An observation-based Galactic Cosmic Ray(GCR)spectral model for heavy nuclei is developed.Zhao and Qin[J.Geophys.Res.Space Phys.118,1837(2013)]proposed an empirical elemental GCR spectra model for nuclear charge 5≤z...An observation-based Galactic Cosmic Ray(GCR)spectral model for heavy nuclei is developed.Zhao and Qin[J.Geophys.Res.Space Phys.118,1837(2013)]proposed an empirical elemental GCR spectra model for nuclear charge 5≤z≤28 over the energy range^30 to 500 Me V/nuc,which is proved to be successful in predicting yearly averaged GCR heavy nuclei spectra.Based on the latest highly statistically precise measurements from ACE/CRIS,a further elemental GCR model with monthly averaged spectra is presented.The model can reproduce the past and predict the future GCR intensity monthly by correlating model parameters with the continuous sunspot number(SSN)record.The effects of solar activity on GCR modulation are considered separately for odd and even solar cycles.Compared with other comprehensive GCR models,our modeling results are satisfyingly consistent with the GCR spectral measurements from ACE/SIS and IMP-8,and have comparable prediction accuracy as the Badhwar&O’Neill 2014 model.A detailed error analysis is also provided.Finally,the GCR carbon and iron nuclei fluxes for the subsequent two solar cycles(SC 25 and 26)are predicted and they show a potential trend in reduced flux amplitude,which is suspected to be relevant to possible weak solar cycles.展开更多
Photofission fragments mass yield for^(232)Th,^(234;238) U,^(237) Np, and^(239;240;242) Pu isotopes are investigated.The calculations are done using a developed approach based on Gorodisskiy's phenomenological for...Photofission fragments mass yield for^(232)Th,^(234;238) U,^(237) Np, and^(239;240;242) Pu isotopes are investigated.The calculations are done using a developed approach based on Gorodisskiy's phenomenological formalism. The Gorodisskiy's method is developed to be applied for the neutron-induced fission. Here we revised it for application to photofission. The effect of emitted neutron prior to fission on the fission fragment mass yields has also been studied. The peak-to-valley ratio is extracted for the240 Pu isotope as a function of energy. Obtained results of the present formalism are compared with the available experimental data. Satisfactory agreement is achieved between the results of present approach and the experimental data.展开更多
By using a simple barrier penetration approach,we predict the α-decay branching ratios to members of ground-state rotational band of heavy even-even No isotopes. We also extend our approach to calculate the α-decay ...By using a simple barrier penetration approach,we predict the α-decay branching ratios to members of ground-state rotational band of heavy even-even No isotopes. We also extend our approach to calculate the α-decay branching ratios to the rotational band of heavy odd-A nuclei. The theoretical branching ratios of α-decays are found in good agreement with the available experimental data.展开更多
The evaporation residue cross sections of synthesizing superheavy nuclei Z=119, 120 are calculated by different sets of master equations with different dynamical variables. Two methods basically predicted similar resu...The evaporation residue cross sections of synthesizing superheavy nuclei Z=119, 120 are calculated by different sets of master equations with different dynamical variables. Two methods basically predicted similar results that the Ca induced hot fusion can 48 produce element 119 easier than produce 120, and the evaporation residue cross sections for 119 are detectable by current advanced techniques, while the evaporation residue cross sections are below 0.1 pb for producing element 120.展开更多
Small modular thorium-based graphite-moderated molten salt reactors (smTMSRs), which combine the advantages of small modular reactors and molten salt reactors, are regarded as a wise development path to speed deployme...Small modular thorium-based graphite-moderated molten salt reactors (smTMSRs), which combine the advantages of small modular reactors and molten salt reactors, are regarded as a wise development path to speed deployment time. In a smTMSR, low enriched uranium and thorium fuels are used in once-through mode, which makes a marked difference in their neutronic properties compared with the case when a conventional molten salt breeder reactor is used. This study investigated the temperature reactivity coefficient (TRC) in a smTMSR, which is mainly affected by the molten salt volume fraction (VF) and the heavy nuclei concentration in the fuel salt (HN). The fourfactor formula method and the reaction rate method were used to indicate the reasons for the TRC change, including the fuel density effect, the fuel Doppler effect, and the graphite thermal scattering effect. The results indicate that only the fuel density has a positive effect on the TRC in the undermoderated region. Thermal scattering from both salt and graphite has a significant negative influence on the TRC in the overmoderated region. The maximal effective multiplication factor, which shows the highest fuel utilization, is located at 10% VF and 12 mol% HN and is still located in the negative TRC region. In addition, on increasing the heavy nuclei amount from 2 mol% HN to 12 mol% HN (VF = 10%), the total TRC undergoes an obvious change from - 11 to - 3 pcm/K, which implies that the change in the HN caused by the fuel feed online should be small to avoid potential trouble in the reactivity control scheme.展开更多
Radioactive decay of super heavy nuclei via the emission of α-particles has been studied theoretically in the preformed cluster model （PCM）. The nucleus-nucleus （NN） potential is obtained by double folding the de...Radioactive decay of super heavy nuclei via the emission of α-particles has been studied theoretically in the preformed cluster model （PCM）. The nucleus-nucleus （NN） potential is obtained by double folding the density distributions of the α-particle and the daughter nucleus with a realistic effective interaction. The M3Y effective interaction, supplemented by a zero-range pseudo-potential for exchange term, is used to calculate the NN potential. The α decay half-lives for 317 nuclei at Z=102 120 are performed in the PCM framework with the theoretical Q values extracted from the MSller-Nix-Kratz and Liran-Marinov-Zeldes mass tables and are compared with the experimental data. The calculated results are also compared with those obtained by using Q values from the Muntian-Hofmann-Patyk-Sobiczewski and Myers-Swiatecki mass estimates.展开更多
The stability of super heavy nuclei（SHN） from Z =104 to Z =126 is analyzed systematically,associated with the following theoretical mass tables： FRDM2012 [At.Data Nucl.Data Tables 109-110（2016）],WS2010 [Phys.Rev....The stability of super heavy nuclei（SHN） from Z =104 to Z =126 is analyzed systematically,associated with the following theoretical mass tables： FRDM2012 [At.Data Nucl.Data Tables 109-110（2016）],WS2010 [Phys.Rev.C 82,044304（2010）],WS-LZ-RBF [J.Phys.G： Nucl.Part.Phys.42,095107（2015）] and the updated experimental data AME2016 [Chinese Physics C 41,040002（2017）].The nucleus with the biggest mean binding energy in each isotopic chain shows systematic regular behavior,indicating that the mean binding energy is a good criterion to classify SHN by their stability.Based on binding energy,the α-decay energy Qα,two-proton separation energy S2p,and two-neutron separation energy S2n are extracted and analyzed.It is found that N =152 and N =162 are sub-magic numbers,N = 184 is a neutron magic number,and Z = 114 is a proton magic number,which may provide useful information for the synthesis and identification of SHN.展开更多
The nuclear and Coulomb potentials between deformed nuclei with octupole deformations and arbitrary orientations are evaluated numerically. The effects of the octupole deformation on the potential between nuclei and t...The nuclear and Coulomb potentials between deformed nuclei with octupole deformations and arbitrary orientations are evaluated numerically. The effects of the octupole deformation on the potential between nuclei and the potential energy surface （PES） used in the description of the production of super-heavy nuclei （SHN） by heavy-ion fusion reactions are investigated in the di-nuclear system model. It is found that the nuclear octupole deformation significantly changes the shape of the PES, which may influence the fusion probability of the SHN. Also, PESs in the tip-belly and belly-belly cases are investigated. Finally, the quasi-fission barriers in the tip-tip and belly-belly cases are evaluated. It is found that the quasi-fission barriers of the belly-belly case are generally larger than those of the tip-tip case.展开更多
We consider the systematics of α-decay half-lives of super-heavy nuclei versus the decay energy and the total α-kinetic energy. We calculate the half-lives using the experimental Qα values. The computed half-lives ...We consider the systematics of α-decay half-lives of super-heavy nuclei versus the decay energy and the total α-kinetic energy. We calculate the half-lives using the experimental Qα values. The computed half-lives are compared with the experimental data and with existing empirical estimates and are found to be in good agreement. Also, we obtain α-preformation factors from the ratio between theoretical and experimental results for some super- heavy nuclei and evaluate the standard deviation. The results indicate the acceptability of the approach.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.41174165,and 41504133)the partial support of the National Science Foundation of USA(Grant Nos.EPSCo R RII-Track-1 Cooperative Agreement OIA-1655280,NASA grants NNX08AJ33G,Subaward 37gvfv102-2,NNX14AC08G,NNX14AJ53G,A99132BT,RR185-447/4944336 and NNX12AB30G)+1 种基金partial support of National Key R&D Program of China(Grant Nos.2018YFC1407304,and 2018YFF01013706)the Open Fund of Key Laboratory(Grant Nos.201801003,and 315030409)
文摘An observation-based Galactic Cosmic Ray(GCR)spectral model for heavy nuclei is developed.Zhao and Qin[J.Geophys.Res.Space Phys.118,1837(2013)]proposed an empirical elemental GCR spectra model for nuclear charge 5≤z≤28 over the energy range^30 to 500 Me V/nuc,which is proved to be successful in predicting yearly averaged GCR heavy nuclei spectra.Based on the latest highly statistically precise measurements from ACE/CRIS,a further elemental GCR model with monthly averaged spectra is presented.The model can reproduce the past and predict the future GCR intensity monthly by correlating model parameters with the continuous sunspot number(SSN)record.The effects of solar activity on GCR modulation are considered separately for odd and even solar cycles.Compared with other comprehensive GCR models,our modeling results are satisfyingly consistent with the GCR spectral measurements from ACE/SIS and IMP-8,and have comparable prediction accuracy as the Badhwar&O’Neill 2014 model.A detailed error analysis is also provided.Finally,the GCR carbon and iron nuclei fluxes for the subsequent two solar cycles(SC 25 and 26)are predicted and they show a potential trend in reduced flux amplitude,which is suspected to be relevant to possible weak solar cycles.
文摘Photofission fragments mass yield for^(232)Th,^(234;238) U,^(237) Np, and^(239;240;242) Pu isotopes are investigated.The calculations are done using a developed approach based on Gorodisskiy's phenomenological formalism. The Gorodisskiy's method is developed to be applied for the neutron-induced fission. Here we revised it for application to photofission. The effect of emitted neutron prior to fission on the fission fragment mass yields has also been studied. The peak-to-valley ratio is extracted for the240 Pu isotope as a function of energy. Obtained results of the present formalism are compared with the available experimental data. Satisfactory agreement is achieved between the results of present approach and the experimental data.
基金National Natural Science Foundation of China(10535010,10735010,10775068)Research Fund for Doctoral Pro-gram of Higher Education of China(20070284016)Major State Basic Research Development Program of China(2007CB815004)
文摘By using a simple barrier penetration approach,we predict the α-decay branching ratios to members of ground-state rotational band of heavy even-even No isotopes. We also extend our approach to calculate the α-decay branching ratios to the rotational band of heavy odd-A nuclei. The theoretical branching ratios of α-decays are found in good agreement with the available experimental data.
基金supported by the National Natural Science Foundation of China (Grant Nos. 1077501, 10875152, 10805061, 10825522 and10975064)the Knowledge Innovation Project of the Chinese Academy of Sciences (Grant No. KJCX2-EW-N01)+1 种基金the Major State Basic Research Development Program (Grant No. 2007CB815000)the support from DFG of Germany
文摘The evaporation residue cross sections of synthesizing superheavy nuclei Z=119, 120 are calculated by different sets of master equations with different dynamical variables. Two methods basically predicted similar results that the Ca induced hot fusion can 48 produce element 119 easier than produce 120, and the evaporation residue cross sections for 119 are detectable by current advanced techniques, while the evaporation residue cross sections are below 0.1 pb for producing element 120.
基金supported by the Chinese TMSR Strategic Pioneer Science and Technology Project(No.XDA02010000)the Frontier Science Key Program of Chinese Academy of Sciences(No.QYZDY-SSW-JSC016)
文摘Small modular thorium-based graphite-moderated molten salt reactors (smTMSRs), which combine the advantages of small modular reactors and molten salt reactors, are regarded as a wise development path to speed deployment time. In a smTMSR, low enriched uranium and thorium fuels are used in once-through mode, which makes a marked difference in their neutronic properties compared with the case when a conventional molten salt breeder reactor is used. This study investigated the temperature reactivity coefficient (TRC) in a smTMSR, which is mainly affected by the molten salt volume fraction (VF) and the heavy nuclei concentration in the fuel salt (HN). The fourfactor formula method and the reaction rate method were used to indicate the reasons for the TRC change, including the fuel density effect, the fuel Doppler effect, and the graphite thermal scattering effect. The results indicate that only the fuel density has a positive effect on the TRC in the undermoderated region. Thermal scattering from both salt and graphite has a significant negative influence on the TRC in the overmoderated region. The maximal effective multiplication factor, which shows the highest fuel utilization, is located at 10% VF and 12 mol% HN and is still located in the negative TRC region. In addition, on increasing the heavy nuclei amount from 2 mol% HN to 12 mol% HN (VF = 10%), the total TRC undergoes an obvious change from - 11 to - 3 pcm/K, which implies that the change in the HN caused by the fuel feed online should be small to avoid potential trouble in the reactivity control scheme.
基金Supported by National Natural Science Foundation of China (10875150, 10775183, 10535010)Major State Basic Research Development Programme in China (2007CB815000)
文摘Radioactive decay of super heavy nuclei via the emission of α-particles has been studied theoretically in the preformed cluster model （PCM）. The nucleus-nucleus （NN） potential is obtained by double folding the density distributions of the α-particle and the daughter nucleus with a realistic effective interaction. The M3Y effective interaction, supplemented by a zero-range pseudo-potential for exchange term, is used to calculate the NN potential. The α decay half-lives for 317 nuclei at Z=102 120 are performed in the PCM framework with the theoretical Q values extracted from the MSller-Nix-Kratz and Liran-Marinov-Zeldes mass tables and are compared with the experimental data. The calculated results are also compared with those obtained by using Q values from the Muntian-Hofmann-Patyk-Sobiczewski and Myers-Swiatecki mass estimates.
基金Supported by National Natural Science Foundation of China(11675066,11647306)Fundamental Research Funds for the Central Universities(lzujbky-2017-ot04)Feitian Scholar Project of Gansu province
文摘The stability of super heavy nuclei（SHN） from Z =104 to Z =126 is analyzed systematically,associated with the following theoretical mass tables： FRDM2012 [At.Data Nucl.Data Tables 109-110（2016）],WS2010 [Phys.Rev.C 82,044304（2010）],WS-LZ-RBF [J.Phys.G： Nucl.Part.Phys.42,095107（2015）] and the updated experimental data AME2016 [Chinese Physics C 41,040002（2017）].The nucleus with the biggest mean binding energy in each isotopic chain shows systematic regular behavior,indicating that the mean binding energy is a good criterion to classify SHN by their stability.Based on binding energy,the α-decay energy Qα,two-proton separation energy S2p,and two-neutron separation energy S2n are extracted and analyzed.It is found that N =152 and N =162 are sub-magic numbers,N = 184 is a neutron magic number,and Z = 114 is a proton magic number,which may provide useful information for the synthesis and identification of SHN.
基金Supported by National Natural Science Foundation of China (10975100,11011130216,10979024,10705014)the financial support from DFG of Germany and Major State Basic Research Development Progrom of China (2007CB81500)
文摘The nuclear and Coulomb potentials between deformed nuclei with octupole deformations and arbitrary orientations are evaluated numerically. The effects of the octupole deformation on the potential between nuclei and the potential energy surface （PES） used in the description of the production of super-heavy nuclei （SHN） by heavy-ion fusion reactions are investigated in the di-nuclear system model. It is found that the nuclear octupole deformation significantly changes the shape of the PES, which may influence the fusion probability of the SHN. Also, PESs in the tip-belly and belly-belly cases are investigated. Finally, the quasi-fission barriers in the tip-tip and belly-belly cases are evaluated. It is found that the quasi-fission barriers of the belly-belly case are generally larger than those of the tip-tip case.
文摘We consider the systematics of α-decay half-lives of super-heavy nuclei versus the decay energy and the total α-kinetic energy. We calculate the half-lives using the experimental Qα values. The computed half-lives are compared with the experimental data and with existing empirical estimates and are found to be in good agreement. Also, we obtain α-preformation factors from the ratio between theoretical and experimental results for some super- heavy nuclei and evaluate the standard deviation. The results indicate the acceptability of the approach.
