Polarization-sensitive photodetectors based on two-dimensional(2D)materials have shown more attractive application prospects compared to traditional thin-film photodetectors due to their atomic thickness,tunable bandg...Polarization-sensitive photodetectors based on two-dimensional(2D)materials have shown more attractive application prospects compared to traditional thin-film photodetectors due to their atomic thickness,tunable bandgap,high mobility and strong light-matter interactions.Among them,2D molybdenum disulfide(MoS_(2))has drawn numerous attentions in photodetection due to its wide spectral range,remarkable photoresponsivity and fast photo-switching rate.However,the isotropic crystal structure of MoS_(2)hampers its application in the polarization-sensitive detection,which is highly desired in military and civilian applications.In this paper,we demonstrated an integration of plasmonic nanocavity with monolayer MoS_(2)to achieve high photoresponsivity and polarization-sensitive photodetector.With the significant enhancement of electromagnetic field provided by the gap-surfaceplasmon(GSP),we achieved a significant photoluminescence(PL)enhancement of 24-fold.Relying on the enhanced light absorption by our plasmonic nanocavity,which generally facilitates photo-generation of electron-hole pairs in MoS_(2),we achieved a high photoresponsivity of 1.88 A/W and degree of linear polarization(DOLP)of 0.8 at the excitation wavelength of 633 nm.Our work provides a feasible and universal solution to realize polarization-sensitive photodetector of MoS_(2)for high-performance and polarization-sensitive photodetectors.展开更多
基金This work was supported by the National Key Research and Development Program of China(No.2021YFA1400700)the National Natural Science Foundation of China(Nos.61888102,62204259,62174179,92265110,11974386,12074420,U21A20140 and 61905274)+4 种基金the Beijing Municipal Science&Technology Commission,Administrative Commission of Zhongguancun Science Park(No.Z211100004821009)the Strategic Priority Research Program of Chinese Academy of Sciences(CAS)(Nos.XDB33000000 and XDB28000000)the Key Research Program of Frontier Sciences of CAS(Nos.QYZDJ-SSWSLH042 and XDPB22)the Project for Young Scientists in Basic Research of CAS(No.YSBR021)This work was also supported by the Synergic Extreme Condition User Facility,China.
文摘Polarization-sensitive photodetectors based on two-dimensional(2D)materials have shown more attractive application prospects compared to traditional thin-film photodetectors due to their atomic thickness,tunable bandgap,high mobility and strong light-matter interactions.Among them,2D molybdenum disulfide(MoS_(2))has drawn numerous attentions in photodetection due to its wide spectral range,remarkable photoresponsivity and fast photo-switching rate.However,the isotropic crystal structure of MoS_(2)hampers its application in the polarization-sensitive detection,which is highly desired in military and civilian applications.In this paper,we demonstrated an integration of plasmonic nanocavity with monolayer MoS_(2)to achieve high photoresponsivity and polarization-sensitive photodetector.With the significant enhancement of electromagnetic field provided by the gap-surfaceplasmon(GSP),we achieved a significant photoluminescence(PL)enhancement of 24-fold.Relying on the enhanced light absorption by our plasmonic nanocavity,which generally facilitates photo-generation of electron-hole pairs in MoS_(2),we achieved a high photoresponsivity of 1.88 A/W and degree of linear polarization(DOLP)of 0.8 at the excitation wavelength of 633 nm.Our work provides a feasible and universal solution to realize polarization-sensitive photodetector of MoS_(2)for high-performance and polarization-sensitive photodetectors.
