In the past decades,machine learning(ML)has impacted the field of electrocatalysis.Modern researchers have begun to take advantage of ML‐based data‐driven techniques to overcome the computational and experimental li...In the past decades,machine learning(ML)has impacted the field of electrocatalysis.Modern researchers have begun to take advantage of ML‐based data‐driven techniques to overcome the computational and experimental limitations to accelerate rational catalyst design.Hence,significant efforts have been made to perform ML to accelerate calculation and aid electrocatalyst design for CO_(2) reduction.This review discusses recent applications of ML to discover,design,and optimize novel electrocatalysts.First,insights into ML aided in accelerating calculation are presented.Then,ML aided in the rational design of the electrocatalyst is introduced,including establishing a data set/data source selection and validation of descriptor selection of ML algorithms validation and predictions of the model.Finally,the opportunities and future challenges are summarized for the future design of electrocatalyst for CO_(2) reduction with the assistance of ML.展开更多
In recent years, network traffic data have become larger and more complex, leading to higher possibilities of network intrusion. Traditional intrusion detection methods face difficulty in processing high-speed network...In recent years, network traffic data have become larger and more complex, leading to higher possibilities of network intrusion. Traditional intrusion detection methods face difficulty in processing high-speed network data and cannot detect currently unknown attacks. Therefore, this paper proposes a network attack detection method combining a flow calculation and deep learning. The method consists of two parts: a real-time detection algorithm based on flow calculations and frequent patterns and a classification algorithm based on the deep belief network and support vector machine(DBN-SVM). Sliding window(SW) stream data processing enables real-time detection, and the DBN-SVM algorithm can improve classification accuracy. Finally, to verify the proposed method, a system is implemented.Based on the CICIDS2017 open source data set, a series of comparative experiments are conducted. The method's real-time detection efficiency is higher than that of traditional machine learning algorithms. The attack classification accuracy is 0.7 percentage points higher than that of a DBN, which is 2 percentage points higher than that of the integrated algorithm boosting and bagging methods. Hence, it is suitable for the real-time detection of high-speed network intrusions.展开更多
基金ANU Futures Scheme,Grant/Award Number:Q4601024National Natural Science Foundation of China,Grant/Award Number:22078054+1 种基金Australian Research Council,Grant/Award Number:DP190100295China Scholarship Council(CSC)Program。
文摘In the past decades,machine learning(ML)has impacted the field of electrocatalysis.Modern researchers have begun to take advantage of ML‐based data‐driven techniques to overcome the computational and experimental limitations to accelerate rational catalyst design.Hence,significant efforts have been made to perform ML to accelerate calculation and aid electrocatalyst design for CO_(2) reduction.This review discusses recent applications of ML to discover,design,and optimize novel electrocatalysts.First,insights into ML aided in accelerating calculation are presented.Then,ML aided in the rational design of the electrocatalyst is introduced,including establishing a data set/data source selection and validation of descriptor selection of ML algorithms validation and predictions of the model.Finally,the opportunities and future challenges are summarized for the future design of electrocatalyst for CO_(2) reduction with the assistance of ML.
基金supported by the National Key Research and Development Program of China(2017YFB1401300,2017YFB1401304)the National Natural Science Foundation of China(61702211,L1724007,61902203)+3 种基金Hubei Provincial Science and Technology Program of China(2017AKA191)the Self-Determined Research Funds of Central China Normal University(CCNU)from the Colleges’Basic Research(CCNU17QD0004,CCNU17GF0002)the Natural Science Foundation of Shandong Province(ZR2017QF015)the Key Research and Development Plan–Major Scientific and Technological Innovation Projects of Shandong Province(2019JZZY020101)。
文摘In recent years, network traffic data have become larger and more complex, leading to higher possibilities of network intrusion. Traditional intrusion detection methods face difficulty in processing high-speed network data and cannot detect currently unknown attacks. Therefore, this paper proposes a network attack detection method combining a flow calculation and deep learning. The method consists of two parts: a real-time detection algorithm based on flow calculations and frequent patterns and a classification algorithm based on the deep belief network and support vector machine(DBN-SVM). Sliding window(SW) stream data processing enables real-time detection, and the DBN-SVM algorithm can improve classification accuracy. Finally, to verify the proposed method, a system is implemented.Based on the CICIDS2017 open source data set, a series of comparative experiments are conducted. The method's real-time detection efficiency is higher than that of traditional machine learning algorithms. The attack classification accuracy is 0.7 percentage points higher than that of a DBN, which is 2 percentage points higher than that of the integrated algorithm boosting and bagging methods. Hence, it is suitable for the real-time detection of high-speed network intrusions.
