In recent years,the gap between the supply and demand of medical radioisotopes has increased,necessitating new methods for producing medical radioisotopes.Photonuclear reactions based on gamma sources have unique adva...In recent years,the gap between the supply and demand of medical radioisotopes has increased,necessitating new methods for producing medical radioisotopes.Photonuclear reactions based on gamma sources have unique advantages in terms of producing high specific activity and innovative medical radioisotopes.However,the lack of experimental data on reaction cross sections for photonuclear reactions of medical radioisotopes of interest has severely limited the development and production of photonuclear transmutation medical radioisotopes.In this study,the entire process of the generation,decay,and measurement of medical radioisotopes was simulated using online gamma activation and offline gamma measurements combined with a shielding gamma-ray spectrometer.Based on a quasi-monochromatic gamma beam from the Shanghai Laser Electron Gamma Source(SLEGS),the feasibility of this measurement of production cross section for surveyed medi-cal radioisotopes was simulated,and specific solutions for measuring medical radioisotopes with ultra-low production cross sections were provided.The feasibility of this method for high-precision measurements of the reaction cross section of medical radioisotopes was demonstrated.展开更多
Two non-destructive analytical techniques (gamma spectrometer and X-ray diffractometer) were employed in the analysis of bauxite and rutile ore and their vicinity soil and control sourced within the Kanam and Wase min...Two non-destructive analytical techniques (gamma spectrometer and X-ray diffractometer) were employed in the analysis of bauxite and rutile ore and their vicinity soil and control sourced within the Kanam and Wase mineral exploration sites. The activity concentrations of natural radionuclides <sup>238</sup>U, <sup>232</sup>Th, and <sup>40</sup>K in the soil samples received from bauxite and rutile mineral mining vicinities revealed high concentrations of <sup>238</sup>U, <sup>232</sup>Th, and <sup>40</sup>K compared to the control soil samples sourced 500 m away from the mineral exploration vicinities. Radiological detriments RLI, AUI, Hin and Hex unveiled values exceeding the radiation standard concentration (>1) for soil. X-ray diffraction characterization of bauxite ore revealed the interlocking minerals of Bauxite (18)%, Albite (11)%, Garnet (15)%, Illite (6)% and Muscovite (43)% in various proportions obtained within the 2θ range (9.18 to 64.4) and a peak value (intensity, cps) of 3400. Pure bauxite percentage in the ore meets metallurgical grade (15 - 25)%. X-ray diffraction of rutile ore revealed the minerals of rutile (40)%, quartz (21.4)%, ilmenite (27)% and garnet (11.8)% found within the 2θ range (27.5 to 35.6) and a peak value intensity of 31.1 - 100.0 cps also meeting the metallurgical grade of 15% - 25%. The major environmental concern associated with the mineral-sands industry is the radiation hazards, pollution of ground-water sources from heavy metals, mineral transport with heavy equipment’s, dredging operations in fragile coastal area and clearing of vegetation.展开更多
Laser-accelerated electrons are promising in producing gamma-photon beams of high peak flux for the study of nuclear photonics,obtaining copious positrons and exploring photon–photon interaction in vacuum.We report o...Laser-accelerated electrons are promising in producing gamma-photon beams of high peak flux for the study of nuclear photonics,obtaining copious positrons and exploring photon–photon interaction in vacuum.We report on the experimental generation of brilliant gamma-ray beams with not only high photon yield but also low divergence,based on picosecond laser-accelerated electrons.The 120 J 1 ps laser pulse drives self-modulated wakefield acceleration in a high-density gas jet and generates tens-of-MeV electrons with 26 nC and divergence as small as 1.51◦.These collimated electrons produce gamma-ray photons through bremsstrahlung radiation when transversing a high-Z solid target.We design a high-energy-resolution Compton-scattering spectrometer and find that a total photon number of 2.2×10^(9)is captured within an acceptance angle of 1.1°for photon energies up to 16 MeV.Comparison between the experimental results and Monte Carlo simulations illustrates that the photon beam inherits the small divergence from electrons,corresponding to a total photon number of 2.2×10^(11)and a divergence of 7.73°.展开更多
Soil samples in and around salt field area have been analyzed for natural radioactivity concentration using gamma ray spectrometer.The activity concentration for ^(232)Th,^(238)U and ^(40)K are ranged from 27.88 to 45...Soil samples in and around salt field area have been analyzed for natural radioactivity concentration using gamma ray spectrometer.The activity concentration for ^(232)Th,^(238)U and ^(40)K are ranged from 27.88 to 45.27 Bq/kg, from BDL to 13.30 Bq/kg,and from 135.54 to 381.28 Bq/kg,respectively.The measured activity concentrations for these radionuclides were compared with world average activity of soil.The average activity concentration of ^(232)Th in the present study is 1.19 times higher than world median value while the activity of ^(238)U and ^(40)K is found to be lower. The absorbed dose rates due to these radionuclides were calculated.The average absorbed gamma dose rate due to the presence of ^(232)Th,^(238)U and ^(40)K in soil samples is 36.99 nGy·h^(-1).These results indicate no radiological anomaly. The data presented in this study will serve as a base line survey for primordial radionuclides concentration in the study area.展开更多
基金supported by the Strategic Priority Research Program of the CAS(No.XDB34030000)National Natural Science Foundation of China(No.11975210 and No.U1832129)+1 种基金National Key Research and Development Program of China(No.2022YFA1602404)Youth Innovation Promotion Association CAS(No.2017309).
文摘In recent years,the gap between the supply and demand of medical radioisotopes has increased,necessitating new methods for producing medical radioisotopes.Photonuclear reactions based on gamma sources have unique advantages in terms of producing high specific activity and innovative medical radioisotopes.However,the lack of experimental data on reaction cross sections for photonuclear reactions of medical radioisotopes of interest has severely limited the development and production of photonuclear transmutation medical radioisotopes.In this study,the entire process of the generation,decay,and measurement of medical radioisotopes was simulated using online gamma activation and offline gamma measurements combined with a shielding gamma-ray spectrometer.Based on a quasi-monochromatic gamma beam from the Shanghai Laser Electron Gamma Source(SLEGS),the feasibility of this measurement of production cross section for surveyed medi-cal radioisotopes was simulated,and specific solutions for measuring medical radioisotopes with ultra-low production cross sections were provided.The feasibility of this method for high-precision measurements of the reaction cross section of medical radioisotopes was demonstrated.
文摘Two non-destructive analytical techniques (gamma spectrometer and X-ray diffractometer) were employed in the analysis of bauxite and rutile ore and their vicinity soil and control sourced within the Kanam and Wase mineral exploration sites. The activity concentrations of natural radionuclides <sup>238</sup>U, <sup>232</sup>Th, and <sup>40</sup>K in the soil samples received from bauxite and rutile mineral mining vicinities revealed high concentrations of <sup>238</sup>U, <sup>232</sup>Th, and <sup>40</sup>K compared to the control soil samples sourced 500 m away from the mineral exploration vicinities. Radiological detriments RLI, AUI, Hin and Hex unveiled values exceeding the radiation standard concentration (>1) for soil. X-ray diffraction characterization of bauxite ore revealed the interlocking minerals of Bauxite (18)%, Albite (11)%, Garnet (15)%, Illite (6)% and Muscovite (43)% in various proportions obtained within the 2θ range (9.18 to 64.4) and a peak value (intensity, cps) of 3400. Pure bauxite percentage in the ore meets metallurgical grade (15 - 25)%. X-ray diffraction of rutile ore revealed the minerals of rutile (40)%, quartz (21.4)%, ilmenite (27)% and garnet (11.8)% found within the 2θ range (27.5 to 35.6) and a peak value intensity of 31.1 - 100.0 cps also meeting the metallurgical grade of 15% - 25%. The major environmental concern associated with the mineral-sands industry is the radiation hazards, pollution of ground-water sources from heavy metals, mineral transport with heavy equipment’s, dredging operations in fragile coastal area and clearing of vegetation.
基金This work was supported by the National Key R&D Program of China(No.2018YFA0404803)the National Natural Science Foundation of China(Nos.12175299,11905278,11975302,and 11935008)+1 种基金the CAS Project for Young Scientists in Basic Research(No.YSBR060)the Youth Innovation Promotion Association of Chinese Academy of Sciences(No.2021242).
文摘Laser-accelerated electrons are promising in producing gamma-photon beams of high peak flux for the study of nuclear photonics,obtaining copious positrons and exploring photon–photon interaction in vacuum.We report on the experimental generation of brilliant gamma-ray beams with not only high photon yield but also low divergence,based on picosecond laser-accelerated electrons.The 120 J 1 ps laser pulse drives self-modulated wakefield acceleration in a high-density gas jet and generates tens-of-MeV electrons with 26 nC and divergence as small as 1.51◦.These collimated electrons produce gamma-ray photons through bremsstrahlung radiation when transversing a high-Z solid target.We design a high-energy-resolution Compton-scattering spectrometer and find that a total photon number of 2.2×10^(9)is captured within an acceptance angle of 1.1°for photon energies up to 16 MeV.Comparison between the experimental results and Monte Carlo simulations illustrates that the photon beam inherits the small divergence from electrons,corresponding to a total photon number of 2.2×10^(11)and a divergence of 7.73°.
文摘Soil samples in and around salt field area have been analyzed for natural radioactivity concentration using gamma ray spectrometer.The activity concentration for ^(232)Th,^(238)U and ^(40)K are ranged from 27.88 to 45.27 Bq/kg, from BDL to 13.30 Bq/kg,and from 135.54 to 381.28 Bq/kg,respectively.The measured activity concentrations for these radionuclides were compared with world average activity of soil.The average activity concentration of ^(232)Th in the present study is 1.19 times higher than world median value while the activity of ^(238)U and ^(40)K is found to be lower. The absorbed dose rates due to these radionuclides were calculated.The average absorbed gamma dose rate due to the presence of ^(232)Th,^(238)U and ^(40)K in soil samples is 36.99 nGy·h^(-1).These results indicate no radiological anomaly. The data presented in this study will serve as a base line survey for primordial radionuclides concentration in the study area.
