We report new results of triple differential cross sections for the single ionization of helium by 1-KeV electron impact at the ejection energy of 10 eV. Investigations have been made for both the perpendicular plane ...We report new results of triple differential cross sections for the single ionization of helium by 1-KeV electron impact at the ejection energy of 10 eV. Investigations have been made for both the perpendicular plane and the plane perpendicular to the momentum transfer geometries. The present calculation is based on the threewCoulomb wave function. Here we have also incorporated the effect of target polarization in the initial state. A comparison is made between the present calculation with the results of other theoretical methods and a recent experiment [Diirr M, Dimopoulou C, Najjari B, Dorn A, Bartschat K, Bray I, Fursa D V, Chen Z, Madison D H and Ullrich J 2008 Phys. Rev. A 77 032717]. At an impact energy of 1 KeV, the target polarization is found to induce a substantial change of the cross section for the ionization process. We observe that the effect of target polarization plays a dominant role in deciding the shape of triple differential cross sections.展开更多
The second-order distorted wave Born aPl6roximation （DWBA） method is employed to investigate the triple differen- tial cross sections （TDCS） of coplanar doubly symmetric （e, 2e） collisions for magnesium at exces...The second-order distorted wave Born aPl6roximation （DWBA） method is employed to investigate the triple differen- tial cross sections （TDCS） of coplanar doubly symmetric （e, 2e） collisions for magnesium at excess energies of 6 eV-20 eV. Comparing with the standard first-order DWBA calculations, the inclusion of the second-order Born term in the scattering amplitude improves the degree of agreement with experiments, especially for backward scattering region of TDCS. This indicates that the present second-order Born term is capable to give a reasonable correction to DWBA model in studying coplanar symmetric （e, 2e） problems of two-valence-electron target in low energy range.展开更多
A dynamically screened three-Coulomb-wave （DS3C） method is applied to study the single ionization of magnesium by electron impact. Triple differential cross sections （TDCS） are calculated in doubly symmetric geome...A dynamically screened three-Coulomb-wave （DS3C） method is applied to study the single ionization of magnesium by electron impact. Triple differential cross sections （TDCS） are calculated in doubly symmetric geometry at incident energies of 13.65, 17.65, 22.65, 27.65, 37.65, 47.65, 57.65, and 67.65 eV. Comparisons are made with experimental data and theoretical predictions from a three-Coulomb-wave function （3C） approach and distorted-wave Born approximation （DWBA）. The overall agreement between the predictions of the DS3C model and the DWBA approach with the experimen- tal data is satisfactory.展开更多
The triple-differential cross section （TDCS） for the （e,2e） ionization of a hydrogen molecule is calculated using the molecule distorted-wave Born approximation （MDWBA）. Distorted waves are obtained by solving m...The triple-differential cross section （TDCS） for the （e,2e） ionization of a hydrogen molecule is calculated using the molecule distorted-wave Born approximation （MDWBA）. Distorted waves are obtained by solving momentum-space coupled-channel Lippmann-Schwinger equations, including the ground state and the lowest-lying electronic state of b3Σu . TDCSs at the incident energy 100 eV in coplanar asymmetric geometry are reported. The present calculations are compared with the available experimental measurements and the theoretical results.展开更多
The standard distorted wave Born approximation （DWBA） method has been extended to second-order Born amplitude in order to describe the multiple interactions between the projectile and the atomic target. Second-order...The standard distorted wave Born approximation （DWBA） method has been extended to second-order Born amplitude in order to describe the multiple interactions between the projectile and the atomic target. Second-order DWBA calculations have been preformed to investigate the triple differential cross sections （TDCS） of coplanar doubly symmetric （e, 2e） collisions for the alkali target potassium at excess energies of 6 eV-60 eV. Compared with the previous first-order DWBA calculations, the present theoretical model improves the degree of agreement with experiments, especially for the backward scattering angle region of TDCS. This indicates that the present second-order Born term is capable of giving a reasonable correction to the DWBA model in studying coplanar symmetric （e, 2e） problems in low and intermediate energy ranges.展开更多
The （e, 2e） triple-differential cross sections of Ag＋ （4p, 4s） are calculated based on the three-body distorted-wave Born approximation considering post-collision interaction in coplanar symmetric geometry. The e...The （e, 2e） triple-differential cross sections of Ag＋ （4p, 4s） are calculated based on the three-body distorted-wave Born approximation considering post-collision interaction in coplanar symmetric geometry. The energy of the outgoing electron is set to be 50, 70, 100, 200, 300,500, 700, and 1000 eV, and the intensity and splitting of forward and backward peaks are discussed in detail. Some new structures are observed around 15° and 85° for 4p and 4s orbitals. Structures in triple-differential cross sections at 15° are reported for the first time. A double-binary collision is proposed to explain the formation of such structures. The structures at 85° are also considered as the result of one kind of double-binary collision.展开更多
本文使用扭曲波波恩近似方法(DWBA)研究了共面对称条件下钙原子的电子碰撞电离反应((e,2e)反应),在DWBA理论的基础上,考虑了原子极化势和离子极化势对三重微分散射截面的影响.采用发展的DWBA方法,我们研究了出射电子能量从6.75 e V到29....本文使用扭曲波波恩近似方法(DWBA)研究了共面对称条件下钙原子的电子碰撞电离反应((e,2e)反应),在DWBA理论的基础上,考虑了原子极化势和离子极化势对三重微分散射截面的影响.采用发展的DWBA方法,我们研究了出射电子能量从6.75 e V到29.25 e V范围内电子与钙原子的碰撞电离过程,计算了电离三重微分截面.通过与已有理论和实验数据进行比较发现,离子极化势对钙原子的共面对称(e,2e)反应散射微分截面有较大的影响,很好的描述了碰撞电离微分截面的结构效应,特别是在散射角度较小时(≦60o),本文计算结果与实验测量非常一致.展开更多
The electron momentum distribution of 3σ_u orbital of carbon dioxide has been measured at high momentum resolution. Through comparation between experimental and theoretical results, the calculation by DFT-B3LYP metho...The electron momentum distribution of 3σ_u orbital of carbon dioxide has been measured at high momentum resolution. Through comparation between experimental and theoretical results, the calculation by DFT-B3LYP method using 6- 311 + +G basis set is more agreement with the experirnental data than other calculations.展开更多
基金Project supported by the Natural Science Foundation of Shanxi Province of China (Grant Nos. 20051008 and 2010011009)the National Natural Science Foundation of China (Grant No. 11047191)+1 种基金the Key Project of Chinese Ministry of Education (Grant No. 211025)the Natural Science Foundation for Young Scientists of Shanxi Province, China (Grant No. 2009021005)
文摘We report new results of triple differential cross sections for the single ionization of helium by 1-KeV electron impact at the ejection energy of 10 eV. Investigations have been made for both the perpendicular plane and the plane perpendicular to the momentum transfer geometries. The present calculation is based on the threewCoulomb wave function. Here we have also incorporated the effect of target polarization in the initial state. A comparison is made between the present calculation with the results of other theoretical methods and a recent experiment [Diirr M, Dimopoulou C, Najjari B, Dorn A, Bartschat K, Bray I, Fursa D V, Chen Z, Madison D H and Ullrich J 2008 Phys. Rev. A 77 032717]. At an impact energy of 1 KeV, the target polarization is found to induce a substantial change of the cross section for the ionization process. We observe that the effect of target polarization plays a dominant role in deciding the shape of triple differential cross sections.
基金supported by the National Natural Science Foundation of China(Grant No.11174066)
文摘The second-order distorted wave Born aPl6roximation （DWBA） method is employed to investigate the triple differen- tial cross sections （TDCS） of coplanar doubly symmetric （e, 2e） collisions for magnesium at excess energies of 6 eV-20 eV. Comparing with the standard first-order DWBA calculations, the inclusion of the second-order Born term in the scattering amplitude improves the degree of agreement with experiments, especially for backward scattering region of TDCS. This indicates that the present second-order Born term is capable to give a reasonable correction to DWBA model in studying coplanar symmetric （e, 2e） problems of two-valence-electron target in low energy range.
基金supported by the National Natural Science Foundation of China(Grant No.11274215)
文摘A dynamically screened three-Coulomb-wave （DS3C） method is applied to study the single ionization of magnesium by electron impact. Triple differential cross sections （TDCS） are calculated in doubly symmetric geometry at incident energies of 13.65, 17.65, 22.65, 27.65, 37.65, 47.65, 57.65, and 67.65 eV. Comparisons are made with experimental data and theoretical predictions from a three-Coulomb-wave function （3C） approach and distorted-wave Born approximation （DWBA）. The overall agreement between the predictions of the DS3C model and the DWBA approach with the experimen- tal data is satisfactory.
基金the National Natural Science Foundation of China(Grant No.11174066)the Key Fund Project of Education Department of Sichuan Province,China(Grant No.13ZA0044)
文摘The triple-differential cross section （TDCS） for the （e,2e） ionization of a hydrogen molecule is calculated using the molecule distorted-wave Born approximation （MDWBA）. Distorted waves are obtained by solving momentum-space coupled-channel Lippmann-Schwinger equations, including the ground state and the lowest-lying electronic state of b3Σu . TDCSs at the incident energy 100 eV in coplanar asymmetric geometry are reported. The present calculations are compared with the available experimental measurements and the theoretical results.
基金Project supported by the National Natural Science Foundation of China (Grant No. 11174066)
文摘The standard distorted wave Born approximation （DWBA） method has been extended to second-order Born amplitude in order to describe the multiple interactions between the projectile and the atomic target. Second-order DWBA calculations have been preformed to investigate the triple differential cross sections （TDCS） of coplanar doubly symmetric （e, 2e） collisions for the alkali target potassium at excess energies of 6 eV-60 eV. Compared with the previous first-order DWBA calculations, the present theoretical model improves the degree of agreement with experiments, especially for the backward scattering angle region of TDCS. This indicates that the present second-order Born term is capable of giving a reasonable correction to the DWBA model in studying coplanar symmetric （e, 2e） problems in low and intermediate energy ranges.
基金Project supported by the Natural Science Foundation of Shandong Province, China (Grant No. Q2008A07)
文摘The （e, 2e） triple-differential cross sections of Ag＋ （4p, 4s） are calculated based on the three-body distorted-wave Born approximation considering post-collision interaction in coplanar symmetric geometry. The energy of the outgoing electron is set to be 50, 70, 100, 200, 300,500, 700, and 1000 eV, and the intensity and splitting of forward and backward peaks are discussed in detail. Some new structures are observed around 15° and 85° for 4p and 4s orbitals. Structures in triple-differential cross sections at 15° are reported for the first time. A double-binary collision is proposed to explain the formation of such structures. The structures at 85° are also considered as the result of one kind of double-binary collision.
文摘本文使用扭曲波波恩近似方法(DWBA)研究了共面对称条件下钙原子的电子碰撞电离反应((e,2e)反应),在DWBA理论的基础上,考虑了原子极化势和离子极化势对三重微分散射截面的影响.采用发展的DWBA方法,我们研究了出射电子能量从6.75 e V到29.25 e V范围内电子与钙原子的碰撞电离过程,计算了电离三重微分截面.通过与已有理论和实验数据进行比较发现,离子极化势对钙原子的共面对称(e,2e)反应散射微分截面有较大的影响,很好的描述了碰撞电离微分截面的结构效应,特别是在散射角度较小时(≦60o),本文计算结果与实验测量非常一致.
文摘The electron momentum distribution of 3σ_u orbital of carbon dioxide has been measured at high momentum resolution. Through comparation between experimental and theoretical results, the calculation by DFT-B3LYP method using 6- 311 + +G basis set is more agreement with the experirnental data than other calculations.
