Novel CexY1-xO washcoats adhered on the cordierite honeycomb, used as supports for Pd catalysts, were prepared by an impregnation method. It was fotmd that the CexY1-xO washcoats had better adhesion and higher adsorpt...Novel CexY1-xO washcoats adhered on the cordierite honeycomb, used as supports for Pd catalysts, were prepared by an impregnation method. It was fotmd that the CexY1-xO washcoats had better adhesion and higher adsorption efficiency of H2PdCl4, and the optimal component of the washcoat was Ce0.8Y0.2O. Model reaction of catalytic combustion of toluene was chosen to evaluate the performance of the developed Pd/CexY1-xO/substrate catalysts. The results showed that the catalytic performance of the Pd/CexY1-xO/substrate catalysts depended on the component of the washcoats, with the Pd/Ce0.8Y0.2O/substrate catalyst giving the best catalytic activity and thermal stability.展开更多
基金the Natural Science Foundation of China (Grant 20473075)
文摘Novel CexY1-xO washcoats adhered on the cordierite honeycomb, used as supports for Pd catalysts, were prepared by an impregnation method. It was fotmd that the CexY1-xO washcoats had better adhesion and higher adsorption efficiency of H2PdCl4, and the optimal component of the washcoat was Ce0.8Y0.2O. Model reaction of catalytic combustion of toluene was chosen to evaluate the performance of the developed Pd/CexY1-xO/substrate catalysts. The results showed that the catalytic performance of the Pd/CexY1-xO/substrate catalysts depended on the component of the washcoats, with the Pd/Ce0.8Y0.2O/substrate catalyst giving the best catalytic activity and thermal stability.