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Mutiparametric Characterization of Atmospheric Particulate in a Heavy-Polluted Area of South Italy
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作者 Carmen De Marco Antonella Boselli +5 位作者 Andrea D’Anna Alessia Sannino gaetano sasso Mariano Sirignano Nicola Spinelli Xuan Wang 《Atmospheric and Climate Sciences》 2022年第2期493-516,共24页
To obtain a real-time image of atmospheric particulate matter (PM) in highly polluted areas and to understand how the anthropogenic component linked to urban activities (industrial activities, domestic heating, road t... To obtain a real-time image of atmospheric particulate matter (PM) in highly polluted areas and to understand how the anthropogenic component linked to urban activities (industrial activities, domestic heating, road traffic, waste disposal) can locally affect near-surface measurement of PM, several measurement campaigns were achieved in the Campania region (Southern Italy) using both Lidar and in-situ instruments. A comparison between the obtained results highlights a good correlation between the data and the potential of remote sensing instruments for air quality monitoring. Data analysis was performed in terms of particle backscattering coefficient profile at 355 nm, PM mass concentration, and size distribution. Wind profiles, which covered a range of altitudes from 40 m to 290 m, were also used to study sources and physical processes involved. Measurement carried out in a rural area with a landfill site highlighted the presence of a homogeneous particulate layer throughout the sounded area due to winds driving aerosol from the landfill to the surrounding areas. The size distribution in mass concentration, highlighted a modal diameter moving towards 0.9 and 2 μm with a larger mass concentration of particles in the morning, before noon and in the afternoon when a large number of trucks delivered solid wastes. Moreover, large concentrations of particulate matter were measured in a small urban town with few industrial activities which peak (211 ± 33 μg&#183;m<sup>-</sup><sup>3</sup>) was measured in the direction of the most urbanized area, probably due to the lighting of the domestic heating systems. Bimodal size distribution in number concentration was measured, indicative of two types of atmospheric particles sources: gas and liquid combustion (particles with sizes below 80 nm), including vehicular traffic and domestic gas-heating, and biomass combustion (particles with sizes of the order of 200 - 500 nm). Finally, data collected in a highly populated and industrialized area highlights the presence of partic 展开更多
关键词 PM Particle Size Distribution Optical Particles Properties Remote Sensing
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