用 NaI 晶体探测器所获取的γ谱可被分解为全能峰,水平连续区和康普顿散射区三个分量.在对 NaI 响应函数的研究工作中,首先用蒙特卡罗方法对晶体中的单次、二次和三次康普顿散射进行拟合.经过改进的函数其参数的物理意义明确,易于在拟...用 NaI 晶体探测器所获取的γ谱可被分解为全能峰,水平连续区和康普顿散射区三个分量.在对 NaI 响应函数的研究工作中,首先用蒙特卡罗方法对晶体中的单次、二次和三次康普顿散射进行拟合.经过改进的函数其参数的物理意义明确,易于在拟合中选取初值.用所选取的总响应函数对6英寸×6英寸的圆柱形NaI 所获取的^(137)的γ谱所作的拟合取得了令人满意的结果.展开更多
The wave packet dynamics of I2^- anions is studied by using the time-dependent wave packet method. Two conclusions can be drawn from the calculations. First, the period of the total photoelectron signal oscillating wi...The wave packet dynamics of I2^- anions is studied by using the time-dependent wave packet method. Two conclusions can be drawn from the calculations. First, the period of the total photoelectron signal oscillating with the propagation of delay time is about 750fs. Second, the photoionization of I2^- anions begin at the time 600 fs, and the time needed for the population of the electronic state of I2 neutral molecule to reach the maximum becomes shorter with the increasing delay time.展开更多
The Na I(Tl) scintillation detector has a number of unique advantages, including wide use, high light yield,and its low price. It is difficult to obtain the decomposition of instrument response spectrum because of lim...The Na I(Tl) scintillation detector has a number of unique advantages, including wide use, high light yield,and its low price. It is difficult to obtain the decomposition of instrument response spectrum because of limitations associated with the Na I(Tl) scintillation detector's energy resolution. This paper, based on the physical process of c photons released from decay nuclides, generating an instrument response spectrum, uses the Monte Carlo method to simulate c photons with Na I(Tl) scintillation detector interaction. The Monte Carlo response matrix is established by different single energy γ-rays with detector effects. The Gold and the improved Boosted-Gold iterative algorithms have also been used in this paper to solve the response matrix parameters through decomposing tests,such as simulating a multi-characteristic energy c-ray spectrum and simulating synthesized overlapping peaks cray spectrum. An inversion decomposition of the c instrument response spectrum for measured samples(U series, Th series and U–Th mixed sources, among others)can be achieved under the response matrix. The decomposing spectrum can be better distinguished between the similar energy characteristic peaks, which improve the error levels of activity analysis caused by the overlapping peak with significant effects.展开更多
NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution ...NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution of these detectors,which detracts from an accurate analysis of the instrument spectra obtained,remains a crucial need.Based on the physical properties and spectrum formation processes of NaI(T1) scintillation detectors,the detector response to gamma photons with different energies is represented by photopeaks that are approximately Gaussian in shape with unique full-width-at-half-maximum(FWHM) values.The FWHM is established as a detector parameter based on resolution calibrations and is used in the construction of a general Gaussian response matrix,which is employed for the inverse decomposition of gamma spectra obtained from the detector.The Gold and Boosted Gold iterative algorithms are employed to accelerate the decomposition of the measured spectrum.Tests of the inverse decomposition method on multiple simulated overlapping peaks and on experimentally obtained U and Th radionuclide series spectra verify the practicability of the method,particularly in the low-energy region of the spectrum,providing for the accurate qualitative and quantitative analysis of radionuclides.展开更多
文摘用 NaI 晶体探测器所获取的γ谱可被分解为全能峰,水平连续区和康普顿散射区三个分量.在对 NaI 响应函数的研究工作中,首先用蒙特卡罗方法对晶体中的单次、二次和三次康普顿散射进行拟合.经过改进的函数其参数的物理意义明确,易于在拟合中选取初值.用所选取的总响应函数对6英寸×6英寸的圆柱形NaI 所获取的^(137)的γ谱所作的拟合取得了令人满意的结果.
基金Supported by the National Natural Science Foundation of China under Grant No 10575017. The code used in our calculation is provided by Professor Ke-Li Han and we appreciate his help and kind advice.
文摘The wave packet dynamics of I2^- anions is studied by using the time-dependent wave packet method. Two conclusions can be drawn from the calculations. First, the period of the total photoelectron signal oscillating with the propagation of delay time is about 750fs. Second, the photoionization of I2^- anions begin at the time 600 fs, and the time needed for the population of the electronic state of I2 neutral molecule to reach the maximum becomes shorter with the increasing delay time.
基金supported by National Natural Science Foundation of China(No.11365001)National Major Scientific Equipment Development Projects(No.041514065)+1 种基金Natural Science Foundation of Jiangxi(No.20161BAB201035)Fundamental Science on Radioactive Geology and Exploration Technology Laboratory,East China Institute of Technology(No.RGET1316)
文摘The Na I(Tl) scintillation detector has a number of unique advantages, including wide use, high light yield,and its low price. It is difficult to obtain the decomposition of instrument response spectrum because of limitations associated with the Na I(Tl) scintillation detector's energy resolution. This paper, based on the physical process of c photons released from decay nuclides, generating an instrument response spectrum, uses the Monte Carlo method to simulate c photons with Na I(Tl) scintillation detector interaction. The Monte Carlo response matrix is established by different single energy γ-rays with detector effects. The Gold and the improved Boosted-Gold iterative algorithms have also been used in this paper to solve the response matrix parameters through decomposing tests,such as simulating a multi-characteristic energy c-ray spectrum and simulating synthesized overlapping peaks cray spectrum. An inversion decomposition of the c instrument response spectrum for measured samples(U series, Th series and U–Th mixed sources, among others)can be achieved under the response matrix. The decomposing spectrum can be better distinguished between the similar energy characteristic peaks, which improve the error levels of activity analysis caused by the overlapping peak with significant effects.
基金supported by the National Natural Science Foundation of China(Grant No.11365001)National Major Scientific Equipment Development Projects(Grant No.041514065)+2 种基金the Educational Commission of Jiangxi Province of China(Grant No.GJJ13464)Plan of Science and Technology of Jiangxi Province(Grant No.20141BBE50024)the Fundamental Science on Radioactive Geology and Exploration Technology Laboratory,East China Institute of Technology(Grant No.RGET1316)
文摘NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution of these detectors,which detracts from an accurate analysis of the instrument spectra obtained,remains a crucial need.Based on the physical properties and spectrum formation processes of NaI(T1) scintillation detectors,the detector response to gamma photons with different energies is represented by photopeaks that are approximately Gaussian in shape with unique full-width-at-half-maximum(FWHM) values.The FWHM is established as a detector parameter based on resolution calibrations and is used in the construction of a general Gaussian response matrix,which is employed for the inverse decomposition of gamma spectra obtained from the detector.The Gold and Boosted Gold iterative algorithms are employed to accelerate the decomposition of the measured spectrum.Tests of the inverse decomposition method on multiple simulated overlapping peaks and on experimentally obtained U and Th radionuclide series spectra verify the practicability of the method,particularly in the low-energy region of the spectrum,providing for the accurate qualitative and quantitative analysis of radionuclides.
