In January 2013, a long-lasting episode of severe haze occurred in central and eastern China, and it attracted attention from all sectors of society. The process and evolution of haze pollution episodes were observed ...In January 2013, a long-lasting episode of severe haze occurred in central and eastern China, and it attracted attention from all sectors of society. The process and evolution of haze pollution episodes were observed by the ＂Forming Mechanism and Con- trol Strategies of Haze in China＂ group using an intensive aerosol and trace gases campaign that simultaneously obtained data at 11 ground-based observing sites in the CARE-China network. The characteristics and formation mechanism of haze pollu- tion episodes were discussed. Five haze pollution episodes were identified in the Beijing-Tianjin-Hebei （Jing-Jin-Ji） area; the two most severe episodes occurred during 9-15 January and 25-31 January. During these two haze pollution episodes, the maximum hourly PMz5 mass concentrations in Beijing were 680 and 530 ~tg m-3, respectively. The process and evolution of haze pollution episodes in other major cities in the Jing-Jin-Ji area, such as Shijiazhuang and Tianjin were almost the same as those observed in Beijing. The external cause of the severe haze episodes was the unusual atmospheric circulation, the depres- sion of strong cold air activities and the very unfavorable dispersion due to geographical and meteorological conditions. How- ever, the internal cause was the quick secondary transformation of primary gaseous pollutants to secondary aerosols, which contributed to the ＂explosive growth＂ and ＂sustained growth＂ of PM2.5. Particularly, the abnormally high amount of nitric ox- ide （NOx） in the haze episodes, produced by fossil fuel combustion and vehicle emissions, played a direct or indirect role in the quick secondary transformation of coal-burning sulphur dioxide （SO2） to sulphate aerosols. Furthermore, gaseous pollutants were transformed into secondary aerosols through heterogeneous reactions on the surface of fine particles, which can change the particle＇s size and chemical composition. Consequently, the proportion of secondary inorganic ions, such as sulphate and nitrate, gradually incr展开更多
In January 2013,a severe fog and haze event(FHE)of strong intensity,long duration,and extensive coverage occurred in eastern China.The present study investigates meteorological conditions for this FHE by diagnosing bo...In January 2013,a severe fog and haze event(FHE)of strong intensity,long duration,and extensive coverage occurred in eastern China.The present study investigates meteorological conditions for this FHE by diagnosing both its atmospheric background fields and daily evolution in January 2013.The results show that a weak East Asian winter monsoon existed in January2013.Over eastern China,the anomalous southerly winds in the middle and lower troposphere are favorable for more water vapor transported to eastern China.An anomalous high at 500 hPa suppresses convection.The weakened surface winds are favorable for the fog and haze concentrating in eastern China.The reduction of the vertical shear of horizontal winds weakens the synoptic disturbances and vertical mixing of atmosphere.The anomalous inversion in near-surface increases the stability of surface air.All these meteorological background fields in January 2013 were conducive to the maintenance and development of fog and haze over eastern China.The diagnosis of the daily evolution of the FHE shows that the surface wind velocity and the vertical shear of horizontal winds in the middle and lower troposphere can exert dynamic effects on fog and haze.The larger(smaller)they are,the weaker(stronger)the fog and haze are.The thermodynamic effects include stratification instability in middle and lower troposphere and the inversion and dew-point deficit in near-surface.The larger(smaller)the stratification instability and the inversion are,the stronger(weaker)the fog and haze are.Meanwhile,the smaller(larger)the dewpoint deficit is,the stronger(weaker)the fog and haze are.Based on the meteorological factors,a multi-variate linear regression model is set up.The model results show that the dynamic and thermodynamic effects on the variance of the fog and haze evolution are almost the same.The contribution of the meteorological factors to the variance of the daily fog and haze evolution reaches 0.68,which explains more than 2/3 of the variance.展开更多
基金supported by the Chinese Academy of Sciences Strategic Priority Research Program(Grant Nos.XDB05020000 and XDA05100100)the National Natural Science Foundation of China(Grant Nos.41230642 and 41021004)
文摘In January 2013, a long-lasting episode of severe haze occurred in central and eastern China, and it attracted attention from all sectors of society. The process and evolution of haze pollution episodes were observed by the ＂Forming Mechanism and Con- trol Strategies of Haze in China＂ group using an intensive aerosol and trace gases campaign that simultaneously obtained data at 11 ground-based observing sites in the CARE-China network. The characteristics and formation mechanism of haze pollu- tion episodes were discussed. Five haze pollution episodes were identified in the Beijing-Tianjin-Hebei （Jing-Jin-Ji） area; the two most severe episodes occurred during 9-15 January and 25-31 January. During these two haze pollution episodes, the maximum hourly PMz5 mass concentrations in Beijing were 680 and 530 ~tg m-3, respectively. The process and evolution of haze pollution episodes in other major cities in the Jing-Jin-Ji area, such as Shijiazhuang and Tianjin were almost the same as those observed in Beijing. The external cause of the severe haze episodes was the unusual atmospheric circulation, the depres- sion of strong cold air activities and the very unfavorable dispersion due to geographical and meteorological conditions. How- ever, the internal cause was the quick secondary transformation of primary gaseous pollutants to secondary aerosols, which contributed to the ＂explosive growth＂ and ＂sustained growth＂ of PM2.5. Particularly, the abnormally high amount of nitric ox- ide （NOx） in the haze episodes, produced by fossil fuel combustion and vehicle emissions, played a direct or indirect role in the quick secondary transformation of coal-burning sulphur dioxide （SO2） to sulphate aerosols. Furthermore, gaseous pollutants were transformed into secondary aerosols through heterogeneous reactions on the surface of fine particles, which can change the particle＇s size and chemical composition. Consequently, the proportion of secondary inorganic ions, such as sulphate and nitrate, gradually incr
基金supported by the National Natural Science Foundation of China(Grant No.41221064)the International S&T Cooperation Project othe Ministry of Science and Technology of China(Grant No.2009-DFA21430)
文摘In January 2013,a severe fog and haze event(FHE)of strong intensity,long duration,and extensive coverage occurred in eastern China.The present study investigates meteorological conditions for this FHE by diagnosing both its atmospheric background fields and daily evolution in January 2013.The results show that a weak East Asian winter monsoon existed in January2013.Over eastern China,the anomalous southerly winds in the middle and lower troposphere are favorable for more water vapor transported to eastern China.An anomalous high at 500 hPa suppresses convection.The weakened surface winds are favorable for the fog and haze concentrating in eastern China.The reduction of the vertical shear of horizontal winds weakens the synoptic disturbances and vertical mixing of atmosphere.The anomalous inversion in near-surface increases the stability of surface air.All these meteorological background fields in January 2013 were conducive to the maintenance and development of fog and haze over eastern China.The diagnosis of the daily evolution of the FHE shows that the surface wind velocity and the vertical shear of horizontal winds in the middle and lower troposphere can exert dynamic effects on fog and haze.The larger(smaller)they are,the weaker(stronger)the fog and haze are.The thermodynamic effects include stratification instability in middle and lower troposphere and the inversion and dew-point deficit in near-surface.The larger(smaller)the stratification instability and the inversion are,the stronger(weaker)the fog and haze are.Meanwhile,the smaller(larger)the dewpoint deficit is,the stronger(weaker)the fog and haze are.Based on the meteorological factors,a multi-variate linear regression model is set up.The model results show that the dynamic and thermodynamic effects on the variance of the fog and haze evolution are almost the same.The contribution of the meteorological factors to the variance of the daily fog and haze evolution reaches 0.68,which explains more than 2/3 of the variance.
