute of Future Environment (QUT).
文摘Continuous processes which allow for large amount of wastewater to be treated to meet drainage standards while reducing treatment time and energy consumption are urgently needed. In this study, a dielectric barrier discharge plasma water bed system was designed and then coupled with granular activated carbon (GAC) adsorption to rapidly remove acid fuchsine (AF) with high efficiency. Effects of feeding gases, treatment time and initial concentration of AF on removal efficiency were investigated. Results showed that compared to the N2 and air plasmas treatments, O2 plasma processing was most effective for AF degradation due to the strong oxidation ability of generated activated species, especially the OH radicals. The addition of GAC significantly enhanced the removal efficiency of AF in aqueous solution and shorten the required time by 50%. The effect was attributed to the ability of porous carbon to trap and concentrate the dye, increasing the time dye molecules were exposed to the plasma discharge zone, and to enhance the production of OH radicals on/in GAC to boost the degradation of dyes by plasma as well as in situ regenerate the exhausted GAC. The study offers a new opportunity for continuous effective remediation of wastewater contaminated with organic dyes using plasma technologies.
