The interfacial diffusive contaminant（phosphorus） release from permeable sediment layer into overlying water column under a unidirectional unsteady（periodic） flow condition was experimentally measured and analyzed...The interfacial diffusive contaminant（phosphorus） release from permeable sediment layer into overlying water column under a unidirectional unsteady（periodic） flow condition was experimentally measured and analyzed. The experimental results indicate that the gross diffusive contaminant release rate is substantially enhanced as compared to that under a steady flow condition, and this enhancement trend is much more pronounced in an immediate release stage. The interfacial diffusive contaminant release rate tends to increase with the increasing flow velocity, decreasing period and augmenting amplitude for the case of the unsteady flow. The additional interfacial diffusive contaminant release under the unsteady flow condition may be related to the hydrodynamic response of the diffusive boundary layer to the flow unsteadiness of the overlying water, depending upon not only the periodic thickness variation of the diffusive boundary layer immediately above the sediment-water interface modulated by the temporal flow velocity of the overlying water column but also the intensified turbulent mixing between the overlying water and the pore-water within the superficial sediment layer induced by an alternate acceleration/deceleration fluctuation during each period.展开更多
A simple modeling approach was suggested to simulate preferential transport of water and contaminants in soil. After saturated hydraulic conductivity was interpolated by means of Krige interpolation method or scaling ...A simple modeling approach was suggested to simulate preferential transport of water and contaminants in soil. After saturated hydraulic conductivity was interpolated by means of Krige interpolation method or scaling method, and then zoned, the locations where saturated hydraulic conductivity was larger represented regions where preferential flow occurred, because heterogeneity of soil, one of the mechanisms resulting in preferential flow, could be reflected through the difference in saturated hydraulic conductivity. The modeling approach was validated through numerical simulation of contaminant transport in a two-dimensional hypothetical soil profile. The results of the numerical simulation showed that the approach suggested in this study was feasible.展开更多
Metal contaminants from surface water pollution events often enter hyporheic zones,under certain conditions,they may be released back into streams,causing secondary pollution to the water quality.The present study inv...Metal contaminants from surface water pollution events often enter hyporheic zones,under certain conditions,they may be released back into streams,causing secondary pollution to the water quality.The present study investigated the effects of adsorption,permeability,and anisotropy of sediment beds on the release of zinc ions(Zn^(2+))from the hyporheic zone into overlying turbulent flows using large-eddy simulations(LES).The volume-averaged Navier-Stokes equations and advection-diffusion equation with adsorption term were used to describe the sediment in-flow,adsorption,and convective diffusion of Zn^(2+) within the sediment layer.The effects of sediment permeability on the Zn^(2+)concentration distribution and mass transfer processes were investigated by time-averaged statistics of flow and concentration fields.The results show that adsorption becomes stronger as the pH value increases,leading to a slow increase in Zn^(2+)concentration in the overlying water layer and reaching a lower steady-state concentration.Higher overall permeability of the sediment layer can enhance mass and momentum exchange near the sediment-water interface(SWI),and intensify the release of Zn^(2+)from the sediment layer into the overlying water.As the wall-normal permeability of the sediment layer increases,the normal turbulent intensity strengthens,momentum transport enhances,the wall-normal Zn^(2+)concentration flux increases,the effective diffusion coefficient increases,and the concentration in the overlying water increases.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11032007,11472168)the Shanghai key Laboratory of mechanics in energy Engineering and Shanghai Program for Innovative Research Team in Universities
文摘The interfacial diffusive contaminant（phosphorus） release from permeable sediment layer into overlying water column under a unidirectional unsteady（periodic） flow condition was experimentally measured and analyzed. The experimental results indicate that the gross diffusive contaminant release rate is substantially enhanced as compared to that under a steady flow condition, and this enhancement trend is much more pronounced in an immediate release stage. The interfacial diffusive contaminant release rate tends to increase with the increasing flow velocity, decreasing period and augmenting amplitude for the case of the unsteady flow. The additional interfacial diffusive contaminant release under the unsteady flow condition may be related to the hydrodynamic response of the diffusive boundary layer to the flow unsteadiness of the overlying water, depending upon not only the periodic thickness variation of the diffusive boundary layer immediately above the sediment-water interface modulated by the temporal flow velocity of the overlying water column but also the intensified turbulent mixing between the overlying water and the pore-water within the superficial sediment layer induced by an alternate acceleration/deceleration fluctuation during each period.
基金Project supported by the National Natural Science Foundation of China (No. 49971041), the National KeyBasic Research and Devel
文摘A simple modeling approach was suggested to simulate preferential transport of water and contaminants in soil. After saturated hydraulic conductivity was interpolated by means of Krige interpolation method or scaling method, and then zoned, the locations where saturated hydraulic conductivity was larger represented regions where preferential flow occurred, because heterogeneity of soil, one of the mechanisms resulting in preferential flow, could be reflected through the difference in saturated hydraulic conductivity. The modeling approach was validated through numerical simulation of contaminant transport in a two-dimensional hypothetical soil profile. The results of the numerical simulation showed that the approach suggested in this study was feasible.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.12172207,92052201).
文摘Metal contaminants from surface water pollution events often enter hyporheic zones,under certain conditions,they may be released back into streams,causing secondary pollution to the water quality.The present study investigated the effects of adsorption,permeability,and anisotropy of sediment beds on the release of zinc ions(Zn^(2+))from the hyporheic zone into overlying turbulent flows using large-eddy simulations(LES).The volume-averaged Navier-Stokes equations and advection-diffusion equation with adsorption term were used to describe the sediment in-flow,adsorption,and convective diffusion of Zn^(2+) within the sediment layer.The effects of sediment permeability on the Zn^(2+)concentration distribution and mass transfer processes were investigated by time-averaged statistics of flow and concentration fields.The results show that adsorption becomes stronger as the pH value increases,leading to a slow increase in Zn^(2+)concentration in the overlying water layer and reaching a lower steady-state concentration.Higher overall permeability of the sediment layer can enhance mass and momentum exchange near the sediment-water interface(SWI),and intensify the release of Zn^(2+)from the sediment layer into the overlying water.As the wall-normal permeability of the sediment layer increases,the normal turbulent intensity strengthens,momentum transport enhances,the wall-normal Zn^(2+)concentration flux increases,the effective diffusion coefficient increases,and the concentration in the overlying water increases.
