Data collected using the micro rain radar(MRR) situated in Jinan city, eastern China, were used to explore the altitudinal and temporal evolution of rainfall microphysical characteristics, and to analyze the bright ba...Data collected using the micro rain radar(MRR) situated in Jinan city, eastern China, were used to explore the altitudinal and temporal evolution of rainfall microphysical characteristics, and to analyze the bright band(BB) characteristics and hydrometeor classification. Specifically, a low-intensity and stable stratiform precipitation event that occurred from 0000 to0550 UTC 15 February 2015 and featured a BB was studied. During this event, the rainfall intensity was less than 2 mm h-1 at a height of 300 m, which was above the radar site level, so the errors caused by the vertical air motion could be ignored.The freezing height from the radiosonde matched well with the top of the BB observed by the MRR. It was also found that the number of 0.5–1 mm diameter drops showed no noticeable variation below the BB. The maximum fall velocity and the maximum gradient fall velocity(GFV) of the raindrops appeared at the bottom of the BB. Meanwhile, a method that uses the GFV and reflectivity to identify the altitude and the thickness of the BB was established, with which the MRR can provide a reliable and real-time estimation of the 0?C isotherm. The droplet fall velocity was used to classify the types of snow crystals above the BB. In the first 20 min of the selected precipitation event, graupel prevailed above the BB; and at an altitude of2000 m, graupel also dominated in the first 250 min. After 150 min, the existence of graupel and dendritic crystals with water droplets above the BB was inferred.展开更多
Two factors that affect satellite retrieval of Aerosol Optical Depth(AOD) are aerosol model assumptions and the separation of surface reflectance.NASA/MODIS Dense Dark Vegetation(DDV) algorithm has been proven valuabl...Two factors that affect satellite retrieval of Aerosol Optical Depth(AOD) are aerosol model assumptions and the separation of surface reflectance.NASA/MODIS Dense Dark Vegetation(DDV) algorithm has been proven valuable in deriving aerosol distribution and properties over land;however,it cannot be applied to bright targets.As a supplement to the DDV algorithm,an algorithm to retrieve AOD over urban areas in North China in winter is developed using MODIS data,including(1) the generation and analysis of adjacent clear-days surface reflectance using MOD09 product from 2007 to 2008,and(2) seasonal aerosol models derived from AERONET data in Beijing and Xianghe sites.Ground-based measurements using sun photometers were used to validate the retrieved AOD,and the correlation coefficient(r) is up to 0.931.Especially for high AOD values(AOD>0.4),more retrievals meet the inversion accuracy.The temporal variations of retrieval errors over urban,rural and mountain regions were examined,and the results indicated that the variation of blue-band surface reflectance is less than 0.02 in a short period except for unusual weather conditions,the retrieval bias is under 0.08,and the relative error decreases as the AOD increases.展开更多
Deep understanding of the inherent luminescence mechanism is essential for the development of aggregation-induced emission(AIE)materials and applications.We first note that the intermolecular excitonic coupling is muc...Deep understanding of the inherent luminescence mechanism is essential for the development of aggregation-induced emission(AIE)materials and applications.We first note that the intermolecular excitonic coupling is much weaker in strength than the intramolecular electron-vibration coupling for a majority of newly termed AIEgens,which leads to the emission peak position insensitive to excitonic coupling,hence the conventional excitonic model for J-aggregation cannot effectively explain their AIE phenomena.Then,using multiscale computational approach coupled with our self-developed thermal vibration correlation function rate formalism and transition-state theory,we quantitatively investigate the aggregation effect on both the radiative and the nonradiative decays of molecular excited states.For radiative decay processes,we propose that the lowest excited state could convert from a transition dipole-forbidden“dark”state to a dipole-allowed“bright”state upon aggregation.For the radiationless processes,we demonstrate the blockage of nonradiative decay via vibration relaxation(BNR-VR)in harmonic region or the removal of nonradiative decay via isomerization(RNR-ISO)or minimum energy crossing point(RNR-MECP)beyond harmonic region in a variety of AIE aggregates.Our theoretical work not only justifies a plethora of experimental results but also makes reliable predictions on molecular design and mechanism that can be experimentally verified.Looking forward,we believe this review will benefit the deep understanding about the universality of AIE phenomenon and further extending the scope of AIE systems with novel applications.展开更多
Data from a long term measurement of Micro Rain Radar （MRR） at a mountain site （Daegwallyeong, DG, one year period of 2005） and a coastal site （Haenam, HN, three years 2004-2006） in South Korea were analyzed to ...Data from a long term measurement of Micro Rain Radar （MRR） at a mountain site （Daegwallyeong, DG, one year period of 2005） and a coastal site （Haenam, HN, three years 2004-2006） in South Korea were analyzed to compare the MRR measured bright band characteristics of stratiform precipitation at the two sites. On average, the bright band was somewhat thicker and the sharpness （average gradient of reflectivity above and below the reflectivity peak） was slightly weaker at DG, compared to those values at HN. The peak reflectivity itself was twice as strong and the relative location of the peak reflectivity within the bright band was higher at HN than at DG. Importantly, the variability of these values was much larger at HN than at DG. The key parameter to cause these differences is suggested to be the difference of the snow particle densities at the two sites, which is related to the degree of riming. Therefore, it is speculated that the cloud microphysical processes at HN may have varied significantly from un-rimed snow growth, producing low density snow particles, to the riming of higher density particles, while snow particle growth at DG was more consistently affected by the riming process, and therefore high density snow particles. Forced uplifting of cloudy air over the mountain area around DG might have resulted in an orographic supercooling effect that led to the enhanced riming of supercooled cloud drops.展开更多
Dear Editor,CRISPR-Cas9 （clustered regularly interspaced short palin- dromic repeats-CRISPR associated） systems have been harnessed for kinds of genome manipulation, including gene editing, transcription regulation,...Dear Editor,CRISPR-Cas9 （clustered regularly interspaced short palin- dromic repeats-CRISPR associated） systems have been harnessed for kinds of genome manipulation, including gene editing, transcription regulation, and chromosome loci imaging （Dominguez et al., 2016; Komor et al., 2017）. A typical engineered CRISPR-Cas9 system is composed of a Cas9 protein and a single guide RNA （sgRNA）, which could form a protein/RNA complex to recognize and cleave DNA sequence （Hsu et al., 2014; Wright et al., 2016）.展开更多
We investigate theoretically waveguides induced by screening-photovoltaic solitons in biased photorefractive-photovoltaic crystals. We show that the number of guided modes in a waveguide induced by a bright screening ...We investigate theoretically waveguides induced by screening-photovoltaic solitons in biased photorefractive-photovoltaic crystals. We show that the number of guided modes in a waveguide induced by a bright screening photovoltaic soliton increases monotonically with the increasing intensity ratio of the soliton, which is the ratio between the peak intensity of the soliton and the dark irradiance. On the other hand, waveguides induced by dark screening-photovoltaic solitons are always single mode for all intensity ratios and the confined energy near the centre of a dark screening-photovoltaic soliton increases monotonically with the increasing intensity ratio. When the bulk photovoltaic effect is neglectable, these waveguides are those induced by screening solitons. When the external field is absent, these waveguides predict those induced by photovoltaic solitons.展开更多
The relationship of hydrogen, GBF （granular bright facet） and very high cycle fatigue properties of high strength spring steels 60Si2CrV with three different hydrogen contents were studied using hydrogen thermal des...The relationship of hydrogen, GBF （granular bright facet） and very high cycle fatigue properties of high strength spring steels 60Si2CrV with three different hydrogen contents were studied using hydrogen thermal desorp- tion analysis and ultrasonic fatigue test. The results showed that the influence of hydrogen on the relationship between fatigue life and the ratio of GBF to inclusion size was obvious, and the expression between fatigue life and with different hydrogen contents can also be obtained. In addition, based on the research of hydrogen diffusion and GBF, it was explained why the GBF cannot form below 106 cycles. At last, the estimated critical fa tigue life of GBF formation can be expressed accurately.展开更多
A new mechanical electrodeposition technology was proposed, and nanocrystalline nickel deposit with bright and smooth surface was prepared in the bath without any additive agents. Unlike traditional methods, the novel...A new mechanical electrodeposition technology was proposed, and nanocrystalline nickel deposit with bright and smooth surface was prepared in the bath without any additive agents. Unlike traditional methods, the novel technology employed dynamical hard particles to continuously polish the cathode surface and disturb the nearby solution during electrodepositing. Experimental results showed that the polishing effect of hard particles can effectively prevent the hydrogen bubbles and impurities from adhering on the deposit surface and avoid the production of pits, pinholes and nodules. Furthermore, comparing with the deposit prepared by traditional methods, the one prepared by the novel technology was substantially refined with grain size ranging from 30 to 80 nm. Every diffraction peak's intensity of the deposit was reduced, the preferential orientation degree of (200) decreased and those of (111) and (220) increased. The microhardness notably increased. The magnetic properties were also changed with decreased saturation magnetization and increased coercive force. It was also found that variation of current density and cathode rotational speed could affect the structure and properties of the nickel deposits prepared by this technology.展开更多
The electrodeposition behaviors of nickel on glassy carbon（GC） and carbon steel（CS） electrodes were investigated in the14.3%-85.7%（mole fraction） betaine.HCl ethylene glycol（EG） ionic liquid using cyclic volta...The electrodeposition behaviors of nickel on glassy carbon（GC） and carbon steel（CS） electrodes were investigated in the14.3%-85.7%（mole fraction） betaine.HCl ethylene glycol（EG） ionic liquid using cyclic voltammetry and chronoamperometry.The results indicated that the reduction of Ni（Ⅱ） on CS electrode via a diffusion-controlled quasi-reversible process was much more facile and easier than that occurred on GC electrode,which followed a diffusion-controlled three-dimensional instantaneous nucleation and growth.Scanning electron microscopy was used to observe that the deposit was dense and contained fine crystallites with average size of（80±4） nm.Energy dispersive spectrometer analysis showed that the obtained deposit was metallic nickel.X-ray diffraction spectroscopy indicated that（111） plane was the most preferred crystal orientation.The nickel deposit was luminous and bright,and had good adhesion with the CS substrate.展开更多
Blue emitting electroluminescent diode using PVCz doped with perylene and BBOT as electron transport has been constructed.The emission spectrum is a mixture of spectra of BBOT and perylene.A luminance of as high as 68...Blue emitting electroluminescent diode using PVCz doped with perylene and BBOT as electron transport has been constructed.The emission spectrum is a mixture of spectra of BBOT and perylene.A luminance of as high as 680cd/m^(2)with lumen efficiency more then 0.0281m/W have been obtained.展开更多
From the observed vector magnetic fields by the Solar Optical Telescope/ Spectro-Polarimeter aboard the satellite Hinode, we have examined whether or not the quiet Sun magnetic fields are non-potential, and how the G-...From the observed vector magnetic fields by the Solar Optical Telescope/ Spectro-Polarimeter aboard the satellite Hinode, we have examined whether or not the quiet Sun magnetic fields are non-potential, and how the G-band filigrees and Ca II network bright points （NBPs） are associated with the magnetic non-potentiality. A sizable quiet region in the disk center is selected for this study. The new findings by the study are as follows. （1） The magnetic fields of the quiet region are obviously non-potential. The region-average shear angle is 40°, the average vertical current is 0.016A m^-2, and the average free magnetic energy density, 2.7× 10^2erg cm^-3. The magnitude of these non-potential quantities is comparable to that in solar active regions. （2） There are overall correlations among current helicity, free magnetic energy and longitudinal fields. The magnetic non-potentiality is mostly concentrated in the close vicinity of network elements which have stronger longitudinal fields. （3） The filigrees and NBPs are magnetically characterized by strong longitudinal fields, large electric helicity, and high free energy density. Because the selected region is away from any enhanced network, these new results can generally be applied to the quiet Sun. The findings imply that stronger network elements play a role in high magnetic non-potentiality in heating the solar atmosphere and in conducting the solar wind.展开更多
This paper discusses the two-dimensional discrete monatomic Fermi- Pasta-Ulam lattice, by using the method of multiple-scale and the quasi-discreteness approach. By taking into account the interaction between the atom...This paper discusses the two-dimensional discrete monatomic Fermi- Pasta-Ulam lattice, by using the method of multiple-scale and the quasi-discreteness approach. By taking into account the interaction between the atoms in the lattice and their nearest neighbours, it obtains some classes of two-dimensional local models as follows： two-dimensional bright and dark discrete soliton trains, two-dimensional bright and dark line discrete breathers, and two-dimensional bright and dark discrete breather.展开更多
基金sponsored by the National Natural Science Foundation of China (Grant Nos. 41475028 and 41530427)
文摘Data collected using the micro rain radar(MRR) situated in Jinan city, eastern China, were used to explore the altitudinal and temporal evolution of rainfall microphysical characteristics, and to analyze the bright band(BB) characteristics and hydrometeor classification. Specifically, a low-intensity and stable stratiform precipitation event that occurred from 0000 to0550 UTC 15 February 2015 and featured a BB was studied. During this event, the rainfall intensity was less than 2 mm h-1 at a height of 300 m, which was above the radar site level, so the errors caused by the vertical air motion could be ignored.The freezing height from the radiosonde matched well with the top of the BB observed by the MRR. It was also found that the number of 0.5–1 mm diameter drops showed no noticeable variation below the BB. The maximum fall velocity and the maximum gradient fall velocity(GFV) of the raindrops appeared at the bottom of the BB. Meanwhile, a method that uses the GFV and reflectivity to identify the altitude and the thickness of the BB was established, with which the MRR can provide a reliable and real-time estimation of the 0?C isotherm. The droplet fall velocity was used to classify the types of snow crystals above the BB. In the first 20 min of the selected precipitation event, graupel prevailed above the BB; and at an altitude of2000 m, graupel also dominated in the first 250 min. After 150 min, the existence of graupel and dendritic crystals with water droplets above the BB was inferred.
基金supported by National Natural Science Foundation of Chinafor Young Scholar (Grant No. 41101400)National Natural Science Foundation of China for Key Program (Grant No. 41130528)Opening Foundation of State Key Laboratory of Remote Sensing Science ofChina (Grant No. OFSLRSS201103)
文摘Two factors that affect satellite retrieval of Aerosol Optical Depth(AOD) are aerosol model assumptions and the separation of surface reflectance.NASA/MODIS Dense Dark Vegetation(DDV) algorithm has been proven valuable in deriving aerosol distribution and properties over land;however,it cannot be applied to bright targets.As a supplement to the DDV algorithm,an algorithm to retrieve AOD over urban areas in North China in winter is developed using MODIS data,including(1) the generation and analysis of adjacent clear-days surface reflectance using MOD09 product from 2007 to 2008,and(2) seasonal aerosol models derived from AERONET data in Beijing and Xianghe sites.Ground-based measurements using sun photometers were used to validate the retrieved AOD,and the correlation coefficient(r) is up to 0.931.Especially for high AOD values(AOD>0.4),more retrievals meet the inversion accuracy.The temporal variations of retrieval errors over urban,rural and mountain regions were examined,and the results indicated that the variation of blue-band surface reflectance is less than 0.02 in a short period except for unusual weather conditions,the retrieval bias is under 0.08,and the relative error decreases as the AOD increases.
基金National Natural Science Foundation of China,Grant/Award Numbers:21788102,21973099,21973043Ministry of Science andTechnology of ChinaNationalKeyR&DPlan,Grant/Award Number:2017YFA0204501。
文摘Deep understanding of the inherent luminescence mechanism is essential for the development of aggregation-induced emission(AIE)materials and applications.We first note that the intermolecular excitonic coupling is much weaker in strength than the intramolecular electron-vibration coupling for a majority of newly termed AIEgens,which leads to the emission peak position insensitive to excitonic coupling,hence the conventional excitonic model for J-aggregation cannot effectively explain their AIE phenomena.Then,using multiscale computational approach coupled with our self-developed thermal vibration correlation function rate formalism and transition-state theory,we quantitatively investigate the aggregation effect on both the radiative and the nonradiative decays of molecular excited states.For radiative decay processes,we propose that the lowest excited state could convert from a transition dipole-forbidden“dark”state to a dipole-allowed“bright”state upon aggregation.For the radiationless processes,we demonstrate the blockage of nonradiative decay via vibration relaxation(BNR-VR)in harmonic region or the removal of nonradiative decay via isomerization(RNR-ISO)or minimum energy crossing point(RNR-MECP)beyond harmonic region in a variety of AIE aggregates.Our theoretical work not only justifies a plethora of experimental results but also makes reliable predictions on molecular design and mechanism that can be experimentally verified.Looking forward,we believe this review will benefit the deep understanding about the universality of AIE phenomenon and further extending the scope of AIE systems with novel applications.
基金funded by the Korean Meteorological Administration Research and Development Program under Grant CATER 2006-2307.
文摘Data from a long term measurement of Micro Rain Radar （MRR） at a mountain site （Daegwallyeong, DG, one year period of 2005） and a coastal site （Haenam, HN, three years 2004-2006） in South Korea were analyzed to compare the MRR measured bright band characteristics of stratiform precipitation at the two sites. On average, the bright band was somewhat thicker and the sharpness （average gradient of reflectivity above and below the reflectivity peak） was slightly weaker at DG, compared to those values at HN. The peak reflectivity itself was twice as strong and the relative location of the peak reflectivity within the bright band was higher at HN than at DG. Importantly, the variability of these values was much larger at HN than at DG. The key parameter to cause these differences is suggested to be the difference of the snow particle densities at the two sites, which is related to the degree of riming. Therefore, it is speculated that the cloud microphysical processes at HN may have varied significantly from un-rimed snow growth, producing low density snow particles, to the riming of higher density particles, while snow particle growth at DG was more consistently affected by the riming process, and therefore high density snow particles. Forced uplifting of cloudy air over the mountain area around DG might have resulted in an orographic supercooling effect that led to the enhanced riming of supercooled cloud drops.
文摘Dear Editor,CRISPR-Cas9 （clustered regularly interspaced short palin- dromic repeats-CRISPR associated） systems have been harnessed for kinds of genome manipulation, including gene editing, transcription regulation, and chromosome loci imaging （Dominguez et al., 2016; Komor et al., 2017）. A typical engineered CRISPR-Cas9 system is composed of a Cas9 protein and a single guide RNA （sgRNA）, which could form a protein/RNA complex to recognize and cleave DNA sequence （Hsu et al., 2014; Wright et al., 2016）.
基金Supported by the National Natural Science Foundation of China under Grant No 10474136.
文摘We investigate theoretically waveguides induced by screening-photovoltaic solitons in biased photorefractive-photovoltaic crystals. We show that the number of guided modes in a waveguide induced by a bright screening photovoltaic soliton increases monotonically with the increasing intensity ratio of the soliton, which is the ratio between the peak intensity of the soliton and the dark irradiance. On the other hand, waveguides induced by dark screening-photovoltaic solitons are always single mode for all intensity ratios and the confined energy near the centre of a dark screening-photovoltaic soliton increases monotonically with the increasing intensity ratio. When the bulk photovoltaic effect is neglectable, these waveguides are those induced by screening solitons. When the external field is absent, these waveguides predict those induced by photovoltaic solitons.
文摘The relationship of hydrogen, GBF （granular bright facet） and very high cycle fatigue properties of high strength spring steels 60Si2CrV with three different hydrogen contents were studied using hydrogen thermal desorp- tion analysis and ultrasonic fatigue test. The results showed that the influence of hydrogen on the relationship between fatigue life and the ratio of GBF to inclusion size was obvious, and the expression between fatigue life and with different hydrogen contents can also be obtained. In addition, based on the research of hydrogen diffusion and GBF, it was explained why the GBF cannot form below 106 cycles. At last, the estimated critical fa tigue life of GBF formation can be expressed accurately.
基金the Natural Science Foundation of Jiangsu Province, China (Grant No. BK2004005)
文摘A new mechanical electrodeposition technology was proposed, and nanocrystalline nickel deposit with bright and smooth surface was prepared in the bath without any additive agents. Unlike traditional methods, the novel technology employed dynamical hard particles to continuously polish the cathode surface and disturb the nearby solution during electrodepositing. Experimental results showed that the polishing effect of hard particles can effectively prevent the hydrogen bubbles and impurities from adhering on the deposit surface and avoid the production of pits, pinholes and nodules. Furthermore, comparing with the deposit prepared by traditional methods, the one prepared by the novel technology was substantially refined with grain size ranging from 30 to 80 nm. Every diffraction peak's intensity of the deposit was reduced, the preferential orientation degree of (200) decreased and those of (111) and (220) increased. The microhardness notably increased. The magnetic properties were also changed with decreased saturation magnetization and increased coercive force. It was also found that variation of current density and cathode rotational speed could affect the structure and properties of the nickel deposits prepared by this technology.
基金Projects(51274108,21263007,51204080)supported by the National Natural Science Foundation of ChinaProject(2011FA009)supported by the Applied Research Foundation of Yunnan Province,ChinaProject(14118441)supported by the Talents Cultivation Foundation of Kunming University of Science and Technology,China
文摘The electrodeposition behaviors of nickel on glassy carbon（GC） and carbon steel（CS） electrodes were investigated in the14.3%-85.7%（mole fraction） betaine.HCl ethylene glycol（EG） ionic liquid using cyclic voltammetry and chronoamperometry.The results indicated that the reduction of Ni（Ⅱ） on CS electrode via a diffusion-controlled quasi-reversible process was much more facile and easier than that occurred on GC electrode,which followed a diffusion-controlled three-dimensional instantaneous nucleation and growth.Scanning electron microscopy was used to observe that the deposit was dense and contained fine crystallites with average size of（80±4） nm.Energy dispersive spectrometer analysis showed that the obtained deposit was metallic nickel.X-ray diffraction spectroscopy indicated that（111） plane was the most preferred crystal orientation.The nickel deposit was luminous and bright,and had good adhesion with the CS substrate.
基金Supported by the National Natural Science Foundation of China.
文摘Blue emitting electroluminescent diode using PVCz doped with perylene and BBOT as electron transport has been constructed.The emission spectrum is a mixture of spectra of BBOT and perylene.A luminance of as high as 680cd/m^(2)with lumen efficiency more then 0.0281m/W have been obtained.
基金supported by the National Natural Science Foundation of China (10873020, 10703007, G10573025, 40674081, 10603008, 10733020 and 40890161)the Chinese Academy of Sciences Project KJCX2-YW-T04the National Basic Research Program of China(G2006CB806303)
文摘From the observed vector magnetic fields by the Solar Optical Telescope/ Spectro-Polarimeter aboard the satellite Hinode, we have examined whether or not the quiet Sun magnetic fields are non-potential, and how the G-band filigrees and Ca II network bright points （NBPs） are associated with the magnetic non-potentiality. A sizable quiet region in the disk center is selected for this study. The new findings by the study are as follows. （1） The magnetic fields of the quiet region are obviously non-potential. The region-average shear angle is 40°, the average vertical current is 0.016A m^-2, and the average free magnetic energy density, 2.7× 10^2erg cm^-3. The magnitude of these non-potential quantities is comparable to that in solar active regions. （2） There are overall correlations among current helicity, free magnetic energy and longitudinal fields. The magnetic non-potentiality is mostly concentrated in the close vicinity of network elements which have stronger longitudinal fields. （3） The filigrees and NBPs are magnetically characterized by strong longitudinal fields, large electric helicity, and high free energy density. Because the selected region is away from any enhanced network, these new results can generally be applied to the quiet Sun. The findings imply that stronger network elements play a role in high magnetic non-potentiality in heating the solar atmosphere and in conducting the solar wind.
基金Project supported by the National Natural Science Foundation of China (Grant No 10574011)Natural Science Foundation of Heilongjiang Province,China (Grant No A200506)
文摘This paper discusses the two-dimensional discrete monatomic Fermi- Pasta-Ulam lattice, by using the method of multiple-scale and the quasi-discreteness approach. By taking into account the interaction between the atoms in the lattice and their nearest neighbours, it obtains some classes of two-dimensional local models as follows： two-dimensional bright and dark discrete soliton trains, two-dimensional bright and dark line discrete breathers, and two-dimensional bright and dark discrete breather.
