提出了通过γ能谱全能峰测量吸收剂量的方法,定义了全能峰角响应函数。采用蒙特卡罗方法计算了50 mm×50 mm NaI(Tl)探测器的平均角响应随射线能量的变化,用标准点源137Cs、60Co、152Eu、133Ba和参考辐射场137Cs、60Co、226Ra、241A...提出了通过γ能谱全能峰测量吸收剂量的方法,定义了全能峰角响应函数。采用蒙特卡罗方法计算了50 mm×50 mm NaI(Tl)探测器的平均角响应随射线能量的变化,用标准点源137Cs、60Co、152Eu、133Ba和参考辐射场137Cs、60Co、226Ra、241Am进行了实验验证。结果证明,在近似各向同性的条件下,对标准点源的测量结果与理论值相比误差小于2%,对参考辐射场的测量结果与电离室测量结果相差小于3%。该方法适合低能到高能的较宽能谱段剂量率测量,不仅能测出某种核素对总剂量率的贡献,且能同时分辨核素种类,无需实验刻度。展开更多
NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution ...NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution of these detectors,which detracts from an accurate analysis of the instrument spectra obtained,remains a crucial need.Based on the physical properties and spectrum formation processes of NaI(T1) scintillation detectors,the detector response to gamma photons with different energies is represented by photopeaks that are approximately Gaussian in shape with unique full-width-at-half-maximum(FWHM) values.The FWHM is established as a detector parameter based on resolution calibrations and is used in the construction of a general Gaussian response matrix,which is employed for the inverse decomposition of gamma spectra obtained from the detector.The Gold and Boosted Gold iterative algorithms are employed to accelerate the decomposition of the measured spectrum.Tests of the inverse decomposition method on multiple simulated overlapping peaks and on experimentally obtained U and Th radionuclide series spectra verify the practicability of the method,particularly in the low-energy region of the spectrum,providing for the accurate qualitative and quantitative analysis of radionuclides.展开更多
文摘提出了通过γ能谱全能峰测量吸收剂量的方法,定义了全能峰角响应函数。采用蒙特卡罗方法计算了50 mm×50 mm NaI(Tl)探测器的平均角响应随射线能量的变化,用标准点源137Cs、60Co、152Eu、133Ba和参考辐射场137Cs、60Co、226Ra、241Am进行了实验验证。结果证明,在近似各向同性的条件下,对标准点源的测量结果与理论值相比误差小于2%,对参考辐射场的测量结果与电离室测量结果相差小于3%。该方法适合低能到高能的较宽能谱段剂量率测量,不仅能测出某种核素对总剂量率的贡献,且能同时分辨核素种类,无需实验刻度。
基金supported by the National Natural Science Foundation of China(Grant No.11365001)National Major Scientific Equipment Development Projects(Grant No.041514065)+2 种基金the Educational Commission of Jiangxi Province of China(Grant No.GJJ13464)Plan of Science and Technology of Jiangxi Province(Grant No.20141BBE50024)the Fundamental Science on Radioactive Geology and Exploration Technology Laboratory,East China Institute of Technology(Grant No.RGET1316)
文摘NaI(T1) scintillation detectors have been widely applied for gamma-ray spectrum measurements owing to advantages such as high detection efficiency and low price.However,the mitigation of the limited energy resolution of these detectors,which detracts from an accurate analysis of the instrument spectra obtained,remains a crucial need.Based on the physical properties and spectrum formation processes of NaI(T1) scintillation detectors,the detector response to gamma photons with different energies is represented by photopeaks that are approximately Gaussian in shape with unique full-width-at-half-maximum(FWHM) values.The FWHM is established as a detector parameter based on resolution calibrations and is used in the construction of a general Gaussian response matrix,which is employed for the inverse decomposition of gamma spectra obtained from the detector.The Gold and Boosted Gold iterative algorithms are employed to accelerate the decomposition of the measured spectrum.Tests of the inverse decomposition method on multiple simulated overlapping peaks and on experimentally obtained U and Th radionuclide series spectra verify the practicability of the method,particularly in the low-energy region of the spectrum,providing for the accurate qualitative and quantitative analysis of radionuclides.
