A yellow continuous wave with beam quality M^2= 4.6 and output power of 4.8 W at 589nm is generated by intracavity sum-frequency mixing of 1064 nm and 1319 nm radiations of a Nd：YAG laser. To achieve high beam qualit...A yellow continuous wave with beam quality M^2= 4.6 and output power of 4.8 W at 589nm is generated by intracavity sum-frequency mixing of 1064 nm and 1319 nm radiations of a Nd：YAG laser. To achieve high beam quality at high power, thermally near-unstable flat-flat resonators with two-rod birefringence compensation are designed to obtain the large fundamental mode size inside the Nd：YAG rods and the same beam width inside the KTP crystal. The optimal intracavity power ratio of both 1064nm and 1319nm beams is also considered. The output power fluctuation of the yellow laser remains less than 5% in four hours.展开更多
The origin of ferromagnetism in epitaxial strained LaCoO_(3-x)films has long been controversial.Here,we investigated the magnetic behavior of a series of oxygen vacancy-ordered LaCoO_(3-x)films on different substrates...The origin of ferromagnetism in epitaxial strained LaCoO_(3-x)films has long been controversial.Here,we investigated the magnetic behavior of a series of oxygen vacancy-ordered LaCoO_(3-x)films on different substrates.Obvious ferromagnetism was observed in perovskite LaCoO_(3)/LSAT(LSAT=(LaAlO_(3))0.3(SrAlTaO_(6))_(0.7))and LaCoO_(3)/SrTiO_(3) films,while LaCoO_(3)/LaAlO_(3)films showed weak ferromagnetic behavior.Meanwhile,LaCoO_(2.67) films exhibited antiferromagnetic behavior.An unexpected low-temperature ferromagnetic phenomenon with a Curie temperature of~83 K and a saturation magnetization of~1.2μB/Co was discovered in 15 nm thick LaCoO_(2.5)/LSAT thin films,which is probably related to the change in the interface CoO_(6) octahedron rotation pattern.Meanwhile,the observed ferromagnetism gradually disappeared as the thickness of the film increased,indicating a relaxation of tensile strain.Analysis suggests that the rotation and rhombohedral distortion of the CoO_(6) octahedron weakened the crystal field splitting and promoted the generation of the ordered high-spin state of Co^(2+).Thus the super-exchange effect between Co^(2+)(high spin state),Co^(2+)(low spin state)and Co^(2+)(high spin state)produced a low-temperature ferromagnetic behavior.However,compressive-strained LaCoO_(2.5)film on a LaAlO_(3)substrate showed normal anti-ferromagnetic behavior.These results demonstrate that both oxygen vacancies and tensile strain are correlated with the emergent magnetic properties in epitaxial LaCoO_(3-x)films and provide a new perspective to regulate the magnetic properties of transition oxide thin films.展开更多
基金Supported by the National Natural Science Foundation of China under Grant No 60508013, and the Knowledge Innovation Programme of Chinese Academy of Sciences under Grant No KJCX1-05.
文摘A yellow continuous wave with beam quality M^2= 4.6 and output power of 4.8 W at 589nm is generated by intracavity sum-frequency mixing of 1064 nm and 1319 nm radiations of a Nd：YAG laser. To achieve high beam quality at high power, thermally near-unstable flat-flat resonators with two-rod birefringence compensation are designed to obtain the large fundamental mode size inside the Nd：YAG rods and the same beam width inside the KTP crystal. The optimal intracavity power ratio of both 1064nm and 1319nm beams is also considered. The output power fluctuation of the yellow laser remains less than 5% in four hours.
基金supported by the National Key Research and Development Program of China(Grant Nos.2020YFA0711502 and 2019YFA0704900)the National Natural Sciences Foundation of China(Grant Nos.52088101,51971240,and 11921004)the Key Program of the Chinese Academy of Sciences and the Strategic Priority Research Program(B)of the Chinese Academy of Sciences(Grant No.XDB33030200)。
文摘The origin of ferromagnetism in epitaxial strained LaCoO_(3-x)films has long been controversial.Here,we investigated the magnetic behavior of a series of oxygen vacancy-ordered LaCoO_(3-x)films on different substrates.Obvious ferromagnetism was observed in perovskite LaCoO_(3)/LSAT(LSAT=(LaAlO_(3))0.3(SrAlTaO_(6))_(0.7))and LaCoO_(3)/SrTiO_(3) films,while LaCoO_(3)/LaAlO_(3)films showed weak ferromagnetic behavior.Meanwhile,LaCoO_(2.67) films exhibited antiferromagnetic behavior.An unexpected low-temperature ferromagnetic phenomenon with a Curie temperature of~83 K and a saturation magnetization of~1.2μB/Co was discovered in 15 nm thick LaCoO_(2.5)/LSAT thin films,which is probably related to the change in the interface CoO_(6) octahedron rotation pattern.Meanwhile,the observed ferromagnetism gradually disappeared as the thickness of the film increased,indicating a relaxation of tensile strain.Analysis suggests that the rotation and rhombohedral distortion of the CoO_(6) octahedron weakened the crystal field splitting and promoted the generation of the ordered high-spin state of Co^(2+).Thus the super-exchange effect between Co^(2+)(high spin state),Co^(2+)(low spin state)and Co^(2+)(high spin state)produced a low-temperature ferromagnetic behavior.However,compressive-strained LaCoO_(2.5)film on a LaAlO_(3)substrate showed normal anti-ferromagnetic behavior.These results demonstrate that both oxygen vacancies and tensile strain are correlated with the emergent magnetic properties in epitaxial LaCoO_(3-x)films and provide a new perspective to regulate the magnetic properties of transition oxide thin films.
基金Supported by Natural Science Foundation of Guangdong Province(8451401501000668)Scientific Research Common Program of Beijing Municipal Commission of Education(KM200910011010)
