A regional surface carbon dioxide （C02） flux inversion system, the Tan-Tracker-Region, was developed by incor- porating an assimilation scheme into the Community Multiscale Air Quality （CMAQ） regional chemical tra...A regional surface carbon dioxide （C02） flux inversion system, the Tan-Tracker-Region, was developed by incor- porating an assimilation scheme into the Community Multiscale Air Quality （CMAQ） regional chemical transport model to resolve fine-scale CO2 variability over East Asia. The proper orthogonal decomposition-based ensemble four-dimensional variational data assimilation approach （POD-4DVar） is the core algorithm for the joint assimilation framework, and simultaneous assimilations of CO2 concentrations and surface CO2 fluxes are applied to help reduce the uncertainty in initial CO2 concentrations. A persistence dynamical model was developed to describe the evolu- tion of the surface CO2 fluxes and help avoid the ＂signal-to-noise＂ problem; thus, CO2 fluxes could be estimated as a whole at the model grid scale, with better use of observation information. The performance of the regional inversion system was evaluated through a group of single-observation-based observing system simulation experiments （OSSEs）. The results of the experiments suggest that a reliable performance of Tan-Tracker-Region is dependent on certain assimilation parameter choices, for example, an optimized window length of approximately 3 h, an ensemble size of approximately 100, and a covariance localization radius of approximately 320 km. This is probably due to the strong diurnal variation and spatial heterogeneity in the fine-scale CMAQ simulation, which could affect the perform- ance of the regional inversion system. In addition, because all observations can be artificially obtained in OSSEs, the performance of Tan-Tracker-Region was further evaluated through different densities of the artificial observation net- work in different CO2 flux situations. The results indicate that more observation sites would be useful to systematic- ally improve the estimation of CO2 concentration and flux in large areas over the model domain. The work presented here forms a foundation for future research in which a thorough estimation o展开更多
基金Supported by the National Natural Science Foundation of China(41130528)National High Technology Research and Development Program of China(2013AA122002)+1 种基金Strategic Priority Research Program-Climate Change:Carbon Budget and Relevant Issues(XDA05040404)National Key Technology Research and Development Program of China(2016YFC0202103)
文摘A regional surface carbon dioxide （C02） flux inversion system, the Tan-Tracker-Region, was developed by incor- porating an assimilation scheme into the Community Multiscale Air Quality （CMAQ） regional chemical transport model to resolve fine-scale CO2 variability over East Asia. The proper orthogonal decomposition-based ensemble four-dimensional variational data assimilation approach （POD-4DVar） is the core algorithm for the joint assimilation framework, and simultaneous assimilations of CO2 concentrations and surface CO2 fluxes are applied to help reduce the uncertainty in initial CO2 concentrations. A persistence dynamical model was developed to describe the evolu- tion of the surface CO2 fluxes and help avoid the ＂signal-to-noise＂ problem; thus, CO2 fluxes could be estimated as a whole at the model grid scale, with better use of observation information. The performance of the regional inversion system was evaluated through a group of single-observation-based observing system simulation experiments （OSSEs）. The results of the experiments suggest that a reliable performance of Tan-Tracker-Region is dependent on certain assimilation parameter choices, for example, an optimized window length of approximately 3 h, an ensemble size of approximately 100, and a covariance localization radius of approximately 320 km. This is probably due to the strong diurnal variation and spatial heterogeneity in the fine-scale CMAQ simulation, which could affect the perform- ance of the regional inversion system. In addition, because all observations can be artificially obtained in OSSEs, the performance of Tan-Tracker-Region was further evaluated through different densities of the artificial observation net- work in different CO2 flux situations. The results indicate that more observation sites would be useful to systematic- ally improve the estimation of CO2 concentration and flux in large areas over the model domain. The work presented here forms a foundation for future research in which a thorough estimation o
