Given the challenge of definitively discriminating between chemical and nuclear explosions using seismic methods alone,surface detection of signature noble gas radioisotopes is considered a positive identification of ...Given the challenge of definitively discriminating between chemical and nuclear explosions using seismic methods alone,surface detection of signature noble gas radioisotopes is considered a positive identification of underground nuclear explosions(UNEs).However,the migration of signature radionuclide gases between the nuclear cavity and surface is not well understood because complex processes are involved,including the generation of complex fracture networks,reactivation of natural fractures and faults,and thermo-hydro-mechanical-chemical(THMC)coupling of radionuclide gas transport in the subsurface.In this study,we provide an experimental investigation of hydro-mechanical(HM)coupling among gas flow,stress states,rock deformation,and rock damage using a unique multi-physics triaxial direct shear rock testing system.The testing system also features redundant gas pressure and flow rate measurements,well suited for parameter uncertainty quantification.Using porous tuff and tight granite samples that are relevant to historic UNE tests,we measured the Biot effective stress coefficient,rock matrix gas permeability,and fracture gas permeability at a range of pore pressure and stress conditions.The Biot effective stress coefficient varies from 0.69 to 1 for the tuff,whose porosity averages 35.3%±0.7%,while this coefficient varies from 0.51 to 0.78 for the tight granite(porosity<1%,perhaps an underestimate).Matrix gas permeability is strongly correlated to effective stress for the granite,but not for the porous tuff.Our experiments reveal the following key engineering implications on transport of radionuclide gases post a UNE event:(1)The porous tuff shows apparent fracture dilation or compression upon stress changes,which does not necessarily change the gas permeability;(2)The granite fracture permeability shows strong stress sensitivity and is positively related to shear displacement;and(3)Hydromechanical coupling among stress states,rock damage,and gas flow appears to be stronger in tight granite than in porous tuff.展开更多
Based on the theories of surface physical chemistry, theoretical formulations for permeability and porosity are presented which include both stress effect and matrix shrinkage in a single equation. Then, a three-dimen...Based on the theories of surface physical chemistry, theoretical formulations for permeability and porosity are presented which include both stress effect and matrix shrinkage in a single equation. Then, a three-dimensional, dual porosity, nonequilibrium adsorption, pseudosteady state mathematical model for gas and water is established and solved by the fully implicit method and the block precondition- ing orthomin algorithm. A history matching for the Qinshui Well TL003 is done. From the results, it is shown that the obvious enhancement of permeability occurs along with the passing time but the reservoir pressure of 15# coal seam cannot fulfill the critical adsorption pressure as a result of the water recharge of the aquifer. Hence, it is suggested to plug the 15# coal seam.展开更多
基金supported by the Laboratory Directed Research&Development(LDRD)program at the Los Alamos National Laboratory(LANL)(Grant No.20220019DR).
文摘Given the challenge of definitively discriminating between chemical and nuclear explosions using seismic methods alone,surface detection of signature noble gas radioisotopes is considered a positive identification of underground nuclear explosions(UNEs).However,the migration of signature radionuclide gases between the nuclear cavity and surface is not well understood because complex processes are involved,including the generation of complex fracture networks,reactivation of natural fractures and faults,and thermo-hydro-mechanical-chemical(THMC)coupling of radionuclide gas transport in the subsurface.In this study,we provide an experimental investigation of hydro-mechanical(HM)coupling among gas flow,stress states,rock deformation,and rock damage using a unique multi-physics triaxial direct shear rock testing system.The testing system also features redundant gas pressure and flow rate measurements,well suited for parameter uncertainty quantification.Using porous tuff and tight granite samples that are relevant to historic UNE tests,we measured the Biot effective stress coefficient,rock matrix gas permeability,and fracture gas permeability at a range of pore pressure and stress conditions.The Biot effective stress coefficient varies from 0.69 to 1 for the tuff,whose porosity averages 35.3%±0.7%,while this coefficient varies from 0.51 to 0.78 for the tight granite(porosity<1%,perhaps an underestimate).Matrix gas permeability is strongly correlated to effective stress for the granite,but not for the porous tuff.Our experiments reveal the following key engineering implications on transport of radionuclide gases post a UNE event:(1)The porous tuff shows apparent fracture dilation or compression upon stress changes,which does not necessarily change the gas permeability;(2)The granite fracture permeability shows strong stress sensitivity and is positively related to shear displacement;and(3)Hydromechanical coupling among stress states,rock damage,and gas flow appears to be stronger in tight granite than in porous tuff.
基金the National High Tech Research and Development Program of China ("863" Project) (Grant No. 2006AA06Z236)the National Basic Research Program ("973" Project) (Grant No. 2002CB11708)
文摘Based on the theories of surface physical chemistry, theoretical formulations for permeability and porosity are presented which include both stress effect and matrix shrinkage in a single equation. Then, a three-dimensional, dual porosity, nonequilibrium adsorption, pseudosteady state mathematical model for gas and water is established and solved by the fully implicit method and the block precondition- ing orthomin algorithm. A history matching for the Qinshui Well TL003 is done. From the results, it is shown that the obvious enhancement of permeability occurs along with the passing time but the reservoir pressure of 15# coal seam cannot fulfill the critical adsorption pressure as a result of the water recharge of the aquifer. Hence, it is suggested to plug the 15# coal seam.