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黑碳团簇及具有包覆水层混合态粒子的光学特性 被引量:6
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作者 徐澍 白连红 +1 位作者 范萌 葛强 《光学学报》 EI CAS CSCD 北大核心 2017年第2期8-16,共9页
基于扩散限制凝聚模型仿真生成了黑碳团簇粒子和具备核-壳结构(核为黑碳团簇,壳为包覆水层)的混合态粒子,并模拟了黑碳团簇粒子的老化过程,利用团簇T矩阵方法计算并研究了粒子形态结构和包覆水层对两种粒子在550nm波长处的光学特性。分... 基于扩散限制凝聚模型仿真生成了黑碳团簇粒子和具备核-壳结构(核为黑碳团簇,壳为包覆水层)的混合态粒子,并模拟了黑碳团簇粒子的老化过程,利用团簇T矩阵方法计算并研究了粒子形态结构和包覆水层对两种粒子在550nm波长处的光学特性。分析表明,新生黑碳团簇粒子的光学特性参数与等体积球形黑碳粒子之间的差异最大,当分形维数Df为1.8时,散射截面和单次散射反照率的相对偏差分别达到61.58%和49.44%,随着黑碳团簇粒子的老化,差异逐渐减小。对于混合态粒子,忽略黑碳核的团簇结构会导致前向散射强度、散射截面、消光截面、单次散射反照率、不对称因子和F_(34)/F_(11)被低估,导致后向散射强度、吸收截面、-F_(12)/F_(11)、F_(33)/F_(11)、F_(44)/F_(11)被高估;包覆水层厚度的增加会加剧混合态粒子散射矩阵中元素随散射角的振荡程度,且忽略黑碳核或球形黑碳核假设所引起的光学特性参数相对偏差呈逐渐减小的趋势。该工作有助于进一步减小黑碳气溶胶辐射强迫估算误差。 展开更多
关键词 大气光学 强迫估算 黑碳团簇 团簇T矩阵 混合态
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燃烧过程中碳烟辐射特性预测方法评述 被引量:4
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作者 刘玉英 李娜娜 黄望全 《推进技术》 EI CAS CSCD 北大核心 2016年第3期479-487,共9页
碳烟辐射特性研究对正确预测火焰连续辐射非常重要。对基于Rayleigh理论的经典碳烟光谱吸收系数和灰体吸收系数预测模型进行了详细综述与分析,并对与预测模型密切相关的碳烟复折射率研究状况和碳烟吸收系数模型常数的应用情况进行了分... 碳烟辐射特性研究对正确预测火焰连续辐射非常重要。对基于Rayleigh理论的经典碳烟光谱吸收系数和灰体吸收系数预测模型进行了详细综述与分析,并对与预测模型密切相关的碳烟复折射率研究状况和碳烟吸收系数模型常数的应用情况进行了分析总结,对碳烟聚合物辐射特性的预测方法进行简要概述。分析认为,目前燃烧碳烟辐射特性预测仍以传统的Rayleigh理论近似方法为主,但需注意模型常数的不确定性及选取。基于分形理论的碳烟聚合物辐射特性预测方法更加准确,但由于其自身的复杂性,目前主要以方法研究为主,鲜见用于燃烧过程中火焰辐射的模拟,因此火焰中碳烟聚合物的辐射特性预测仍有待进一步开展研究。 展开更多
关键词 燃烧 辐射特性 吸收系数 复折射率 碳烟聚合物 Rayleigh理论
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Application of WSGSA Model in Predicting Temperature and Soot in C_(2)H_(4)/Air Turbulent Diffusion Flame 被引量:1
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作者 HE Zhenzong ZHU Ruihan +2 位作者 DONG Chuanhui MAO Junkui FU Yao 《Transactions of Nanjing University of Aeronautics and Astronautics》 EI CSCD 2022年第4期482-492,共11页
Soot,a product of insufficient combustion,is usually in the form of aggregate. The multi-scattering of soot fractal aggregates has been proved to play an important role in studying the soot radiative properties,which ... Soot,a product of insufficient combustion,is usually in the form of aggregate. The multi-scattering of soot fractal aggregates has been proved to play an important role in studying the soot radiative properties,which is rarely considered in predicting the radiative heat transfer in combustion flame. In the present study,based on the weighted sum of gray soot fractal aggregate(WSGSA) model,which is used to predict the temperature field and soot aggregates in turbulent diffusion flame,the flame temperature distribution and soot volume fraction distribution under the conditions of the model without considering radiation,the default radiation model in Fluent software and the WSGSA model are calculated respectively. The results show that the flame temperature will be seriously overestimated without considering radiation and the maximum relative discrepancy of flame centerline temperature is about 64.5%. The accuracy will be improved by the default radiation model in the Fluent software,but the flame temperature is still overestimated and the maximum relative discrepancy of flame centerline temperature is about 42.1%. However,more satisfactory results can be obtained by the WSGSA model,and the maximum relative discrepancy of flame centerline temperature is no more than 15.3%. Similar conclusions can also be obtained in studying the temperature distribution along different flame heights. Moreover,the soot volume fraction can be predicted more accurately with the application of the WSGSA model. Both without considering radiation and using the default radiation model in the Fluent software will result in the underestimating of soot volume fraction. All the results reveal that the WSGSA model can be used to predict the temperature and soot aggregates in the CH/air turbulent diffusion flame. 展开更多
关键词 radiative heat transfer WSGSA model soot radiation turbulent diffusion flame soot aggregate
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基于散射光强度的碳黑团聚体分形结构和粒径分布同时反演
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作者 张俊友 齐宏 +2 位作者 王一飞 任亚涛 阮立明 《北京航空航天大学学报》 EI CAS CSCD 北大核心 2020年第5期925-932,共8页
利用散射光信号实现碳黑团聚体分形结构和粒径分布参数的同时反演,在火焰辐射换热模拟和污染物测定方面有着重要应用价值。反演的正问题基于瑞利-德拜-甘斯多分散分形团聚体(RDG-PFA)散射理论,研究了2种信号方案,包括多角度散射及多角... 利用散射光信号实现碳黑团聚体分形结构和粒径分布参数的同时反演,在火焰辐射换热模拟和污染物测定方面有着重要应用价值。反演的正问题基于瑞利-德拜-甘斯多分散分形团聚体(RDG-PFA)散射理论,研究了2种信号方案,包括多角度散射及多角度散射-准直透射率。反演前,对比2种信号方案的残余适应度值分布发现,散射与透射信号同时使用有效减弱了反问题的病态性。反演过程基于协方差矩阵自适应的演化策略(CMA-ES)算法,该算法具有很强的局部搜索能力,为快速且稳定地反演各个目标参数提供了保障。反演结果表明了CMA-ES算法较大搜索空间内的可行性和普适性,同时也证明了采用多角度散射-准直透射率的组合信号有效提高了目标参数的反演精度。 展开更多
关键词 光散射 碳黑 团聚体 分形维度 反问题 优化算法
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Scattering and propagation of terahertz pulses in random soot aggregate systems 被引量:1
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作者 李海英 吴振森 +1 位作者 白璐 李正军 《Chinese Physics B》 SCIE EI CAS CSCD 2014年第5期277-282,共6页
Scattering and propagation of terahertz pulses in random soot aggregate systems are studied by using the generalized multi-particle Mie-solution (GMM) and the pulse propagation theory. Soot aggregates are obtained b... Scattering and propagation of terahertz pulses in random soot aggregate systems are studied by using the generalized multi-particle Mie-solution (GMM) and the pulse propagation theory. Soot aggregates are obtained by the diffusion-limited aggregation (DLA) model. For a soot aggregate in soot aggregate systems, scattering characteristics are analyzed by using the GMM. Scattering intensities versus scattering angles are given. The effects of different positions of the aggregate on the scattering intensities, scattering cross sections, extinction cross sections, and absorption cross sections are computed and compared. Based on pulse propagation in random media, the transmission of terahertz pulses in random soot aggregate systems is determined by the two-frequency mutual coherence function. Numerical simulations and analysis are given for terahertz pulses (0.7956 THz). 展开更多
关键词 soot aggregate systems terahertz pulse scattering and propagation
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