Monitoring and modeling of airborne particulate matter(PM)from low-altitude sources is becoming an important regulatory target as the adverse health consequences of PM become better understood.However,application of m...Monitoring and modeling of airborne particulate matter(PM)from low-altitude sources is becoming an important regulatory target as the adverse health consequences of PM become better understood.However,application of models not specifically designed for simulation of PM from low-altitude emissions may bias predictions.To address this problem,we describe the modification and validation of an air dispersion model for the simulation of lowaltitude PM dispersion from a typical cotton ginning facility.We found that the regulatory recommended model(AERMOD)overestimated pollutant concentrations by factors of 64.7,6.97 and 7.44 on average for PM 2.5,PM 10,and TSP,respectively.Pollutant concentrations were negatively correlated with height(p<0.05),distance from source(p<0.05)and standard deviation of wind direction(p<0.001),and positively correlated with average wind speed(p<0.001).Based on these results,we developed dispersion correction factors for AERMOD and cross-validated the revised model against independent observations,reducing overestimation factors to 3.75,1.52 and 1.44 for PM 2.5,PM 10 and TSP,respectively.Further reductions in model error may be obtained from use of additional observations and refinement of dispersive correction factors.More generally,the correction permits the validated adjustment and application of pre-existing models for risk assessment and development of remediation techniques.The same approach may also be applied to improve simulations of other air pollutants and environmental conditions of concern.展开更多
Abrupt air pollution accidents can endanger people’s health and destroy the local ecological environment.The appropriate emergency response can minimize the harmful effects of accidents and protect people’s lives an...Abrupt air pollution accidents can endanger people’s health and destroy the local ecological environment.The appropriate emergency response can minimize the harmful effects of accidents and protect people’s lives and property.This paper provides an overview of the key emergency response technologies for abrupt air pollution accidents around the globe with emphasis on the major achievements that China has obtained in recent years.With decades of effort,China has made significant progress in emergency monitoring technologies and equipment,source estimation technologies,pollutant dispersion simulation technologies and others.Many effective domestic emergency monitoring instruments(e.g.,portable DOAS/FT-IR systems,portable FID/PID systems,portable GC-MS systems,scanning imaging remote sensing systems,and emergency monitoring vehicles)had been developed which can meet the demands for routine emergency response activities.A monitoring layout technique combining air dispersion simulation,fuzzy comprehensive evaluation,and a post-optimality analysis was proposed to identify the optimal monitoring layout scheme under the constraints of limited monitoring resources.Multiple source estimation technologies,including the forward method and the inversion method,have been established and evaluated under various scenarios.Multi-scale dynamic pollution dispersion simulation systems with high temporal and spatial resolution were further developed.A comprehensive emergency response platform integrating database support,source estimation,monitoring schemes,fast monitoring of pollutants,pollution predictions and risk assessment was developed based on the technical idea of"source identification-model simulation-environmental monitoring"dynamic interactive feedback.It is expected that the emergency response capability for abrupt air pollution accidents will gradually improve in China.展开更多
基金provided by National Programs 306,Product Quality and New Uses,and 212,Soil and Air
文摘Monitoring and modeling of airborne particulate matter(PM)from low-altitude sources is becoming an important regulatory target as the adverse health consequences of PM become better understood.However,application of models not specifically designed for simulation of PM from low-altitude emissions may bias predictions.To address this problem,we describe the modification and validation of an air dispersion model for the simulation of lowaltitude PM dispersion from a typical cotton ginning facility.We found that the regulatory recommended model(AERMOD)overestimated pollutant concentrations by factors of 64.7,6.97 and 7.44 on average for PM 2.5,PM 10,and TSP,respectively.Pollutant concentrations were negatively correlated with height(p<0.05),distance from source(p<0.05)and standard deviation of wind direction(p<0.001),and positively correlated with average wind speed(p<0.001).Based on these results,we developed dispersion correction factors for AERMOD and cross-validated the revised model against independent observations,reducing overestimation factors to 3.75,1.52 and 1.44 for PM 2.5,PM 10 and TSP,respectively.Further reductions in model error may be obtained from use of additional observations and refinement of dispersive correction factors.More generally,the correction permits the validated adjustment and application of pre-existing models for risk assessment and development of remediation techniques.The same approach may also be applied to improve simulations of other air pollutants and environmental conditions of concern.
基金supported by the National Key Research and Development Program of China(No.2017YFC0209900)Beijing Nova Program from Beijing Municipal Science&Technology Commission(No.Z201100006820098)the Youth Science and Technology Talents Support Program(2020)by Anhui Association for Science and Technology(No.RCTJ202002)。
文摘Abrupt air pollution accidents can endanger people’s health and destroy the local ecological environment.The appropriate emergency response can minimize the harmful effects of accidents and protect people’s lives and property.This paper provides an overview of the key emergency response technologies for abrupt air pollution accidents around the globe with emphasis on the major achievements that China has obtained in recent years.With decades of effort,China has made significant progress in emergency monitoring technologies and equipment,source estimation technologies,pollutant dispersion simulation technologies and others.Many effective domestic emergency monitoring instruments(e.g.,portable DOAS/FT-IR systems,portable FID/PID systems,portable GC-MS systems,scanning imaging remote sensing systems,and emergency monitoring vehicles)had been developed which can meet the demands for routine emergency response activities.A monitoring layout technique combining air dispersion simulation,fuzzy comprehensive evaluation,and a post-optimality analysis was proposed to identify the optimal monitoring layout scheme under the constraints of limited monitoring resources.Multiple source estimation technologies,including the forward method and the inversion method,have been established and evaluated under various scenarios.Multi-scale dynamic pollution dispersion simulation systems with high temporal and spatial resolution were further developed.A comprehensive emergency response platform integrating database support,source estimation,monitoring schemes,fast monitoring of pollutants,pollution predictions and risk assessment was developed based on the technical idea of"source identification-model simulation-environmental monitoring"dynamic interactive feedback.It is expected that the emergency response capability for abrupt air pollution accidents will gradually improve in China.
