In this paper, we demonstrated trace of dye molecules in living plants. The NaGdF4:Yb^(3+),Er^(3+) nanoparticles probe was used to detect the rhodamine B(RhB) in bean sprout. It is found that the fluorescencedye can b...In this paper, we demonstrated trace of dye molecules in living plants. The NaGdF4:Yb^(3+),Er^(3+) nanoparticles probe was used to detect the rhodamine B(RhB) in bean sprout. It is found that the fluorescencedye can be efficiently imbibed during the growing process and the absorbance presented a position dependence effect, which was supported by the upconversion spectra and the fluorescent image characterization. In addition, the concentration of the residual RhB in bean sprout can be efficiently traced by the synthesized probe based on the fluorescent resonant energy transfer. Finally, the relation between the excitation power, concentration and the ratio of yellow to green emission are discussed in detail. These results can be helpful in understanding the RhB dye molecules absorbance process in vegetable growth and provide an efficient way to trace the residual dyes in vivo plant.展开更多
Optical biosensors with a high sensitivity and a low detection limit play a highly significant role in extensive scenarios related to our daily life. Combined with a specific numerical simulation based on the transfer...Optical biosensors with a high sensitivity and a low detection limit play a highly significant role in extensive scenarios related to our daily life. Combined with a specific numerical simulation based on the transfer matrix and resonance condition, the idea of novel single-waveguide-based microresonators with a double-spiral-race- track (DSR) shape is proposed and their geometry optimizations and sensing characteristics are also investigated based on the Vernier effect. The devices show good sensing performances, such as a high quality factor of 1.23 x 105, a wide wavelength range of over 120 nm, a high extinction ratio (ER) over 62.1 dB, a high sensitivity of 698.5 nm/RIU, and a low detection limit of 1.8 × 10^-5. Furthermore, single-waveguide-based resonators can also be built by cascading two DSR structures in series, called twin-DSRs, and the results show that the sensing properties are enhanced in terms of quasi free spectral range (FSR) and ER due to the double Vernier effect. Excellent features indicate that our novel single-waveguide-based resonators have the potential for future compact and highly integrated biosensors.展开更多
基金Project supported by the National Natural Science Foundation of China(61675067,51675174,61575062,61474042)the Scientific Research Fund of Hunan Provincial Education Department(16C0627,17B090)the Natural Science Foundation of Hunan Province,China(2016JJ2059,2018JJ3138)
文摘In this paper, we demonstrated trace of dye molecules in living plants. The NaGdF4:Yb^(3+),Er^(3+) nanoparticles probe was used to detect the rhodamine B(RhB) in bean sprout. It is found that the fluorescencedye can be efficiently imbibed during the growing process and the absorbance presented a position dependence effect, which was supported by the upconversion spectra and the fluorescent image characterization. In addition, the concentration of the residual RhB in bean sprout can be efficiently traced by the synthesized probe based on the fluorescent resonant energy transfer. Finally, the relation between the excitation power, concentration and the ratio of yellow to green emission are discussed in detail. These results can be helpful in understanding the RhB dye molecules absorbance process in vegetable growth and provide an efficient way to trace the residual dyes in vivo plant.
基金supported in part by the National Natural Science Foundation of China(No.61575038)the Fundamental Research Funds for the Central Universities(No.ZYGX2015J052)
文摘Optical biosensors with a high sensitivity and a low detection limit play a highly significant role in extensive scenarios related to our daily life. Combined with a specific numerical simulation based on the transfer matrix and resonance condition, the idea of novel single-waveguide-based microresonators with a double-spiral-race- track (DSR) shape is proposed and their geometry optimizations and sensing characteristics are also investigated based on the Vernier effect. The devices show good sensing performances, such as a high quality factor of 1.23 x 105, a wide wavelength range of over 120 nm, a high extinction ratio (ER) over 62.1 dB, a high sensitivity of 698.5 nm/RIU, and a low detection limit of 1.8 × 10^-5. Furthermore, single-waveguide-based resonators can also be built by cascading two DSR structures in series, called twin-DSRs, and the results show that the sensing properties are enhanced in terms of quasi free spectral range (FSR) and ER due to the double Vernier effect. Excellent features indicate that our novel single-waveguide-based resonators have the potential for future compact and highly integrated biosensors.