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Review of Black Carbon in the Arctic—Origin, Measurement Methods, and Observations
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作者 Nicole Mö lders Stanley G. Edwin 《Open Journal of Air Pollution》 2018年第2期181-213,共33页
Current knowledge about black carbon (BC) emission estimates, state-of-the-art measurement methods, near-surface BC concentrations ([BC]), and mixing ratios in snow is consolidated for the Arctic. Since no direct meth... Current knowledge about black carbon (BC) emission estimates, state-of-the-art measurement methods, near-surface BC concentrations ([BC]), and mixing ratios in snow is consolidated for the Arctic. Since no direct method exists to measure [BC], results from modern indirect methods differ among devices. Pan-Arctic wide [BC] and changes are hard to access;monitoring often ends once national ambient air quality standards are met. Few remote sites have long records. Past measurements showed distinct differences among the various Arctic climate regions. Past and own observations in communities permit qualitative discussion of the diurnal course, response to weather, season, or different emission situations like weekdays and weekends at a given site and/or among sites. Comparison of data from collocated aethalometer indicated more similar accuracy than found in mid- and low-latitudes despite of much lower ambient temperatures and [BC]. Snow samples give an incomplete glimpse at the removal and input into ecosystems. 展开更多
关键词 BLACK CARBON Emissions in the ARCTIC ARCTIC BLACK CARBON OBSERVATIONS Measuring BLACK CARBON in the ARCTIC BLACK CARBON DEPOSITION in the ARCTIC
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On the Limits to Manage Air-Quality in Glacier Bay 被引量:2
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作者 Nicole Mölders Scott Gende 《Journal of Environmental Protection》 2016年第12期1923-1955,共34页
In Glacier Bay National Park, about 95% of the visitors come on board of cruise ships. The National Park Service has the mandate to manage park resources like air quality and visibility, while ensuring visitation. To ... In Glacier Bay National Park, about 95% of the visitors come on board of cruise ships. The National Park Service has the mandate to manage park resources like air quality and visibility, while ensuring visitation. To understand the impact of cruise-ship emissions on the overall concentrations in Glacier Bay, emission-source contribution ratios (ESCR) and the interaction of pollutant from local and/or distant sources were determined using results from four WRF/Chem simulations of the 2008 tourist season (May 15 to September 15). These simulations only differed by the emissions considered: Biogenic emissions only (CLN), biogenic plus activity-based cruise-ship emissions (REF), biogenic plus all anthropogenic emissions except cruise-ship emissions (RETRO), and all aforementioned emissions (ALL). In general, ESCRs differed among pollutants. Interaction between pollutants from cruise-ship emissions and species from other sources including those advected into the bay decreased towards the top of the atmospheric boundary layer. Pollutants from different sources interacted strongest (lowest) in the west arm of the fjord where ships berthed for glacier viewing (in areas of the bay without cruise-ship travel). Pollutant interaction both enhanced/reduced NO<sub>2</sub> concentrations by 10% (4 - 8 ppt absolute). Except for ozone, cruise-ship emissions on average governed air quality in the bay. On days with cruise-ship visits, they contributed between 60% and 80% of the bay-wide daily mean SO<sub>2</sub> and NO<sub>2</sub> concentrations below 1 km height. On days without visits, cruise-ship contributions still reached 40% due to previous visits. Highest cruise-ship ESCRs occurred during stagnant weather conditions. Despite the fact that all coarse particulate matter was due to anthropogenic sources, worst visibility conditions were due to meteorology. The results suggest limits as well as windows for managing air quality and visibility in Glacier Bay. 展开更多
关键词 Glacier Bay National Park Emission-Source Contribution Cruise-Ship Emissions Air-Quality Management Interaction of Pollutants
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Sustainability of Wind Energy under Changing Wind Regimes—A Case Study 被引量:2
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作者 Nicole Mölders Dinah Khordakova +1 位作者 Ralph Dlugi Gerhard Kramm 《Atmospheric and Climate Sciences》 2016年第2期158-173,共16页
A method was introduced to assess the sustainability of energy production over the lifetime (~20 y) of wind turbines. Community Earth System Model simulations were downscaled for the tourist seasons (mid-May to mid-Se... A method was introduced to assess the sustainability of energy production over the lifetime (~20 y) of wind turbines. Community Earth System Model simulations were downscaled for the tourist seasons (mid-May to mid-September) of 2006 to 2012 (CESM-P1) and 2026 to 2032 (CESM-P2) to obtain a reference and projected wind-speed climatology, respectively. The wind speeds served to calculate the potential power output and capacity factors of seven turbine types. CESM-P1 wind-speed climatology, power output, and capacity factors were compared to those derived from wind speeds obtained by numerical weather forecasts for reference to known standard to wind-farm managers. Juneau, Alaska served as a virtual testbed as this region is known to experience changes in wind speeds in response to the Pacific Decadal Oscillation. CESM-P2 suggested about 2% decrease for wind speeds between the speeds at cut-in and rated power, and about 8% - 10% decrease in potential wind-power output. This means that in regions of decadal climate variations, the sustainability of wind-energy production should be part of the decision-making process. The study demonstrated that using mean values of wind-speeds can provide qualitative knowledge about decreases/increases in potential energy production, but not about the magnitude. Using the total individual wind-speed data of all seasons provided the same amount of total power output than summing up the power outputs of individual seasons. The main advantage of calculating individual seasonal wind-power outputs, however, is that it theoretically permits assessment of interannual variability in power output and capacity factors. Comparison to a known standard may help stakeholders in understanding of uncertainty and interpretation of projected changes. 展开更多
关键词 Sustainability of Wind Energy Sensitivity of Wind Energy to Decadal Climate Variations CESM DOWNSCALING Interannual Variability
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June to October Aerosol Optical Depth over the Arctic at Various Spatial and Temporal Scales in MODIS, MAIAC, CALIOP and GOES Data
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作者 Nicole Mölders Mariel Friberg 《Open Journal of Air Pollution》 CAS 2023年第1期1-29,共29页
The accuracy of the cloud-aerosol lidar with orthogonal polarization (CALIOP), moderate resolution imaging spectroradiometer (MODIS), Multi-Angle Implementation of Atmospheric Correction (MAIAC), and Geostationary Ope... The accuracy of the cloud-aerosol lidar with orthogonal polarization (CALIOP), moderate resolution imaging spectroradiometer (MODIS), Multi-Angle Implementation of Atmospheric Correction (MAIAC), and Geostationary Operational Environmental Satellite (GOES) aerosol optical depth (AOD) products for the Arctic north of 59.75°N was examined by means of 35 aerosol robotic network (AERONET) AOD sites. The assessment for June to October 2006 to 2020 showed MAIAC AOD agreed the best with AERONET AOD;CALIOP AOD differed the strongest from the AERONET AOD. Cross-correlations of CALIOP AOD along the satellite path indicated that AOD-values 40 km up-and-down the path often failed to represent the AERONET AOD-values within ±30 min of the overpass in this region dominated by easterly winds. Typically, CALIOP AOD was lower than AERONET AOD and MAIAC AOD at the sites, especially, at sites with mean AOD below 0.1. Generally, MODIS AOD values exceeded those of MAIAC. Comparison of CALIOP, MAIAC, and MODIS products resampled on a 0.25° × 0.25° grid revealed differences among the products caused by their temporal and spatial resolution, sample habit and size. Typically, the MODIS AOD-product showed the most details in AOD distribution. Despite differences in AOD-values, all products provided similar temporal evolution of elevated and lower AOD. 展开更多
关键词 Inter-Comparison of MAIAC CALIOP MODIS C6.1 GOES AOD-Products Long-Term Evaluation of AOD-Products with AERONET Observations AOD Distribution over the Arctic Changes in Arctic AOD
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Inventory of the Thermo-Physiological Behavior of Fabrics—A Review
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作者 Nicole Mölders 《Journal of Textile Science and Technology》 2023年第2期127-150,共24页
A comprehensive literature review was performed to create an inventory of thermal-physiological quantities for fabrics from different fiber materials, material blends, and fabric structures. The goal was to derive ove... A comprehensive literature review was performed to create an inventory of thermal-physiological quantities for fabrics from different fiber materials, material blends, and fabric structures. The goal was to derive over-arching concepts that cannot be seen by the individual studies alone. Equations of best fits suggest non-linear changes for fabric thickness, thermal and water-vapor resistance with changes in material blend ratio. Air permeability decreases with increasing fabric density and fabric weight wherein the degree of decrease differs among fabric materials, blend ratio, and fabric structure. Water-vapor transmission rates strongly depend on fabric thickness, material, and blend, but marginally depend on fabric structure as long as the fabric and material thickness remain the same. 展开更多
关键词 Thermal Resistance of Fabrics Thermal Conductivity of Fabrics Water-Vapor Resistance of Fabrics Water-Vapor Transmission Rate Inventory of Thermal-Physiological Characteristics of Fabrics Energetics of Fabrics
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Changes in Aerosol Optical Depth over the Arctic Ocean as Seen by CALIOP, MAIAC, and MODIS C6.1
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作者 Nicole Mölders Mariel Friberg 《Journal of Environmental Protection》 2023年第6期419-440,共22页
Due to the recent increase in Arctic shipping, 2006-2020 June to October Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 (C6.1), and Mult... Due to the recent increase in Arctic shipping, 2006-2020 June to October Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 (C6.1), and Multi-Angle Implementation of Atmospheric Correction (MAIAC) retrieved aerosol optical depth (AOD) data were examined for changes in AOD from period 1 (P1, 2006-2012) to period 2 (P2, 2014-2020 (P2). Herein, AOD was statistically analyzed on a 0.25° × 0.25° grid and in the airsheds over the various ocean basins over the Arctic north of 59.75°N. According to heatmaps of the correlation between AOD and ship traffic, and AOD and fire emissions for the airsheds, all three AOD products captured the observed inter-annual variability in wildfire occurrence well, and showed wildfire emissions over Siberia were more severe in P2 than P1. Except for the Atlantic, North, and Baltic Seas, Beaufort Sea, and Barents Sea, all three AOD products indicated that AOD was higher over the various basins in P2 than P1, but disagreed on the magnitude. This fact suggests that the detection of changes in the typical low AOD over the Arctic Ocean might be rather qualitative than quantitative. While all products captured increases in AOD due to ships at berth, only MODIS C6.1 caught the elevated AOD due to shipping on the Siberian rivers. Obviously, sub-daily resolutions are required to capture increased AOD due to short-term events like a traveling ship or short-interval fire. 展开更多
关键词 Arctic Aerosol Optical Depth Changes in Aerosol Optical Depth Arctic Ship-Emissions Impacts on AOD Boreal Wildfire Impacts on AOD
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On the Maximum of Wind Power Efficiency
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作者 Gerhard Kramm Gary Sellhorst +3 位作者 Hannah K. Ross John Cooney Ralph Dlugi Nicole Mölders 《Journal of Power and Energy Engineering》 2016年第1期1-39,共39页
In our paper we demonstrate that the filtration equation used by Gorban’ et al. for determining the maximum efficiency of plane propellers of about 30 percent for free fluids plays no role in describing the flows in ... In our paper we demonstrate that the filtration equation used by Gorban’ et al. for determining the maximum efficiency of plane propellers of about 30 percent for free fluids plays no role in describing the flows in the atmospheric boundary layer (ABL) because the ABL is mainly governed by turbulent motions. We also demonstrate that the stream tube model customarily applied to derive the Rankine-Froude theorem must be corrected in the sense of Glauert to provide an appropriate value for the axial velocity at the rotor area. Including this correction leads to the Betz-Joukowsky limit, the maximum efficiency of 59.3 percent. Thus, Gorban’ et al.’s 30% value may be valid in water, but it has to be discarded for the atmosphere. We also show that Joukowsky’s constant circulation model leads to values of the maximum efficiency which are higher than the Betz-Jow-kowsky limit if the tip speed ratio is very low. Some of these values, however, have to be rejected for physical reasons. Based on Glauert’s optimum actuator disk, and the results of the blade-element analysis by Okulov and S&oslashrensen we also illustrate that the maximum efficiency of propeller-type wind turbines depends on tip-speed ratio and the number of blades. 展开更多
关键词 Wind Power Power Efficiency General Momentum Theory Axial Momentum Theory Blade Element Analysis Betz-Joukowsky Limit Joukowsky’s Constant Circulation Model Glauert’s Optimum Actuator Disk Balance Equation for Momentum Equation of Continuity Balance Equation for Kinetic Energy Reynolds’ Average Hesselberg’s Average Favre’s Average Bernoulli’s Equation Integral Equations
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Using MAN and Coastal AERONET Measurements to Assess the Suitability of MODIS C6.1 Aerosol Optical Depth for Monitoring Changes from Increased Arctic Shipping
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作者 Nicole Mölders Mariel Friberg 《Open Journal of Air Pollution》 2020年第4期77-104,共28页
Collocated data of the moderate resolution imaging spectroradiometer (MO<span style="font-family:Verdana;">-</span><span style="font-family:Verdana;">DIS) Collection 6.1 aerosol o... Collocated data of the moderate resolution imaging spectroradiometer (MO<span style="font-family:Verdana;">-</span><span style="font-family:Verdana;">DIS) Collection 6.1 aerosol optical depths (AOD) at 3 km × 3 km north of 59.9</span><span style="font-family:Verdana;">°</span><span style="font-family:Verdana;">N over ocean were assessed at 550 nm by aerosol robotic network (AERONET) data from coastal sites and marine aerosol network (MAN) data from vessels during June to October 2006 to 2018. Typically, MODIS AOD w</span><span style="font-family:Verdana;">as</span><span style="font-family:Verdana;"> higher at low and lower at high values than the AERONET AOD. Discrepancies were largest for sites where the Earth’s surface around the site is very heterogeneous (Canadian Archipelago, coast of Greenland). Due to the higher likelihood for sea-ice, MAN and MODIS AOD differed stronger west of Greenland and over the Beaufort Sea than at location in the Greenland and Norwegian Seas and Atlantic. MODIS AOD well captured the inter-seasonal variability found in the AERONET AOD data (R = 0.933). At all sites, MO</span><span style="font-family:Verdana;">-</span><span style="font-family:Verdana;">DIS and AERONET AOD agreement improved as time progressed in the shipping season, hinting at errors in sea-ice vs. open water classification. Overall 75.3% of the MODIS AOD data fell within the limits of the error envelops of the AERONET/MAN AOD data with MAN ranging between 87.5% and 100%. Changes in both MODIS and AERONET mean AOD between two periods of same length (2006-2011, 2013-2018) were explainable by changes in emissions for all sites</span><span style="font-family:Verdana;">.</span> 展开更多
关键词 Aerosol Optical Depth over the Arctic Ocean MODIS Evaluation by AERONET and MAN Data Changes in Arctic Aerosol Optical Depth over the Ocean North of 59.9°N Arctic Shipping Season Aerosol Optical Depths
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On the Solar Climate of the Moon and the Resulting Surface Temperature Distribution
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作者 Gerhard Kramm Nicole Mölders +1 位作者 Martina Berger Ralph Dlugi 《Natural Science》 CAS 2022年第9期386-420,共35页
The solar climate of our Moon is analyzed using the results of numerical simulations and the recently released data of the Diviner Lunar Radiometer Experiment (DLRE) to assess (a) the resulting distribution of the sur... The solar climate of our Moon is analyzed using the results of numerical simulations and the recently released data of the Diviner Lunar Radiometer Experiment (DLRE) to assess (a) the resulting distribution of the surface temperature, (b) the related global mean surface temperature T<sub>s</sub>>, and (c) the effective radiation temperature T<sub>e</sub> <sub></sub>often considered as a proxy for T<sub>s</sub>> of rocky planets and/or their natural satellites, where T<sub>e</sub> <sub></sub>is based on the global radiation budget of the well-known “thought model” of the Earth in the absence of its atmosphere. Because the Moon consists of similar rocky material like the Earth, it comes close to this thought model. However, the Moon’s astronomical features (e.g., obliquity, angular velocity of rotation, position relative to the disc of the solar system) differ from that of the Earth. Being tidally locked to the Earth, the Moon’s orbit around the Sun shows additional variation as compared to the Earth’s orbit. Since the astronomical parameters affect the solar climate, we predicted the Moon’s orbit coordinates both relative to the Sun and the Earth for a period of 20 lunations starting May 24, 2009, 00:00 UT1 with the planetary and lunar ephemeris DE430 of the Jet Propulsion Laboratory of the California Institute of Technology. The results revealed a mean heliocentric distance for the Moon and Earth of 1.00124279 AU and 1.00166376 AU, respectively. The mean geocentric distance of the Moon was 384792 km. The synodic and draconic months deviated from their respective means in a range of -5.7 h to 6.9 h and ±3.4 h, respectively. The deviations of the anomalistic months from their mean range between -2.83 d and 0.97 d with the largest negative deviations occurring around the points of inflection in the curve that represents the departure of the synodic month from its mean. Based on the two successive passages of the Sun through the ascending node of the lunar equator plane, the time interval between them co 展开更多
关键词 Solar Climate Temperature Inequality Hölder’s Inequility Global Radiation Budget Local Radiation Budget Global Energy Budget Local Energy Budget Global Albedo Global Averaging Effective Radiation Temperature Surface Temperature Slab Temperature Multilayer-Force-Restore Method
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Indoor and Outdoor Particulate Matter Exposure of Rural Interior Alaska Residents
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作者 Stanley G. Edwin Nicole Mölders 《Open Journal of Air Pollution》 2020年第3期37-60,共24页
To assess the exposure of residents in rural communities in the Yukon Flats to particulate matter of 2.5 μm or less in diameter (PM<sub><span style="font-family:Verdana;">2.5</span></su... To assess the exposure of residents in rural communities in the Yukon Flats to particulate matter of 2.5 μm or less in diameter (PM<sub><span style="font-family:Verdana;">2.5</span></sub><span style="font-family:Verdana;">), both indoor and outdoor concentration observations were carried out from March to September 2019 in Ft. Yukon, Alaska. Indoor concentrations were measured at 0.61 m (breathing level during sleeping) in homes and at 1.52 m heights (breathing level of standing adult) in homes and office/commercial buildings. Air quality was better at both heights in cabins than frame homes both during times with and without surface-based inversions. In frame houses, concentrations were higher at 0.61 m than 1.52 m, while the opposite is true typically for cabins. Differences between shoulder season and summer indoor concentrations in residences were related to changes in heating, subsistence lifestyle and mosquito repellents. In summer, office and commercial buildings, air quality decreased due to increased indoor emissions related to increased use of equipment and mosquito pics as well as more merchandise. During summer indoor concentrations reached unhealthy for sensitive groups to hazardous conditions for extended times that even exceeded the high outdoor concentrations. Due to nearby wildfires, July mean outdoor concentrations were 55.3 μg·m<sup>-</sup></span><sup><span style="font-family:Verdana;">3</span></sup><span style="font-family:Verdana;"> which exceeds the 24-h US National Ambient Air Quality Standard of 35 μg·m</span><span style="font-family:Verdana;"><sup>-3</sup></span><span style="font-family:Verdana;">. Indoor and outdoor concentrations correlated the strongest with each other for office/commercial buildings, followed by frame houses and cabins. Office/commercial buildings with temperature monitors had one to two orders of magnitude lower concentrations than those without.</span> 展开更多
关键词 Indoor Air Quality Yukon Flats Alaska Fine Particulate Matter PM2.5 Exposure in Rural Alaska Tribal Air Quality Study
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