Based on the experimental results, three basic conclusions are summarized for the thermal/electric-field poling (TEFP) silica materials, with which the second-order nonlinear optical coefficient in the bulk silica gla...Based on the experimental results, three basic conclusions are summarized for the thermal/electric-field poling (TEFP) silica materials, with which the second-order nonlinear optical coefficient in the bulk silica glass after TEFP is calculated, and relationships between the coefficient and the applied voltage V 0 in the poling process and the thickness of the nonlinear layer created from the poling are obtained. Theoretical results show that the second-order susceptibility χ(2) and the second-harmonic efficiency η in the poled bulk glass are proportional to √V 0 and V 0 2 , respectively; χ(2)~0.2?1.6 pm/V for the bulk glass after the typical TEFP; χ(2) decreases with an increase in the poling time after the TEFP silica glass approximately reaches the steady state. Theoretical results are well consistent with the experimental reports.展开更多
文摘Based on the experimental results, three basic conclusions are summarized for the thermal/electric-field poling (TEFP) silica materials, with which the second-order nonlinear optical coefficient in the bulk silica glass after TEFP is calculated, and relationships between the coefficient and the applied voltage V 0 in the poling process and the thickness of the nonlinear layer created from the poling are obtained. Theoretical results show that the second-order susceptibility χ(2) and the second-harmonic efficiency η in the poled bulk glass are proportional to √V 0 and V 0 2 , respectively; χ(2)~0.2?1.6 pm/V for the bulk glass after the typical TEFP; χ(2) decreases with an increase in the poling time after the TEFP silica glass approximately reaches the steady state. Theoretical results are well consistent with the experimental reports.