PM2.5 and PM10 samples were collected at four major cities in the Pearl River Delta （PRD）, South China, during winter and summer in 2002. Six water-soluble ions, Na^＋, NH4＋, K^＋, Cl^-, NO3^- and SO4^2- were measu...PM2.5 and PM10 samples were collected at four major cities in the Pearl River Delta （PRD）, South China, during winter and summer in 2002. Six water-soluble ions, Na^＋, NH4＋, K^＋, Cl^-, NO3^- and SO4^2- were measured using ion chromatography. On average, ionic species accounted for 53.3% and 40.5% for PM2.5 and PM10, respectively in winter and 39.4% and 35.2%, respectively in summer. Secondary ions such as sulfate, nitrate and ammonium accounted for the major part of the total ionic species. Sulfate was the most abundant species followed by nitrate. Overall, a regional pollution tendency was shown that there were higher concentrations of sulfate, nitrate and ammonium in Guangzhou City than those in the other PRD cities. Significant seasonal variations were also observed with higher levels of species in winter but lower in summer. The Asian monsoon system was favorable for removal and diffusion of air pollutants in PRD in summer while highly loading of local industrial emissions tended to deteriorate the air quality as well. NO3^-/SO4^2- ratio indicated that mobile sources have considerably contribution to the urban aerosol, and stationary sources should not be neglected. Besides the primary emissions, complex atmospheric reactions under favorable weather conditions should be paid more attention for the control of primary emission in the PRD region.展开更多
This study analyzed the temporal precipitation variations in the arid Central Asia （ACA） and their regional differences during 1930-2009 using monthly gridded precipitation from the Climatic Research Unit （CRU）. O...This study analyzed the temporal precipitation variations in the arid Central Asia （ACA） and their regional differences during 1930-2009 using monthly gridded precipitation from the Climatic Research Unit （CRU）. Our results showed that the annual precipitation in this westerly circulation dominated arid region is generally increasing during the past 80 years, with an apparent increasing trend （0.7 mm/10 a） in winter. The precipitation variations in ACA also differ regionally, which can be divided into five distinct subregions （Ⅰ West Kazakhstan region, Ⅱ East Kazakhstan region, ⅢCentral Asia Plains region, Ⅳ Kyrgyzstan region, and V Iran Plateau region）. The annual precipitation falls fairly even on all seasons in the two northern subregions （regions Ⅰ and Ⅱ, approximately north of 45°N）, whereas the annual precipitation is falling mainly on winter and spring （accounting for up to 80% of the annual total precipitation） in the three southern subregions. The annual precipitation is increasing on all subregions except the southwestern ACA （subregion Ⅴ） during the past 80 years. A significant increase in precipitation appeared in subregions Ⅰ and Ⅲ. The long-term trends in annual precipitation in all subregions are determined mainly by trends in winter precipitation. Additionally, the precipitation in ACA has significant interannual variations. The 2-3-year cycle is identified in all subregions, while the 5-6-year cycle is also found in the three southern subregions. Besides the inter-annual variations, there were 3-4 episodic precipitation variations in all subregions, with the latest episodic change that started in the mid- to late 1970s. The precipitations in most of the study regions are fast increasing since the late 1970s. Overall, the responses of ACA precipitation to global warming are complicated. The variations of westerly circulation are likely the major factors that influence the precipitation variations in the study region.展开更多
Along the meridian of 105°E, the Chinese region are divided into two parts, east and west. The results show that in the east part of China the temperate extratropical belt, the warm extratropical belt, and the no...Along the meridian of 105°E, the Chinese region are divided into two parts, east and west. The results show that in the east part of China the temperate extratropical belt, the warm extratropical belt, and the northern subtropical belt shift northward significantly, whereas the middle subtropical belt and the southern subtropical belt have less or no change. As for the northern subtropical belt, the maximal northward shift can reach 3.7 degrees of latitude. As for the warm extratropical belt, along the meridian of 120°-125°E, the maximal northward shift can reach 3-4 degrees. In the west part of China, each climatic belt changes little. Only in the Xinjiang area are the significant northward shifts. Correspondingly, it is found that in the last 50 years the traditional seasons have changed. For Beijing, Hailar, and Lanzhou, in general, summer becomes longer and winter shorter over the last 50 years. Summer begins early and ends late with respect to early 1950s. Contrary to the summer, winter begins late and ends early with respect to early 1950s. Furthermore, spring and autumn have changed over the last 50 years: with respect to early 1950s spring begins early and autumn begins late.展开更多
A new North Atlantic Oscillation (NAO) index, the NAOI, is defined as the differences of normalized sea level pressures regionally zonal-averaged over a broad range of longitudes 80°W-30°E. A comprehensive c...A new North Atlantic Oscillation (NAO) index, the NAOI, is defined as the differences of normalized sea level pressures regionally zonal-averaged over a broad range of longitudes 80°W-30°E. A comprehensive comparison of six NAO indices indicates that the new NAOI provides a more faithful representation of the spatial-temporal variability associated with the NAO on all timescales. A very high signal-to-noise ratio for the NAOI exists for all seasons, and the life cycle represented by the NAOI describes well the seasonal migration for action centers of the NAO. The NAOI captures a larger fraction of the variance of sea level pressure over the North Atlantic sector (20°-90°N, 80°W-30°E), on average 10% more than any other NAO index. There are quite different relationships between the NAOI and surface air temperature during winter and summer. A novel feature, however, is that the NAOI is significantly negative correlated with surface air temperature over the North Atlantic Ocean between 10°-25°N and 70°-30°W, whether in winter or summer. From 1873, the NAOI exhibits strong interannual and decadal variability. Its interannual variability of the twelve calendar months is obviously phase-locked with the seasonal cycle. Moreover, the annual NAOI exhibits a clearer decadal variability in amplitude than the winter NAOI. An upward trend is found in the annual NAOI between the 1870s and 1910s, while the other winter NAO indices fail to show this tendency. The annual NAOI exhibits a strongly positive epoch of 50 years between 1896 and 1950. After 1950, the variability of the annual NAOI is very similar to that of the winter NAO indices.展开更多
Zhengzhou is a developing city in China, that is heavily polluted by high levels of particulate matter. In this study, fine particulate matter （PM2.5） was collected and analyzed for their chemical composition （solu...Zhengzhou is a developing city in China, that is heavily polluted by high levels of particulate matter. In this study, fine particulate matter （PM2.5） was collected and analyzed for their chemical composition （soluble ions, elements, elemental carbon （EC） and organic carbon （OC）） in an industrial district of Zhengzhou in 2010. The average concentrations of PM2.5 were 181, 122, 186 and 211 μg/m3 for spring, summer, autumn and winter, respectively, with an annual average of 175 μg/m3, far exceeding the PM2.5 regulation of USA National Air Quality Standards （15 μg/m3）. The dominant components of PM2.5 in Zhengzhou were secondary ions （sulphate and nitrate） and carbon fractions. Soluble ions, total carbon and elements contributed 41%, 13% and 3% of PM2.5 mass, respectively. Soil dust, secondary aerosol and coal combustion, each contributing about 26%, 24% and 23% of total PM2.5 mass, were the major sources of PM2.5, according to the result of positive matrix factorization analysis. A mixed source of biomass burning, oil combustion and incineration contributed 13% of PM2.5. Fine particulate matter arising from vehicles and industry contributed about 10% and 4% of PM2.5, respectively.展开更多
目的比较症状总分(total symptom score,TSS)及视觉模拟量表(visual analog scale,VAS)在变应性鼻炎(AR)疗效评估中的相关性及适用性。方法对200例AR患者进行问卷调查,包括TSS、各症状VAS(Multi-VAS)、总症状VAS(Uni-VAS)及鼻结膜炎相...目的比较症状总分(total symptom score,TSS)及视觉模拟量表(visual analog scale,VAS)在变应性鼻炎(AR)疗效评估中的相关性及适用性。方法对200例AR患者进行问卷调查,包括TSS、各症状VAS(Multi-VAS)、总症状VAS(Uni-VAS)及鼻结膜炎相关生活质量问卷(rhinoconjunctivitis quality of lifequestionnaire,RQLQ),比较其相关性及适用性。结果198例患者问卷完整,统计分析显示,TSS与Multi-VAS相关性,r=0.79,P<0.001;两者与RQLQ相关性分别为r=0.66,P<0.001和r=0.62,P<0.001。28例(14%)患者认为TSS与VAS难易程度相当,161例(81.3%)患者认为TSS较难填,主要原因是界定症状分级需要更多思考,9例(4.5%)患者认为VAS评分较难,原因为抽象、不容易理解。Uni-VAS患者接受性最好,与RQLQ相关性r=0.55,P<0.001。结论 TSS、VAS均可反映AR患者生活质量,两者相关性好。Multi-VAS可以较详尽反映患者各症状的情况,Uni-VAS评分患者更易接受,简单适用。不同评分方法适用于不同研究目的。展开更多
By use of the NCEP/ NCAR reanalysis data, the seasonal variation of the South Asia high (SAH) is analyzed. The influences of temporal and spatial variations of the middle and upper level atmospheric temperatures, the ...By use of the NCEP/ NCAR reanalysis data, the seasonal variation of the South Asia high (SAH) is analyzed. The influences of temporal and spatial variations of the middle and upper level atmospheric temperatures, the visible heat sources, and the diabatic heating rates in the whole atmospheric column on the seasonal variation of the SAH are discussed. Results show that the SAH has two seasonal balancing modes, one of which is the land high in summer and the other the ocean high in winter. The land high itself can be divided into two patterns as well, that is the Tibetan high and the Iranian high. Heating fields have important impacts on the seasonal variation of the SAH. The SAH is a warm high and its center has the property of heat preference, usually locating over or moving to an area with relatively larger heating rates. The annual cycle of the SAH is mainly controlled by the seasonal process of the latent and sensible heating in South Asia. Strong shortwave radiative heating in the north at high latitudes and over the Tibetan Plateau also has an effects on the northward movement and maintenance of the SAH. The cooling effect of infrared radiation is an important cause in weakening the SAH.展开更多
基金Project supported by the National Natural Science Founding of China(No.20347003,40121303)the Research Grants Council of Hong Kong(No.PolyU5038/01E,PolyU5145/03E)the Area of Strategic Development on Atmospheric and Urban Air Pollution of The Hong Kong Polytechnic University(No.A516,A510).
文摘PM2.5 and PM10 samples were collected at four major cities in the Pearl River Delta （PRD）, South China, during winter and summer in 2002. Six water-soluble ions, Na^＋, NH4＋, K^＋, Cl^-, NO3^- and SO4^2- were measured using ion chromatography. On average, ionic species accounted for 53.3% and 40.5% for PM2.5 and PM10, respectively in winter and 39.4% and 35.2%, respectively in summer. Secondary ions such as sulfate, nitrate and ammonium accounted for the major part of the total ionic species. Sulfate was the most abundant species followed by nitrate. Overall, a regional pollution tendency was shown that there were higher concentrations of sulfate, nitrate and ammonium in Guangzhou City than those in the other PRD cities. Significant seasonal variations were also observed with higher levels of species in winter but lower in summer. The Asian monsoon system was favorable for removal and diffusion of air pollutants in PRD in summer while highly loading of local industrial emissions tended to deteriorate the air quality as well. NO3^-/SO4^2- ratio indicated that mobile sources have considerably contribution to the urban aerosol, and stationary sources should not be neglected. Besides the primary emissions, complex atmospheric reactions under favorable weather conditions should be paid more attention for the control of primary emission in the PRD region.
基金supported by National Basic Research Program of China (Grant No. 2010CB950202)National Natural Science Foundation of China (Grant Nos. 40971056 and 41021091)Fundamental Research Funds for the Central Universities (Grant No. LZUJBKY-2009-82)
文摘This study analyzed the temporal precipitation variations in the arid Central Asia （ACA） and their regional differences during 1930-2009 using monthly gridded precipitation from the Climatic Research Unit （CRU）. Our results showed that the annual precipitation in this westerly circulation dominated arid region is generally increasing during the past 80 years, with an apparent increasing trend （0.7 mm/10 a） in winter. The precipitation variations in ACA also differ regionally, which can be divided into five distinct subregions （Ⅰ West Kazakhstan region, Ⅱ East Kazakhstan region, ⅢCentral Asia Plains region, Ⅳ Kyrgyzstan region, and V Iran Plateau region）. The annual precipitation falls fairly even on all seasons in the two northern subregions （regions Ⅰ and Ⅱ, approximately north of 45°N）, whereas the annual precipitation is falling mainly on winter and spring （accounting for up to 80% of the annual total precipitation） in the three southern subregions. The annual precipitation is increasing on all subregions except the southwestern ACA （subregion Ⅴ） during the past 80 years. A significant increase in precipitation appeared in subregions Ⅰ and Ⅲ. The long-term trends in annual precipitation in all subregions are determined mainly by trends in winter precipitation. Additionally, the precipitation in ACA has significant interannual variations. The 2-3-year cycle is identified in all subregions, while the 5-6-year cycle is also found in the three southern subregions. Besides the inter-annual variations, there were 3-4 episodic precipitation variations in all subregions, with the latest episodic change that started in the mid- to late 1970s. The precipitations in most of the study regions are fast increasing since the late 1970s. Overall, the responses of ACA precipitation to global warming are complicated. The variations of westerly circulation are likely the major factors that influence the precipitation variations in the study region.
基金supported by the National Natural Science Foundation of China(Grant No.40231006)the Key Innovation Project of the Chinese Academy of Sciences(ZKCX2 SW-210,KZCX1-10-07)the National Key Program for De-veloping Basic Sciences(G1999043408).
文摘Along the meridian of 105°E, the Chinese region are divided into two parts, east and west. The results show that in the east part of China the temperate extratropical belt, the warm extratropical belt, and the northern subtropical belt shift northward significantly, whereas the middle subtropical belt and the southern subtropical belt have less or no change. As for the northern subtropical belt, the maximal northward shift can reach 3.7 degrees of latitude. As for the warm extratropical belt, along the meridian of 120°-125°E, the maximal northward shift can reach 3-4 degrees. In the west part of China, each climatic belt changes little. Only in the Xinjiang area are the significant northward shifts. Correspondingly, it is found that in the last 50 years the traditional seasons have changed. For Beijing, Hailar, and Lanzhou, in general, summer becomes longer and winter shorter over the last 50 years. Summer begins early and ends late with respect to early 1950s. Contrary to the summer, winter begins late and ends early with respect to early 1950s. Furthermore, spring and autumn have changed over the last 50 years: with respect to early 1950s spring begins early and autumn begins late.
基金supported jointly by the NOAA Arctic Research,CAS Project ZKCX2-SW-210the National Natural Science Foundation of China(Grant No.40275025)
文摘A new North Atlantic Oscillation (NAO) index, the NAOI, is defined as the differences of normalized sea level pressures regionally zonal-averaged over a broad range of longitudes 80°W-30°E. A comprehensive comparison of six NAO indices indicates that the new NAOI provides a more faithful representation of the spatial-temporal variability associated with the NAO on all timescales. A very high signal-to-noise ratio for the NAOI exists for all seasons, and the life cycle represented by the NAOI describes well the seasonal migration for action centers of the NAO. The NAOI captures a larger fraction of the variance of sea level pressure over the North Atlantic sector (20°-90°N, 80°W-30°E), on average 10% more than any other NAO index. There are quite different relationships between the NAOI and surface air temperature during winter and summer. A novel feature, however, is that the NAOI is significantly negative correlated with surface air temperature over the North Atlantic Ocean between 10°-25°N and 70°-30°W, whether in winter or summer. From 1873, the NAOI exhibits strong interannual and decadal variability. Its interannual variability of the twelve calendar months is obviously phase-locked with the seasonal cycle. Moreover, the annual NAOI exhibits a clearer decadal variability in amplitude than the winter NAOI. An upward trend is found in the annual NAOI between the 1870s and 1910s, while the other winter NAO indices fail to show this tendency. The annual NAOI exhibits a strongly positive epoch of 50 years between 1896 and 1950. After 1950, the variability of the annual NAOI is very similar to that of the winter NAO indices.
基金part of the Science and Technology Plan Project in Zhengzhou funded by Henan Administration of Foreign Experts Affairs and Science and Technology Bureau of Zhengzhou City (grant no.094SYJH36069)support from Peking University and Taiwan Yunlin University of Science and Technology
文摘Zhengzhou is a developing city in China, that is heavily polluted by high levels of particulate matter. In this study, fine particulate matter （PM2.5） was collected and analyzed for their chemical composition （soluble ions, elements, elemental carbon （EC） and organic carbon （OC）） in an industrial district of Zhengzhou in 2010. The average concentrations of PM2.5 were 181, 122, 186 and 211 μg/m3 for spring, summer, autumn and winter, respectively, with an annual average of 175 μg/m3, far exceeding the PM2.5 regulation of USA National Air Quality Standards （15 μg/m3）. The dominant components of PM2.5 in Zhengzhou were secondary ions （sulphate and nitrate） and carbon fractions. Soluble ions, total carbon and elements contributed 41%, 13% and 3% of PM2.5 mass, respectively. Soil dust, secondary aerosol and coal combustion, each contributing about 26%, 24% and 23% of total PM2.5 mass, were the major sources of PM2.5, according to the result of positive matrix factorization analysis. A mixed source of biomass burning, oil combustion and incineration contributed 13% of PM2.5. Fine particulate matter arising from vehicles and industry contributed about 10% and 4% of PM2.5, respectively.
文摘目的比较症状总分(total symptom score,TSS)及视觉模拟量表(visual analog scale,VAS)在变应性鼻炎(AR)疗效评估中的相关性及适用性。方法对200例AR患者进行问卷调查,包括TSS、各症状VAS(Multi-VAS)、总症状VAS(Uni-VAS)及鼻结膜炎相关生活质量问卷(rhinoconjunctivitis quality of lifequestionnaire,RQLQ),比较其相关性及适用性。结果198例患者问卷完整,统计分析显示,TSS与Multi-VAS相关性,r=0.79,P<0.001;两者与RQLQ相关性分别为r=0.66,P<0.001和r=0.62,P<0.001。28例(14%)患者认为TSS与VAS难易程度相当,161例(81.3%)患者认为TSS较难填,主要原因是界定症状分级需要更多思考,9例(4.5%)患者认为VAS评分较难,原因为抽象、不容易理解。Uni-VAS患者接受性最好,与RQLQ相关性r=0.55,P<0.001。结论 TSS、VAS均可反映AR患者生活质量,两者相关性好。Multi-VAS可以较详尽反映患者各症状的情况,Uni-VAS评分患者更易接受,简单适用。不同评分方法适用于不同研究目的。
基金This research was jointly sponsored by "The National Key Programme for Developing Basic Sciences"project (1998040900)Part Ⅰ, and the National Natural Science Foundation of China Project:"Studies on Interaction between the South Asia High and the Asian Monsoon and lts Mechanisms"under Grant No.40175021.
文摘By use of the NCEP/ NCAR reanalysis data, the seasonal variation of the South Asia high (SAH) is analyzed. The influences of temporal and spatial variations of the middle and upper level atmospheric temperatures, the visible heat sources, and the diabatic heating rates in the whole atmospheric column on the seasonal variation of the SAH are discussed. Results show that the SAH has two seasonal balancing modes, one of which is the land high in summer and the other the ocean high in winter. The land high itself can be divided into two patterns as well, that is the Tibetan high and the Iranian high. Heating fields have important impacts on the seasonal variation of the SAH. The SAH is a warm high and its center has the property of heat preference, usually locating over or moving to an area with relatively larger heating rates. The annual cycle of the SAH is mainly controlled by the seasonal process of the latent and sensible heating in South Asia. Strong shortwave radiative heating in the north at high latitudes and over the Tibetan Plateau also has an effects on the northward movement and maintenance of the SAH. The cooling effect of infrared radiation is an important cause in weakening the SAH.
