This paper presents a 2.5D scattering of incident plane SV waves by a canyon in a layered half-space by using the indirect boundary element method (IBEM). A free field response analysis is performed to provide the d...This paper presents a 2.5D scattering of incident plane SV waves by a canyon in a layered half-space by using the indirect boundary element method (IBEM). A free field response analysis is performed to provide the displacements and stresses on the boundary of the canyon where fictitious uniform moving loads are applied to calculate the Green's fi.mctions for the displacements and stresses. The amplitudes of the loads are determined by the boundary conditions. The free field displacements are added to the fictitious uniform moving loads induced displacements and the total response is obtained. Numerical calculations are performed for a canyon with homogenous and in one layer over bedrock. The effects of the thickness and stiffness of the layer on the amplification are studied and discussed.展开更多
A simple method for the controllable hydrothermal synthesis of nanocrystalline anatase TiO2(nc-TiO2) particles involving the selection of suitable organic alkali peptizing agents is reported.A dye-sensitized solar cel...A simple method for the controllable hydrothermal synthesis of nanocrystalline anatase TiO2(nc-TiO2) particles involving the selection of suitable organic alkali peptizing agents is reported.A dye-sensitized solar cell(DSSC) with square-like nc-TiO2 particles with side lengths about 8-13 nm-prepared using tetraethylammonium hydroxide(TEAOH)-in the photoelectrode showed higher photovoltaic performance than two other DSSCs with square-like nc-TiO2 particles with side lengths about 7-10 nm-prepared using tetrabutylammonium hydroxide-or elongated nc-TiO2 particles with lengths about 18-35 nm and width about 10 18 nm-prepared using tetramethylammonium hydroxide(TMAOH)-in the photoelectrodes.When a scattering layer prepared from sub-micron size spheres or cone-like nc-TiO2 particles-synthesized using a higher concentration of TMAOH-was added on top of the photoelectrode fabricated from nc-TiO2 synthesized with TEAOH,the energy conversion efficiency of the DSSC was markedly increased from 6.77% to 8.18%.展开更多
Although ultrablack surfaces are urgently needed in wide applications owing to their extremely low reflectance over a broadband wavelength,obtaining simultaneously the ultrablackness and mechanical robustness by simpl...Although ultrablack surfaces are urgently needed in wide applications owing to their extremely low reflectance over a broadband wavelength,obtaining simultaneously the ultrablackness and mechanical robustness by simple process technique is still a great challenge.Herein,by decoupling different light extinction effects to different layers of coating,we design an ultrablack coating that is all-sprayable in whole process.This coating presents low reflectance over visible–mid-infrared(VIS–MIR)wavelength(av.R≈1%in VIS),low multi-angle scattering(bidirectional reflection distribution function(BRDF)=10-2–10-3 sr-1),together with good substrate adhesion grade and self-cleaning ability,which are superior to most reported sprayable ultrablack surfaces.The light extinction effects of each layer are discussed.This method is also applicable in other material systems.展开更多
The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unav...The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unavoidable in online measurements, we present in this work a multiple scattering calculation method, in which a layer model is employed. The three-dimensional particle system is divided into a pile of layers the number of which is automatically determined, depending on the obscuration of the particle system. The calculation is found to be fast, reasonable and reliable.展开更多
Forward-/backward-facing steps in boundary-layer flows are often seen in engineering applications, and they have potential impacts on laminar-turbulent transition through scattering of the oncoming instability modes(e...Forward-/backward-facing steps in boundary-layer flows are often seen in engineering applications, and they have potential impacts on laminar-turbulent transition through scattering of the oncoming instability modes(e.g., Tollmien-Schlichting(T-S) waves). This issue is studied in the present paper by applying a local scattering framework, which is a rather generic mathematical framework on describing the mode scattering process. In this framework, a high-Reynolds-number triple-deck formalism is employed, and a transmission coefficient, defined as the ratio of the asymptotic amplitude of the instability mode downstream of the step to that upstream, is introduced. Through the systematical study, it has been found that both the forward-and backward-facing steps have a destabilizing effect on the oncoming T-S waves in subsonic boundary layers, this effect increases with the height of the step and/or the frequency of the T-S wave, and a backward-facing step(BFS) always has a greater impact than a forward-facing step(FFS). These facts agree with most of the previous investigations.However, one numerical study(WORNER, A., RIST, U., and WAGNER, S. Humps/steps influence on stability characteristics of two-dimensional laminar boundary layer. AIAA Journal, 41, 192–197(2003)), which was based on an ad-hoc configuration, showed an opposite impact of an FFS. Through the investigation on the specific configuration, it is revealed that the wrong conclusion was drawn by misinterpreting the numerical results.展开更多
文章通过Stober法合成粒径为300 nm的SiO_(2)纳米球,将该纳米球以乙醇为溶剂配置成一定浓度的悬浮液,通过旋涂法使其在染料敏化太阳能电池(dye-sensitized solar cells,DSSCs)的光阳极P25上形成一层薄膜,再将形成的P25-SiO_(2)复合膜放...文章通过Stober法合成粒径为300 nm的SiO_(2)纳米球,将该纳米球以乙醇为溶剂配置成一定浓度的悬浮液,通过旋涂法使其在染料敏化太阳能电池(dye-sensitized solar cells,DSSCs)的光阳极P25上形成一层薄膜,再将形成的P25-SiO_(2)复合膜放入TiO_(2)溶胶中浸泡一定时间,使得光阳极上的SiO_(2)纳米球被TiO_(2)纳米粒子包裹,形成SiO_(2)-TiO_(2)核壳结构薄膜。与没有散射层的DSSCs相比,以该核壳结构薄膜作为DSSCs的光散射层电池的光电转换效率提高了18%。展开更多
In this paper,a node-based smoothed finite element method(NS-FEM)with linear gradient fields(NS-FEM-L)is presented to solve elastic wave scattering by a rigid obstacle.By using Helmholtz decomposition,the problem is t...In this paper,a node-based smoothed finite element method(NS-FEM)with linear gradient fields(NS-FEM-L)is presented to solve elastic wave scattering by a rigid obstacle.By using Helmholtz decomposition,the problem is transformed into a boundary value problem with coupled boundary conditions.In numerical analysis,the perfectly matched layer(PML)and transparent boundary condition(TBC)are introduced to truncate the unbounded domain.Then,a linear gradient is constructed in a node-based smoothing domain(N-SD)by using a complete order of polynomial.The unknown coefficients of the smoothed linear gradient function can be solved by three linearly independent weight functions.Further,based on the weakened weak formulation,a system of linear equation with the smoothed gradient is established for NS-FEM-L with PML or TBC.Some numerical examples also demonstrate that the presented method possesses more stability and high accuracy.It turns out that the modified gradient makes the NS-FEM-L-PML and NS-FEM-L-TBC possess an ideal stiffness matrix,which effectively overcomes the instability of original NS-FEM.Moreover,the convergence rates of L 2 and H1 semi-norm errors for the two NS-FEM-L models are also higher.展开更多
Two sets of laser-damage experiments on large-aperture fused silica optics have been carried out in a high-power laser facility. Severe damage has been found on the grating which presented dense craters on the front s...Two sets of laser-damage experiments on large-aperture fused silica optics have been carried out in a high-power laser facility. Severe damage has been found on the grating which presented dense craters on the front surface. This phenomenon is quite different from other fused silica optics, which are damaged on the rear surface. The damage possibility due to the redeposition layer was ruled out by acid-etching the grating's front surface. The remarkable stimulated Brillouin scattering (SBS) effect was observed in grating and the reason for the front surface damage is thought to be the backward SBS.展开更多
Three-dimensional TiO2 microspheres doped with N were synthesized by a simple single-step solvothermal method and the sample treated for 15 h (hereafter called TMF) was then used as scattering layers in the photoano...Three-dimensional TiO2 microspheres doped with N were synthesized by a simple single-step solvothermal method and the sample treated for 15 h (hereafter called TMF) was then used as scattering layers in the photoanodes of dye-sensitized solar cells (DSSCs). The TMF was characterized using scanning electron micro- scopy, high resolution transmission electron microscopy, Brunauer-Emmett-Teller measurements, X-ray diffraction, and X-ray photoelectron spectroscopy. The TMF had a high surface area of 93.2 m2. g-~ which was beneficial for more dye-loading. Five photoanode films with different internal structures were fabricated by printing different numbers of TMF scattering layers on fluorine-doped tin oxide glass. UV-vis diffuse reflection spectra, incident photon-to-current efficiencies, photocurrent-voltage curves and electrochemical impedance spectroscopy were used to investigate the optical and electrochemical proper- ties of these photoanodes in DSSCs. The presence of nitrogen in the TMF changed the TMF microstructure, which led to a higher open circuit voltage and a longer electron lifetime. In addition, the presence of the nitrogen significantly improved the light utilization and photocur- rent. The highest photoelectric conversion efficiency achieved was 8.08%, which is much higher than that derived from typical P25 nanoparticles (6.52%).展开更多
This work was done in Summer of 1988, 1989 and 1992, at three different stations (34, 39 and 44 m under sea level), in the south Yellow Sea using narrow band acoustic pulses with center frequencies of 120, 160 and 200...This work was done in Summer of 1988, 1989 and 1992, at three different stations (34, 39 and 44 m under sea level), in the south Yellow Sea using narrow band acoustic pulses with center frequencies of 120, 160 and 200 kHz.The pulses were echoed back from three different depths. We used CTD to record the temperature and salinity of different depth day and night, and the plankton samples at different layers were hauled up for comparison. We applied the numerical method introduced by R. Kind to calculate reflected plane wave spectrum, measured temperature and salinity in vertical direction of non-uniform layer distribution and obtained the numerical simulation signals of backward scattering sound waves from thermocline layers. We then compared them with the experimental data. Through the experiments of the same periords of three years we have confimed that the measured time that layer-scattering-waves to reach our recorders agreed well with that obtained by temperature sectional simulated data. On the other hand, there is no apparent effects of plankton distribution. This indicates that acoustic scattering mainly depends on physical non-uniformity property of the media (sea water).展开更多
An analytical solution for scattering of incident plane SV waves by a circular-arc canyon with a covering layer was derived by Fourier-Bessel series expansion technique, and the solution was utilized to analyze the ef...An analytical solution for scattering of incident plane SV waves by a circular-arc canyon with a covering layer was derived by Fourier-Bessel series expansion technique, and the solution was utilized to analyze the effects of the covering layer on incident plane SV waves. It was shown that the covering layer in a canyon, even if it is very thin, amplifies incident plane SV waves tremendously, and the amplification can be two and half times more than that for a simple canyon; the stiffness and thickness of the covering layer also have great effects on incident plane SV waves.展开更多
Using linear water wave theory,three-dimensional problems concerning the interaction of waves with spherical structures in a fluid which contains a three-layer fluid consisting of a layer of finite depth bounded above...Using linear water wave theory,three-dimensional problems concerning the interaction of waves with spherical structures in a fluid which contains a three-layer fluid consisting of a layer of finite depth bounded above by freshwater of finite depth with free surface and below by an infinite layer of water of greater density are considered.In such a situation timeharmonic waves with a given frequency can propagate with three wavenumbers.The sphere is submerged in either of the three layers.Each problem is reduced to an infinite system of linear equations by employing the method of multipoles and the system of equations is solved numerically by standard technique.The hydrodynamic forces(vertical and horizontal forces)are obtained and depicted graphically against the wavenumber.When the density ratio of the upper and middle layer is made to approximately one,curves for vertical and horizontal forces almost coincide with the corresponding curves for the case of a two-layer fluid with a free surface.This means that in the limit,the density ratio of the upper and middle layer goes to approximately one,the solution agrees with the solution for the case of a two-layer fluid with a free surface.展开更多
The indirect boundary element method (IBEM) is used to study the surface motion of an alluvial valley in layered half-space for incident plane P-waves based on Wolf’s theory. Firstly, the free field response can be s...The indirect boundary element method (IBEM) is used to study the surface motion of an alluvial valley in layered half-space for incident plane P-waves based on Wolf’s theory. Firstly, the free field response can be solved by the direct stiffness method, and the scattering wave response is calculated by Green’s functions of distributed loads acting on inclined lines in a layered half-space. The method is verified by comparing its results with literature and numerical analyses are performed by taking the amplification of incident plane P-waves by an alluvial valley in one soil layer resting on bedrock as an example. The results show that there exist distinct differences between the wave amplification by an alluvial valley embedded in layered half-space and that in homogeneous half-space and there is interaction between the valley and the soil layer. The amplitudes are relatively large when incident frequencies are close to the soil layer’s resonant frequencies.展开更多
基金National Natural Science Foundation of China Under Grant No.50908156 and 50978183Tianjin Natural Science Foundation Under Grant No. 07JCZDJC10100
文摘This paper presents a 2.5D scattering of incident plane SV waves by a canyon in a layered half-space by using the indirect boundary element method (IBEM). A free field response analysis is performed to provide the displacements and stresses on the boundary of the canyon where fictitious uniform moving loads are applied to calculate the Green's fi.mctions for the displacements and stresses. The amplitudes of the loads are determined by the boundary conditions. The free field displacements are added to the fictitious uniform moving loads induced displacements and the total response is obtained. Numerical calculations are performed for a canyon with homogenous and in one layer over bedrock. The effects of the thickness and stiffness of the layer on the amplification are studied and discussed.
基金supported by the National Key Basic Research Program of China(973)(2006CB202605)High-Tech Research and Development Program of China(983)(2007AA05Z439)National Natural Science Foundation of China(20973183)~~
基金supported by the National High Technology Research and Development of China (863 Program,2009AA03Z217)the National Natural Science Foundation of China (90922028,51002053)+1 种基金the Natural Science Foundation of Fujian Province (2010J05115)the Fundamental Research Funds for the Central Universities (JB-SJ1001)
文摘A simple method for the controllable hydrothermal synthesis of nanocrystalline anatase TiO2(nc-TiO2) particles involving the selection of suitable organic alkali peptizing agents is reported.A dye-sensitized solar cell(DSSC) with square-like nc-TiO2 particles with side lengths about 8-13 nm-prepared using tetraethylammonium hydroxide(TEAOH)-in the photoelectrode showed higher photovoltaic performance than two other DSSCs with square-like nc-TiO2 particles with side lengths about 7-10 nm-prepared using tetrabutylammonium hydroxide-or elongated nc-TiO2 particles with lengths about 18-35 nm and width about 10 18 nm-prepared using tetramethylammonium hydroxide(TMAOH)-in the photoelectrodes.When a scattering layer prepared from sub-micron size spheres or cone-like nc-TiO2 particles-synthesized using a higher concentration of TMAOH-was added on top of the photoelectrode fabricated from nc-TiO2 synthesized with TEAOH,the energy conversion efficiency of the DSSC was markedly increased from 6.77% to 8.18%.
基金supported by the National Natural Science Foundation of China(Nos.11832010,11890682 and 21721002)the National Key Basic Research Program of China(No.2018YFA0208403)the Austrian-Chinese Cooperative Research and Development Projects(No.GJHZ2043),Chinese Academy of Sciences.
文摘Although ultrablack surfaces are urgently needed in wide applications owing to their extremely low reflectance over a broadband wavelength,obtaining simultaneously the ultrablackness and mechanical robustness by simple process technique is still a great challenge.Herein,by decoupling different light extinction effects to different layers of coating,we design an ultrablack coating that is all-sprayable in whole process.This coating presents low reflectance over visible–mid-infrared(VIS–MIR)wavelength(av.R≈1%in VIS),low multi-angle scattering(bidirectional reflection distribution function(BRDF)=10-2–10-3 sr-1),together with good substrate adhesion grade and self-cleaning ability,which are superior to most reported sprayable ultrablack surfaces.The light extinction effects of each layer are discussed.This method is also applicable in other material systems.
基金support from the National Natural Science Foundation of China (No. 50876069)the Ministry of Education of the People’s Republic of China (No.208041)from the Shanghai Municipal Education Commis-sion (No. 07ZZ88)
文摘The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unavoidable in online measurements, we present in this work a multiple scattering calculation method, in which a layer model is employed. The three-dimensional particle system is divided into a pile of layers the number of which is automatically determined, depending on the obscuration of the particle system. The calculation is found to be fast, reasonable and reliable.
基金supported by the National Natural Science Foundation of China(Nos.11472189 and11772224)
文摘Forward-/backward-facing steps in boundary-layer flows are often seen in engineering applications, and they have potential impacts on laminar-turbulent transition through scattering of the oncoming instability modes(e.g., Tollmien-Schlichting(T-S) waves). This issue is studied in the present paper by applying a local scattering framework, which is a rather generic mathematical framework on describing the mode scattering process. In this framework, a high-Reynolds-number triple-deck formalism is employed, and a transmission coefficient, defined as the ratio of the asymptotic amplitude of the instability mode downstream of the step to that upstream, is introduced. Through the systematical study, it has been found that both the forward-and backward-facing steps have a destabilizing effect on the oncoming T-S waves in subsonic boundary layers, this effect increases with the height of the step and/or the frequency of the T-S wave, and a backward-facing step(BFS) always has a greater impact than a forward-facing step(FFS). These facts agree with most of the previous investigations.However, one numerical study(WORNER, A., RIST, U., and WAGNER, S. Humps/steps influence on stability characteristics of two-dimensional laminar boundary layer. AIAA Journal, 41, 192–197(2003)), which was based on an ad-hoc configuration, showed an opposite impact of an FFS. Through the investigation on the specific configuration, it is revealed that the wrong conclusion was drawn by misinterpreting the numerical results.
文摘文章通过Stober法合成粒径为300 nm的SiO_(2)纳米球,将该纳米球以乙醇为溶剂配置成一定浓度的悬浮液,通过旋涂法使其在染料敏化太阳能电池(dye-sensitized solar cells,DSSCs)的光阳极P25上形成一层薄膜,再将形成的P25-SiO_(2)复合膜放入TiO_(2)溶胶中浸泡一定时间,使得光阳极上的SiO_(2)纳米球被TiO_(2)纳米粒子包裹,形成SiO_(2)-TiO_(2)核壳结构薄膜。与没有散射层的DSSCs相比,以该核壳结构薄膜作为DSSCs的光散射层电池的光电转换效率提高了18%。
基金supported by the National Natural Science Foundation of China(Grant Nos.11901423,12002290 and 11771321)the Youth Science and the Technology Research Foundation of Shanxi Province(Grant Nos.201901D211104 and 201901D211107)the Shanxi Youth Top-Notch Talent Support Program(Grant No.DT18100306).
文摘In this paper,a node-based smoothed finite element method(NS-FEM)with linear gradient fields(NS-FEM-L)is presented to solve elastic wave scattering by a rigid obstacle.By using Helmholtz decomposition,the problem is transformed into a boundary value problem with coupled boundary conditions.In numerical analysis,the perfectly matched layer(PML)and transparent boundary condition(TBC)are introduced to truncate the unbounded domain.Then,a linear gradient is constructed in a node-based smoothing domain(N-SD)by using a complete order of polynomial.The unknown coefficients of the smoothed linear gradient function can be solved by three linearly independent weight functions.Further,based on the weakened weak formulation,a system of linear equation with the smoothed gradient is established for NS-FEM-L with PML or TBC.Some numerical examples also demonstrate that the presented method possesses more stability and high accuracy.It turns out that the modified gradient makes the NS-FEM-L-PML and NS-FEM-L-TBC possess an ideal stiffness matrix,which effectively overcomes the instability of original NS-FEM.Moreover,the convergence rates of L 2 and H1 semi-norm errors for the two NS-FEM-L models are also higher.
文摘Two sets of laser-damage experiments on large-aperture fused silica optics have been carried out in a high-power laser facility. Severe damage has been found on the grating which presented dense craters on the front surface. This phenomenon is quite different from other fused silica optics, which are damaged on the rear surface. The damage possibility due to the redeposition layer was ruled out by acid-etching the grating's front surface. The remarkable stimulated Brillouin scattering (SBS) effect was observed in grating and the reason for the front surface damage is thought to be the backward SBS.
文摘Three-dimensional TiO2 microspheres doped with N were synthesized by a simple single-step solvothermal method and the sample treated for 15 h (hereafter called TMF) was then used as scattering layers in the photoanodes of dye-sensitized solar cells (DSSCs). The TMF was characterized using scanning electron micro- scopy, high resolution transmission electron microscopy, Brunauer-Emmett-Teller measurements, X-ray diffraction, and X-ray photoelectron spectroscopy. The TMF had a high surface area of 93.2 m2. g-~ which was beneficial for more dye-loading. Five photoanode films with different internal structures were fabricated by printing different numbers of TMF scattering layers on fluorine-doped tin oxide glass. UV-vis diffuse reflection spectra, incident photon-to-current efficiencies, photocurrent-voltage curves and electrochemical impedance spectroscopy were used to investigate the optical and electrochemical proper- ties of these photoanodes in DSSCs. The presence of nitrogen in the TMF changed the TMF microstructure, which led to a higher open circuit voltage and a longer electron lifetime. In addition, the presence of the nitrogen significantly improved the light utilization and photocur- rent. The highest photoelectric conversion efficiency achieved was 8.08%, which is much higher than that derived from typical P25 nanoparticles (6.52%).
文摘This work was done in Summer of 1988, 1989 and 1992, at three different stations (34, 39 and 44 m under sea level), in the south Yellow Sea using narrow band acoustic pulses with center frequencies of 120, 160 and 200 kHz.The pulses were echoed back from three different depths. We used CTD to record the temperature and salinity of different depth day and night, and the plankton samples at different layers were hauled up for comparison. We applied the numerical method introduced by R. Kind to calculate reflected plane wave spectrum, measured temperature and salinity in vertical direction of non-uniform layer distribution and obtained the numerical simulation signals of backward scattering sound waves from thermocline layers. We then compared them with the experimental data. Through the experiments of the same periords of three years we have confimed that the measured time that layer-scattering-waves to reach our recorders agreed well with that obtained by temperature sectional simulated data. On the other hand, there is no apparent effects of plankton distribution. This indicates that acoustic scattering mainly depends on physical non-uniformity property of the media (sea water).
基金State Natural Science Foundation of China (No.59878032).
文摘An analytical solution for scattering of incident plane SV waves by a circular-arc canyon with a covering layer was derived by Fourier-Bessel series expansion technique, and the solution was utilized to analyze the effects of the covering layer on incident plane SV waves. It was shown that the covering layer in a canyon, even if it is very thin, amplifies incident plane SV waves tremendously, and the amplification can be two and half times more than that for a simple canyon; the stiffness and thickness of the covering layer also have great effects on incident plane SV waves.
文摘Using linear water wave theory,three-dimensional problems concerning the interaction of waves with spherical structures in a fluid which contains a three-layer fluid consisting of a layer of finite depth bounded above by freshwater of finite depth with free surface and below by an infinite layer of water of greater density are considered.In such a situation timeharmonic waves with a given frequency can propagate with three wavenumbers.The sphere is submerged in either of the three layers.Each problem is reduced to an infinite system of linear equations by employing the method of multipoles and the system of equations is solved numerically by standard technique.The hydrodynamic forces(vertical and horizontal forces)are obtained and depicted graphically against the wavenumber.When the density ratio of the upper and middle layer is made to approximately one,curves for vertical and horizontal forces almost coincide with the corresponding curves for the case of a two-layer fluid with a free surface.This means that in the limit,the density ratio of the upper and middle layer goes to approximately one,the solution agrees with the solution for the case of a two-layer fluid with a free surface.
基金Supported by National Natural Science Foundation of China (No. 50978156 and No. 50908183)
文摘The indirect boundary element method (IBEM) is used to study the surface motion of an alluvial valley in layered half-space for incident plane P-waves based on Wolf’s theory. Firstly, the free field response can be solved by the direct stiffness method, and the scattering wave response is calculated by Green’s functions of distributed loads acting on inclined lines in a layered half-space. The method is verified by comparing its results with literature and numerical analyses are performed by taking the amplification of incident plane P-waves by an alluvial valley in one soil layer resting on bedrock as an example. The results show that there exist distinct differences between the wave amplification by an alluvial valley embedded in layered half-space and that in homogeneous half-space and there is interaction between the valley and the soil layer. The amplitudes are relatively large when incident frequencies are close to the soil layer’s resonant frequencies.