In this paper a projectile ion-recoil ion coincidence technique is used to investigate the transfer ionization processes in collisions of 0.22-6.30 MeV Cq+ ions and 0.25-6.35 MeV 0q+ ions (q=1, 2, 3, 4) with the H...In this paper a projectile ion-recoil ion coincidence technique is used to investigate the transfer ionization processes in collisions of 0.22-6.30 MeV Cq+ ions and 0.25-6.35 MeV 0q+ ions (q=1, 2, 3, 4) with the He atom separately. The cross section ratio f of transfer ionization to single electron transfer is measured, and the dependence of f on both charge state q and energy E of the projectiles is investigated. The electron-structure and the mechanisms leading to transfer ionization affect the dependence of f on q and E. Our measurements, along with other data published previously, suggest a similar dependence of f on charge state and energy of projectile for partially stripped ions over a large energy range. The maximum value of f is approximately 0.17q^0.60; the energy corresponding to maximum f is about 160q^0.60 keV/u.展开更多
The ratios of transfer ionization (TI) to single-electron capture (SC) cross sections have been measured for the collisions of partially stripped C^q+ ions (q = 1-4) with He. The collision velocity ranges from ...The ratios of transfer ionization (TI) to single-electron capture (SC) cross sections have been measured for the collisions of partially stripped C^q+ ions (q = 1-4) with He. The collision velocity ranges from 0.7 to 4.4 vo (vo is the Bohr velocity). The projectile-ion and recoil-ion coincidence technique is used to separate the processes of TI and SC. The ratios reach the maximum when the velocity is about 3.7 vo. This can be explained qualitatively based on the two-step mechanism. The experimental results are also compared with the results calculated using the classical trajectory Monte Carlo (CTMC) method. The CTMC results are in agreement with the experimental data basically. The discrepancies in higher velocity region are interpreted by the effective charge effect.展开更多
The dependence of the ratio R1 for transfer ionization to single capture for Cq+, Nq+, Oq+, Neq+ ions on Ne target upon the electronic structure of the projectile is studied. For Aq+-Ne collisions the ratio R1 decreas...The dependence of the ratio R1 for transfer ionization to single capture for Cq+, Nq+, Oq+, Neq+ ions on Ne target upon the electronic structure of the projectile is studied. For Aq+-Ne collisions the ratio R1 decreases as the atomic number Z of the projectile increases for q=4,5,6,7 sequences which provides strong evidence for the increase of the binding energy of the target valence electron after single electron capture. The increase in binding energy depends both upon the atomic number of the projectile and the target atom.展开更多
Multiple electron transfer processes are studied for Arq+ + Ne (q = 8, 9, 11, 12) collisions by using multi-parameter coincidence techniques. Various electron transfer processes are identified experimentally and the r...Multiple electron transfer processes are studied for Arq+ + Ne (q = 8, 9, 11, 12) collisions by using multi-parameter coincidence techniques. Various electron transfer processes are identified experimentally and the related cross-sections are measured. The dependence of transfer ionization cross-sections on the recoil charge states is compared with the results from the modified molecular classical overbarrier model. It is found that the modified model described the experimental results reasonably.展开更多
The ratios of the cross section of the transfer-ionization to the single-electron-capture of Argon induced by Cq+ (q=1,2,3) ions are measured by means of position sensitive and time-of-flight techniques. Our experimen...The ratios of the cross section of the transfer-ionization to the single-electron-capture of Argon induced by Cq+ (q=1,2,3) ions are measured by means of position sensitive and time-of-flight techniques. Our experimental results are compared with the data of Heq+ (q=1,2)-Ar of DuBois. A qualitative interpretation is presented based on the Classical-Over-Barrier Model of Bohr.展开更多
文摘In this paper a projectile ion-recoil ion coincidence technique is used to investigate the transfer ionization processes in collisions of 0.22-6.30 MeV Cq+ ions and 0.25-6.35 MeV 0q+ ions (q=1, 2, 3, 4) with the He atom separately. The cross section ratio f of transfer ionization to single electron transfer is measured, and the dependence of f on both charge state q and energy E of the projectiles is investigated. The electron-structure and the mechanisms leading to transfer ionization affect the dependence of f on q and E. Our measurements, along with other data published previously, suggest a similar dependence of f on charge state and energy of projectile for partially stripped ions over a large energy range. The maximum value of f is approximately 0.17q^0.60; the energy corresponding to maximum f is about 160q^0.60 keV/u.
文摘The ratios of transfer ionization (TI) to single-electron capture (SC) cross sections have been measured for the collisions of partially stripped C^q+ ions (q = 1-4) with He. The collision velocity ranges from 0.7 to 4.4 vo (vo is the Bohr velocity). The projectile-ion and recoil-ion coincidence technique is used to separate the processes of TI and SC. The ratios reach the maximum when the velocity is about 3.7 vo. This can be explained qualitatively based on the two-step mechanism. The experimental results are also compared with the results calculated using the classical trajectory Monte Carlo (CTMC) method. The CTMC results are in agreement with the experimental data basically. The discrepancies in higher velocity region are interpreted by the effective charge effect.
文摘The dependence of the ratio R1 for transfer ionization to single capture for Cq+, Nq+, Oq+, Neq+ ions on Ne target upon the electronic structure of the projectile is studied. For Aq+-Ne collisions the ratio R1 decreases as the atomic number Z of the projectile increases for q=4,5,6,7 sequences which provides strong evidence for the increase of the binding energy of the target valence electron after single electron capture. The increase in binding energy depends both upon the atomic number of the projectile and the target atom.
基金The authors would like to thank the ECR team for providing us with good beamThis work was supported by the National Natural Science Foundation of China (Grant No. 19704012)CAS-Bairen Plan.
文摘Multiple electron transfer processes are studied for Arq+ + Ne (q = 8, 9, 11, 12) collisions by using multi-parameter coincidence techniques. Various electron transfer processes are identified experimentally and the related cross-sections are measured. The dependence of transfer ionization cross-sections on the recoil charge states is compared with the results from the modified molecular classical overbarrier model. It is found that the modified model described the experimental results reasonably.
文摘The ratios of the cross section of the transfer-ionization to the single-electron-capture of Argon induced by Cq+ (q=1,2,3) ions are measured by means of position sensitive and time-of-flight techniques. Our experimental results are compared with the data of Heq+ (q=1,2)-Ar of DuBois. A qualitative interpretation is presented based on the Classical-Over-Barrier Model of Bohr.