The traditional anomaly （TA） reference frame and its corresponding anomaly for a given data span changes with the extension of data length. In this study, the modulated annual cycle （MAC）, instead of the widely us...The traditional anomaly （TA） reference frame and its corresponding anomaly for a given data span changes with the extension of data length. In this study, the modulated annual cycle （MAC）, instead of the widely used climatological mean annual cycle, is used as an alternative reference frame for computing climate anomalies to study the multi-timescale variability of surface air temperature （SAT） in China based on homogenized daily data from 1952 to 2004. The Ensemble Empirical Mode Decomposition （EEMD） method is used to separate daily SAT into a high frequency component, a MAC component, an interannual component, and a decadal-to-trend component. The results show that the EEMD method can reflect historical events reasonably well, indicating its adaptive and temporally local characteristics. It is shown that MAC is a temporally local reference frame and will not be altered over a particular time span by an exten-sion of data length, thereby making it easier for physical interpretation. In the MAC reference frame, the low frequency component is found more suitable for studying the interannual to longer timescale variability （ILV） than a 13-month window running mean, which does not exclude the annual cycle. It is also better than other traditional versions （annual or summer or winter mean） of ILV, which contains a portion of the annual cycle. The analysis reveals that the variability of the annual cycle could be as large as the magnitude of interannual variability. The possible physical causes of different timescale variability of SAT in China are further discussed.展开更多
Knowledge of particle number size distribution（PND） and new particle formation（NPF）events in Southern China is essential for mitigation strategies related to submicron particles and their effects on regional air q...Knowledge of particle number size distribution（PND） and new particle formation（NPF）events in Southern China is essential for mitigation strategies related to submicron particles and their effects on regional air quality,haze,and human health.In this study,seven field measurement campaigns were conducted from December 2013 to May 2015 using a scanning mobility particle sizer（SMPS） at four sites in Southern China,including three urban sites and one background site.Particles were measured in the size range of15-515 nm,and the median particle number concentrations（PNCs） were found to vary in the range of 0.3× 10~4-2.2 × 10~4 cn^（-3） at the urban sites and were approximately 0.2 × 10~4 cm^（-3） at the background site.The peak diameters at the different sites varied largely from 22 to 102 nm.The PNCs in the Aitken mode（25-100 nm） at the urban sites were up to 10 times higher than they were at the background site,indicating large primary emissions from traffic at the urban sites.The diurnal variations of PNCs were significantly influenced by both rush hour traffic at the urban sites and NPF events.The frequencies of NPF events at the different sites were0%-30%,with the highest frequency occurring at an urban site during autumn.With higher SO_2 concentrations and higher ambient temperatures being necessary,NPF at the urban site was found to be more influenced by atmospheric oxidizing capability,while NPF at the background site was limited by the condensation sink.This study provides a unique dataset of particle number and size information in various environments in Southern China,which can help understand the sources,formation,and the climate forcing of aerosols in this quickly developing region,as well as help constrain and validate NPF modeling.展开更多
基金supported by Grant 2006CB400504 from the National Basic Research Program of ChinaGrant LCS-2006-03 fromthe Laboratory for Climate Studies, China MeteorologicalAdministration+1 种基金sponsored by the National Science Foundation of USA (ATM-0653136, ATM-0917743)sponsored by National Key Technologies R&D Pro-gram under Grant No. 2007BAC29B03
文摘The traditional anomaly （TA） reference frame and its corresponding anomaly for a given data span changes with the extension of data length. In this study, the modulated annual cycle （MAC）, instead of the widely used climatological mean annual cycle, is used as an alternative reference frame for computing climate anomalies to study the multi-timescale variability of surface air temperature （SAT） in China based on homogenized daily data from 1952 to 2004. The Ensemble Empirical Mode Decomposition （EEMD） method is used to separate daily SAT into a high frequency component, a MAC component, an interannual component, and a decadal-to-trend component. The results show that the EEMD method can reflect historical events reasonably well, indicating its adaptive and temporally local characteristics. It is shown that MAC is a temporally local reference frame and will not be altered over a particular time span by an exten-sion of data length, thereby making it easier for physical interpretation. In the MAC reference frame, the low frequency component is found more suitable for studying the interannual to longer timescale variability （ILV） than a 13-month window running mean, which does not exclude the annual cycle. It is also better than other traditional versions （annual or summer or winter mean） of ILV, which contains a portion of the annual cycle. The analysis reveals that the variability of the annual cycle could be as large as the magnitude of interannual variability. The possible physical causes of different timescale variability of SAT in China are further discussed.
基金supported by the National Natural Science Foundation of China(Nos.U1301234,21277003)the Shenzhen Science&Technology Plan,and the Ministry of Science and Technology of China(No.2013CB228503)
文摘Knowledge of particle number size distribution（PND） and new particle formation（NPF）events in Southern China is essential for mitigation strategies related to submicron particles and their effects on regional air quality,haze,and human health.In this study,seven field measurement campaigns were conducted from December 2013 to May 2015 using a scanning mobility particle sizer（SMPS） at four sites in Southern China,including three urban sites and one background site.Particles were measured in the size range of15-515 nm,and the median particle number concentrations（PNCs） were found to vary in the range of 0.3× 10~4-2.2 × 10~4 cn^（-3） at the urban sites and were approximately 0.2 × 10~4 cm^（-3） at the background site.The peak diameters at the different sites varied largely from 22 to 102 nm.The PNCs in the Aitken mode（25-100 nm） at the urban sites were up to 10 times higher than they were at the background site,indicating large primary emissions from traffic at the urban sites.The diurnal variations of PNCs were significantly influenced by both rush hour traffic at the urban sites and NPF events.The frequencies of NPF events at the different sites were0%-30%,with the highest frequency occurring at an urban site during autumn.With higher SO_2 concentrations and higher ambient temperatures being necessary,NPF at the urban site was found to be more influenced by atmospheric oxidizing capability,while NPF at the background site was limited by the condensation sink.This study provides a unique dataset of particle number and size information in various environments in Southern China,which can help understand the sources,formation,and the climate forcing of aerosols in this quickly developing region,as well as help constrain and validate NPF modeling.
