Solid-state lithium metal batteries are one of the most promising options for next-generation batteries pursuing high-energy density and high-safety.However,the inevitable volatilization of lithium compounds during si...Solid-state lithium metal batteries are one of the most promising options for next-generation batteries pursuing high-energy density and high-safety.However,the inevitable volatilization of lithium compounds during sintering leads to low relative density and low ionic conductivity of solid-state electrolytes.Herein,the dynamic lithium-compensation mechanism is proposed to facilitate the densification of Ta-substituted garnet-type electrolyte(Li_(6.5)La_(3)Zr_(1.5)Ta_(0.5)O_(12)(LLZT))through the reversible manipulating of Li_(2)O atmosphere.Li_(2)ZrO_(3)is used as mother powder additive,which reacts with Li_(2)O in sintering atmosphere and forms Li_(6)Zr_(2)O_(7).Li_(2)ZrO_(3)/Li_(6)Zr_(2)O_(7)buffer pair manipulates the sintering Li_(2)O atmosphere,which is vital for LLZT,within the Li_(2)O partial pressure range corresponding to Li_(2)ZrO_(3)and Li_(6)Zr_(2)O_(7).Furthermore,the reversibility mechanism of buffer pair for Li_(2)O absorption and release is revealed.The obtained LLZT exhibits a relative density of over 96%and an ionic conductivity exceeding 7×10^(−4)S·cm^(−1)with no abnormal grain growth.The symmetric cell demonstrates an excellent lithium dendrite suppressing ability(stable cycling at a current density of 0.3 mA·cm^(−2)for over 1000 h).Such dynamic lithium-compensation strategy has been successfully applied in atmosphere manipulation of LLZT sintering process,which reduces the dependence of LLZT on the Li_(2)O atmosphere,making it conducive to large-scale preparation of electrolyte ceramics.展开更多
Abstract A simple scheme for teleporting an unknown M-qubit cat-like state is proposed. The steps of this scheme can be summarized simply： disentangle-teleport-reconstruct entanglement. If proper unitary operations a...Abstract A simple scheme for teleporting an unknown M-qubit cat-like state is proposed. The steps of this scheme can be summarized simply： disentangle-teleport-reconstruct entanglement. If proper unitary operations and measurements from senders are given, the teleportation of an unknown M-qubit cat-like state can be converted into single qubit teleportation. In the meantime, the receiver should also carry out right unitary operations with the introduction of appropriate ancillary qubits to confirm the successful teleportation of the demanded entangled state. The present scheme can be generalized to teleport an unknown M-quNit state, i.e., an M-quNit state can be teleported by a single quNit entangled pair.展开更多
Attosecond transient absorption(ATA)has been developed as an all-optical technique for probing electron dynamics in matter.Here we present a scheme that can modify the laserinduced state and the corresponding ATA spec...Attosecond transient absorption(ATA)has been developed as an all-optical technique for probing electron dynamics in matter.Here we present a scheme that can modify the laserinduced state and the corresponding ATA spectrum via excitation by a pair of XUV attosecond pulses and by a time-delayed mid-infrared(MIR)laser probe.Different from the scheme of the electronic excitation by a single XUV attosecond pulse,the application of a pair of XUV pulses provides extra degrees of freedom,such as the time delay and the intensity ratio between two XUV pulses,which make it possible to adjust the pump process,resulting in the modification of the ATA spectrum.We show that by varying the time delay between the two XUV pulses,the population of the dark state and the ATA spectrum of the laser-induced state have periodic modulations.We also demonstrate that the peak of the ATA spectrum of the laser-induced state appears at a fixed time delay between the XUV pair and the MIR laser when the intensity ratio is large,and it changes with the time delay when the intensity ratio is small,which can be related to either one of two peaks in the population of the dark state.展开更多
A Cooper-pair box biased by a classical voltage and also irradiated by a squeezed state field is considered in order to find new ways to quantum communication and calculation. The quantum dynamics of the Cooper-pair b...A Cooper-pair box biased by a classical voltage and also irradiated by a squeezed state field is considered in order to find new ways to quantum communication and calculation. The quantum dynamics of the Cooper-pair box and the entanglement which is the core theoretics of quantum communication and calculation is investigated in this system, which is related to the squeezing parameter of the squeezed state, A model of Hamiltonian which represents the interaction between box and quantum field is introduced. Finally, the relationship between the entanglement and the squeezing parameter of the squeezed state is demonstrated.展开更多
This paper examines the quantization of mesoscopic circuit including Josephson junctions. Following Feynman＇s assumption, via the Hamilton dynamic approach and by virtue of the entangled state representation, it cons...This paper examines the quantization of mesoscopic circuit including Josephson junctions. Following Feynman＇s assumption, via the Hamilton dynamic approach and by virtue of the entangled state representation, it constructs Hamiltonian operator for the double-Josephson-junction mesoscopic circuit coupled by a capacitor. Then it uses the Heisenberg equation of motion to derive the induction voltage across each Josephson junction. The result manifestly shows how the voltage is affected by the capacitance coupling.展开更多
The existence of a single topologically protected edge state in the first bulk bandgap for acoustic/elastic valley Hall insulators(VHIs)with zigzag interface configurations(ZICs)is well known.However,in this work,we s...The existence of a single topologically protected edge state in the first bulk bandgap for acoustic/elastic valley Hall insulators(VHIs)with zigzag interface configurations(ZICs)is well known.However,in this work,we show that an ultra-broadband edgestate pair in this bandgap can be created using the inverse design by topology optimization.The valley Hall insulator design increases the operational bandwidth 121%compared with an existing valley Hall insulator from recent literature and exhibits extreme field confinement,where more than 99%of the field intensity is concentrated within three unit-cells from the interface.One-way propagation and topological robustness towards small cavity defects are confirmed for the full bandwidth.The exploitation of such edge-state pairs of valley Hall insulators opens an avenue for realizing broadband confined edge modes.In tests for disorder and bend defects,we show that the additional ZIC,with a different operational frequency interval,encountered at the defects,degrades the transmission for bend and disorder defects which may prove significant for the application of VHIs.Through an alternative topology optimization method based on two ZICs,we further increase their common operational bandwidth.展开更多
fragments, F- and Cl- including two isotope species 35Cl- and 37Cl-, are observed in the photoexcitations of CFC13. The ion-pair anion efficiency spectra of 35Cl- and 37Cl- are recorded in the photon energy range of 7...fragments, F- and Cl- including two isotope species 35Cl- and 37Cl-, are observed in the photoexcitations of CFC13. The ion-pair anion efficiency spectra of 35Cl- and 37Cl- are recorded in the photon energy range of 7.75-22.00 eV. The threshold of ion-pair dissociation CFCl3-CFC12＋＋Cl- is experimentally determined to be 7.944-0.04 eV. With the references of the high-resolution photoabsorption spectra reported in the literatures, we make tentative assignments of the electron valence-to-Rydberg transitions. Furthermore, the multibody ion-pair fragmentation processes to Cl- are discussed by comparison between the calculated thermochemical thresholds and the experimental efficiency spectrum.展开更多
A state-dependent proof of Bell's theorem without inequalities using the product state of any two maximally entangled states (Bell states) of two qubits for two observers in an ideal condition, each of which posse...A state-dependent proof of Bell's theorem without inequalities using the product state of any two maximally entangled states (Bell states) of two qubits for two observers in an ideal condition, each of which possesses two qubits,is proposed. It is different from the other proofs in which there exists a fundamental requirement that certain specific suitable Bell states have been chosen. Moreover, in any non-ideal situation, a common Bell inequality independent of the choices of the 16-product states is derived, which is used to test the contradiction between quantum mechanics and local reality theory in the reach of current experimental technology.展开更多
As an innovative theory and technology,quantum network coding has become the research hotspot in quantum network communications.In this paper,a quantum remote state preparation scheme based on quantum network coding i...As an innovative theory and technology,quantum network coding has become the research hotspot in quantum network communications.In this paper,a quantum remote state preparation scheme based on quantum network coding is proposed.Comparing with the general quantum remote state preparation schemes,our proposed scheme brings an arbitrary unknown quantum state finally prepared remotely through the quantum network,by designing the appropriate encoding and decoding steps for quantum network coding.What is worth mentioning,from the network model,this scheme is built on the quantum k-pair network which is the expansion of the typical bottleneck network—butterfly network.Accordingly,it can be treated as an efficient quantum network preparation scheme due to the characteristics of network coding,and it also makes the proposed scheme more applicable to the large-scale quantum networks.In addition,the fact of an arbitrary unknown quantum state remotely prepared means that the senders do not need to know the desired quantum state.Thus,the security of the proposed scheme is higher.Moreover,this scheme can always achieve the success probability of 1 and 1-max flow of value k.Thus,the communication efficiency of the proposed scheme is higher.Therefore,the proposed scheme turns out to be practicable,secure and efficient,which helps to effectively enrich the theory of quantum remote state preparation.展开更多
基金financially supported by the National Key Research and Development Program of China(No.2022YFB3807700)the National Natural Science Foundation of China(Nos.U20A20248 and U1930208)+1 种基金the Key-Area Research and Development Program of Guangdong Province(No.2020B090919001)the Shanghai Engineering Research Center of Inorganic Energy Materials and Electric Power Sources(No.18DZ2280800).
文摘Solid-state lithium metal batteries are one of the most promising options for next-generation batteries pursuing high-energy density and high-safety.However,the inevitable volatilization of lithium compounds during sintering leads to low relative density and low ionic conductivity of solid-state electrolytes.Herein,the dynamic lithium-compensation mechanism is proposed to facilitate the densification of Ta-substituted garnet-type electrolyte(Li_(6.5)La_(3)Zr_(1.5)Ta_(0.5)O_(12)(LLZT))through the reversible manipulating of Li_(2)O atmosphere.Li_(2)ZrO_(3)is used as mother powder additive,which reacts with Li_(2)O in sintering atmosphere and forms Li_(6)Zr_(2)O_(7).Li_(2)ZrO_(3)/Li_(6)Zr_(2)O_(7)buffer pair manipulates the sintering Li_(2)O atmosphere,which is vital for LLZT,within the Li_(2)O partial pressure range corresponding to Li_(2)ZrO_(3)and Li_(6)Zr_(2)O_(7).Furthermore,the reversibility mechanism of buffer pair for Li_(2)O absorption and release is revealed.The obtained LLZT exhibits a relative density of over 96%and an ionic conductivity exceeding 7×10^(−4)S·cm^(−1)with no abnormal grain growth.The symmetric cell demonstrates an excellent lithium dendrite suppressing ability(stable cycling at a current density of 0.3 mA·cm^(−2)for over 1000 h).Such dynamic lithium-compensation strategy has been successfully applied in atmosphere manipulation of LLZT sintering process,which reduces the dependence of LLZT on the Li_(2)O atmosphere,making it conducive to large-scale preparation of electrolyte ceramics.
基金supported by National Natural Science Foundation of China under Grant No.10574060
文摘Abstract A simple scheme for teleporting an unknown M-qubit cat-like state is proposed. The steps of this scheme can be summarized simply： disentangle-teleport-reconstruct entanglement. If proper unitary operations and measurements from senders are given, the teleportation of an unknown M-qubit cat-like state can be converted into single qubit teleportation. In the meantime, the receiver should also carry out right unitary operations with the introduction of appropriate ancillary qubits to confirm the successful teleportation of the demanded entangled state. The present scheme can be generalized to teleport an unknown M-quNit state, i.e., an M-quNit state can be teleported by a single quNit entangled pair.
基金supported by the National Natural Science Foundation of China(Grant Nos.91950102 and 11834004)the Natural Science Foundation of Jiangsu Province(Grant No.BK20220925)the Funding of Nanjing University of Science and Technology(NJUST)(Grant No.TSXK2022D005)
文摘Attosecond transient absorption(ATA)has been developed as an all-optical technique for probing electron dynamics in matter.Here we present a scheme that can modify the laserinduced state and the corresponding ATA spectrum via excitation by a pair of XUV attosecond pulses and by a time-delayed mid-infrared(MIR)laser probe.Different from the scheme of the electronic excitation by a single XUV attosecond pulse,the application of a pair of XUV pulses provides extra degrees of freedom,such as the time delay and the intensity ratio between two XUV pulses,which make it possible to adjust the pump process,resulting in the modification of the ATA spectrum.We show that by varying the time delay between the two XUV pulses,the population of the dark state and the ATA spectrum of the laser-induced state have periodic modulations.We also demonstrate that the peak of the ATA spectrum of the laser-induced state appears at a fixed time delay between the XUV pair and the MIR laser when the intensity ratio is large,and it changes with the time delay when the intensity ratio is small,which can be related to either one of two peaks in the population of the dark state.
文摘A Cooper-pair box biased by a classical voltage and also irradiated by a squeezed state field is considered in order to find new ways to quantum communication and calculation. The quantum dynamics of the Cooper-pair box and the entanglement which is the core theoretics of quantum communication and calculation is investigated in this system, which is related to the squeezing parameter of the squeezed state, A model of Hamiltonian which represents the interaction between box and quantum field is introduced. Finally, the relationship between the entanglement and the squeezing parameter of the squeezed state is demonstrated.
基金Project supported by the National Natural Science Foundation of China (Grant No 10574060)the Natural Science Foundation(Grant No Y2004A09) of Shandong Province,China
文摘This paper examines the quantization of mesoscopic circuit including Josephson junctions. Following Feynman＇s assumption, via the Hamilton dynamic approach and by virtue of the entangled state representation, it constructs Hamiltonian operator for the double-Josephson-junction mesoscopic circuit coupled by a capacitor. Then it uses the Heisenberg equation of motion to derive the induction voltage across each Josephson junction. The result manifestly shows how the voltage is affected by the capacitance coupling.
基金supported by the China Scholarship Council(CSC)the Danmarks Grundforskningsfond(Grant No.DNRF147)。
文摘The existence of a single topologically protected edge state in the first bulk bandgap for acoustic/elastic valley Hall insulators(VHIs)with zigzag interface configurations(ZICs)is well known.However,in this work,we show that an ultra-broadband edgestate pair in this bandgap can be created using the inverse design by topology optimization.The valley Hall insulator design increases the operational bandwidth 121%compared with an existing valley Hall insulator from recent literature and exhibits extreme field confinement,where more than 99%of the field intensity is concentrated within three unit-cells from the interface.One-way propagation and topological robustness towards small cavity defects are confirmed for the full bandwidth.The exploitation of such edge-state pairs of valley Hall insulators opens an avenue for realizing broadband confined edge modes.In tests for disorder and bend defects,we show that the additional ZIC,with a different operational frequency interval,encountered at the defects,degrades the transmission for bend and disorder defects which may prove significant for the application of VHIs.Through an alternative topology optimization method based on two ZICs,we further increase their common operational bandwidth.
文摘fragments, F- and Cl- including two isotope species 35Cl- and 37Cl-, are observed in the photoexcitations of CFC13. The ion-pair anion efficiency spectra of 35Cl- and 37Cl- are recorded in the photon energy range of 7.75-22.00 eV. The threshold of ion-pair dissociation CFCl3-CFC12＋＋Cl- is experimentally determined to be 7.944-0.04 eV. With the references of the high-resolution photoabsorption spectra reported in the literatures, we make tentative assignments of the electron valence-to-Rydberg transitions. Furthermore, the multibody ion-pair fragmentation processes to Cl- are discussed by comparison between the calculated thermochemical thresholds and the experimental efficiency spectrum.
文摘A state-dependent proof of Bell's theorem without inequalities using the product state of any two maximally entangled states (Bell states) of two qubits for two observers in an ideal condition, each of which possesses two qubits,is proposed. It is different from the other proofs in which there exists a fundamental requirement that certain specific suitable Bell states have been chosen. Moreover, in any non-ideal situation, a common Bell inequality independent of the choices of the 16-product states is derived, which is used to test the contradiction between quantum mechanics and local reality theory in the reach of current experimental technology.
基金This work is supported by the National Natural Science Foundation of China(Grant Nos.61370188,62176273,61962009)the Scientific Research Common Program of Beijing Municipal Commission of Education(KM202010015009,KM202110015004)+4 种基金Initial Funding for the Doctoral Program of BIGC(27170121001/009)the Open Foundation of State key Laboratory of Networking and Switching Technology(Beijing University of Posts and Telecommunications)(SKLNST-2021-1-16)the Open Fund of Advanced Cryptography and System Security Key Laboratory of Sichuan Province(Grant No.SKLACSS-202101)the Fundamental Research Funds for Beijing Municipal Commission of Education,Beijing Urban Governance Research Base of North China University of Technologythe Natural Science Foundation of Inner Mongolia(2021MS06006).
文摘As an innovative theory and technology,quantum network coding has become the research hotspot in quantum network communications.In this paper,a quantum remote state preparation scheme based on quantum network coding is proposed.Comparing with the general quantum remote state preparation schemes,our proposed scheme brings an arbitrary unknown quantum state finally prepared remotely through the quantum network,by designing the appropriate encoding and decoding steps for quantum network coding.What is worth mentioning,from the network model,this scheme is built on the quantum k-pair network which is the expansion of the typical bottleneck network—butterfly network.Accordingly,it can be treated as an efficient quantum network preparation scheme due to the characteristics of network coding,and it also makes the proposed scheme more applicable to the large-scale quantum networks.In addition,the fact of an arbitrary unknown quantum state remotely prepared means that the senders do not need to know the desired quantum state.Thus,the security of the proposed scheme is higher.Moreover,this scheme can always achieve the success probability of 1 and 1-max flow of value k.Thus,the communication efficiency of the proposed scheme is higher.Therefore,the proposed scheme turns out to be practicable,secure and efficient,which helps to effectively enrich the theory of quantum remote state preparation.
