采用对比和分析的方法,研究了黑龙江省带岭凉水国家级自然保护区温带森林生态系统磷沉降、溪流、河流和渗透水输出磷含量动态特征,以及磷沉降和水系统磷输出对红松人工林、落叶松人工林、椴树红松混交林、枫桦红松混交林和白桦次生林5...采用对比和分析的方法,研究了黑龙江省带岭凉水国家级自然保护区温带森林生态系统磷沉降、溪流、河流和渗透水输出磷含量动态特征,以及磷沉降和水系统磷输出对红松人工林、落叶松人工林、椴树红松混交林、枫桦红松混交林和白桦次生林5种林型土壤全磷和有效磷的影响。结果表明,研究区域通过降雨产生的年磷沉降量约为0.888 kg hm-2,7月除红松人工林外,其他4个林型穿透雨磷浓度均高于大气降雨的磷浓度。7月枫桦红松林、8月白桦次生林和红松人工林A层土壤渗透水磷浓度低于林内雨磷浓度,表层土壤对穿透雨中磷有固定作用。在凉水自然保护区森林生态系统内,森林系统内小溪流、凉水河和凉水森林系统外永翠河水磷浓度均较林外降雨及穿透降雨磷浓度高,表现为永翠河水>土壤A层渗透水>凉水河>小溪>穿透雨>大气降雨。表明土壤中部分磷素通过地表径流和壤中流流出森林生态系统,并汇集于林中小溪,最后进入河流,造成磷在小溪和河流中的富集。大气磷沉降、森林水系统磷输出均与椴树红松林A0层土壤全磷含量呈显著负相关,与红松人工林B层土壤全磷含量呈极显著正相关,与落叶松人工林A0层土壤有效磷含量呈极显著正相关。展开更多
To understand the migration mechanisms of phosphorus(P)during coal-based reduction,a high-phosphorus oolitic iron ore was reduced by coal under various experimental conditions.The migration characteristics and kinetic...To understand the migration mechanisms of phosphorus(P)during coal-based reduction,a high-phosphorus oolitic iron ore was reduced by coal under various experimental conditions.The migration characteristics and kinetics of P were investigated by a field-emission electron probe microanalyzer(FE-EPMA)and using the basic principle of solid phase mass transfer,respectively.Experimental results showed that the P transferred from the slag to the metallic phase during reduction,and the migration process could be divided into three stages:phosphorus diffusing from the slag to the metallic interface,the formation of Fe P compounds at the slag metal interface and P diffusing from the slag metal interface to the metallic interior.The reduction time and temperature significantly influenced the phosphorus content of the metallic and slag phases.The P content of the metallic phase increased with increasing reduction time and temperature,while that of the slag phase gradually decreased.The P diffusion constant and activation energy were determined and a migration kinetics model of P in coal-based reduction was proposed.P diffusion in the metallic phase was the controlling step of the P migration.展开更多
文摘采用对比和分析的方法,研究了黑龙江省带岭凉水国家级自然保护区温带森林生态系统磷沉降、溪流、河流和渗透水输出磷含量动态特征,以及磷沉降和水系统磷输出对红松人工林、落叶松人工林、椴树红松混交林、枫桦红松混交林和白桦次生林5种林型土壤全磷和有效磷的影响。结果表明,研究区域通过降雨产生的年磷沉降量约为0.888 kg hm-2,7月除红松人工林外,其他4个林型穿透雨磷浓度均高于大气降雨的磷浓度。7月枫桦红松林、8月白桦次生林和红松人工林A层土壤渗透水磷浓度低于林内雨磷浓度,表层土壤对穿透雨中磷有固定作用。在凉水自然保护区森林生态系统内,森林系统内小溪流、凉水河和凉水森林系统外永翠河水磷浓度均较林外降雨及穿透降雨磷浓度高,表现为永翠河水>土壤A层渗透水>凉水河>小溪>穿透雨>大气降雨。表明土壤中部分磷素通过地表径流和壤中流流出森林生态系统,并汇集于林中小溪,最后进入河流,造成磷在小溪和河流中的富集。大气磷沉降、森林水系统磷输出均与椴树红松林A0层土壤全磷含量呈显著负相关,与红松人工林B层土壤全磷含量呈极显著正相关,与落叶松人工林A0层土壤有效磷含量呈极显著正相关。
基金financially supported by the National Natural Science Foundation of China (No.51604063)
文摘To understand the migration mechanisms of phosphorus(P)during coal-based reduction,a high-phosphorus oolitic iron ore was reduced by coal under various experimental conditions.The migration characteristics and kinetics of P were investigated by a field-emission electron probe microanalyzer(FE-EPMA)and using the basic principle of solid phase mass transfer,respectively.Experimental results showed that the P transferred from the slag to the metallic phase during reduction,and the migration process could be divided into three stages:phosphorus diffusing from the slag to the metallic interface,the formation of Fe P compounds at the slag metal interface and P diffusing from the slag metal interface to the metallic interior.The reduction time and temperature significantly influenced the phosphorus content of the metallic and slag phases.The P content of the metallic phase increased with increasing reduction time and temperature,while that of the slag phase gradually decreased.The P diffusion constant and activation energy were determined and a migration kinetics model of P in coal-based reduction was proposed.P diffusion in the metallic phase was the controlling step of the P migration.
